arXiv subjects

Ryan van Mastrigt

Publications and source records attributed to Ryan van Mastrigt.

5 recordsLinked to original sources

arXiv2026

Machine learned designs of functional colloidal foldamers

A protein's function follows from the structure it adopts, and in some cases which structure that is depends on the pathway taken. In programmable matter the target is fixed before assembly, and whatever else forms is treated as error. Here we show that pathways themselves form a design space. Using reinforcement learning, we fold model DNA-coated droplet chains into rigid two-dimensional geometries, uncovering two classes of pathways: downhill, in which bonds are only added, and detour, in which bonds are broken and remade before the target is reached: for some the only route that exists. Coarse-graining pathways by interactions gives experimentally realizable protocols. Some produce one geometry, others several: structures sharing a detour route can be cycled between, while those that coexist assemble into superstructures inaccessible to a uniform product. Function emerges from the pathways rather than being designed. Designing the process instead of the components could give colloidal materials that reconfigure on demand.

cond-mat.soft↗

arXiv2025

Metamaterials that learn to change shape

Learning to change shape is a fundamental strategy of adaptation and evolution of living organisms, from bacteria and cells to tissues and animals. Human-made materials can also exhibit advanced shape morphing capabilities, but lack the ability to learn. Here, we build metamaterials that can learn complex shape-changing responses using a contrastive learning scheme. By being shown examples of the target shape changes, our metamaterials are able to learn those shape changes by progressively updating internal learning degrees of freedom -- the local stiffnesses. Unlike traditional materials that are designed once and for all, our metamaterials have the ability to forget and learn new shape changes in sequence, to learn multiple shape changes that break reciprocity, and to learn multistable shape changes, which in turn allows them to perform reflex gripping actions and locomotion. Our findings establish metamaterials as an exciting platform for physical learning, which in turn opens avenues for the use of physical learning to design adaptive materials and robots.

cond-mat.soft↗

arXiv2024

Prospecting for Pluripotency in Metamaterial Design

From self-assembly and protein folding to combinatorial metamaterials, a key challenge in material design is finding the right combination of interacting building blocks that yield targeted properties. Such structures are fiendishly difficult to find; not only are they rare, but often the design space is so rough that gradients are useless and direct optimization is hopeless. Here, we design ultra rare combinatorial metamaterials capable of multiple desired deformations by introducing a two-fold strategy that avoids the drawbacks of direct optimization. We first combine convolutional neural networks with genetic algorithms to prospect for metamaterial designs with a potential for high performance. In our case, these metamaterials have a high number of spatially extended modes; they are pluripotent. Second, we exploit this library of pluripotent designs to generate metamaterials with multiple target deformations, which we finally refine by strategically placing defects. Our pluripotent, multishape metamaterials would be impossible to design through trial-and-error or standard optimization. Instead, our data-driven approach is systematic and ideally suited to tackling the large and intractable combinatorial problems that are pervasive in material science.

cond-mat.soft↗

arXiv2023

Emergent Nonlocal Combinatorial Design Rules for Multimodal Metamaterials

Combinatorial mechanical metamaterials feature spatially textured soft modes that yield exotic and useful mechanical properties. While a single soft mode often can be rationally designed by following a set of tiling rules for the building blocks of the metamaterial, it is an open question what design rules are required to realize multiple soft modes. Multimodal metamaterials would allow for advanced mechanical functionalities that can be selected on the fly. Here we introduce a transfer matrix-like framework to design multiple soft modes in combinatorial metamaterials composed of aperiodic tilings of building blocks. We use this framework to derive rules for multimodal designs for a specific family of building blocks. We show that such designs require a large number of degeneracies between constraints, and find precise rules on the real space configuration that allow such degeneracies. These rules are significantly more complex than the simple tiling rules that emerge for single-mode metamaterials. For the specific example studied here, they can be expressed as local rules for tiles composed of pairs of building blocks in combination with a nonlocal rule in the form of a global constraint on the type of tiles that are allowed to appear together anywhere in the configuration. This nonlocal rule is exclusive to multimodal metamaterials and exemplifies the complexity of rational design of multimode metamaterials. Our framework is a first step towards a systematic design strategy of multimodal metamaterials with spatially textured soft modes.

cond-mat.soft↗

arXiv2022

Machine Learning of Implicit Combinatorial Rules in Mechanical Metamaterials

Combinatorial problems arising in puzzles, origami, and (meta)material design have rare sets of solutions, which define complex and sharply delineated boundaries in configuration space. These boundaries are difficult to capture with conventional statistical and numerical methods. Here we show that convolutional neural networks can learn to recognize these boundaries for combinatorial mechanical metamaterials, down to finest detail, despite using heavily undersampled training sets, and can successfully generalize. This suggests that the network infers the underlying combinatorial rules from the sparse training set, opening up new possibilities for complex design of (meta)materials.

cond-mat.soft↗