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Rudolf Grimm

Publications and source records attributed to Rudolf Grimm.

At least 37 records · Page 2Linked to original sources

Decoherence of Impurities in a Fermi Sea of Ultracold Atoms

We investigate the decoherence of $^{40}$K impurities interacting with a three-dimensional Fermi sea of $^{6}$Li across an interspecies Feshbach resonance. The decoherence is measured as a function of the interaction strength and temperature using a spin-echo atom interferometry method. For weak to moderate interaction strengths, we interpret our measurements in terms of scattering of K quasiparticles by the Fermi sea and find very good agreement with a Fermi liquid calculation. For strong interactions, we observe significant enhancement of the decoherence rate, which is largely independent of temperature, pointing to behavior that is beyond the Fermi liquid picture.

cond-mat.quant-gas↗

Finite-temperature effects on a triatomic Efimov resonance in ultracold cesium

We report a thorough investigation of finite-temperature effects on three-body recombination near a triatomic Efimov resonance in an ultracold gas of cesium atoms. Our measurements cover a wide range from a near-ideal realization of the zero-temperature limit to a strongly temperature-dominated regime. The experimental results are analyzed within a recently introduced theoretical model based on a universal zero-range theory. The temperature-induced shift of the resonance reveals a contribution that points to an energy-dependence of the three-body parameter. We interpret this contribution in terms of the finite range of the van der Waals interaction in real atomic systems and we quantify it in an empirical way based on length scale arguments. A universal character of the corresponding resonance shift is suggested by observations related to other Efimov resonances and the comparison with a theoretical finite-temperature approach that explicitly takes the van der Waals interaction into account. Our findings are of importance for the precise determination of Efimov resonance positions from experiments at finite temperatures.

cond-mat.quant-gas↗

Ultracold dense samples of dipolar RbCs molecules in the rovibrational and hyperfine ground state

We produce ultracold dense trapped samples of 87Rb133Cs molecules in their rovibrational ground state, with full nuclear hyperfine state control, by stimulated Raman adiabatic passage (STIRAP) with efficiencies of 90%. We observe the onset of hyperfine-changing collisions when the magnetic field is ramped so that the molecules are no longer in the hyperfine ground state. A strong quadratic shift of the transition frequencies as a function of applied electric field shows the strongly dipolar character of the RbCs ground-state molecule. Our results open up the prospect of realizing stable bosonic dipolar quantum gases with ultracold molecules.

cond-mat.quant-gas↗

The three-body parameter for Efimov states in lithium-6

We present a state-of-the-art reanalysis of experimental results on Efimov resonances in the three-fermion system of $^6$Li. We discuss different definitions of the 3-body parameter (3BP) for Efimov states, and adopt a definition that excludes effects due to deviations from universal scaling for low-lying states. We develop a finite-temperature model for the case of three distinguishable fermions and apply it to the excited-state Efimov resonance to obtain the most accurate determination to date of the 3BP in an atomic three-body system. Our analysis of ground-state Efimov resonances in the same system yields values for the three-body parameter that are consistent with the excited-state result. Recent work has suggested that the reduced 3BP for atomic systems is a near-universal quantity, almost independent of the particular atom involved. However, the value of the 3BP obtained for $^6$Li is significantly ($\sim 20$%) different from that previously obtained from the excited-state resonance in Cs. The difference between these values poses a challenge for theory.

cond-mat.quant-gas↗

Resonant atom-dimer collisions in cesium: Testing universality at positive scattering lengths

We study the collisional properties of an ultracold mixture of cesium atoms and dimers close to a Feshbach resonance near 550G in the regime of positive $s$-wave scattering lengths. We observe an atom-dimer loss resonance that is related to Efimov's scenario of trimer states. The resonance is found at a value of the scattering length that is different from a previous observation at low magnetic fields. This indicates non-universal behavior of the Efimov spectrum for positive scattering lengths. We compare our observations with predictions from effective field theory and with a recent model based on the van der Waals interaction. We present additional measurements on pure atomic samples in order to check for the presence of a resonant loss feature related to an avalanche effect as suggested by observations in other atomic species. We could not confirm the presence of such a feature.

