arXiv subjects

Sébastien Petit-Watelot

Publications and source records attributed to Sébastien Petit-Watelot.

At least 19 recordsLinked to original sources

arXiv2026

Magneto-optical signal from $\mathrm{Co_2Mn}$-based Heusler thin films in MOKE and BLS

$\mathrm{Co_2Mn}$-based Heusler compounds offer a versatile, composition-tunable platform for magnonics and spintronics. Among them, the half-metallic $\mathrm{Co_2MnSi}$ is of particular interest for magnonics owing to its ultralow Gilbert damping, yet its weak magneto-optical response in the visible challenges optical probing such as Brillouin light scattering (BLS). We study the magneto-optical response of epitaxial $\mathrm{Co_2Mn}X$ films ($X = \{\mathrm{Al}_x\mathrm{Si}_{1-x}, \mathrm{Ga}_x\mathrm{Ge}_{1-x}, \mathrm{Sn}\}$) by magneto-optical Kerr effect (MOKE) spectroscopy and BLS. Angle-resolved MOKE resolves a significant, wavelength-dependent quadratic MOKE (QMOKE) only for $\mathrm{Co_2MnSi}$, whereas $\mathrm{Co_2MnAl}$, $\mathrm{Co_2MnGa}$ and $\mathrm{Co_2MnSn}$ respond dominantly linearly. Comparing BLS intensities of thermal magnons at two wavelengths, $\mathrm{Co_2MnSi}$ gives the weakest signal at 532 nm yet among the strongest at 457 nm, tracking the spectral dependence of its Kerr angle. These results emphasise the relation between the two magneto-optical techniques, guiding the choice of probing wavelength for $\mathrm{Co_2Mn}$-based Heusler compounds.

cond-mat.mes-hall↗

arXiv2026

Interface-Controlled Spin-Orbit Torques in Rare-Earth Synthetic Ferrimagnets Probed by Sagnac Magneto-Optics and Harmonic Hall Measurements

Spin-orbit torque (SOT) provides an efficient route for manipulating magnetization in spintronic devices, and its accurate quantification is essential. Here, we investigate Co/Gd-based synthetic ferrimagnets using complementary magnetotransport and magneto-optical techniques. We use a Sagnac magneto-optical interferometry method to directly quantify current-induced magnetization tilting and extract the damping-like SOT effective field. The Sagnac measurements show good agreement with harmonic Hall analysis across different Co/Gd and Gd/Pt/Co heterostructures, providing a quantitative determination of the damping-like SOT effective field that does not rely on electrical transport signatures. By varying the Gd thickness and multilayer stacking order, we demonstrate that the damping-like torque is strongly influenced by spin transport and angular momentum conversion at rare-earth and heavy-metal interfaces. The observation of a finite torque in Gd/Pt/Co/Pt structures, where conventional Pt spin Hall contributions are expected to compensate, highlights the active role of the Gd layer in SOT generation. Furthermore, interface engineering enables perpendicular magnetic anisotropy in Gd/Pt/Co/Al heterostructures with a 2-nm-thick Co layer, allowing current-induced SOT switching at current densities of 8-10 MA/cm$^2$. These results establish rare-earth-based synthetic ferrimagnets as a versatile platform for engineering spin-orbit phenomena and optimizing low-power spintronic devices.

cond-mat.mtrl-sci↗

arXiv2026

Epitaxial $\mathrm{Co_2MnSi}$ with intrinsic magnetocrystalline anisotropy as a route to bias-field-free nonlinear half-metal magnonics at the nanoscale

Half-metallic Heusler compounds like $\mathrm{Co_2MnSi}$ allow to bridge magnonic and spintronic functionality for hybrid unconventional computing approaches with sought-after properties like 100% spin polarization and associated low Gilbert damping $α\leq 10^{-3}$. However, the desirable material parameters are inherently tied to the crystal lattice with a particularly critical dependence on structural order in $\mathrm{Co_2MnSi}$. To date, the successful fabrication of nanoscale devices with robust structural integrity remains yet a challenge, and consequently the impact of the material parameters on the resulting nonlinear spin-wave dynamics remains largely unexplored. Here, we report on a study of linear and nonlinear spin-wave dynamics in transversally magnetized $\mathrm{Co_2MnSi}$ waveguides with impeccable crystalline ordering. We show that epitaxial, $\mathrm{L2}_1$-ordered $\mathrm{Co_2MnSi}$ exhibits an intrinsic cubic anisotropy with first- and second-order contributions, stabilizing a magnetization alignment along the crystal $\langle110\rangle$ directions. We confirm the implication of an unaffected crystal structure resulting in preserved magnetic properties in the patterned structures. Herein, the persistent magnetocrystalline anisotropy reshapes the spin-wave dispersion which yields a first-order nonlinear instability suppression range extending over several GHz - even for vanishing bias fields. Moreover, the intrinsic magnetocrystalline anisotropy can be exploited to counteract shape demagnetization for a stabilized low bias field operation in the favourable Damon-Eshbach geometry with high group velocities and decay lengths. Together with the proven half-metallicity and ultralow Gilbert damping, this research establishes $\mathrm{Co_2MnSi}$ as a robust, scalable platform towards bias-field-free nonlinear half-metal magnonics.

