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Ruixian Liu

Publications and source records attributed to Ruixian Liu.

14 recordsLinked to original sources

$d$-spacing distributions as a probe of nematoelastic response in iron-based superconductors

Electronic nematicity in iron-based superconductors (FeSCs) couples bilinearly to orthorhombic strain, allowing nematic correlations to appear in the lattice response. Here we use neutron Larmor diffraction to measure the temperature-dependent distribution of relative $d$ spacings in electron-doped Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$, hole-doped Ba$_{0.83}$K$_{0.17}$Fe$_2$As$_2$, FeSe, and Fe$_{1.07}$Te. In Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ crystals without intentionally applied uniaxial stress, the in-plane distribution width, $\varepsilon_{\rm FWHM}$, increases on cooling in the tetragonal phase and can be described phenomenologically by a Curie--Weiss-like form. The fitted scale $T^*$ decreases with Co doping and evolves similarly to the nematic phase diagram inferred from elastoresistance, although the two experiments probe different response functions. Related broadening in Ba$_{0.83}$K$_{0.17}$Fe$_2$As$_2$ and FeSe supports extending this interpretation beyond electron-doped BaFe$_2$As$_2$. By contrast, Fe$_{1.07}$Te shows no extended Curie--Weiss-like regime without applied stress, whereas uniaxial pressure produces a strongly anisotropic broadening that can contain contributions from both the field-biased lattice response and inhomogeneous loading. A mean-field model with bilinear nematoelastic coupling and spatially varying symmetry-breaking stress explains the Curie--Weiss-like broadening in terms of the renormalized orthorhombic compliance. Neutron Larmor diffraction therefore provides a bulk-sensitive probe of nematic-related lattice broadening that complements electronic and elastic measurements.

cond-mat.supr-con

Winding feature and thermal evolution of the Dirac magnons in CrI$_3$

Two-dimensional honeycomb lattice ferromagnet chromium tri-iodide (CrI$_3$) has attracted tremendous interest because it retains ferromagnetism down to the monolayer limit and hosts intriguing topological magnons. As a prototypical van der Waals magnet, CrI$_3$ provides an ideal platform for exploring the interplay between reduced dimensionality, magnetic order, and nontrivial spin excitations. Here, using inelastic neutron scattering together with improved sample quality, we uncover the magnon winding feature around the $K$-point of the hexagonal Brillouin zone, a key signature of Dirac magnons. In addition, we find that the magnon energy follows a $T^2$-renormalization behavior at elevated temperatures, consistent with magnon-magnon interactions. These results provide previously missing information on the magnon spectrum of CrI$_3$ and further consolidate the topological nature of its spin excitations.

cond-mat.mtrl-sci

Uniaxial strain tuned magnetism of the altermagnet candidate h-FeS

Altermagnets are collinear magnetic materials with 'alter'nating local crystalline environments, characterized by joint spin and crystalline symmetries that enable ferromagnetic-like transport properties but with vanishing net magnetization. Hexagonal FeS (h-FeS) is a recently identified altermagnet candidate that shows a spontaneous anomalous Hall effect (AHE) accompanied by a tiny net magnetization. Here, we show that both the spontaneous AHE and magnetization can be effectively suppressed by an in-plane compressive strain. Since neutron diffraction measurements show that the applied uniaxial strain only modifies the in-plane domain population but does not affect the in-plane magnetic structure, the major effect of the applied strain is to tune the small $c$-axis ferromagnetic moment. Our results demonstrate a strong correlation between the tiny net magnetization and the spontaneous AHE in h-FeS, and show that uniaxial strain provides an effective knob to tune both properties in this altermagnet candidate for spintronic applications.

cond-mat.mtrl-sci

Magnetic excitations in biaxial-strain detwinned $\alpha$-RuCl$_{3}$

The honeycomb magnet $\alpha$-RuCl$_{3}$ has been a leading candidate for realizing the Kitaev quantum spin liquid (QSL), but its intrinsic spin dynamics have remained obscured by crystal twinning. Here we apply biaxial anisotropic strain to detwin $\alpha$-RuCl$_{3}$ single crystals and directly visualize the intrinsic magnetic excitations using inelastic neutron scattering. We discover that the low-energy spin waves emerge from the $M$ points -- transverse to the magnetic Bragg peaks -- providing direct evidence of anisotropic magnetic interactions in $\alpha$-RuCl$_{3}$. The intrinsic spin-wave spectrum imposes stringent constraints on the extended Kitaev Hamiltonian, yielding a refined, quantitatively consistent set of exchange couplings for the zigzag ground state and its low-energy dynamics. Above the magnon band, we uncover broad excitation continua: while a twofold-symmetric feature near 6 meV at $\Gamma$ is consistent with bimagnon scattering, the dominant spectral weight forms a sixfold-symmetric continuum extending up to $\sim 16$ meV that cannot be explained by conventional magnons. This strongly supports the presence of fractionalized excitations-a hallmark of Kitaev QSL physics. Our findings establish biaxial strain as a powerful symmetry-breaking probe to access the intrinsic spin dynamics of Kitaev materials and provide critical benchmarks for refining theoretical models of quantum magnetism in $\alpha$-RuCl$_{3}$.