cond-mat.quant-gas↗

Observation of the Second Triatomic Resonance in Efimov's Scenario

We report the observation of a three-body recombination resonance in an ultracold gas of cesium atoms at a very large negative value of the $s$-wave scattering length. The resonance is identified as the second triatomic Efimov resonance, which corresponds to the situation where the first excited Efimov state appears at the threshold of three free atoms. This observation, together with a finite-temperature analysis and the known first resonance, allows the most accurate demonstration to date of the discrete scaling behavior at the heart of Efimov physics. For the system of three identical bosons, we obtain a scaling factor of $21.0(1.3)$, close to the ideal value of $22.7$.

cond-mat.quant-gas↗

Observation of a Strong Atom-Dimer Attraction in a Mass-Imbalanced Fermi-Fermi Mixture

We investigate a mixture of ultracold fermionic $^{40}$K atoms and weakly bound $^{6}$Li$^{40}$K dimers on the repulsive side of a heteronuclear atomic Feshbach resonance. By radio-frequency spectroscopy we demonstrate that the normally repulsive atom-dimer interaction is turned into a strong attraction. The phenomenon can be understood as a three-body effect in which two heavy $^{40}$K fermions exchange the light $^{6}$Li atom, leading to attraction in odd partial-wave channels (mainly p-wave). Our observations show that mass imbalance in a fermionic system can profoundly change the character of interactions as compared to the well-established mass-balanced case.

cond-mat.quant-gas↗

Quantum degenerate mixtures of strontium and rubidium atoms

We report on the realization of quantum degenerate gas mixtures of the alkaline-earth element strontium with the alkali element rubidium. A key ingredient of our scheme is sympathetic cooling of Rb by Sr atoms that are continuously laser cooled on a narrow linewidth transition. This versatile technique allows us to produce ultracold gas mixtures with a phase-space density of up to 0.06 for both elements. By further evaporative cooling we create double Bose-Einstein condensates of 87Rb with either 88Sr or 84Sr, reaching more than 10^5 condensed atoms per element for the 84Sr-87Rb mixture. These quantum gas mixtures constitute an important step towards the production of a quantum gas of polar, open-shell RbSr molecules.

cond-mat.quant-gas↗

Higher-nodal collective modes in a resonantly interacting Fermi gas

We report on experimental investigations of longitudinal collective oscillations in a highly elongated, harmonically trapped two-component Fermi gas with resonantly tuned s-wave interactions ('unitary Fermi gas'). We focus on higher-nodal axial modes, which in contrast to the elementary modes have received little attention so far. We show how these modes can be efficiently excited using a resonant local excitation scheme and sensitively analyzed by a Fourier transformation of the detected time evolution of the axial density profile. We study the temperature dependence of the mode frequencies across the superfluid phase transition. The behavior is qualitatively different from the elementary modes, where the mode frequencies are independent of the temperature as long as the gas stays in the hydrodynamic regime. Our results are compared to theoretical predictions based on Landau's two-fluid theory and available experimental knowledge of the equation of state. The comparison shows excellent agreement and thus both represents a sensitive test for the validity of the theoretical approach and provides an independent test of the equation of state. The present results obtained on modes of first-sound character represent benchmarks for the observation of second-sound propagation and corresponding oscillation modes.

cond-mat.quant-gas↗

Feshbach resonances, weakly bound molecular states and coupled-channel potentials for cesium at high magnetic fields

We explore the scattering properties of ultracold ground-state Cs atoms at magnetic fields between 450 G (45 mT) and 1000 G. We identify 17 new Feshbach resonances, including two very broad ones near 549 G and 787 G. We measure the binding energies of several different dimer states by magnetic field modulation spectroscopy. We use least-squares fitting to these experimental results, together with previous measurements at lower field, to determine a new 6-parameter model of the long-range interaction potential, designated M2012. Coupled-channels calculations using M2012 provide an accurate mapping between the s-wave scattering length and the magnetic field over the entire range of fields considered. This mapping is crucial for experiments that rely on precise tuning of the scattering length, such as those on Efimov physics.

