arXiv subjects

Ryan E. Baumbach

Publications and source records attributed to Ryan E. Baumbach.

At least 19 recordsLinked to original sources

arXiv2026

Easy-plane anisotropy of magnetic fluctuations in UTe2

The large directional anisotropy of superconducting UTe2 along the lattice a, b, c directions in magnetic susceptibility, upper critical fields, and Knight shift suggests spin-triplet Cooper pairing. If spin fluctuations bind the Cooper pair, one needs to determine their anisotropy in spin space to characterize the superconducting state. Here we use polarised and unpolarised inelastic neutron scattering (INS) experiments to show that antiferromagnetic (AFM) spin fluctuations at the Y point are highly isotropic within the ac-plane but have no observable magnitude along the b-axis. Our results rule out the assumed Ising anisotropy and constrain the possible pairing channels. AFM exchange is no longer pair forming in the triplet channel and the d vector along b is strongly favoured. We capture the experimental observations within a microscopic framework that encompasses the dual nature of 5f electrons. We include itinerant and localized 5f-moments in a tight-binding model fitted to quantum oscillations data. In congruence with INS, the exchange between localized moments generically consists of a strong FM intra-dimer interaction, maxima close to the Y and T points, mediated by 5p_y and 6d_{3z^2-r^2} orbitals respectively, and magnetically decoupled ab-planes. We find that anisotropy and dimerization of the moments can lead to gapped excitations that, in combination with Landau damping, can produce the observed overdamped response at the Y point. We suggest that enhancement of the response and its observed near-O(2)-symmetry could both be driven by proximity to a quantum critical point where the dimer excitation gap closes and gives place to incommensurate helical order. Analysis of the linearized gap equation for a nearest-neighbour pairing interaction favours the B1u triplet with a dominant d-vector component along b, although the possibility of spin singlet pairing cannot be ruled out.

cond-mat.str-el↗

arXiv2025

Evolution of magnetic bubble domains in the uniaxial ferromagnet CeRu$_2$Ga$_2$B inferred from the Hall effect and ac magnetic susceptibility

We study the Hall effect, AC magnetic susceptibility ($χ_{\rm ac}$), and magnetic force microscopy of the uniaxial ferromagnet CeRu$_2$Ga$_2$B with a centrosymmetric crystal structure. We observe a finite topological Hall effect (THE) within the ordered phase before the magnetization is polarized by applied field. By comparing the field dependences of the area fraction of the magnetic bubbles, the derivative of $χ_{\rm ac}$, and the THE signal, we deduce that the magnetic bubbles of CeRu$_2$Ga$_2$B evolve from the trivial to topological spin texture with field. Our findings will be utilized to expand the search for magnetic materials hosting the topological spin textures to ones with uniaxial anisotropy, and open a new possibility to tailor the topological spin texture.

cond-mat.str-el↗

arXiv2025

Large Kohn anomaly and phonon collapse induced by charge density wave in UPt$_2$Si$_2$

Using high-energy-resolution inelastic x-ray scattering, we observe anomalous softening and damping of the transverse acoustic phonon in UPt$_2$Si$_2$ as the system is cooled towards the charge density wave (CDW) transition temperature, T$_{\rm{CDW}}$. The phonon exhibits a marked Kohn-type anomaly around the CDW wave vector, Q$_{\rm{CDW}}$, and becomes overdamped within a finite momentum range already well above T$_{\rm{CDW}}$. The dispersion anomaly is consistent with potential Fermi surface nesting, which together with the extended phonon collapse indicate strong electron-phonon coupling. The transition temperature estimated from the phonon softening is markedly lower than T$_{\rm{CDW}}$, consistent with a primarily electronic instability rather than a phonon-driven transition. Our results establish UPt$_2$Si$_2$ as a prime example of a strongly correlated electron CDW system with exceptionally strong electron-phonon coupling driving phonon softening and collapse.

