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Ronnie Kosloff

Publications and source records attributed to Ronnie Kosloff.

At least 19 recordsLinked to original sources

An experimental pathway towards an exact theory of strong coupling

We employ a mathematically equivalent form of the GKLS master equation to arrive at an exact theoretical description of a two-level system strongly coupled to the environment. The framework, while intuitive, shedding light on the physics of the problem, and agreeing with existing results, such as thermalisation to a non-canonical state, is based around three parameters that are unknown outside of the weak coupling regime -- the analogue to the detailed balance relation, and two coupling strength constants. As a way forward, we propose a feasible experimental protocol based on a solid-state electronic quantum dot device, through which the fundamental parameters of the problem can be revealed, which would further the fundamental understanding of strong coupling.

quant-ph

Memory-Scalable and Hardware-Adaptive Matrix-Free Quantum Simulation

The core step in quantum simulations is typically matrix vector multiplication $\phi = \Hmat \psi$. Executing this step is limited by memory requirement to store the Hamiltonian. We present a memory-scalable, hardware-adaptive matrix-free framework for applying large operators on vectors without materializing the full matrix on a single accelerator. The operator is represented through a block-procedural interface: blocks may be generated, loaded, cached, distributed, or applied directly only when their action is needed. For quantum simulation, it provides the core kernel for quantum operations. An adaptive planner selects block size, cache strategy, GPU grouping, row distribution, and task parallelization from memory and workload estimates. We describe analytic, measured, and learned planning strategies that choose between procedural generation, partial caching, full caching, and row-distributed caching. The method removes the requirement that the full dense matrix fit in the accelerator memory. This shifts large simulations from a fixed memory barrier to a tunable balance between block generation, cache reuse, data movement, parallel scheduling, and numerical accuracy.

quant-ph

Revealing the physical structure of the general quantum master equation

The Lindblad (GKLS) master equation, which represents the mathematical form for the general evolution of a density matrix, is a versatile and widely-used tool in open quantum systems. In contrast with the typical approach of imposing additional conditions on the system, such as weak coupling or energy conservation, we explore the structure of the equation with no assumptions. We demonstrate that general quantum dynamics can be expressed through a combination of free evolution, exchanges of some physical quantities (generalised charges), not necessarily commuting with the Hamiltonian, between the system and the bath, and pure dephasing. This result comprises a novel perspective on quantum master equations, employing physical processes as elemental parts. We use it to explore the dynamics and stationary states of a two-level system and show that strong coupling, particle exchange, and non-Abelian effects all share the same physical origin. Moreover, we demonstrate that the generalised Gibbs state for all three cases contains a non-commutation term, which has not been previously considered.

quant-ph

Quantum dot thermal machines -- a guide to engineering

Continuous particle exchange thermal machines require no time-dependent driving, can be realised in solid-state electronic devices, and miniaturised to nanometre scale. Quantum dots, providing a narrow energy filter and allowing to manipulate particle flow between the hot and cold reservoirs are at the heart of such devices. It has been theoretically shown that by mitigating passive heat flow, Carnot efficiency can be approached arbitrarily closely in a quantum dot heat engine, and experimentally, values of 0.7ηC have been reached. However, for practical applications, other parameters of a thermal machine, such as maximum power, efficiency at maximum power, and noise - stability of the power output or heat extraction - take precedence over maximising efficiency. We explore the effect of internal microscopic dynamics of a quantum dot on these quantities and demonstrate that its performance as a thermal machine depends on few parameters - the overall conductance and three inherent asymmetries of the dynamics. These parameters will act as a guide to engineering the quantum states of the quantum dot, allowing to optimise its performance beyond that of the simplest case of a two-fold spin-degenerate transmission level.

cond-mat.mes-hall

Optimal Control of thermally noisy quantum gates in a multilevel system

Quantum systems are inherently sensitive to environmental noise and imperfections in external control fields, which pose a significant challenge for the practical implementation of quantum technologies. These noise sources degrade the fidelity of quantum gates, making their mitigation a key requirement for realizing reliable quantum computing. In this study, we apply Optimal Control Theory (OCT) within a thermodynamically consistent Markovian framework to design high-fidelity quantum gates in the presence of thermal relaxation. Such a description is essential for realistic modeling and optimization of noisy quantum gates in near-term quantum technologies, where strong control fields and thermal environments act simultaneously. Our approach combines OCT with a control-dependent dissipative generator derived from the non-adiabatic master equation framework based on time-dependent invariants of the free evolution. As a result, the driving fields modify both the unitary and dissipative parts of the evolution. We implement the scheme for one- and two-qubit gates embedded in larger Hilbert spaces and compare direct-control and ancilla-assisted architectures. Using logical-subspace-resolved diagnostics, we quantify how the optimized dynamics redistributes the dissipative action between logical and ancillary sectors in the model systems studied here. In particular, we show that ancilla-assisted control can reduce the effective thermal-noise burden on the logical subspace in the relevant parameter regime, while direct control remains the most effective route when available. High-precision propagation of the full open-system dynamics reveals substantial fidelity improvements, in some cases by orders of magnitude, while clarifying the limits of mitigation at large relaxation rates and temperatures.

