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Rustam Rysov

Publications and source records attributed to Rustam Rysov.

6 recordsLinked to original sources

Generation of high-fluence and high-intensity hard x-ray attosecond pulses at European XFEL

By combining hard x-ray attosecond pulses from the European XFEL with total-reflection focusing x-ray optics, we generated nanofocused hard x-ray attosecond pulses with intensities and fluences comparable to the highest values attained in the hard x-ray regime. A peak intensity on the order of 10$^{20}$ W/cm$^2$ is confirmed through the observation of saturation in amplified spontaneous emission from copper atoms. These x-ray pulses enable new scientific opportunities, including the exploration of higher-order nonlinear light--matter interactions, damage-free structure determination, and coherent control of atoms and molecules.

physics.optics

Spatio-temporal migration of antiferromagnetic domain walls in Sr2IrO4

By laser pump-probe time-resolved coherent magnetic X-ray diffraction imaging, we have measured the migration velocity of antiferromagnetic domain walls in the Mott insulator Sr2IrO4 at 100 K. During the laser-induced demagnetization, we observe domain walls moving at 3x10^6 m/s, significantly faster than acoustic velocities. This is understood to arise from a purely electronic spin contribution to the magnetic structure without any role for coupling to the crystal lattice.

cond-mat.str-el

Probing the Linewidth of the 12.4-keV Solid-State $^{45}$Sc Isomeric Resonance

The $^{45}$Sc nuclear transition from the ground to the isomeric state at 12.389~keV, with a lifetime of 0.46~s, exhibits an extraordinarily narrow natural width of 1.4~feV and a quality factor $\simeq 10^{19}$ -- surpassing those of the most precise atomic clocks -- making $^{45}$Sc a compelling platform for advanced metrology and nuclear clocks. Here we investigate how closely the spectral width and quality factor of the solid-state $^{45}$Sc resonance can approach these natural limits. Using the European X-ray Free-Electron Laser, we confirm the isomer's lifetime via time-delayed incoherent $K_{\alpha,\beta}$ fluorescence and observe previously unreported elastic fluorescence, yielding a partial internal conversion coefficient of 390(60). The absence of a clear nuclear forward scattering signal beyond a 2-ms delay implies environmental broadening of at least $500~\Gamma_{0}$ under experimental conditions, placing bounds on solid-state decoherence mechanisms. These findings set new experimental benchmarks for solid-state nuclear clock development.

quant-ph

Ultrafast X-ray sonography reveals the spatial heterogeneity of the laser-induced magneto-structural phase transition in FeRh

Phase transitions are governed by both intrinsic and extrinsic heterogeneities, yet capturing their spatio-temporal dynamics remains a challenge. While ultrafast techniques track phase changes on femtosecond timescales, the spatial complexity and stochastic nature of the processes often remain hidden. Here, we present an experimental approach that combines well-established ultrafast hard-X-ray diffraction with a propagating strain pulse as a universal and non-invasive probe. This ultrafast X-ray sonography can capture the spatio-temporal phase heterogeneity in great detail by resolving the phase-specific strain response. We apply this approach to the antiferromagnetic-to-ferromagnetic magneto-structural phase transition in FeRh and identify the ferromagnetic phase to nucleate at the surface as narrow columnar domains of approximately $30\,\text{nm}$ diameter. Besides reconciling the diverse experimental results in the literature on FeRh, X-ray sonography offers a versatile platform for investigating a wide range of phase transitions accompanied by structural changes.

cond-mat.mtrl-sci

Softness and Hydrodynamic Interactions Regulate Lipoprotein Transport in Crowded Yolk Environments

Low-density lipoproteins (LDLs) serve as nutrient reservoirs in egg yolk for embryonic development and as promising drug carriers. Both roles critically depend on their mobility in densely crowded biological environments. Under these crowded conditions, diffusion is hindered by transient confinement within dynamic cages formed by neighboring particles, driven by solvent-mediated hydrodynamic interactions and memory effects -- phenomena that have remained challenging to characterize computationally and experimentally. Here, we employ megahertz X-ray photon correlation spectroscopy to directly probe the cage dynamics of LDLs in yolk-plasma across various concentrations. We find that LDLs undergo anomalous diffusion, experiencing $\approx$ 100-fold reduction in self-diffusion at high concentrations compared to dilute solutions. This drastic slowing-down is attributed to a combination of hydrodynamic interactions, direct particle-particle interactions, and the inherent softness of LDL particles. Despite reduced dynamics, yolk-plasma remains as a liquid, yet sluggish, balancing dense packing, structural stability, and fluidity essential for controlled lipid release during embryogenesis.

cond-mat.soft

Dynamic X-ray coherent diffraction analysis: bridging the timescales between imaging and photon correlation spectroscopy

The advent of diffraction limited sources and developments in detector technology opens up new possibilities for the study of materials in situ and operando. Coherent X-ray diffraction techniques such as coherent X-ray diffractive imaging (CXDI) and X-ray photon correlation spectroscopy (XPCS) are capable for this purpose and provide complimentary information, although due to signal-to-noise requirements, their simultaneous demonstration has been limited. Here, we demonstrate a strategy for the simultaneous use of CXDI and XPCS to study in situ the Brownian motion of colloidal gold nanoparticles of 200 nm diameter suspended in a glycerol-water mixture. We visualise the process of agglomeration, examine the spatiotemporal space accessible with the combination of techniques, and demonstrate CXDI with 22 ms temporal resolution.

cond-mat.mes-hall