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Ryan Kim

Publications and source records attributed to Ryan Kim.

8 recordsLinked to original sources

Real-time Multi-instrument Autonomous Discovery of Novel Phase-change Memory Materials

Autonomous labs enable the integration of automated experiment execution, data analysis and decision making. The main challenge remains the integration of diverse data streams from multiple instruments, where the data is often heterogeneous and unsynchronized. The standard learning process of undetermined synthesis-process-structure-property relationships (SPSPR) usually relies on post-experiment analysis after data is fully collected, not during live experiments, and decision making is carried out independently across characterization equipment. Here, we demonstrate the Multi-instrument Autonomous Discovery (MAD) framework -- combining structural property mapping and functional property optimization simultaneously in a closed-loop manner. As an example, we applied MAD to phase change memory (PCM) materials, and, in particular on the Mn-Sb-Te ternary, a previously unexplored materials system for PCM. A multi-output model is employed to merge data from x-ray diffraction (XRD) and electrical resistance measurements simultaneously through a co-regionalization kernel that models the relationship between them. The output probabilistic posterior and uncertainty quantification facilitate decision making with shared knowledge, while the goals are different across tasks. We aimed to maximize the knowledge of crystal structure distribution using non-negative matrix factorization (NMF), while in parallel, we find the composition with the maximum resistance value, an important figure of merit for PCM. Leveraging MAD, we found promising electrical PCMs and identified the SPSPR within 25 closed-loop iterations, corresponding to a seven-fold speed-up. The framework opens a new path of study in large-scale autonomous facilities, where future experiments can be run in parallel together, not independently.

cond-mat.mtrl-sci

Combinatorial Survey of Structural Phase Distribution and Magnetism in Fe-Ge-Te Composition-spread Thin Film Libraries

Recently, magnetic 2-dimensional (2D) van der Waals (vdW) materials have garnered tremendous attention. The vdW ferromagnet Fe5Ge1Te2 has a Curie temperature Tc of ~ 270 K, which is tailorable by tuning the stoichiometry and the Fe deficiency to reach room temperature. To explore the expanded compositional space, we implemented combinatorial synthesis and high-throughput characterization to investigate the structural phase distribution and ferromagnetism of a Fe-Ge-Te thin film library. The library was prepared by magnetron co-sputtering followed by annealing in vacuum or in an inert environment. Composition and structural phase distribution of the 177 pads in the library were characterized using high-throughput wavelength dispersive spectroscopy (WDS), X-ray diffraction (XRD), and two-point probe resistance measurements. We leverage unsupervised machine learning to cluster the XRD dataset into groups of compositions with similar structural phases, and further study the ferromagnetic properties via SQUID magnetometry and X-ray magnetic circular dichroism (XMCD) across different clusters. The results are compared against magnetization and structural models calculated using DFT. Our results demonstrate that the hexagonal crystal structure is a critical prerequisite for ferromagnetism in this system, and that unexplored materials adopting this structure can be efficiently identified as possible ferromagnetic materials using our high-throughput, ML-assisted framework. This workflow based on the combinatorial strategy allows us to rapidly capture the composition-structure-magnetic property map across a broad compositional landscape of novel magnetic materials.

cond-mat.mtrl-sci

Humanity's Last Exam

Benchmarks are important tools for tracking the rapid advancements in large language model (LLM) capabilities. However, benchmarks are not keeping pace in difficulty: LLMs now achieve over 90\% accuracy on popular benchmarks like MMLU, limiting informed measurement of state-of-the-art LLM capabilities. In response, we introduce Humanity's Last Exam (HLE), a multi-modal benchmark at the frontier of human knowledge, designed to be the final closed-ended academic benchmark of its kind with broad subject coverage. HLE consists of 2,500 questions across dozens of subjects, including mathematics, humanities, and the natural sciences. HLE is developed globally by subject-matter experts and consists of multiple-choice and short-answer questions suitable for automated grading. Each question has a known solution that is unambiguous and easily verifiable, but cannot be quickly answered via internet retrieval. State-of-the-art LLMs demonstrate low accuracy and calibration on HLE, highlighting a significant gap between current LLM capabilities and the expert human frontier on closed-ended academic questions. To inform research and policymaking upon a clear understanding of model capabilities, we publicly release HLE at https://lastexam.ai.