cond-mat.str-el↗

arXiv2025

High-Magnetic Field Phases in U$_{1-x}$Th$_x$Te$_2$

At temperatures much lower than its superconducting critical temperature $T_c$ of 2.1 K, the heavy fermion superconductor UTe$_2$ has a remarkable phase diagram of magnetic field $H$ vs. angles $ϕ$ and $θ$ at which $H$ is tilted away from the $b$-axis toward the $a$- and $c$-axes, respectively, in the orthorhombic unit cell. The phase diagram appears to contain three superconducting phases: (1) a low field superconducting phase SC$_{\mathrm{LF}}$ extending over all values of $ϕ$ and $θ$ with an upper critical field $H_{c2}$ with a maximum value of 15 T at $ϕ= θ= 0^\circ$; (2) a high field superconducting phase SC$_{\mathrm{HF}}$ located in a region between $ϕ\approx 7^\circ$ and $θ\approx 4^\circ$ in fields from $H_{c2\mathrm{LF}}$ of the SC$_{\mathrm{LF}}$ phase and the metamagnetic transition at $H_m$ at $\sim 35$ T marking the onset of the magnetic field polarized FP phase: and (3) a SC$_{\mathrm{FP}}$ superconducting phase that resides entirely within the FP phase in a pocket of superconductivity extending from $θ\approx 20^\circ$ to $40^\circ$ in fields from $\sim 40$ T to above 60 T. In this work, we studied the $H$ vs $θ$ phase diagram at a base temperature of $\sim 0.6$ K as a function of Th concentration $x$ in U$_{1-x}$Th$_x$Te$_2$ pseudobinary compounds for $0.5\% \lesssim x \lesssim 4.7\%$. We find that for all values of $x$ within this range, the SC$_{\mathrm{LF}}$ phase is retained with a reduced value of $H_{c2}$ of $\sim 10$ T at $ϕ= θ= 0^\circ$ for $x = 4.7\%$, while the SC$_{\mathrm{HF}}$ phase is suppressed. The SC$_{\mathrm{FP}}$ and FP phases are unaffected to values of $x = 2\%$ but are completely suppressed in the region $x = 2.5$ to $4.7\%$ where the residual resistance ratio RRR has decreased from $\sim 14$ at $x = 1.5\%$ to values of $\sim 3$, indicating a significant increase in disorder.

cond-mat.str-el↗

arXiv2024

Structural transition and uranium valence change in UTe$_2$ at high pressure revealed by x-ray diffraction and spectroscopy

High pressure x-ray diffraction up to 30 GPa and resonant emission x-ray spectroscopy and partial fluorescence yield x-ray absorption spectroscopy up to 52 GPa were used to study how the structural and electronic properties of UTe$_2$ evolve with pressure at room temperature. An orthorhombic to tetragonal phase transition was observed to occur between 5 and 7 GPa, with a large volume collapse of nearly 11% and a nearest U-U distance increase by about 4%. This lower to higher symmetry transition suggests less 5f electron participation in bonding when the weakly correlated superconducting phase in the tetragonal structure of UTe$_2$ appears. Beyond 7 GPa, no new structural transitions were found up to 30 GPa. The resonant x-ray emission spectra clearly demonstrate an intermediate valence of U, nearly +3.74 at 1.8 GPa and room temperature, and reveal that the U valence shifts towards 4+, passes through a peak at 2.8 GPa, and then decreases towards 3+ and settles down to a nearly constant value above 15 GPa. These experiments reveal that some fundamental structural and valence changes occur in UTe2 at relatively low pressures, which could be responsible for the interplay between unconventional superconductivity, magnetic ordering, and weakly correlated superconductivity that is manifested in the temperature-pressure phase diagram of UTe2.

cond-mat.str-el↗

arXiv2023

Observation of odd-parity superconductivity in UTe2

Symmetry properties of the order parameter are among the most fundamental characteristics of a superconductor. The pairing symmetry of recently discovered heavy fermion superconductor UTe2 featuring an exceedingly large upper critical field has attracted a great deal of attention. Even though it is widely believed that UTe2 possesses an odd-parity, spin-triplet pairing symmetry, direct evidence for it is lacking, especially at zero or low magnetic fields. We report here the selection-rule results of Josephson coupling between In, an s-wave superconductor, and UTe2. The orientation dependence of the Josephson coupling suggests very strongly that UTe2 possess an odd-parity pairing state of B_1u in zero magnetic fields. We also report the formation of Andreev surface bound states on the (1-10) surface of UTe2.

cond-mat.supr-con↗

arXiv2022

Thickness and twist angle dependent interlayer excitons in metal monochalcogenide heterostructures