cond-mat.mes-hall↗

arXiv2026

Spin-polarization of the electric current in half-metallic Co$_2$MnSi Heusler thin films

Using propagating spin wave spectroscopy we measure the spin wave Doppler shift in patterned MgO/Co$_2$MnSi/MgO thin films and determine the degree of spin-polarization of the electric current. Our measurements reveal that the current is fully spin-polarized in the devices. This shows that the half-metallic character of the electron band structure translates into a fully spin polarized current flowing across the patterned films. Additionally, we measure a current-induced change of the spin-wave attenuation from which we estimate the non-adiabatic spin-transfer-torque parameter.

cond-mat.mtrl-sci↗

arXiv2026

Unconventional views on orbitronics supported by experimental results

Emerging orbitronics assumes long-range orbital current transport, analogous to spin currents. However, recent theory and experiments challenge this view, showing rather local characters for orbital polarization and orbit-spin conversions. We study angular momentum generated by ferromagnetic resonance and thermal gradients in Ni/(Pt)Ti/Au heterostructures. The observed charge current produced is independent of Ti thickness up to 60 nm, incompatible with orbital transport in Ti. Instead, its magnitude depends on both Ti interfaces, evidencing spin-mediated transport in between after and before local orbit-spin interconversions.

cond-mat.mtrl-sci↗

arXiv2026

RF field characterization and rectification effects in spin pumping and spin-torque FMR for spin-orbitronics

Quantifying spin-orbital-to-charge conversion efficiency is crucial for spin-orbitronics. Two widely used methods for determining these efficiencies are based on ferromagnetic resonance (FMR), spin pumping FMR for the inverse effect, and spin-torque FMR for the direct effect. A key parameter to achieve accurate quantification, especially for spin-pumping FMR, is the RF field strength, $h_{\mathrm{RF}}$. We present a comprehensive theoretical model and experimental protocol that allow a correct quantification of $h_{\mathrm{RF}}$. It was validated by extensive experimental results and it was rigorously tested across various antennas geometries and ferromagnetic systems. We demonstrate that odd-symmetric Lorentzian voltages-which perfectly mimic spin-pumping or spin-torque FMR signals-can arise purely from rectification effects (due to anisotropic magnetoresistance) when $h_{\mathrm{RF}}$ orientation is parallel to the ferromagnetic surface. Through a systematic study of various 10-nm-thick ferromagnetic layers, such as Ni, NiFe, Fe, and CoFeB, we find that while Fe and CoFeB exhibit minimal rectification, Ni and NiFe generate strong rectified signals that must be corrected. We further demonstrate that these rectification effects become negligible for ferromagnetic thicknesses $\leq$ 6 nm, as validated in NiFe/Pt bilayers, providing an important guideline for the design of future heterostructures.

cond-mat.mtrl-sci↗

arXiv2025

Spin current symmetries generated by GdFeCo ferrimagnet across its magnetisation compensation temperature

Ferrimagnets, composed of antiferromagnetically coupled magnetic sublattices whose net magnetisation can be tuned by temperature, offer a unique platform for probing the symmetry of the spin currents they generate and for identifying the sublattice contributions to these currents. Here, we investigate the spin current symmetries produced by GdFeCo ferrimagnet at a fixed concentration and across a broad temperature range, including the magnetisation compensation point. Using complementary techniques based on spin-torque ferromagnetic resonance spectroscopy, we separate the contributions of the spin Hall effect (SHE) and the spin anomalous Hall effect (SAHE). We show that the torques arising from both mechanisms retain their sign across the magnetisation compensation temperature, and that the SAHE-driven damping-like torque has the opposite sign to the SHE-driven term. We suggest that both effects originates from distinct electronic subsystems: the SHE emerging from Gd 5d electrons, and the SAHE from FeCo 3d electrons. Consequently, the SHE sign remains insensitive to the magnetisation state, whereas the SAHE sign does not invert at compensation, reproducing our observations. Together, these insights clarify the interplay between sublattices in ferrimagnetic spin transport and highlight the potential of ferrimagnetic spin currents to generate spin torques in adjacent layers or within the ferrimagnet itself.