cond-mat.str-el

Signatures of three-state Potts nematicity in spin excitations of the van der Waals antiferromagnet FePSe$_3$

In two-dimensional (2D) nearly square-lattice quantum materials, electron correlations can induce an electronic nematic phase with twofold rotational ($C_2$) symmetry that profoundly impacts their properties. For 2D materials with threefold rotational ($C_3$) symmetry, such as the honeycomb lattice, a vestigial three-state Potts nematic order has been observed in the van der Waals antiferromagnet (AFM) FePSe$_3$ via optical and thermodynamic methods under uniaxial strain. Here, we use neutron scattering to study the magnetic order and spin excitations of FePSe$_3$ under uniaxial strain. In the AFM ordered state, we find that $\sim$0.6% tensile strain significantly suppresses one zigzag domain and promotes the other two, lowering the AFM order and spin waves to $C_2$ symmetry. The broken $C_3$ symmetry in spin excitations persists slightly above $T_{\rm{N}}\approx 108.6$ K, where the zigzag AFM order is absent. Our results thus provide direct evidence of magnetoelastic coupling and suggest that the three-state Potts nematicity in paramagnetic spin excitations arises from the vestigial order associated with the low-temperature zigzag AFM order.

cond-mat.str-el

Spin correlations in La$_3$Ni$_2$O$_7$ thin films

The discovery of ambient-pressure superconductivity with $T_{c,\text{onset}} > 40$ K in La$_3$Ni$_2$O$_7$ (LNO) thin films grown on the SrLaAlO$_4$ (SLAO) substrate with compressive ($\varepsilon\approx-2\%$) epitaxial strain provides a unique platform for investigating the superconducting mechanism in nickelate superconductors. Here, we use resonant inelastic X-ray scattering (RIXS) to unveil the dispersive spin excitations in the LNO/SLAO thin film and establish the strain dependence of the electronic and spin excitations in LNO thin films with strain ranging from $\varepsilon\approx-2\%$ to $+1.9\%$. Compared with bulk LNO, LNO/SLAO exhibits similar $dd$ excitations and spin dynamics, but with a larger spin-excitation bandwidth, whereas tensile-strained LNO/SrTiO$_3$ exhibits a marked suppression of both the spin excitations and the Ni $3d_{z^2}$-derived $dd$ excitations. This evolution reflects a strain-tuned interlayer exchange interaction $J_z$ and Ni $3d_{z^2}$-O 2$p_z$ hybridization. Our results demonstrate how epitaxial strain modulates the interlayer magnetic coupling and are consistent with scenarios in which the interlayer antiferromagnetic superexchange interaction promotes interlayer pairing in bilayer nickelates.

cond-mat.supr-con

Evolution of pairing symmetry in FeSe$_{1-x}$S$_x$ as probed by uniaxial-strain tuning of $T_c$

In iron-based superconductors (FeSCs), the interplay between electronic nematicity and superconductivity is essential for understanding the exotic superconducting ground state. In the nematic regime, uniaxial-strain ($\varepsilon$) tuning of the superconducting transition temperature $T_c$ [$\Delta T_c(\varepsilon)=\alpha\varepsilon+\beta\varepsilon^2$] offers a unique approach to investigating the evolution of pairing symmetry if both $s$ and $d$ wave pairing instabilities are relevant. Here, we employ uniaxial strain to tune the $T_c$ of FeSe$_{1-x}$S$_x$, in which both nematicity and superconductivity undergo significant changes with doping. While $T_c$ is usually suppressed quadratically with $\varepsilon$ in optimally doped BaFe$_2$As$_2$, $\Delta T_c(\varepsilon)$ in FeSe$_{1-x}$S$_x$ dominated by $\Delta T_c(\varepsilon)=\beta\varepsilon^2$ changes its sign from $\beta$ < $0$ in FeSe to $\beta$ > $0$ in FeSe$_{1-x}$S$_x$ ($x\gtrsim0.10$), indicating an evolution of the pairing symmetry from an $s_{\pm}$ state towards an $s+d$ wave state. These findings highlight the $\Delta T_c(\varepsilon)$ as a powerful probe for elucidating the superconducting pairing symmetry in the nematic regime of FeSCs and provide new insights into the evolution of pairing symmetry in FeSCs.