Interlayer excitons, or bound electron-hole pairs whose constituent quasiparticles are located in distinct stacked semiconducting layers, are being intensively studied in heterobilayers of two dimensional semiconductors. They owe their existence to an intrinsic type-II band alignment between both layers that convert these into p-n junctions. Here, we unveil a pronounced interlayer exciton (IX) in heterobilayers of metal monochalcogenides, namely gamma-InSe on epsilon-GaSe, whose pronounced emission is adjustable just by varying their thicknesses given their number of layers dependent direct bandgaps. Time-dependent photoluminescense spectroscopy unveils considerably longer interlayer exciton lifetimes with respect to intralayer ones, thus confirming their nature. The linear Stark effect yields a bound electron-hole pair whose separation d is just (3.6 \pm 0.1) Å with d being very close to dSe = 3.4 Å which is the calculated interfacial Se separation. The envelope of IX is twist angle dependent and describable by superimposed emissions that are nearly equally spaced in energy, as if quantized due to localization induced by the small moiré periodicity. These heterostacks are characterized by extremely flat interfacial valence bands making them prime candidates for the observation of magnetism or other correlated electronic phases upon carrier doping.

cond-mat.mes-hall↗

arXiv2022

Magnetic properties of equiatomic CrMnFeCoNi

Magnetic, specific heat, and structural properties of the equiatomic Cantor alloy system are reported for temperatures between 5 kelvin and 300 kelvin, and up to fields of 70 kilo-oersted. Magnetization measurements performed on as-cast, annealed, and cold-worked samples reveal a strong processing history dependence and that high-temperature annealing after cold-working does not restore the alloy to a pristine state. Measurements on known precipitates show that the two transitions, detected at 43 kelvin and 85 kelvin, are intrinsic to the Cantor alloy and not the result of an impurity phase. Experimental and ab initio density functional theory (DFT) computational results suggest that these transitions are a weak ferrimagnetic transition and a spin-glass-like transition, respectively, and magnetic and specific heat measurements provide evidence of significant Stoner enhancement and electron-electron interactions within the material.

cond-mat.mtrl-sci↗

arXiv2020

Charge density wave with anomalous temperature dependence in UPt2Si2

Using single crystal neutron and x-ray diffraction, we discovered a charge density wave (CDW) below 320 K, which accounts for the long-sought origin of the heat capacity and resistivity anomalies in UPt2Si2. The modulation wavevector, Qmod, is intriguingly similar to the Fermi surface nesting wavevector of URu2Si2. Qmod shows an unusual temperature dependence, shifting from commensurate to incommensurate position upon cooling and becoming locked at ~ (0.42 0 0) near 180 K. Bulk measurements indicate a cross-over toward a correlated coherent state around the same temperature, suggesting an interplay between the CDW and Kondo-lattice-like coherence before coexisting antiferromagnetic order sets in at TN = 35 K.

cond-mat.supr-con↗

arXiv2019

Magnetoelastic coupling in URu2Si2: Probing multipolar correlations in the hidden order state

Time reversal symmetry and magnetoelastic correlations are probed by means of high-resolution volume dilatometry in URu2Si2 at cryogenic temperatures and magnetic fields more than enough to suppress the hidden order state at H_HO(T = 0.66 K) approximately 35 T. We report a significant crystal lattice volume expansion at and above H_HO(T), and even above T_HO, possibly a consequence of field-induced f-electron localization, and hysteresis at some high field phase boundaries that confirm volume involvement. We investigate in detail the magnetostriction and magnetization as the temperature is reduced over two decades from 50 K where the system is paramagnetic, to 0.5 K in the realms of the hidden order state. We find a dominant quadratic-in-field dependence delta L/L proportional to H^2, a result consistent with a state that is symmetric under time reversal. The data shows, however, an incipient yet unmistakable asymptotic approach to linear (delta L/L proportional to 1-H/H_0) for 15 T < H < H_HO(0.66 K) approximately 35 T at the lowest temperatures. We discuss these results in the framework of a Ginzburg-Landau formalism that proposes a complex order parameter for the HO to model the (H,T,p) phase diagram.

cond-mat.str-el↗

arXiv2018

Imaging the magnetic states in an actinide ferromagnet UMn$_2$Ge$_2$

We present studies of the magnetic domain structure of UMn$_2$Ge$_2$ single crystals using a home-built low temperature magnetic force microscope. The material has two distinct magnetic ordering temperatures, originating from the Mn and U moments. At room temperature, where the Mn moments dominate, there are flower-like domain patterns similar to those observed in uniaxial ferromagnets. After exposing the sample to a one-tesla magnetic field near 40 K, the evolution of the magnetic domains are imaged through zero-field warming up to 200 K. Near the ordering temperature of the uranium moments a clear change in the domain wall motion is observed. The domain size analysis of the flower-like pattern reveals that the domain structure is consistent with a model of branching domains.

