arXiv subjects

Ruokai Xu

Publications and source records attributed to Ruokai Xu.

3 recordsLinked to original sources

arXiv2024

Possible gapless quantum spin liquid behavior in the triangular-lattice Ising antiferromagnet PrMgAl$_{11}$O$_{19}$

Quantum spin liquids (QSLs) represent a novel state where spins are highly entangled but do not order even at zero temperature due to strong quantum fluctuations. Such a state is mostly studied in Heisenberg models defined on geometrically frustrated lattices. Here, we turn to a new triangular-lattice antiferromagnet PrMgAl$_{11}$O$_{19}$, in which the interactions are believed to be of Ising type. Magnetic susceptibility measured with an external field along the $c$ axis is two orders of magnitude larger than that with a field in the $ab$ plane, displaying an ideal easy-axis behavior. Meanwhile, there is no magnetic phase transition or spin freezing observed down to 1.8 K. Ultralow-temperature specific heat measured down to 50 mK does not capture any phase transition either, but a hump at 4.5 K, below which the magnetic specific heat exhibits a quasi-quadratic temperature dependence that is consistent with a Dirac QSL state. Inelastic neutron scattering technique is also employed to elucidate the nature of its ground state. In the magnetic excitation spectra, there is a gapless broad continuum at the base temperature 55~mK, in favor of the realization of a gapless QSL. Our results provide a scarce example for the QSL behaviors observed in an Ising-type magnet, which can serve as a promising platform for future research on QSL physics based on an Ising model.

cond-mat.str-el↗

arXiv2023

Signatures of a gapless quantum spin liquid in the Kitaev material Na$_3$Co$_{2-x}$Zn$_x$SbO$_6$

The honeycomb-lattice cobaltate Na$_3$Co$_2$SbO$_6$ has recently been proposed to be a proximate Kitaev quantum spin liquid~(QSL) candidate. However, non-Kitaev terms in the Hamiltonian lead to a zigzag-type antiferromagnetic~(AFM) order at low temperatures. Here, we partially substitute magnetic Co$^{2+}$ with nonmagnetic Zn$^{2+}$ and investigate the chemical doping effect in tuning the magnetic ground states of Na$_3$Co$_{2-x}$Zn$_x$SbO$_6$. X-ray diffraction characterizations reveal no structural transition but quite tiny changes on the lattice parameters over our substitution range $0\leq x\leq0.4$. Magnetic susceptibility and specific heat results both show that AFM transition temperature is continuously suppressed with increasing Zn content $x$ and neither long-range magnetic order nor spin freezing is observed when $x\geq0.2$. More importantly, a linear term of the specific heat representing fermionic excitations is captured below 5~K in the magnetically disordered regime, as opposed to the $C_{\rm m}\propto T^3$ behavior expected for bosonic excitations in the AFM state. Based on the data above, we establish a magnetic phase diagram of Na$_3$Co$_{2-x}$Zn$_x$SbO$_6$. Our results indicate the presence of gapless fractional excitations in the samples with no magnetic order, evidencing a potential QSL state induced by doping in a Kitaev system.

cond-mat.str-el↗

arXiv2023

Suppression of the antiferromagnetic order by Zn doping in a possible Kitaev material Na$_2$Co$_2$TeO$_6$

Very recently, a 3$d$ based honeycomb cobaltate Na$_2$Co$_2$TeO$_6$ has garnered tremendous attention due to the proposed proximity to the Kitaev spin-liquid state as its 4$d$/5$d$ counterparts. Here, we use Zn to substitute Co in a broad range and perform systematic studies on Na$_2$Co$_{2-x}$Zn$_x$TeO$_6$ by structural, magnetic, and thermodynamic measurements, and track the doping evolution of its magnetic ground states. Due to the extremely close radii of Zn$^{2+}$ and high-spin Co$^{2+}$ ions, the substitution can be easily achieved. X-ray diffractions reveal no structural transition but only minor changes on the lattice parameter $c$ over a wide substitution range $0 \leq x \leq 1.5$. Magnetic susceptibility and specific heat measurements both suggest an antiferromagnetic ground state which is gradually suppressed with doping. It can survive with $x$ up to $\sim1.0$. Then it evolves into a spin-glass phase with short-range order that is rapidly supplanted by a magnetically disordered state when $x \geq 1.3$. By summarizing all these data, we construct a magnetic phase diagram of Na$_2$Co$_{2-x}$Zn$_x$TeO$_6$. Our results demonstrate that the Zn doping can effectively suppress the magnetic order and induce a possibe quantum paramagnetic state. These may serve as a platform to investigate the Kitaev physics in this system.

cond-mat.str-el↗