arXiv subjects

Ruihuan Duan

Publications and source records attributed to Ruihuan Duan.

12 recordsLinked to original sources

arXiv2026

Probing mesoscopic nonlocal screening in van der Waals heterostructures with polaritons

Predictive optical modelling of van der Waals (vdW) heterostructures is critical for meta-optics, near-field photonics and quantum technologies. At their buried interfaces, charge transfer and spatially extended screening challenge local descriptions based on layer-by-layer stacking of fixed permittivity tensors. However, such nonlocal corrections have been established mainly for plasmonic systems at ångström-nanometre scales and are often assumed negligible on optical-wavelength scales. Here we challenge this view by uncovering a mesoscopic nonlocal screening regime, extending up to ~140 nm, at buried charge-transfer interfaces in transition-metal dichalcogenide/α-molybdenum trioxide (TMDC/α-MoO3) phonon-polaritonic heterostructures. Using phonon polaritons as an ultrasensitive probe, we quantify charge transfer from polariton-wavelength shifts and find a thickness-independent saturated response as α-MoO3 is thinned. Rather than merely complicating optical modelling, this nonlocal saturation turns a design-level correction into an opportunity by yielding a transferable cross-material metric. Across more than 120 devices, this metric scales linearly with the work-function difference between the TMDC and α-MoO3. We further identify a lattice-mismatch-set energy threshold for charge transfer, revising Anderson-type band alignment for vdW interfaces.

physics.optics↗

arXiv2025

Electric-field Control of Giant Ferronics

Ferrons are quantum excitations of electric polarization in ferroelectrics and electric analogues of magnons but have lacked direct experimental verification at room temperature. We harness the coupling of soft phonons and ferroelectric order in layered NbOX2 (X = I, Br, Cl) to generate, detect, and control giant ferrons, creating a new class of ultralow-power, chip-scale terahertz (THz) sources. Multiple ferron modes produce intense, narrowband THz emission with quality factors up to 228 and radiation efficiencies up to five orders of magnitude greater than state of the art semiconductor emitters. Resonant excitation of a high-Q ferron mode achieves efficiencies two orders of magnitude higher than intense lithium niobate THz sources. We further demonstrate direct, non-volatile electric-field control of ferron oscillations. These findings provide evidence for multiple ferrons and establish Ferronics as a foundational platform for light- and field-driven control of quantum order, with broad impact on ultrafast electronics, photonics, quantum technologies, and next-generation wireless communication.

cond-mat.mtrl-sci↗

arXiv2025

Optical Switching of Moiré Chern Ferromagnet

Optical manipulation of quantum matter offers a non-contact, high-precision and fast control. Fractional Chern ferromagnet states in moiré superlattices are promising for topological quantum computing, but an effective optical control protocol has remained elusive. Here, we demonstrate robust optical switching of integer and fractional Chern ferromagnets in twisted MoTe2 bilayers using circularly polarized light. Highly efficient optical manipulation of spin orientations in the topological ferromagnet regime is realized at zero field using a pump light power as low as 28 nanowatts per square micrometer. Utilizing this optically induced transition, we also demonstrate magnetic bistate cycling and spatially resolved writing of ferromagnetic domain walls. This work establishes a reliable and efficient optical control scheme for moiré Chern ferromagnets, paving the way for dissipationless spintronics and quantized Chern junction devices.

cond-mat.mes-hall↗

arXiv2025

Strain Induced Robust Skyrmion lattice at Room Temperature in van der Waals Ferromagnet

Manipulating topological magnetic orders of two-dimensional (2D) magnets by strain, once achieved, offers enormous potential for future low-power flexible spintronic applications. In this work, by placing Fe3GaTe2 (FGaT), a room-temperature 2D ferromagnet, on flexible substrate, we demonstrate a field-free and robust formation of skyrmion lattice induced by strain. By applying a minimal strain of ~0.80% to pre-annealed FGaT flakes, the Magnetic Force Microscopy (MFM) tip directly triggers the transition from maze-like domains to an ordered skyrmion lattice while scanning the sample surface. The skyrmion lattice is rather stable against extensive cyclic mechanical testing (stretching, bending, and twisting over 2000 cycles each). It also exhibited stability across a wide range of magnetic fields (~2.9 kOe) and temperatures (~ 323 K), as well as long-term retention stability, highlighting its robustness and field free stabilization. The strain effect reduces the lattice symmetry and enhances the Dzyaloshinskii-Moriya interaction (DMI) of FGaT, thus stabilizing the skyrmion lattice. Our findings highlight the potential of FGaT for integrating magnetic skyrmions into future low-power-consumption flexible spintronics devices.

