arXiv subjects

Rudolf Gross

Publications and source records attributed to Rudolf Gross.

At least 19 recordsLinked to original sources

arXiv2026

Nonreciprocal Magnon Hanle Effect in Antiferromagnetic $\alpha$-Fe$_2$O$_3$

The precession of the magnon pseudospin about the equilibrium pseudofield, the latter capturing the nature of magnonic eigenexcitations in an antiferromagnet, gives rise to the magnon Hanle effect. Its realization via electrically injected and detected spin transport in an antiferromagnetic insulator demonstrates its high potential for devices and as a convenient probe for magnon eigenmodes and the underlying spin interactions in the antiferromagnet. Here, we observe a non-reciprocity in the Hanle signal measured in alpha-Fe2O3 using two spatially separated Pt electrodes as spin injector and detector. Interchanging their roles alters the detected magnon spin signal. The recorded difference depends on the applied magnetic field and reverses sign when the signal passes its nominal maximum at the so-called compensation field. Our findings unlock the high potential of antiferromagnetic magnonics towards the realization of electronics-inspired phenomena.

cond-mat.mes-hall↗

arXiv2026

Spin Hall Magnetoresistance in Antiferromagnetic Insulators

Antiferromagnetic materials promise improved performance for spintronic applications, as they are robust against external magnetic field perturbations and allow for faster magnetization dynamics compared to ferromagnets. The direct observation of the antiferromagnetic state, however, is challenging due to the absence of a macroscopic magnetization. We show that the spin Hall magnetoresistance (SMR) is a versatile tool to probe the antiferromagnetic spin structure via simple electrical transport experiments by investigating the easy-plane antiferromagnetic insulators alpha-Fe2O3 (hematite) and NiO in bilayer heterostructures with a Pt heavy-metal top electrode. While rotating an external magnetic field in three orthogonal planes, we record the longitudinal and the transverse resistivities of Pt and observe characteristic resistivity modulations consistent with the SMR effect. We analyze both their amplitude and phase and compare the data to the results from a prototypical collinear ferrimagnetic Y3Fe5O12/Pt bilayer. The observed magnetic field dependence is explained in a comprehensive model, based on two magnetic sublattices and taking into account magnetic field-induced modifications of the domain structure. Our results show that the SMR effect allows to readout the spin configuration and to investigate magnetoelastic effects in antiferromagnetic multi-domain materials. We demonstrate that the SMR amplitude scales with the sum of the absolute sublattice magnetizations in ferrimagnetic and antiferromagnetic materials. In alpha-Fe2O3/Pt bilayers, we find an unexpectedly large SMR amplitude of 2.5E-3, twice as high as for prototype Y3Fe5O12/Pt bilayers, making the system particularly interesting for room-temperature antiferromagnetic spintronic applications.

cond-mat.mtrl-sci↗

arXiv2026

Temperature dependence of the magnon-phonon coupling in yttrium iron garnet/gadolinium gallium garnet high overtone bulk acoustic resonators

Weexperimentally study the temperature dependence of the magnon-phonon coupling in a yttrium iron garnet (YIG)/gadolinium gallium garnet (GGG) heterostructure. More specifically, we use broadband ferromagnetic resonance to investigate the magneto-elastic coupling between the Kittel mode of a YIG thin film and the transverse acoustic phonon modes of the YIG/GGG high overtone bulk acoustic wave acoustic resonator for in and out-of-plane field directions in the temperature range between T = 5K and 300K. We find that for a magnetic field applied normal to the film surface, magneto-elastic coupling decreases with decreasing temperature, whereas it increases for the in-plane magnetic field configuration. The observed temperature dependence differs from earlier observations on bulk YIG samples, which might be due to the temperature dependent stress imposed by the GGG substrate.

cond-mat.mtrl-sci↗

arXiv2026

Impact of Stoichiometry of MoSi Thin Films for Enhanced Sensitivity of Superconducting Nanowire Single-Photon Detectors