cond-mat.mtrl-sci↗

arXiv2018

Topological Excitations of Hidden Order in URu$_2$Si$_2$ Under Extreme Electric Fields

Quantum materials are epitomized by the influence of collective modes upon their macroscopic properties. Relatively few examples exist, however, whereby coherence of the ground-state wavefunction directly contributes to the conductivity. Notable examples include the quantizing effects of high magnetic fields upon the 2D electron gas, the collective sliding of charge density waves subject to high electric fields, and perhaps most notably the macroscopic phase coherence that enables superconductors to carry dissipationless currents. Here we reveal that the low temperature hidden order state of URu$_2$Si$_2$ exhibits just such a connection between the quantum and macroscopic worlds -- under large voltage bias we observe non-linear contributions to the conductivity that are directly analogous to the manifestation of phase slips in one-dimensional superconductors [1], suggesting a complex order parameter for hidden order

cond-mat.str-el↗

arXiv2018

Uncovering the Origin of Divergence in the CsM(CrO$_4$)$_2$ (M = La, Pr, Nd, Sm, Eu; Am) Family through Examination of the Chemical Bonding in a Molecular Cluster and by Band Structure Analysis

A series of f-block chromates, CsM(CrO$_4$)$_2$ (M = La, Pr, Nd, Sm, Eu; Am), were prepared revealing notable differences between the AmIII derivatives and their lanthanide analogs. While all compounds form similar layered structures, the americium compound exhibits polymorphism and adopts both a structure isomorphous with the early lanthanides as well as one that possesses lower symmetry. Both polymorphs are dark red and possess band gaps that are smaller than the LnIII compounds. In order to probe the origin of these differences, the electronic structure of $α$-CsSm(CrO$_4$)$_2$, $α$-CsEu(CrO$_4$)$_2$ and $α$-CsAm(CrO$_4$)$_2$ were studied using both a molecular cluster approach featuring hybrid density functional theory and QTAIM analysis, and by the periodic LDA+GA and LDA+DMFT methods. Notably, the covalent contributions to bonding by the f orbitals was found to be more than twice as large in the AmIII chromate than in the SmIII and EuIII compounds, and even larger in magnitude than the Am-5f spin-orbit splitting in this system. Our analysis indicates also that the Am-O covalency in $α$-CsAm(CrO$_4$)$_2$ is driven by the degeneracy of the 5f and 2p orbitals, and not by orbital overlap.

cond-mat.str-el↗

arXiv2017

Investigation of the commensurate magnetic structure in heavy fermion CePt2In7 using magnetic resonant X-ray diffraction

We investigated the magnetic structure of the heavy fermion compound CePt$_2$In$_7$ below $T_N~=5.34(2)$ K using magnetic resonant X-ray diffraction at ambient pressure. The magnetic order is characterized by a commensurate propagation vector ${k}_{1/2}~=~\left( \frac{1}{2} , \frac{1}{2}, \frac{1}{2}\right)$ with spins lying in the basal plane. Our measurements did not reveal the presence of an incommensurate order propagating along the high symmetry directions in reciprocal space but cannot exclude other incommensurate modulations or weak scattering intensities. The observed commensurate order can be described equivalently by either a single-${k}$ structure or by a multi-${k}$ structure. Furthermore we explain how a commensurate-only ordering may explain the broad distribution of internal fields observed in nuclear quadrupolar resonance experiments (Sakai et al. 2011, Phys. Rev. B 83 140408) that was previously attributed to an incommensurate order. We also report powder X-ray diffraction showing that the crystallographic structure of CePt$_2$In$_7$ changes monotonically with pressure up to $P~=~7.3$ GPa at room temperature. The determined bulk modulus $B_0~=~81.1(3)$ GPa is similar to the ones of the Ce-115 family. Broad diffraction peaks confirm the presence of pronounced strain in polycrystalline samples of CePt$_2$In$_7$. We discuss how strain effects can lead to different electronic and magnetic properties between polycrystalline and single crystal samples.