cond-mat.supr-con

Cryogenic Digital Image Correlation as a Probe of Strain in Iron-Based Superconductors

Uniaxial strain is a powerful tuning parameter that can control symmetry and anisotropic electronic properties in iron-based superconductors. However, accurately characterizing anisotropic strain can be challenging and complex. Here, we utilize a cryogenic optical system equipped with a high-spatial-resolution microscope to characterize surface strains in iron-based superconductors using the digital image correlation method. Compared with other methods such as high-resolution X-ray diffraction, strain gauge, and capacitive sensor, digital image correlation offers a non-contact, full-field measurement approach, acting as an optical virtual strain gauge that provides high spatial resolution. The results measured on detwinned {\BFA} are quantitatively consistent with the distortion measured by X-ray diffraction and neutron Larmor diffraction. These findings highlight the potential of cryogenic digital image correlation as an effective and accessible tool for probing the isotropic and anisotropic strains, facilitating the application of uniaxial strain tuning in the study of quantum materials.

cond-mat.supr-con

Nematic quantum disordered state in FeSe

The unusual quantum-disordered magnetic ground state intertwined with superconductivity and electronic nematicity in FeSe has been a research focus in iron-based superconductors. However, the intrinsic spin excitations across the entire Brillouin zone in detwinned FeSe, which forms the basis for a microscopic understanding of the magnetic state and superconductivity, remain to be determined. Here, we use inelastic neutron scattering to map out the spin excitations of FeSe dewtinned with a uniaxial-strain device. We find that the stripe spin excitations (Q=(1, 0)/(0, 1)) exhibit the $C_2$ symmetry up to $E\approx120$ meV, while the N{\'e}el spin excitations (Q=(1, 1)) retain their $C_4$ symmetry in the nematic state. The temperature dependence of the difference in the spin excitations at Q=(1, 0) and (0, 1) for temperatures above the structural phase transition unambiguously shows the establishment of the nematic quantum disordered state. The similarity of the N\'eel excitations in FeSe and NaFeAs suggests that the N\'eel excitations are driven by the enhanced electron correlations in the $3d_{xy}$ orbital. By determining the key features of the stripe excitations and fitting their dispersions using a Heisenberg Hamiltonian with biquadratic interaction ($J_1$-$K$-$J_2$), we establish a spin-interaction phase diagram and conclude that FeSe is close to a crossover region between the antiferroquadrupolar, N\'eel, and stripe ordering regimes. The results provide an experimental basis for establishing a microscopic theoretical model to describe the origin and intertwining of the emergent orders in iron-based superconductors.

cond-mat.supr-con

Nematic charge-density-wave correlations in FeSe$_{1-x}$S$_{x}$

The occurrence of charge-density-wave (CDW) order is a common thread in the phase diagram of cuprate high-transition-temperature ($T_c$) superconductors. In iron-based superconductors (FeSCs), nematic order and fluctuations play a decisive role in driving other emergent orders. CDW order has been observed by scanning tunneling microscopy for various FeSCs such as FeSe thin films, uniaxially strained LiFeAs, and tetragonal FeSe$_{0.81}$S$_{0.19}$. However, it remains elusive if the CDW in these materials is a bulk phenomenon as well as if and how it intertwines with the electronic nematicity. Using energy-resolved resonant X-ray scattering at the Fe-L$_3$ edge, we report the discovery of a local-strain-induced incommensurate isotropic CDW order in FeSe$_{0.82}$S$_{0.18}$. A highly anisotropic CDW response under uniaxial strain unambiguously manifests that the CDW is directly coupled to the nematicity. Transforming part of Fe$^{2+}$ to Fe$^{3+}$ on the surface of FeSe$_{1-x}$S$_{x}$ reveals that the same isotropic CDW can be induced, enhanced, and stabilized in the whole nematic regime measured ($x=0-0.19$). As Fe$^{3+}$ can create local lattice distortions on the surface, the CDW could arise from the interaction between the local strain around Fe$^{3+}$ and the nematic electron correlations. Our experimental observation of a local-strain-induced CDW gives vital information for understanding the interplay between electron correlations and the electronic nematicity in FeSCs.

cond-mat.supr-con

Deep Learning based Spatially Dependent Acoustical Properties Recovery

The physics-informed neural network (PINN) is capable of recovering partial differential equation (PDE) coefficients that remain constant throughout the spatial domain directly from physical measurements. In this work, we propose a spatially dependent physics-informed neural network (SD-PINN), which enables the recovery of coefficients in spatially-dependent PDEs using a single neural network, eliminating the requirement for domain-specific physical expertise. We apply the SD-PINN to spatially-dependent wave equation coefficients recovery to reveal the spatial distribution of acoustical properties in the inhomogeneous medium. The proposed method exhibits robustness to noise owing to the incorporation of a loss function for the physical constraint that the assumed PDE must be satisfied. For the coefficients recovery of spatially two-dimensional PDEs, we store the PDE coefficients at all locations in the 2D region of interest into a matrix and incorporate the low-rank assumption for such a matrix to recover the coefficients at locations without available measurements.

