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Rui-Jian Liang

Publications and source records attributed to Rui-Jian Liang.

6 recordsLinked to original sources

Room-Temperature Storage of Entanglement in a Silicon Carbide Quantum Node

Robust entanglement at room temperature is a central challenge for solid-state quantum information processing and quantum-enhanced sensing. Here we demonstrate room-temperature storage of entanglement in a silicon carbide (SiC) quantum node by coherently transferring an electron-nuclear entangled state onto long-lived nuclear-spin memory qubits. Using a shallow single color center in 4H-SiC, conventionally denoted PL6, we realize a fully addressable three-qubit register composed of one electron-spin processor and two strongly coupled $^{29}$Si nuclear-spin memory qubits. This platform enables the deterministic generation of high-fidelity entangled states, including a nuclear-spin Bell state with a fidelity of $94 \pm 2\%$ and a three-qubit Greenberger-Horne-Zeilinger (GHZ)-type state with a fidelity of $89 \pm 4\%$. By implementing a SWAP-gate protocol in the strong hyperfine-coupling regime, the electron-nuclear entanglement is transferred to the nuclear-spin memory with a fidelity of $92.5 \pm 2.5\%$, extending the entanglement lifetime by a factor of 240. We further confirm the generality of this approach in an additional heterogeneous $^{29}$Si-$^{13}$C nuclear-spin register and, through a statistical survey of 200 single PL6 centers, show that multi-nuclear-spin registers occur naturally with probabilities above 10%. These results position shallow SiC color centers as a powerful platform for entanglement-assisted quantum sensing and scalable room-temperature quantum technologies.

quant-ph

High-yield engineering and identification of oxygen-related modified divacancies in 4H-SiC

Modified divacancies in the 4H polytype of silicon carbide (SiC) exhibit enhanced charge stability and spin addressability at room temperature, making them attractive for quantum applications. However, their low formation yield and lack of direct structural identification have hindered progress. Here, we demonstrate a controllable method for high-yield engineering and identification of oxygen-related modified divacancy color centers in 4H-SiC via oxygen-ion implantation. Based on their distinct optical and spin-resonance characteristics, we experimentally resolve four types of modified divacancies. Furthermore, by measuring isotope-resolved 17O hyperfine interactions, we identify them as the four crystallographic configurations of oxygen-vacancy (OV) complexes. Remarkably, single OV centers account for over 90% of the total defect population and exhibit superior optical properties and spin coherence compared with defects created by conventional carbon or nitrogen implantation. We characterize the zero-phonon lines of these OV centers and reveal distinct temperature-dependent behavior in spin-readout contrast. By optimizing implantation dose and annealing temperature, we achieve high-density ensembles and observe Rabi-oscillation beating patterns associated with different orientations of basal-type defects. These results establish a high-yield route for scalable engineering of these four oxygen-related modified divacancies in 4H-SiC and clarify their atomic structure, opening new opportunities for solid-state quantum technologies.

quant-ph

Coherent Spin-Photon Interface of single PL6 Color Centers in Silicon Carbide

The PL6 color center in silicon carbide has recently emerged as a promising platform for quantum information processing, yet its coherent spin--photon interface has remained largely unexplored. Here we present a comprehensive investigation of single PL6 centers, combining spectroscopy with theoretical analysis. The excited-state fine structure is fully resolved using group-theoretical modeling and strain-dependent measurements. Under resonant excitation, we achieve a spin initialization fidelity of $99.69 \pm 0.03\%$ and a readout contrast of $98.31 \pm 1.03\%$. The spin--photon--entangled $A_2$ transition exhibits narrow optical linewidths ($\sim 180$~MHz) and a polarization visibility of $\sim 82\%$. Coherent optical driving enables Rabi frequencies up to $2.895$~GHz, while dynamical decoupling extends the spin coherence time from $0.5$~ms to $5.70$~ms. Our results establish PL6 as a competitive solid-state spin--photon interface hosted in a commercially available semiconductor platform.

quant-ph

Decoherence-protected entangling gates in a silicon carbide quantum node

Solid-state color centers are promising candidates for nodes in quantum network architectures. However, realizing scalable and fully functional quantum nodes, comprising both processor and memory qubits with high-fidelity universal gate operations, remains a central challenge in this field. Here, we demonstrate a fully functional quantum node in silicon carbide, where electron spins act as quantum processors and nuclear spins serve as quantum memory. Specifically, we design a pulse sequence that combines dynamical decoupling with hyperfine interactions to realize decoherence-protected universal gate operations between the processor and memory qubits. Leveraging this gate, we deterministically prepare entangled states within the quantum node, achieving a fidelity of 90%, which exceeds the fault-tolerance threshold of certain quantum network architectures. These results open a pathway toward scalable and fully functional quantum nodes based on silicon carbide.

quant-ph

Robust single divacancy defects near stacking faults in 4H-SiC under resonant excitation

Color centers in silicon carbide (SiC) have demonstrated significant promise for quantum information processing. However, the undesirable ionization process that occurs during optical manipulation frequently causes fluctuations in the charge state and performance of these defects, thereby restricting the effectiveness of spin-photon interfaces. Recent predictions indicate that divacancy defects near stacking faults possess the capability to stabilize their neutral charge states, thereby providing robustness against photoionization effects. In this work, we present a comprehensive protocol for the scalable and targeted fabrication of single divacancy arrays in 4H-SiC using a high-resolution focused helium ion beam. Through photoluminescence emission (PLE) experiments, we demonstrate long-term emission stability with minimal linewidth shift ($\sim$ 50 MHz over 3 hours) for the single c-axis divacancies within stacking faults. By measuring the ionization rate for different polytypes of divacancies, we found that the divacancies within stacking faults are more robust against resonant excitation. Additionally, angle-resolved PLE spectra reveal their two resonant-transition lines with mutually orthogonal polarizations. Notably, the PLE linewidths are approximately 7 times narrower and the spin-coherent times are 6 times longer compared to divacancies generated via carbon-ion implantation. These findings highlight the immense potential of SiC divacancies for on-chip quantum photonics and the construction of efficient spin-to-photon interfaces, indicating a significant step forward in the development of quantum technologies.

quant-ph

Plasmonic-enhanced bright single spin defects in silicon carbide membranes

Optically addressable spin defects in silicon carbide (SiC) have emerged as attractable platforms for various quantum technologies. However, the low photon count rate significantly limits their applications. We strongly enhanced the brightness by 7 times and spin-control strength by 14 times of single divacancy defects in 4H-SiC membranes using surface plasmon generated by gold film coplanar waveguides. The mechanism of the plasmonic-enhanced effect is further studied by tuning the distance between single defects and the surface of the gold film. A three-energy-level model is used to determine the corresponding transition rates consistent with the enhanced brightness of single defects. Lifetime measurements also verified the coupling between defects and surface plasmons. Our scheme is low-cost, without complicated microfabrication and delicate structures, which is applicable for other spin defects in different materials. This work would promote developing spin defect-based quantum applications in mature SiC materials.

physics.optics