cond-mat.mes-hall↗

arXiv2023

Magnetic SAW RFID Sensor Based on Love Wave for Detection of Magnetic Field and Temperature

Magnetic field measurement including a temperature compensation is essential for a magnetic field sensor. This study investigates a magnetic surface acoustic wave (MSAW) sensor in a reflective delay line configuration with two acoustic propagation paths with and without magnetic field sensitive layer. The delay in path with sensitive layer leads to magnetic field detection and the one without enable temperature measurement and thus compensation for the first path. The developed sensor is based on a ZnO/LiNbO$_3$ Ycut (X-direction) layered structure as Love wave platform. Love wave as a shear wave being more favorable for magnetic detection. Co-Fe-B is considered as sensitive layer to detect magnetic field changes and is deposited on the top of ZnO, but only on one of the two paths. We combined an original configuration of connected IDTs with a high electromechanical coupling coefficient (K$^2$) mode to improve the signal amplitude. The achieved sensor exhibits a high temperature and magnetic field sensitivity of -63 ppm/$^\circ$C and -781 ppm/mT, respectively. The temperature compensation method for magnetic field measurement is demonstrated using a differential measurement by subtracting the delay times obtained for the two paths with and without the sensitive layer. Finally, The sensor exhibited good repeatability at various temperatures. Moreover, the device developed allows in addition to the multisensor functionality, the radio frequency identification (RFID) which is necessary for the deployment of sensor networks.

eess.SP↗

arXiv2023

Spin transport properties of spinel vanadate-based heterostructures

Spin-orbit coupling and breaking of inversion symmetry are necessary ingredients to enable a pure spin current-based manipulation of the magnetization via the spin-orbit torque effect. Currently, magnetic insulator oxides with non-dissipative characteristics are being explored. When combined with non-magnetic heavy metals, known for their large spin-orbit coupling, they offer promising potential for energy-efficient spin-orbitronics applications. The intrinsic electronic correlations characterizing those strongly correlated oxides hold the promises to add extra control-knobs to the desired efficient spin-wave propagation and abrupt magnetization switching phenomena. Spinel vanadate FeV2O4 (FVO) exhibits several structural phase transitions which are accompanied by an intricate interplay of magnetic, charge and orbital orderings. When grown as a thin film onto SrTiO3, the compressive strain state induces a perpendicular magnetic anisotropy, making FVO-based heterostructures desirable for spin-orbitronics applications. In this study, we have optimised the deposition of stoichiometric and epitaxial Pt/FVO heterostructures by Pulsed Laser Deposition and examined their spin-related phenomena. From angle-dependent magnetotransport measurements, we observed both Anisotropic Magnetoresistance (AMR) and Spin Hall Magnetoresistance (SMR) effects. Our findings show the SMR component as the primary contributor to the overall magnetoresistance, whose high value of 0.12% is only comparable to properly optimized oxide-based systems.

cond-mat.mtrl-sci↗

arXiv2023

Spin-to-charge conversion by spin pumping in sputtered polycrystalline Bi$_x$Se$_{1-x}$

Topological materials are of high interest due to the promise to obtain low power and fast memory devices based on efficient spin-orbit torque switching or spin-orbit magnetic state read-out. In particular, sputtered polycrystalline Bi$_x$Se$_{1-x}$ is one of the materials with more potential for this purpose since it is relatively easy to fabricate and has been reported to have a very high spin Hall angle. We study the spin-to-charge conversion in Bi$_x$Se$_{1-x}$ using the spin pumping technique coming from the ferromagnetic resonance in a contiguous permalloy thin film. We put a special emphasis on the interfacial properties of the system. Our results show that the spin Hall angle of Bi$_x$Se$_{1-x}$ has an opposite sign to the one of Pt. The charge current arising from the spin-to-charge conversion is, in contrast, lower than Pt by more than one order of magnitude. We ascribe this to the interdiffusion of Bi$_x$Se$_{1-x}$ and permalloy and the changes in chemical composition produced by this effect, which is an intrinsic characteristic of the system and is not considered in many other studies.

cond-mat.mtrl-sci↗

arXiv2022

Thermal spin current generation in the multifunctional ferrimagnet Ga$_{0.6}$Fe$_{1.4}$O$_{3}$