cs.LG

Analysis of Modern Computer Vision Models for Blood Cell Classification

The accurate classification of white blood cells and related blood components is crucial for medical diagnoses. While traditional manual examinations and automated hematology analyzers have been widely used, they are often slow and prone to errors. Recent advancements in deep learning have shown promise for addressing these limitations. Earlier studies have demonstrated the viability of convolutional neural networks such as DenseNet, ResNet, and VGGNet for this task. Building on these foundations, our work employs more recent and efficient models to achieve rapid and accurate results. Specifically, this study used state-of-the-art architectures, including MaxVit, EfficientVit, EfficientNet, EfficientNetV2, and MobileNetV3. This study aimed to evaluate the performance of these models in WBC classification, potentially offering a more efficient and reliable alternative to current methods. Our approach not only addresses the speed and accuracy concerns of traditional techniques but also explores the applicability of innovative deep learning models in hematological analysis.

eess.IV

Implementing a Hybrid Quantum-Classical Neural Network by Utilizing a Variational Quantum Circuit for Detection of Dementia

Magnetic resonance imaging (MRI) is a common technique to scan brains for strokes, tumors, and other abnormalities that cause forms of dementia. However, correctly diagnosing forms of dementia from MRIs is difficult, as nearly 1 in 3 patients with Alzheimer's were misdiagnosed in 2019, an issue neural networks can rectify. Quantum computing applications This proposed novel neural network architecture uses a fully-connected (FC) layer, which reduces the number of features to obtain an expectation value by implementing a variational quantum circuit (VQC). The VQC created in this study utilizes a layer of Hadamard gates, Rotation-Y gates that are parameterized by tanh(intensity) * (pi/2) of a pixel, controlled-not (CNOT) gates, and measurement operators to obtain the expected values. This study found that the proposed hybrid quantum-classical convolutional neural network (QCCNN) provided 97.5% and 95.1% testing and validation accuracies, respectively, which was considerably higher than the classical neural network (CNN) testing and validation accuracies of 91.5% and 89.2%. Additionally, using a testing set of 100 normal and 100 dementia MRI images, the QCCNN detected normal and demented images correctly 95% and 98% of the time, compared to the CNN accuracies of 89% and 91%. With hospitals like Massachusetts General Hospital beginning to adopt machine learning applications for biomedical image detection, this proposed architecture would approve accuracies and potentially save more lives. Furthermore, the proposed architecture is generally flexible, and can be used for transfer-learning tasks, saving time and resources.

quant-ph

Aerodynamic Optimization of the Angle of Attack of the Wing Design of a MQ-9 Reaper UAV

In this paper I present the aerodynamic optimization of the angle of attack of MQ-9 Reaper wings under turbulent airflow conditions. The background discusses the evolution of UAVs such as the Hunter and their usages for different tasks, specifically within the last decade. The main procedural stage consists of creating a criterion for choosing the most aerodynamic wing design by considering certain aerodynamic properties and analyzing the lift and drag coefficients using computer software. At the end of the paper, the final optimized MQ-9 wing design, along with its respective design parameters, are presented and discussed.

physics.flu-dyn

Development of a conversing and body temperature scanning autonomously navigating robot to help screen for COVID-19

Throughout the COVID-19 pandemic, the most common symptom displayed by patients has been a fever, leading to the use of temperature scanning as a preemptive measure to detect potential carriers of the virus. Human employees with handheld thermometers have been used to fulfill this task, however this puts them at risk as they cannot be physically distanced and the sequential nature of this method leads to great inconveniences and inefficiency. The proposed solution is an autonomously navigating robot capable of conversing and scanning people's temperature to detect fevers and help screen for COVID-19. To satisfy this objective, the robot must be able to (1) navigate autonomously, (2) detect and track people, and (3) get individuals' temperature reading and converse with them if it exceeds 38{\deg}C. An autonomously navigating mobile robot is used with a manipulator controlled using a face tracking algorithm, and an end effector consisting of a thermal camera, smartphone, and chatbot. The goal is to develop a functioning solution that performs the above tasks. In addition, technical challenges encountered and their engineering solutions will be presented, and recommendations will be made for enhancements that could be incorporated when approaching commercialization.

cs.RO

Automatic calibration of time of flight based non-line-of-sight reconstruction

Time of flight based Non-line-of-sight (NLOS) imaging approaches require precise calibration of illumination and detector positions on the visible scene to produce reasonable results. If this calibration error is sufficiently high, reconstruction can fail entirely without any indication to the user. In this work, we highlight the necessity of building autocalibration into NLOS reconstruction in order to handle mis-calibration. We propose a forward model of NLOS measurements that is differentiable with respect to both, the hidden scene albedo, and virtual illumination and detector positions. With only a mean squared error loss and no regularization, our model enables joint reconstruction and recovery of calibration parameters by minimizing the measurement residual using gradient descent. We demonstrate our method is able to produce robust reconstructions using simulated and real data where the calibration error applied causes other state of the art algorithms to fail.

eess.IV