cond-mat.mtrl-sci↗

arXiv2025

Boosting classical and quantum nonlinear processes in ultrathin van der Waals materials

Understanding and controlling nonlinear processes is crucial for engineering light-matter interaction and generating non-classical light. A significant challenge in ultra-thin nonlinear materials is the marked diminution of the nonlinear conversion efficiency due to the reduced light-matter interaction length and, in many cases, the centrosymmetric crystalline structures. Here we relax these limitations and report a giant boost of classical and quantum nonlinear processes in ultrathin van der Waals materials. Specifically, with a metal-nonlinear material heterostructure we enhance classical second-harmonic generation in h-BN flakes by two-orders of magnitude. Moreover, we have engineered a metal-SiO2-nonlinear material heterostructure resulting in a remarkable two orders of magnitude augmentation of the quantum spontaneous parametric down-conversion (SPDC) in NbOCl2 flakes. Notably, we demonstrate SPDC in a 16 nm-thick NbOCl2 flake integrated into the proposed structure. These findings simplify on-chip quantum state engineering and accelerate the use of van der Waals materials in nonlinear optoelectronics.

quant-ph↗

arXiv2024

Fundamental scaling laws of water window X-rays from free electron-driven van der Waals structures

Water-window X-rays are crucial in medical and biological applications, enabling natural contrast imaging of biological cells in their near-native states without external staining. However, water-window X-ray sources whose output photon energy can be arbitrarily specified - a crucial feature in many high-contrast imaging applications - are still challenging to obtain except at large synchrotron facilities. Here, we present a solution to this challenge by demonstrating table-top, water-window X-ray generation from free electron-driven van der Waals materials, resulting in output photon energies that can be continuously tuned across the entire water window regime. In addition, we present a truly predictive theoretical framework that combines first-principles electromagnetism with Monte Carlo simulations to accurately predict the photon flux and brightness in absolute numbers. Using this framework, we theoretically obtain fundamental scaling laws for the tunable photon flux, showing good agreement with experimental results and providing a path to the design of powerful emitters based on free electron-driven quantum materials. We show that we can achieve photon fluxes needed for imaging and spectroscopy applications (over 1E8 photons per second on sample) where compactness is important, and the ultrahigh fluxes of synchrotron sources are not needed. Importantly, our theory highlights the critical role played by the large mean free paths and interlayer atomic spacings unique to van der Waals structures, showing the latter's advantages over other materials in generating water window X-rays. Our results should pave the way to advanced techniques and new modalities in water-window X-ray generation and high-resolution biological imaging.

physics.optics↗

arXiv2024

Room-temperature tunable tunneling magnetoresistance in Fe3GaTe2/WSe2/Fe3GaTe2 van der Waals heterostructures

The exceptional properties of two-dimensional (2D) magnet materials present a novel approach to fabricate functional magnetic tunnel junctions (MTJ) by constructing full van der Waals (vdW) heterostructures with atomically sharp and clean interfaces. The exploration of vdW MTJ devices with high working temperature and adjustable functionalities holds great potential for advancing the application of 2D materials in magnetic sensing and data storage. Here, we report the observation of highly tunable room-temperature tunneling magnetoresistance through electronic means in a full vdW Fe3GaTe2/WSe2/Fe3GaTe2 MTJ. The spin valve effect of the MTJ can be detected even with the current below 1 nA, both at low and room temperatures, yielding a tunneling magnetoresistance (TMR) of 340% at 2 K and 50% at 300 K, respectively. Importantly, the magnitude and sign of TMR can be modulated by a DC bias current, even at room temperature, a capability that was previously unrealized in full vdW MTJs. This tunable TMR arises from the contribution of energy-dependent localized spin states in the metallic ferromagnet Fe3GaTe2 during tunnel transport when a finite electrical bias is applied. Our work offers a new perspective for designing and exploring room-temperature tunable spintronic devices based on vdW magnet heterostructures.

cond-mat.mes-hall↗

arXiv2023

Exciton-exciton Interaction in Monolayer MoSe$_2$ from Mutual Screening of Coulomb Binding

The potential for low-threshold optical nonlinearity has received significant attention in the fields of photonics and conceptual optical neuron networks. Excitons in two-dimensional (2D) semiconductors are particularly promising in this regard as reduced screening and dimensional confinement foster their pronounced many-body interactions towards nonlinearity. However, experimental determination of the interactions remains ambiguous, as optical pumping in general creates a mixture of excitons and unbound carriers, where the impacts of band gap renormalization and carrier screening on exciton energy counteract each other. Here by comparing the influences on exciton ground and excited states energies in the photoluminescence spectroscopy of monolayer MoSe$_2$, we are able to identify separately the screening of Coulomb binding by the neutral excitons and by charge carriers. The energy difference between exciton ground state (A-1s) and excited state (A-2s) red-shifts by 5.5 meV when the neutral exciton density increases from 0 to $4\times 10^{11}$ cm$^{-2}$, in contrast to the blue shifts with the increase of either electron or hole density. This energy difference change is attributed to the mutual screening of Coulomb binding of neutral excitons, from which we extract an exciton polarizability of $α_{2D}^{\rm exciton} = 2.55\times 10^{-17}$ eV(m/V)$^2$. Our finding uncovers a new mechanism that dominates the repulsive part of many-body interaction between neutral excitons.