quant-ph

From the Bloch equation to a thermodynamically consistent master equation

The Bloch equation that set the foundation for open quantum systems, was conceived by pure physical reasoning. Since then, the Lindblad (GKLS) form of a quantum master equation, its most general mathematical representation, became an established staple in the open quantum systems toolbox. It allows to describe a multitude of quantum phenomena, however its universality comes at a cost - without additional constraints, the resultant dynamics are not necessarily thermodynamically consistent, and the equation itself lacks an intuitive interpretation. We present a mathematically equivalent form of the Lindblad master equation under a single constraint of strict energy conservation. The "elemental Bloch" equation separates the system dynamics into its elemental parts, making an explicit distinction between thermal mixing, dephasing, and energy relaxation, and thus reinstating the physical intuition in the equation. We derive the equation for a many-level system by accounting for all relevant transitions between pairs of levels. Finally, the formalism is illustrated by calculating the fixed point of the dynamics and exploring the conditions for canonical invariance in quantum systems.

quant-ph

Mitigating controller noise in quantum gates using optimal control theory

All quantum systems are subject to noise from the environment or external controls. This noise is a major obstacle to the realization of quantum technology. For example, noise limits the fidelity of quantum gates. Employing optimal control theory, we study the generation of quantum single and two-qubit gates. Specifically, we explore a Markovian model of phase and amplitude noise, leading to the degradation of the gate fidelity. We show that optimal control with such noise models generates control solutions to mitigate the loss of gate fidelity. The problem is formulated in Liouville space employing an extremely accurate numerical solver and the Krotov algorithm for solving the optimal control equations.

quant-ph

Inertial geometric quantum logic gates

We present rapid and robust protocols for STIRAP and quantum logic gates. Our gates are based on geometric phases acquired by instantaneous eigenstates of a slowly accelerating inertial Hamiltonian. To begin, we establish the criteria for inertial evolution and subsequently engineer pulse shapes that fulfill these conditions. These tailored pulses are then used to optimize geometric logic gates. We analyze a realization of our protocols with $^{87}$Rb atoms, resulting in gate fidelity that approaches the current state-of-the-art, with marked improvements in robustness.

quant-ph

Simulating photo-dissociation in strong field by the random phase thermal wavefunction approach

Simulating photo-dissociation processes is a challenging task when the number of states involved is significantly large. We present an ab-initio quantum model for strong field photo-dissociation processes which incorporates rotational dynamics. The computational complexity was reduced by employing the random phase thermal wavefunction method. The simulation outcome are analogous to experimental observable, such as the momentum angular distribution of the photo-fragments. We studied the convergence of these observables at two field intensities. The simulation method can be applied to wide-ranging time-domain spectroscopy at experimental conditions far beyond the reach of accurate direct numerical methods.

quant-ph

Unification of the first law of quantum thermodynamics

Underlying the classical thermodynamic principles are analogous microscopic laws, arising from the fundamental axioms of quantum mechanics. These define quantum thermodynamic variables such as quantum work and heat and characterize the possible transformations of open quantum systems. The foremost quantum thermodynamic law is a simple statement concerning the conservation of energy. Nevertheless, there exist ambiguity and disagreement regarding the precise partition of a quantum system's energy change to work and heat. By treating quantum mechanics as a comprehensive theory, applicable to both the micro and macroscopic domains, and employing dynamical symmetries, we bridge the gaps between five popular thermodynamic approaches to the first law. These include both autonomous and semi-classical formulations, which define work in terms of an ensemble average, as well as the single shot paradigm, where work is defined as a deterministic quantity.

quant-ph

Controlling the uncontrollable: Quantum control of open system dynamics

Quantum control of an open system is demonstrated employing a thermodynamically consistent master equation. In this framework, the open system dynamics depend on the control protocol due to the dressing of the system by the drive. This interrelation serves as the key element for control. The influence of the external drive is incorporated within the dynamical equation, enabling an indirect control of the dissipation. The control paradigm is displayed by analyzing entropy changing state to state transformations, heating and cooling N-level systems. Following, we study the generation of quantum non-unitary maps via coherent control. These include both reset maps with complete memory loss and single-qubit unitary maps under dissipative conditions.