cond-mat.quant-gas↗

Second sound and the superfluid fraction in a resonantly interacting Fermi gas

Superfluidity is a macroscopic quantum phenomenon, which shows up below a critical temperature and leads to a peculiar behavior of matter, with frictionless flow, the formation of quantized vortices, and the quenching of the moment of inertia being intriguing examples. A remarkable explanation for many phenomena exhibited by a superfluid at finite temperature can be given in terms of a two-fluid mixture comprised of a normal component that behaves like a usual fluid and a superfluid component with zero viscosity and zero entropy. Important examples of superfluid systems are liquid helium and neutron stars. More recently, ultracold atomic gases have emerged as new superfluid systems with unprecedented possibilities to control interactions and external confinement. Here we report the first observation of `second sound' in an ultracold Fermi gas with resonant interactions. Second sound is a striking manifestation of the two-component nature of a superfluid and corresponds to an entropy wave, where the superfluid and the non-superfluid components oscillate in opposite phase, different from ordinary sound (`first sound'), where they oscillate in phase. The speed of second sound depends explicitly on the value of the superfluid fraction, a quantity sensitive to the spectrum of elementary excitations. Our measurements allow us to extract the temperature dependence of the superfluid fraction, which in strongly interacting quantum gases has been an inaccessible quantity so far.

cond-mat.quant-gas↗

Collective Modes in a Unitary Fermi Gas across the Superfluid Phase Transition

We provide a joint theoretical and experimental investigation of the temperature dependence of the collective oscillations of first sound nature exhibited by a highly elongated harmonically trapped Fermi gas at unitarity, including the region below the critical temperature for superfluidity. Differently from the lowest axial breathing mode, the hydrodynamic frequencies of the higher nodal excitations show a temperature dependence, which is calculated starting from Landau two-fluid theory and using the available experimental knowledge of the equation of state. The experimental results agree with high accuracy with the predictions of theory and provide the first evidence for the temperature dependence of the collective frequencies near the superfluid phase transition.

cond-mat.quant-gas↗

Laser cooling to quantum degeneracy

We report on Bose-Einstein condensation (BEC) in a gas of strontium atoms, using laser cooling as the only cooling mechanism. The condensate is formed within a sample that is continuously Doppler cooled to below 1\muK on a narrow-linewidth transition. The critical phase-space density for BEC is reached in a central region of the sample, in which atoms are rendered transparent for laser cooling photons. The density in this region is enhanced by an additional dipole trap potential. Thermal equilibrium between the gas in this central region and the surrounding laser cooled part of the cloud is established by elastic collisions. Condensates of up to 10^5 atoms can be repeatedly formed on a timescale of 100ms, with prospects for the generation of a continuous atom laser.

cond-mat.quant-gas↗

Production of quantum degenerate strontium gases: Larger, better, faster, colder

We report on an improved scheme to generate Bose-Einstein condensates (BECs) and degenerate Fermi gases of strontium. This scheme allows us to create quantum gases with higher atom number, a shorter time of the experimental cycle, or deeper quantum degeneracy than before. We create a BEC of 84-Sr exceeding 10^7 atoms, which is a 30-fold improvement over previously reported experiments. We increase the atom number of 86-Sr BECs to 2.5x10^4 (a fivefold improvement), and refine the generation of attractively interacting 88-Sr BECs. We present a scheme to generate 84-Sr BECs with a cycle time of 2s, which, to the best of our knowledge, is the shortest cycle time of BEC experiments ever reported. We create deeply-degenerate 87-Sr Fermi gases with T/T_F as low as 0.10(1), where the number of populated nuclear spin states can be set to any value between one and ten. Furthermore, we report on a total of five different double-degenerate Bose-Bose and Bose-Fermi mixtures. These studies prepare an excellent starting point for applications of strontium quantum gases anticipated in the near future.