cond-mat.str-el↗

arXiv2016

Quasiparticle interference of heavy fermions in resonant X-ray scattering

Resonant X-ray scattering (RXS) has recently become an increasingly important tool for the study of ordering phenomena in correlated electron systems. Yet, the interpretation of the RXS experiments remains theoretically challenging due to the complexity of the RXS cross-section. Central to this debate is the recent proposal that impurity-induced Friedel oscillations, akin to quasiparticle interference signals observed with the scanning tunneling microscope (STM), can lead to scattering peaks in the RXS experiments. The possibility that quasiparticle properties can be probed in RXS measurements opens up a new avenue to study the bulk band structure of materials with the orbital and element selectivity provided by RXS. Here, we test these ideas by combining RXS and STM measurements of the heavy fermion compound CeMIn$_5$ (M = Co, Rh). Temperature and doping dependent RXS measurements at the Ce-M$_4$ edge show a broad scattering enhancement that correlates with the appearance of heavy f-electron bands in these compounds. The scattering enhancement is consistent with the measured quasiparticle interference signal in the STM measurements, indicating that quasiparticle interference can be probed through the momentum distribution of RXS signals. Overall, our experiments demonstrate new opportunities for studies of correlated electronic systems using the RXS technique.

cond-mat.str-el↗

arXiv2015

Non-stoichiometry and Defects in the Weyl Semimetals TaAs, TaP, NbP, and NbAs

We report a structural study of the Weyl semimetals TaAs, TaP, NbP, and NbAs, utilizing diffraction techniques (single crystal x-ray diffraction and energy dispersive spectroscopy) and imaging techniques (transmission electron microscopy/scanning transmission electron microscopy). We observe defects of various degrees, leading to non-stoichiometric single crystals of all four semimetals. While TaP displays a large pnictide deficiency with composition TaP$_{0.83(3)}$, and stacking faults accompanied by anti-site disorder and site vacancies, TaAs displays transition metal deficiency with composition Ta$_{0.92(2)}$As and a high density of stacking faults. NbP also displays pnictide deficiency, yielding composition NbP$_{0.95(2)}$, and lastly, NbAs display very little deviation from a 1:1 composition, NbAs$_{1.00(3)}$, and is therefore recommended to serve as the model compound for these semimetals.

cond-mat.mtrl-sci↗

arXiv2013

Visualizing Nodal Heavy Fermion Superconductivity in CeCoIn5

Understanding the origin of superconductivity in strongly correlated electron systems continues to be at the forefront of unsolved problems in all of physics. Among the heavy f-electron systems, CeCoIn5 is one of the most fascinating, as it shares many of the characteristics of correlated d-electron high-Tc cuprate and pnictide superconductors, including the competition between antiferromagnetism and superconductivity. While there has been evidence for unconventional pairing in this compound, high-resolution spectroscopic measurements of the superconducting state have been lacking. Previously, we have used high-resolution scanning tunneling microscopy techniques to visualize the emergence of heavy-fermion excitations in CeCoIn5 and demonstrate the composite nature of these excitations well above Tc. Here we extend these techniques to much lower temperatures to investigate how superconductivity develops within a strongly correlated band of composite excitations. We find the spectrum of heavy excitations to be strongly modified just prior to the onset of superconductivity by a suppression of the spectral weight near the Fermi energy, reminiscent of the pseudogap state in the cuprates. By measuring the response of superconductivity to various perturbations, through both quasiparticle interference and local pair-breaking experiments, we demonstrate the nodal d-wave character of superconducting pairing in CeCoIn5.

cond-mat.supr-con↗

arXiv2013

Detection of electronic nematicity using scanning tunneling microscopy

Electronic nematic phases have been proposed to occur in various correlated electron systems and were recently claimed to have been detected in scanning tunneling microscopy (STM) conductance maps of the pseudogap states of the cuprate high-temperature superconductor Bi2Sr2CaCu2O8+x (Bi-2212). We investigate the influence of anisotropic STM tip structures on such measurements and establish, with a model calculation, the presence of a tunneling interference effect within an STM junction that induces energy-dependent symmetry-breaking features in the conductance maps. We experimentally confirm this phenomenon on different correlated electron systems, including measurements in the pseudogap state of Bi-2212, showing that the apparent nematic behavior of the imaged crystal lattice is likely not due to nematic order but is related to how a realistic STM tip probes the band structure of a material. We further establish that this interference effect can be used as a sensitive probe of changes in the momentum structure of the sample's quasiparticles as a function of energy.

cond-mat.str-el↗