We report on the impact of the stoichiometry of superconducting MoSi thin films on the performance of superconducting nanowire single-photon detectors (SNSPDs). Specifically, we investigate the relation between the film parameters critical temperature Tc , sheet resistance Rs and superconductor thickness d and observe a universal scaling behavior. To benchmark the performance of SNSPDs fabricated from films having different stoichiometry, we measure the bias dependent count rate curves, while the detector is illuminated with wavelengths between 780 nm and 1550 nm. The detector performance as a function photon energy for different nanowire widths reveals a linear relation between the detection current and the photon energy. Furthermore, we determine the interfacial thermal boundary conductance $\beta$ between the superconducting thin film and the substrate, by measuring the return current of the SNSPD and find an increase of $\beta$ with increasing Mo concentration. The highest sensitivity amongst all compared devices is achieved for Mo$_{0.53}$Si$_{0.47}$, with low Tc (4.1 K) and high Rs (397$\Omega$/sq) at a film thickness of 5.4 nm.

cond-mat.supr-con↗

arXiv2026

Experimental setup for the combined study of spin ensembles and superconducting quantum circuits

A hybrid quantum computing architecture combining quantum processors and quantum memory units allows for exploiting each component's unique properties to enhance the overall performance of the total system. However, superconducting qubits are highly sensitive to magnetic fields, while spin ensembles require finite fields for control, creating a major integration challenge. In this work, we demonstrate the first experimental setup that satisfies these constraints and provides verified qubit stability. Our cryogenic setup comprises two spatially and magnetically decoupled sample volumes inside a single dilution refrigerator: one hosting flux-tunable superconducting qubits and the other a spin ensemble equipped with a superconducting solenoid generating fields up to 50 mT. We show that several layers of Cryophy shielding and an additional superconducting aluminum shield suppress magnetic crosstalk by more than eight orders of magnitude, ensuring stability of the qubit's performance. Moreover, the operation of the solenoid adds minimal thermal load on the relevant stages of the dilution refrigerator. Our results enable scalable hybrid quantum architectures with low-loss integration, marking a key step toward scalable hybrid quantum computing platforms.

physics.app-ph↗

arXiv2026

Practical quantum tokens: challenges and perspectives

The concept of quantum tokens dates back alongside quantum cryptography to Stephen Wiesner's seminal work in 1983[1]. Already this initial work proposes society-relevant applications such as secure quantum banknotes, which can be exchanged between a bank and a customer. This quantum currency is based on various physical states that can be easily verified but is protected from being copied by the fundamental quantum laws. Four decades later, these ideas have flourished in the field of quantum information, and the concept of quantum banknotes has not only adopted many varying names, such as quantum money, quantum coins, quantum-digital payments, and quantum tokens, but also reached its first experimental demonstrations. In this perspective article, we discuss the current state-of-the-art of quantum tokens in the field of quantum information, as well as their future perspectives. We present a number of physical realizations of quantum tokens with integrated quantum memories and their applicability scenarios in detail. Finally, we discuss how quantum tokens fit into the information security ecosystem and consider their relationship to post-quantum cryptography.

quant-ph↗

arXiv2025

Resolving Abrikosov vortex entry in superconducting nano-string resonators via displacement-noise spectroscopy in cavity-optomechanics

Abrikosov vortices in type-II superconductors critically influence current flow and coherence, thereby imposing fundamental limits on superconducting quantum technologies. Quantum circuits employ superconducting elements at micro- and mesoscopic scales, where individual vortices can significantly impact device performance, necessitating investigation of vortex entry, motion, and pinning in these constrained geometries. Cavity-optomechanical platforms combining flux-tunable microwave resonators with superconducting nanomechanical elements offer a promising route to the single-photon strong-coupling regime and enable highly sensitive probing of the mechanical degree of freedom under elevated magnetic fields. Here, we exploit this platform to investigate vortex entry processes at the single-event level. We observe discrete jumps of the mechanical resonance frequency attributable to individual vortex entry, corresponding to attonewton-scale forces and allowing quantitative extraction of single-vortex pinning energies. These signatures are superimposed on a smooth power-law background characteristic of the collective Campbell-regime of vortex elasticity. Our results establish optomechanics-inspired sensing as a powerful method for exploring fundamental superconducting properties and identifying decoherence pathways in quantum circuits. Beyond advancing vortex physics, this work opens new opportunities for integrating mechanical sensing into superconducting device architectures, bridging condensed matter physics and quantum information science.