cond-mat.quant-gas↗

Creation of ultracold Sr2 molecules in the electronic ground state

We report on the creation of ultracold 84Sr2 molecules in the electronic ground state. The molecules are formed from atom pairs on sites of an optical lattice using stimulated Raman adiabatic passage (STIRAP). We achieve a transfer efficiency of 30% and obtain 4x10^4 molecules with full control over the external and internal quantum state. STIRAP is performed near the narrow 1S0-3P1 intercombination transition, using a vibrational level of the 0u potential as intermediate state. In preparation of our molecule association scheme, we have determined the binding energies of the last vibrational levels of the 0u, 1u excited-state, and the 1Σ_g^+ ground-state potentials. Our work overcomes the previous limitation of STIRAP schemes to systems with Feshbach resonances, thereby establishing a route that is applicable to many systems beyond bi-alkalis.

cond-mat.quant-gas↗

Towards the production of ultracold ground-state RbCs molecules: Feshbach resonances, weakly bound states, and coupled-channel model

We have studied interspecies scattering in an ultracold mixture of $^{87}$Rb and $^{133}$Cs atoms, both in their lowest-energy spin states. The three-body loss signatures of 30 incoming s- and p-wave magnetic Feshbach resonances over the range 0 to 667 G have been catalogued. Magnetic field modulation spectroscopy was used to observe molecular states bound by up to 2.5 MHz$\times h$. Magnetic moment spectroscopy along the magneto-association pathway from 197 to 182 G gives results consistent with the observed and calculated dependence of the binding energy on magnetic field strength. We have created RbCs Feshbach molecules using two of the resonances. We have set up a coupled-channel model of the interaction and have used direct least-squares fitting to refine its parameters to fit the experimental results from the Feshbach molecules, in addition to the Feshbach resonance positions and the spectroscopic results for deeply bound levels. The final model gives a good description of all the experimental results and predicts a large resonance near 790 G, which may be useful for tuning the interspecies scattering properties. Quantum numbers and vibrational wavefunctions from the model can also be used to choose optimal initial states of Feshbach molecules for their transfer to the rovibronic ground state using stimulated Raman adiabatic passage (STIRAP).

physics.atom-ph↗

Metastability and Coherence of Repulsive Polarons in a Strongly Interacting Fermi Mixture

Ultracold Fermi gases with tuneable interactions represent a unique test bed to explore the many-body physics of strongly interacting quantum systems. In the past decade, experiments have investigated a wealth of intriguing phenomena, and precise measurements of ground-state properties have provided exquisite benchmarks for the development of elaborate theoretical descriptions. Metastable states in Fermi gases with strong repulsive interactions represent an exciting new frontier in the field. The realization of such systems constitutes a major challenge since a strong repulsive interaction in an atomic quantum gas implies the existence of a weakly bound molecular state, which makes the system intrinsically unstable against decay. Here, we exploit radio-frequency spectroscopy to measure the complete excitation spectrum of fermionic 40K impurities resonantly interacting with a Fermi sea of 6Li atoms. In particular, we show that a well-defined quasiparticle exists for strongly repulsive interactions. For this "repulsive polaron" we measure its energy and its lifetime against decay. We also probe its coherence properties by measuring the quasiparticle residue. The results are well described by a theoretical approach that takes into account the finite effective range of the interaction in our system. We find that a non-zero range of the order of the interparticle spacing results in a substantial lifetime increase. This major benefit for the stability of the repulsive branch opens up new perspectives for investigating novel phenomena in metastable, repulsively interacting fermion systems.

cond-mat.quant-gas↗

Detection and manipulation of nuclear spin states in fermionic strontium

Fermionic 87Sr has a nuclear spin of I=9/2, higher than any other element with similar electronic structure. This large nuclear spin has many applications in quantum simulation and computation, for which preparation and detection of the spin state are requirements. For an ultracold 87Sr cloud, we show two complementary methods to characterize the spin-state mixture: optical Stern-Gerlach state separation and state-selective absorption imaging. We use these methods to optimize the preparation of a variety of spin-state mixtures by optical pumping and to measure an upper bound of the 87Sr spin relaxation rate.

cond-mat.quant-gas↗