arXiv subjects

Rong-Chun Ge

Publications and source records attributed to Rong-Chun Ge.

At least 19 recordsLinked to original sources

arXiv2023

Cavity induced many-body localization

In this manuscript, we explore the feasibility of achieving many-body localization in the context of cavity quantum electrodynamics at strong coupling. Working with a spinless electronic Hubbard chain sitting coupled to a single-mode cavity, we show that the global coupling between electrons and photons -- which generally would be expected to delocalize the fermionic excitations -- can instead favor the appearance of localization. This is supported by a novel high-frequency expansion that correctly accounts for electron-photon interaction at strong coupling, as well as numerical calculations in both single particle and many-bod regimes. We find evidence that many-body localization may survive strong quantum fluctuations of the photon number by exploring energy dependence, seeing signatures of localization down to photon numbers as small as $n\sim2$.

cond-mat.mes-hall↗

arXiv2023

Coherent control of an ultrabright single spin in hexagonal boron nitride at room temperature

Hexagonal boron nitride (hBN) is a remarkable two-dimensional (2D) material that hosts solid-state spins and has great potential to be used in quantum information applications, including quantum networks. However, in this application, both the optical and spin properties are crucial for single spins but have not yet been discovered simultaneously for hBN spins. Here, we realize an efficient method for arraying and isolating the single defects of hBN and use this method to discover a new spin defect with a high probability of 85%. This single defect exhibits outstanding optical properties and an optically controllable spin, as indicated by the observed significant Rabi oscillation and Hahn echo experiments at room temperature. First principles calculations indicate that complexes of carbon and oxygen dopants may be the origin of the single spin defects. This provides a possibility for further addressing spins that can be optically controlled.

physics.optics↗

arXiv2021

Floquet engineering of lattice structure and dimensionality in twisted moiré heterobilayers

We present an experimental proposal to tune the effective lattice structure in twisted transition metal dichalcogenide (TMD) heterobilayers with time-periodic Floquet drive. We show that elliptically polarized light with sub-terahertz frequencies $\hbarω\sim 1$ meV and moderate electric fields $E\sim0.2$~MV/cm allows tuning between the native triangular lattice and a square lattice, while linearly polarized light enables dimensional reduction to a quasi-one-dimensional geometry. Without drive, these twisted TMDs simulate the single band Fermi-Hubbard model; we show that this approximation still holds in the presence of drive. This control opens the door to explore a rich variety of correlated phases of matter, such as spin liquids and d-wave superconductivity.

cond-mat.mes-hall↗

arXiv2016

Reply to "Comment on "Normalization of quasinormal modes in leaky optical cavities and plasmonic resonators" " by E. A. Muljarov and W. Langbein

We refute all claims of the "Comment on "Normalization of quasinormal modes in leaky optical cavities and plasmonic resonators" " by E. A. Muljarov and W. Langbein (arXiv:1602.07278v1). Based entirely on information already contained in our original article (P. T. Kristensen, R.-C. Ge and S. Hughes, Physical Review A 92, 053810 (2015)), we dismiss every point of criticism as being completely unjustified and point out how important parts of our argumentation appear to have been overlooked by the Comment Authors. In addition, we provide additional calculations showing directly the link between the normalizations by Sauvan et al. and Muljarov et al., which were not included in our original article.

cond-mat.mes-hall↗

arXiv2016

Quasinormal mode theory and modelling of electron energy loss spectroscopy for plasmonic nanostructures

Understanding light-matter interactions using localized surface plasmons (LSPs) is of fundamental interest in classical and quantum plasmonics and has a wide range of applications. In order to understand the spatial properties of LSPs, electron energy loss spectroscopy (EELS) is a common and powerful method of spatially resolving the extreme localized fields that can be obtained with metal resonators. However, modelling EELS for general shaped resonators presents a major challenge in computational electrodynamics, requiring the full photon Green function as a function of two space points and frequency. Here we present an intuitive and computationally simple method for computing EELS maps of plasmonic resonators using a quasinormal mode (QNM) expansion technique. By separating the contribution of the QNM and the bulk material, we give closed-form analytical formulas for the plasmonic QNM contribution to the EELS maps. We exemplify our technique for a split ring resonator, a gold nanorod, and a nanorod dimer structure. The method is accurate, intuitive, and gives orders of magnitude improvements over direct dipole simulations that numerically solve the full 3D Maxwell equations. We also show how the same QNM Green function can be used to obtain the Purcell factor (and projected local density of optical states) from quantum dipole emitters or two level atoms, and we demonstrate how the spectral features differ in general to the EELS spectrum.

cond-mat.mes-hall↗

arXiv2015

Normalization of quasinormal modes in leaky optical cavities and plasmonic resonators