cond-mat.mes-hall↗

arXiv2025

Charge, heat, and spin transport phenomena in metallic conductors

In solid state materials, gradients of the electro-chemical potential, the temperature, or the spin-chemical potential drive the flow of charge, heat, and spin angular momentum, resulting in a net transport of energy. Beyond the primary transport processes - such as the flow of charge, heat, and spin angular momentum driven by gradients in their respective potentials - a wide range of coupled or cross-linked transport responses can occur, giving rise to a rich variety of transport phenomena. These transport phenomena are commonly categorized under (anomalous) thermoelectric, thermomagnetic, and galvanomagnetic effects, along with their spin-dependent counterparts. However, establishing a systematic classification and comparison among them remains a complex and nontrivial task. This paper attempts a didactic overview of the different transport phenomena, by categorizing and briefly discussing each of them based on charge, heat, and spin transport in conducting solids. The phenomena are structured in three categories: collinear, transverse, and so-called `planar' transport effects. The resulting overview attempts to categorize all effects in a consistent manner.

cond-mat.mtrl-sci↗

arXiv2025

Broadband electron paramagnetic resonance spectroscopy of $^{167}$Er:$^{7}$LiYF$_4$ at mK temperatures

Rare-earth spin ensembles are a promising platform for microwave quantum memory applications due to their hyperfine transitions, which can exhibit exceptionally long coherence times when using an operation point with zero first-order Zeeman (ZEFOZ) shift. In this work, we use broadband electron paramagnetic resonance (EPR) spectroscopy on $^{167}$Er:$^{7}$LiYF$_4$ single crystals at sub-Kelvin temperatures. By fitting the spin Hamiltonian to the zero-field spectrum, we obtain refined parameters of the magnetic field-independent interactions, such as the hyperfine and quadrupole interaction. We also study the influence of the quadrupole interaction on the hyperfine splitting in the zero and low magnetic field range by analyzing EPR-spectra between 0 mT and 50 mT. Our findings highlight the broadband EPR spectroscopy approach as a powerful tool for the precise determination of the spin Hamiltonian parameters and for the characterization of hyperfine transitions in terms of their selection rules and linewidth.

quant-ph↗

arXiv2024

Planar scanning probe microscopy enables vector magnetic field imaging at the nanoscale

Planar scanning probe microscopy is a recently emerging alternative approach to tip-based scanning probe imaging. It can scan an extended planar sensor, such as a polished bulk diamond doped with magnetic-field-sensitive nitrogen-vacancy (NV) centers, in nanometer-scale proximity of a planar sample. So far, this technique has been limited to optical near-field microscopy, and has required nanofabrication of the sample of interest. Here we extend this technique to magnetometry using NV centers, and present a modification that removes the need for sample-side nanofabrication. We harness this new ability to perform a hitherto infeasible measurement - direct imaging of the three-dimensional vector magnetic field of magnetic vortices in a thin film magnetic heterostructure, based on repeated scanning with NV centers with different orientations within the same scanning probe. Our result opens the door to quantum sensing using multiple qubits within the same scanning probe, a prerequisite for the use of entanglement-enhanced and massively parallel schemes.

cond-mat.mes-hall↗

arXiv2024

Electronic correlations and spin frustration in the molecular conductors $\kappa$-(BEDT-TTF)$_2$X probed by magnetic quantum oscillations

The layered molecular conductors $\kappa$-(BEDT-TTF)$_2$X are a perfect experimental platform for studying the physics of the Mott transition and related exotic electronic states. In these materials, the subtle balance between various instabilities of the normal metallic state can be efficiently changed by applying a very moderate external pressure or by subtle chemical modifications, e.g. by a replacement of the insulating anion X$^{-}$, frequently referred to as ``chemical pressure''. A crucially important but still unsettled issue is an exact understanding of the influence of physical and chemical pressure on the electronic structure. Here, we use magnetic quantum oscillations to explore in a broad pressure range the behavior of the key parameters governing the Mott physics, the electronic correlation strength ratio $U/t$ and the spin frustration ratio $t'/t$ in two $\kappa$ salts, the ambient-pressure antiferromagnetic insulator with X = Cu[N(CN)$_2$]Cl and the ambient-pressure superconductor with X = Cu(NCS)$_2$. Our analysis shows that pressure effectively changes not only the conduction bandwidth but also the degree of spin frustration, thus weakening both the electronic correlation strength and the magnetic ordering instability. At the same time, we find that the replacement of the anion Cu[N(CN)$_2$]Cl$^-$ by Cu(NCS)$_2^-$ results in a significant increase of the frustration parameter $t'/t$, leaving the correlation strength essentially unchanged.