cond-mat.mtrl-sci↗

arXiv2022

Visualizing bulk and edge photocurrent flow in anisotropic Weyl semimetals

Materials that rectify light into current in their bulk are desired for optoelectronic applications. In inversion-breaking Weyl semimetals, bulk photocurrents may arise due to nonlinear optical processes that are enhanced near the Weyl nodes. However, the photoresponse of these materials is commonly studied by scanning photocurrent microscopy (SPCM), which convolves the effects of photocurrent generation and collection. Here, we directly image the photocurrent flow inside the type-II Weyl semimetals WTe2 and TaIrTe4 using high-sensitivity quantum magnetometry with nitrogen-vacancy center spins. We elucidate an unknown mechanism for bulk photocurrent generation termed the anisotropic photothermoelectric effect (APTE), where unequal thermopowers along different crystal axes drive intricate circulations of photocurrent around the photoexcitation. Using simultaneous SPCM and magnetic imaging at the sample's interior and edges, we visualize how the APTE stimulates the long-range photocurrent collected in our Weyl semimetal devices through the Shockley-Ramo theorem. Our results highlight an overlooked, but widely relevant source of current flow and inspire novel photodetectors using homogeneous materials with anisotropy.

cond-mat.mtrl-sci↗

arXiv2022

Enhanced versatility of table-top X-rays from van der Waals structures

Van der Waals (vdW) materials have attracted much interest for their myriad unique electronic, mechanical and thermal properties. In particular, they are promising candidates for monochromatic, table-top X-ray sources. This work reveals that the versatility of the table-top vdW X-ray source goes beyond what has been demonstrated so far. By introducing a tilt angle between the vdW structure and the incident electron beam, it is theoretically and experimentally shown that the accessible photon energy range is more than doubled. This allows for greater versatility in real-time tuning of the vdW X-ray source. Furthermore, this work shows that the accessible photon energy range is maximized by simultaneously controlling both the electron energy and the vdW structure tilt. These results should pave the way for highly tunable, compact X-ray sources, with potential applications including hyperspectral X-ray fluoroscopy and X-ray quantum optics.

physics.optics↗

arXiv2021

Controlled synthesis of MoxW1-xTe2 atomic layers with emergent quantum states

Recently, new states of matter like superconducting or topological quantum states were found in transition metal dichalcogenides (TMDs) and manifested themselves in a series of exotic physical behaviors. Such phenomena have been demonstrated to exist in a series of transition metal tellurides including MoTe2, WTe2 and alloyed MoxW1-xTe2. However, the behaviors in the alloy system have been rarely addressed due to their difficulty in obtaining atomic layers with controlled composition, albeit the alloy offers a great platform to tune the quantum states. Here, we report a facile CVD method to synthesize the MoxW1-xTe2 with controllable thickness and chemical composition ratios. The atomic structure of monolayer MoxW1-xTe2 alloy was experimentally confirmed by scanning transmission electron microscopy (STEM). Importantly, two different transport behaviors including superconducting and Weyl semimetal (WSM) states were observed in Mo-rich Mo0.8W0.2Te2 and W-rich Mo0.2W0.8Te2 samples respectively. Our results show that the electrical properties of MoxW1-xTe2 can be tuned by controlling the chemical composition, demonstrating our controllable CVD growth method is an efficient strategy to manipulate the physical properties of TMDCs. Meanwhile, it provides a perspective on further comprehension and shed light on the design of device with topological multicomponent TMDCs materials.

cond-mat.mtrl-sci↗

arXiv2020

Many-body effect in optical properties of monolayer molybdenum diselenide

Excitons in monolayer transition metal dichalcogenide (TMD) provide a paradigm of composite Boson in 2D system. This letter reports a photoluminescence and reflectance study of excitons in monolayer molybdenum diselenide (MoSe2) with electrostatic gating. We observe the repulsive and attractive Fermi polaron modes of the band edge exciton, its excited state and the spin-off excitons. Our data validate the polaronic behavior of excitonic states in the system quantitatively where the simple three-particle trion model is insufficient to explain.

cond-mat.mes-hall↗