cs.LG

Nematic spin correlations pervading the phase diagram of FeSe$_{1-x}$S$_{x}$

We use resonant inelastic X-ray scattering (RIXS) at the Fe-L$_3$ edge to study the spin excitations of uniaxial-strained and unstrained FeSe$_{1-x}$S$_{x}$ ($0\leq x\leq0.21$) samples. The measurements on unstrained samples reveal dispersive spin excitations in all doping levels, which show only minor doping dependence in energy dispersion, lifetime, and intensity, indicating that high-energy spin excitations are only marginally affected by sulfur doping. RIXS measurements on uniaxial-strained samples reveal that the high-energy spin-excitation anisotropy observed previously in FeSe is also present in the doping range $0< x\leq0.21$ of FeSe$_{1-x}$S$_{x}$. The spin-excitation anisotropy persists to a high temperature up to $T>200$ K in $x=0.18$ and reaches a maximum around the nematic quantum critical doping ($x_c\approx0.17$). Since the spin-excitation anisotropy directly reflects the existence of nematic spin correlations, our results indicate that high-energy nematic spin correlations pervade the regime of nematicity in the phase diagram and are enhanced by the nematic quantum criticality. These results emphasize the essential role of spin fluctuations in driving electronic nematicity and open the door for uniaxial strain tuning of spin excitations in quantum materials hosting strong magnetoelastic coupling and electronic nematicity.

cond-mat.str-el

Spin-excitation anisotropy in the nematic state of detwinned FeSe

The origin of the electronic nematicity in FeSe is one of the most important unresolved puzzles in the study of iron-based superconductors. In both spin- and orbital-nematic models, the intrinsic magnetic excitations at $\mathbf{Q}_1=(1, 0)$ and $\mathbf{Q}_2=(0, 1)$ of twin-free FeSe are expected to provide decisive criteria for clarifying this issue. Although a spin-fluctuation anisotropy below 10 meV between $\mathbf{Q}_1$ and $\mathbf{Q}_2$ has been observed by inelastic neutron scattering around $T_c\sim 9$ K ($<<T_s\sim 90$ K), it remains unclear whether such an anisotropy also persists at higher energies and associates with the nematic transition $T_{\rm s}$. Here we use resonant inelastic x-ray scattering (RIXS) to probe the high-energy magnetic excitations of uniaxial-strain detwinned FeSe and {\BFA}. A prominent anisotropy between the magnetic excitations along the $H$ and $K$ directions is found to persist to $\sim200$ meV in FeSe, which is even more pronounced than the anisotropy of spin waves in {\BFA}. This anisotropy decreases gradually with increasing temperature and finally vanishes at a temperature around the nematic transition temperature $T_{\rm s}$. Our results reveal an unprecedented strong spin-excitation anisotropy with a large energy scale well above the $d_{xz}/d_{yz}$ orbital splitting, suggesting that the nematic phase transition is primarily spin-driven. Moreover, the measured high-energy spin excitations are dispersive and underdamped, which can be understood from a local-moment perspective. Our findings provide the much-needed understanding of the mechanism for the nematicity of FeSe and points to a unified description of the correlation physics across seemingly distinct classes of Fe-based superconductors.

cond-mat.supr-con

Computational analysis of pathological image enables interpretable prediction for microsatellite instability

Microsatellite instability (MSI) is associated with several tumor types and its status has become increasingly vital in guiding patient treatment decisions. However, in clinical practice, distinguishing MSI from its counterpart is challenging since the diagnosis of MSI requires additional genetic or immunohistochemical tests. In this study, interpretable pathological image analysis strategies are established to help medical experts to automatically identify MSI. The strategies only require ubiquitous Haematoxylin and eosin-stained whole-slide images and can achieve decent performance in the three cohorts collected from The Cancer Genome Atlas. The strategies provide interpretability in two aspects. On the one hand, the image-level interpretability is achieved by generating localization heat maps of important regions based on the deep learning network; on the other hand, the feature-level interpretability is attained through feature importance and pathological feature interaction analysis. More interestingly, both from the image-level and feature-level interpretability, color features and texture characteristics are shown to contribute the most to the MSI predictions. Therefore, the classification models under the proposed strategies can not only serve as an efficient tool for predicting the MSI status of patients, but also provide more insights to pathologists with clinical understanding.

stat.ML