cond-mat.str-el↗

arXiv2024

Onset of transmon ionization in microwave single-photon detection

By strongly driving a transmon-resonator system, the transmon qubit may eventually escape from its cosine-shaped potential. This process is called transmon ionization (TI) and known to be detrimental to the qubit coherence and operation. In this work, we investigate the onset of TI in an irreversible, parametrically-driven, frequency conversion process in a system consisting of a superconducting 3D-cavity coupled to a fixed-frequency transmon qubit. Above a critical pump power we find a sudden increase in the transmon population. Using Renyi entropy, Floquet modes, and Husimi Q functions, we infer that this abrupt change can be attributed to a quantum-to-classical phase transition. Furthermore, in the context of the single-photon detection, we measure a TI-uncorrected detection efficiency of up to 86% and estimate a TI-corrected value of up to 78% by exploiting the irreversible frequency conversion. Our numerical simulations suggest that increasing the detuning between the pump and qubit frequencies and increasing the qubit anharmonicity can suppress the TI impact. Our findings highlight the general importance of the TI process when operating coupled qubit-cavity systems.

quant-ph↗

arXiv2024

Remote sensing of a levitated superconductor with a flux-tunable microwave cavity

We present a cavity-electromechanical system comprising a superconducting quantum interference device which is embedded in a microwave resonator and coupled via a pick-up loop to a 6 $\mu$g magnetically-levitated superconducting sphere. The motion of the sphere in the magnetic trap induces a frequency shift in the SQUID-cavity system. We use microwave spectroscopy to characterize the system, and we demonstrate that the electromechanical interaction is tunable. The measured displacement sensitivity of $10^{-7} \, \mathrm{m} / \sqrt{\mathrm{Hz}}$, defines a path towards ground-state cooling of levitated particles with Planck-scale masses at millikelvin environment temperatures.

quant-ph↗

arXiv2023

Temperature dependence of the magnon-phonon interaction in high overtone bulk acoustic resonator-ferromagnetic thin film hybrids

Tailored magnon-phonon hybrid systems, where high overtone bulk acoustic resonators couple resonantly to the magnonic mode of a ferromagnetic thin film, are considered optimal for the creation of acoustic phonons with a defined circular polarization. This class of devices is therefore ideal for the investigation of phonon propagation properties and assessing their capacity to transport angular momentum in the classical and potentially even in the quantum regime. Here, we study the coupling between the magnons in a ferromagnetic \ch{Co25Fe75} thin film and the transverse acoustic phonons in a bulk acoustic wave resonators formed by the sapphire substrate onto which the film is deposited. Using broadband ferromagnetic resonance experiments as a function of temperature, we investigate the strength of the coherent magnon-phonon interaction and the individual damping rates of the magnons and phonons participating in the process. This demonstrates that this coupled magnon-phonon system can reach a cooperativity $C\approx 1$ at cryogenic temperatures. Our experiments also showcase the potential of strongly coupled magnon-phonon systems for strain sensing applications.

cond-mat.mes-hall↗

arXiv2023

Electrically induced angular momentum flow between separated ferromagnets

Converting angular momentum between different degrees of freedom within a magnetic material results from a dynamic interplay between electrons, magnons and phonons. This interplay is pivotal to implementing spintronic device concepts that rely on spin angular momentum transport. We establish a new concept for long-range angular momentum transport that further allows to address and isolate the magnonic contribution to angular momentum transport in a nanostructured metallic ferromagnet. To this end, we electrically excite and detect spin transport between two parallel and electrically insulated ferromagnetic metal strips on top of a diamagnetic substrate. Charge-to-spin current conversion within the ferromagnetic strip generates electronic spin angular momentum that is transferred to magnons via electron-magnon coupling. We observe a finite angular momentum flow to the second ferromagnetic strip across a diamagnetic substrate over micron distances, which is electrically detected in the second strip by the inverse charge-to-spin current conversion process. We discuss phononic and dipolar interactions as the likely cause to transfer angular momentum between the two strips. Moreover, our work provides the experimental basis to separate the electronic and magnonic spin transport and thereby paves the way towards magnonic device concepts that do not rely on magnetic insulators.