We discuss three formally different formulas for normalization of quasinormal modes currently in use for modeling optical cavities and plasmonic resonators and show that they are complementary and provide the same result. Regardless of the formula used for normalization, one can use the norm to define an effective mode volume for use in Purcell factor calculations.

physics.optics↗

arXiv2015

Quantum dynamics of two quantum dots coupled through localized plasmons: An intuitive and accurate quantum optics approach using quasinormal modes

We study the quantum dynamics of two quantum dots (QDs) or artificial atoms coupled through the fundamental localized plasmon of a gold nanorod resonator. We derive an intuitive and efficient time-local master equation, in which the effect of the metal nanorod is taken into consideration self-consistently using a quasinormal mode (QNM) expansion technique of the photon Green function. Our efficient QNM technique offers an alternative and more powerful approach over the standard Jaynes-Cummings model, where the radiative decay, nonradiative decay, and spectral reshaping effect of the electromagnetic environment is rigorously included in a clear and transparent way. We also show how one can use our approach to compliment the approximate Jaynes-Cummings model in certain spatial regimes where it is deemed to be valid. We then present a study of the quantum dynamics and photoluminescence spectra of the two plasmon-coupled QDs. We first explore the non-Markovian regime, which is found to be important only on the ultrashort time scale of the plasmon mode which is about 40$\,$fs. For the field free evolution case of excited QDs near the nanorod, we demonstrate how spatially separated QDs can be effectively coupled through the plasmon resonance and we show how frequencies away from the plasmon resonance can be more effective for coherently coupling the QDs. Despite the strong inherent dissipation of gold nanoresonators, we show that qubit entanglements as large as 0.7 can be achieved from an initially separate state, which has been limited to less than 0.5 in previous work for weakly coupled reservoirs. We also study the superradiance and subradiance decay dynamics of the QD pair. Finally, we investigate the rich quantum dynamics of QDs that are incoherently pumped, ...

cond-mat.mes-hall↗

arXiv2015

Quasi-normal mode approach to the local-field problem in quantum optics

The local-field (LF) problem of a finite-size dipole emit- ter radiating inside a lossy inhomogeneous structure is a long-standing and challenging quantum optical problem, and it now is becoming more important due to rapid advances in solid-state fabrication technologies. Here we introduce a simple and accurate quasi-normal mode (QNM) technique to solve this problem analyti- cally by separating the scattering problem into contribu- tions from the QNM and an image dipole. Using a real- cavity model to describe an artificial atom inside a lossy and dispersive gold nanorod, we show when the contri- bution of the QNM to LFs will dominate over the homo- geneous contribution. We also show how to accurately describe surface scattering for real cavities that are close to the metal interface and explore regimes when the surface scattering dominates. Our results offer an intui- tive picture of the underlying physics for the LF problem and facilitate the understanding of novel photon sources within lossy structures.

cond-mat.mes-hall↗

arXiv2015

Design of an efficient single photon source from a metallic nanorod dimer: a quasinormal mode finite-difference time-domain approach

We describe how the finite-difference time-domain (FDTD) technique can be used to compute the quasinormal mode (QNM) for metallic nano-resonators, which is important for describing and understanding light-matter interactions in nanoplasmonics. We use the QNM to model the enhanced spontaneous emission rate for dipole emitters near a gold nanorod dimer structure using a newly developed QNM expansion technique. Significant enhanced photon emission factors of around 1500 are obtained with large output $β$-factors of about $60\%$.

cond-mat.mes-hall↗

arXiv2014

Quasinormal mode approach to modelling light-emission and propagation in nanoplasmonics

We describe a powerful and intuitive technique for modeling light-matter interactions in classical and quantum nanoplasmonics. Our approach uses a quasinormal mode expansion of the Green function within a metal nanoresonator of arbitrary shape, together with a Dyson equation, to derive an expression for the spontaneous decay rate and far field propagator from dipole oscillators outside resonators. For a single quasinormal mode, at field positions outside the quasi-static coupling regime, we give a closed form solution for the Purcell factor and generalized effective mode volume. We augment this with an analytic expression for the divergent LDOS very near the metal surface, which allows us to derive a simple and highly accurate expression for the electric field outside the metal resonator at distances from a few nanometers to infinity. This intuitive formalism provides an enormous simplification over full numerical calculations and fixes several pending problems in quasinormal mode theory.

quant-ph↗

arXiv2013

Accessing quantum nanoplasmonics in a hybrid quantum-dot metal nanosystem: Mollow triplet of a quantum dot near a metal nanoparticle