quant-ph

Non-Markovian dynamics under time-translation symmetry

A dynamical symmetry is employed to determine the structure of the quantum non-Markovian time-local master equation. Such a structure is composed from two components: scalar kinetic coefficients and the standard quantum Markovian operator form. The kinetic coefficients are generally time-dependent and incorporate information on the kinematics and memory effects, while the operators manifest the dynamical symmetry. Specifically, we focus on time-translation symmetric dynamics, where the Lindblad jump operators constitute the eigenoperators of the free dynamics. This symmetry is motivated by thermodynamic microscopic considerations, where strict energy conservation between system and environment imposes the time-translation symmetry. The construction is generalized to other symmetries, and to driven quantum systems. The formalism is illustrated by three exactly solvable non-Markovian models, where the exact reduced description exhibits a dynamical symmetric structure. The formal structure of the master equation leads to a first principle calculation of the exact kinetic coefficients. This opens the possibility to simulate in a modular fashion non-Markovian dynamics.

quant-ph

Quantum optimal control in quantum technologies. Strategic report on current status, visions and goals for research in Europe

Quantum optimal control, a toolbox for devising and implementing the shapes of external fields that accomplish given tasks in the operation of a quantum device in the best way possible, has evolved into one of the cornerstones for enabling quantum technologies. The last few years have seen a rapid evolution and expansion of the field. We review here recent progress in our understanding of the controllability of open quantum systems and in the development and application of quantum control techniques to quantum technologies. We also address key challenges and sketch a roadmap for future developments.

quant-ph

Controlling the uncontrollable: Quantum control of open system dynamics

Control of open quantum systems is an essential ingredient to the realization of contemporary quantum science and technology. We demonstrate such control by employing a thermodynamically consistent framework, taking into account the fact that the drive can modify the interaction with environment. Such an effect is incorporated within the dynamical equation, leading to control dependent dissipation, this relation serves as the key element for open system control. Thermodynamics of the control process is reflected by a unidirectional flow of energy to the environment resulting in large entropy production. The control paradigm is displayed by analyzing entropy changing state to state transformations, such as heating and cooling. In addition, the generation of quantum gates under dissipative conditions is demonstrated for both non-unitary reset maps with complete memory loss and a universal set of single and double qubit unitary gates.

quant-ph

Employing Typicality in Optimal Control Theory

Controlling the dynamics of quantum systems is a crucial task in quantum science and technology. Obtaining the driving field that transforms the quantum systems to its objective is a typical control task. This task is hard, scaling unfavorably with the size of Hilbert space. To tackle this issue we employ typicality to assist in finding the control field for such systems. To demonstrate the method we choose the control task of cooling the fine structure states of the AlF molecule, from relatively high temperatures which results in large Hilbert space. Using quantum typicality, we demonstrate that we can simulate an ensemble of states, enabling a control task addressing simultaneously many states. We employ this method to find a control field for cooling molecules with large number of internal sates, corresponding to high initial temperatures.

quant-ph

Quantum thermo-dynamical construction for driven open quantum systems

Quantum dynamics of driven open systems should be compatible with both quantum mechanic and thermodynamic principles. By formulating the thermodynamic principles in terms of a set of postulates we obtain a thermodynamically consistent master equation. Following an axiomatic approach, we base the analysis on an autonomous description, incorporating the drive as a large transient control quantum system. In the appropriate physical limit, we derive the semi-classical description, where the control is incorporated as a time-dependent term in the system Hamiltonian. The transition to the semi-classical description reflects the conservation of global coherence and highlights the crucial role of coherence in the initial control state. We demonstrate the theory by analyzing a qubit controlled by a single bosonic mode in a coherent state.

quant-ph

Experimental verification of the inertial theorem control protocols

An experiment based on a trapped Ytterbium ion validates the inertial theorem for the SU(2) algebra. The qubit is encoded within the hyperfine states of the atom and controlled by RF fields. The inertial theorem generates analytical solutions for non-adiabatically driven systems that are `accelerated' slowly, bridging the gap between the sudden and adiabatic limits. These solutions are shown to be stable to small deviations, both experimentally and theoretically. As a result, the inertial solutions pave the way to rapid quantum control of closed, as well as open quantum systems. For large deviations from the inertial condition, the amplitude diverges while the phase remains accurate.

quant-ph

Coherent Control of Ultrafast Bond Making and Subsequent Molecular Dynamics: Demonstration of Final-State Branching Ratio Control

Quantum coherent control of ultrafast bond making and the subsequent molecular dynamics is crucial for the realization of a new photochemistry, where a shaped laser field is actively driving the chemical system in a coherent way from the thermal initial state of the reactants to the final state of the desired products. We demonstrate here coherent control over the relative yields of Mg$_2$ molecules that are generated via photoassociation and subsequently photodriven into different groups of final states. The strong-field process involves non-resonant multiphoton femtosecond photoassociation of a pair of thermally hot magnesium atoms into a bound Mg$_{2}$ molecule and subsequent molecular dynamics on electronically excited states. The branching-ratio control is achieved with linearly chirped laser pulses, utilizing the different chirp dependence that various groups of final molecular states display for their post-pulse population. Our study establishes the feasibility of high degree coherent control over quantum molecular dynamics that is initiated by femtosecond photoassociation of thermal atoms.

physics.atom-ph