cond-mat.mes-hall↗

arXiv2023

Single-crystalline YIG flakes with uniaxial in-plane anisotropy and diverse crystallographic orientations

We study Y3Fe5O12 (YIG) flakes that we produce via mechanical cleaving and exfoliation of YIG single crystals. By characterizing their structural and magnetic properties, we find that these YIG nanoflakes have surfaces oriented along unusual crystallographic axes and uniaxial in-plane magnetic anisotropy due to their shape, both of which are not commonly available in YIG thin films. These physical properties, combined with the possibility of picking up the YIG flakes and stacking them onto flakes of other van der Waals materials or pre-patterned electrodes or waveguides, open unexplored possibilities for magnonics and for the realization of novel YIG-based heterostructures and devices.

cond-mat.mtrl-sci↗

arXiv2023

High-Q magnetic levitation and control of superconducting microspheres at millikelvin temperatures

We report the levitation of a superconducting lead-tin sphere with 100 micrometer diameter (corresponding to a mass of 5.6 micrograms) in a static magnetic trap formed by two coils in an anti-Helmholtz configuration, with adjustable resonance frequencies up to 240 hertz. The center-of-mass motion of the sphere is monitored magnetically using a dc superconducting quantum interference device as well as optically and exhibits quality factors of up to 2.6e7. We also demonstrate 3D magnetic feedback control of the sphere's motion. The setup is housed in a dilution refrigerator operating at 15 millikelvin. By implementing a cryogenic vibration isolation system we can attenuate environmental vibrations at 200 hertz by approximately seven orders of magnitude. The combination of low temperature, large mass and high quality factor as well as adjustable resonance frequencies provides a promising platform for testing quantum physics in previously unexplored regimes with high mass and long coherence times.

quant-ph↗

arXiv2023

Impact of magnetic anisotropy on the magnon Hanle effect in $α$-Fe$_2$O$_3$

In easy-plane antiferromagnets, the nature of the elementary excitations of the spin system is captured by the precession of the magnon pseudospin around its equilibrium pseudofield, manifesting itself in the magnon Hanle effect. Here, we investigate the impact of growth-induced changes in the magnetic anisotropy on this effect in the antiferromagnetic insulator $α$-Fe$_2$O$_3$ (hematite). To this end, we compare the structural, magnetic, and magnon-based spin transport properties of $α$-Fe$_2$O$_3$ films with different thicknesses grown by pulsed laser deposition in molecular and atomic oxygen atmospheres. While in films grown with molecular oxygen a spin-reorientation transition (Morin transition) is absent down to $10\,$K, we observe a Morin transition for those grown by atomic-oxygen-assisted deposition, indicating a change in magnetic anisotropy. Interestingly, even for a $19\,$nm thin $α$-Fe$_2$O$_3$ film grown with atomic oxygen we still detect a Morin transition at $125\,$K. We characterize the magnon Hanle effect in these $α$-Fe$_2$O$_3$ films via all-electrical magnon transport measurements. The films grown with atomic oxygen show a markedly different magnon spin signal from those grown in molecular oxygen atmospheres. Most importantly, the maximum magnon Hanle signal is significantly enhanced and the Hanle peak is shifted to lower magnetic field values for films grown with atomic oxygen. These observations suggest a change of magnetic anisotropy for $α$-Fe$_2$O$_3$ films fabricated by atomic-oxygen-assisted deposition resulting in an increased oxygen content in these films. Our findings provide new insights into the possibility to fine-tune the magnetic anisotropy in $α$-Fe$_2$O$_3$ and thereby to engineer the magnon Hanle effect.

cond-mat.mes-hall↗