We present a theoretical study of the resonance fluorescence spectra of an optically driven quantum dot placed near a single metal nanoparticle. The metallic reservoir coupling is calculated for an 8-nm metal nanoparticle using a time-convolutionless master equation approach where the exact photon reservoir function is included using Green function theory. By exciting the system coherently near the nanoparticle dipole mode, we show that the driven Mollow spectrum becomes highly asymmetric due to internal coupling effects with higher-order plasmons. We also highlight regimes of resonance squeezing and broadening as well as spectral reshaping through light propagation. Our master equation technique can be applied to any arbitrary material system, including lossy inhomogeneous structures, where mode expansion techniques are known to break down.

cond-mat.mes-hall↗

arXiv2013

Mollow "quintuplets" from coherently-excited quantum dots

Charge-neutral excitons in semiconductor quantum dots have a small finite energy separation caused by the anisotropic exchange splitting. Coherent excitation of neutral excitons will generally excite both exciton components, unless the excitation is parallel to one of the dipole axes. We present a polaron master equation model to describe two-exciton pumping using a coherent continuous wave pump field in the presence of a realistic anisotropic exchange splitting. We predict a five-peak incoherent spectrum, thus generalizing the Mollow triplet to become a Mollow quintuplet. We experimentally confirm such spectral quintuplets for In(Ga)As quantum dots and obtain very good agreement with theory.

cond-mat.mes-hall↗

arXiv2012

Efficient Quantum Ratchet

Quantum resonance is one of the main characteristics of the quantum kicked rotor, which has been used to induce accelerated ratchet current of the particles with a generalized asymmetry potential. Here we show that by desynchronizing the kicked potentials of the flashing ratchet [Phys. Rev. Lett. 94, 110603 (2005)], new quantum resonances are stimulated to conduct directed currents more efficiently. Most distinctly, the missed resonances $κ=1.0π$ and $κ=3.0π$ are created out to induce even larger currents. At the same time, with the help of semiclassical analysis, we prove that our result is exact rather than phenomenon induced by errors of the numerical simulation. Our discovery may be used to realize directed transport efficiently, and may also lead to a deeper understanding of symmetry breaking for the dynamical evolution.

quant-ph↗

arXiv2011

Non-classical correlation of cascaded photon pairs emitted from quantum dot

We studied the quantum correlation between the photon pairs generated by biexciton cascade decays of self-assembled quantum dots, and determined the temperature behavior associated with so-called sudden change of the quantum correlation. The relationship between the fine structure splitting and the sudden change temperature is also provided. Our study indicates that this correlation behavior sudden change temperature is independent on the back ground noise in the system and far lower than entanglement sudden death temperature, therefore it should be easier to observe the phenomenon of correlation sudden change in experiments than to observe entanglement sudden death.

quant-ph↗

arXiv2011

Violation of Leggett-Garg inequalities in single quantum dot

We investigate the violation of Leggett-Garg (LG) inequalities inquantum dots with the stationarity assumption. By comparing two types of LG inequalities, we find a better one which is easier to be tested in experiment. In addition, we show that the fine-structure splitting, background noise and temperature of quantum dots all influence the violation of LG inequalities.

quant-ph↗

arXiv2010

Non-Markovian Dynamics of Quantum and Classical Correlations in the Presence of System-Bath Coherence

We present a detailed study of the dynamics of correlations in non-Markovian environments, applying the hierarchy equations approach. This theoretical treatment is able to take the system-bath interaction into consideration carefully. It is shown that crosses and sudden changes of classical and quantum correlations can happen if we gradually reduce the strength of the interactions between qubits. For some special initial states, sudden transitions between classical and quantum correlations even occur.

quant-ph↗

arXiv2010

Spin dynamics in the XY model

We study the evolution of entanglement, quantum correlation and classical correlation for the one dimensional XY model in external transverse magnetic field. The system is initialized in the full polarized state along the z axis, after annealing, different sites will become entangled. We study the three kinds of correlation for both the nearest and the next-nearest neighbor sites. We find that for large anisotropy parameter the quantum phase transition can be indicated by the dynamics of classical correlation between the nearest neighbor sites. We find that the dynamics of entanglement for both the nearest and next-nearest neighbor sites show significantly different behaviors with different values of magnetic field. We also find that the evolution of quantum correlation and classical correlation of the nearest neighbor sites are obviously different from those of the next-nearest neighbor sites.

quant-ph↗

arXiv2010

Non-Markovian Entanglement Sudden Death and Rebirth of a Two-Qubit System in the Presence of System-Bath Coherence

We present a detailed study of the entanglement dynamics of a two-qubit system coupled to independent non-Markovian environments, employing hierarchy equations. This recently developed theoretical treatment can conveniently solve non-Markovian problems and take into consideration the correlation between the system and bath in an initial state. We concentrate on calculating the death and rebirth time points of the entanglement to obtain a general view of the concurrence curve and explore the behavior of entanglement dynamics with respect to the coupling strength, the characteristic frequency of the noise bath and the environment temperature.

quant-ph↗