In recent years, multifunctional materials have attracted increasing interest for magnetic memories and energy harvesting applications. Magnetic insulating materials are of special interest for this purpose, since they allow the design of more efficient devices due to the lower Joule heat losses. In this context, Ga$_{0.6}$Fe$_{1.4}$O$_3$ (GFO) is a good candidate for spintronics applications, since it can exhibit multiferroicity and presents a spin Hall magnetoresistance similar to the one observed in a yttrium iron garnet (YIG)/Pt bilayer. Here, we explore GFO utilizing thermo-spin measurements in an on-chip approach. By carefully considering the geometry of our thermo-spin devices we are able to quantify the spin Seebeck effect and the spin current generation in a GFO/Pt bilayer, obtaining a value comparable to that of YIG/Pt. This further confirms the promises of an efficient spin current generation with the possibility of an electric-field manipulation of the magnetic properties of the system in an insulating ferrimagnetic material.

cond-mat.mtrl-sci↗

arXiv2022

Ferrimagnet GdFeCo characterization for spin-orbitronics: large field-like and damping-like torques

Spintronics is showing promising results in the search for new materials and effects to reduce energy consumption in information technology. Among these materials, ferrimagnets are of special interest, since they can produce large spin currents that trigger the magnetization dynamics of adjacent layers or even their own magnetization. Here, we present a study of the generation of spin current by GdFeCo in a GdFeCo/Cu/NiFe trilayer where the FeCo sublattice magnetization is dominant at room temperature. Magnetic properties such as the saturation magnetization are deduced from magnetometry measurements while damping constant is estimated from spin-torque ferromagnetic resonance (ST-FMR). We show that the overall damping-like (DL) and field-like (FL) effective fields as well as the associated spin Hall angles can be reliably obtained by performing the dependence of ST-FMR by an added dc current. The sum of the spin Hall angles for both the spin Hall effect (SHE) and the spin anomalous Hall effect (SAHE) symmetries are: $θ_{DL}^{SAHE} + θ_{DL}^{SHE}=-0.15 \pm 0.05$ and $θ_{FL}^{SAHE} + θ_{FL}^{SHE}=0.026 \pm 0.005$. From the symmetry of ST-FMR signals we find that $θ_{DL}^{SHE}$ is positive and dominated by the negative $θ_{DL}^{SAHE}$. The present study paves the way for tuning the different symmetries in spin conversion in highly efficient ferrimagnetic systems.

cond-mat.mes-hall↗

arXiv2021

Spin current transport in hybrid Pt / multifunctional magnetoelectric Ga0.6Fe1.4O3 bilayers

The low power manipulation of magnetization is currently a highly sought-after objective in spintronics. Non ferromagnetic large spin-orbit coupling heavy metal (NM) / ferromagnet (FM) heterostructures offer interesting elements of response to this issue, by granting the manipulation of the FM magnetization by the NM spin Hall effect (SHE) generated spin current. Additional functionalities, such as the electric field control of the spin current generation, can be offered using multifunctional ferromagnets. We have studied the spin current transfer processes between Pt and the multifunctional magnetoelectric Ga0.6Fe1.4O3 (GFO). In particular, via angular dependent magnetotransport measurements, we were able to differentiate between magnetic proximity effect (MPE)-induced anisotropic magnetoresistance (AMR) and spin Hall magnetoresistance (SMR). Our analysis shows that SMR is the dominant phenomenon at all temperatures and is the only one to be considered near room temperature, with a magnitude comparable to those observed in Pd/YIG or Pt/YIG heterostructures. These results indicate that magnetoelectric GFO thin films show promises for achieving an electric-field control of the spin current generation in NM/FM oxide-based heterostructures.

cond-mat.mtrl-sci↗

arXiv2021

Nanocontact vortex oscillators based on Co$_2$MnGe pseudo-spin valves

We present an experimental study of vortex dynamics in magnetic nanocontacts based on pseudo spin valves comprising the Co$_2$MnGe Heusler compound. The films were grown by molecular beam epitaxy, where precise stoichiometry control and tailored stacking order allowed us to define the bottom ferromagnetic layer as the reference layer, with minimal coupling between the free and reference layers. 20-nm diameter nanocontacts were fabricated using a nano-indentation technique, leading to self-sustained gyration of the vortex generated by spin-transfer torques above a certain current threshold. By combining frequency- and time-domain measurements, we show that different types of spin-transfer induced dynamics related to different modes associated to the magnetic vortex configuration can be observed, such as mode hopping, mode coexistence and mode extinction appear in addition to the usual gyration mode.

cond-mat.mes-hall↗

arXiv2020

Current-induced spin torques on single GdFeCo magnetic layers

Spintronics exploits spin-orbit coupling (SOC) to generate spin currents, spin torques, and, in the absence of inversion symmetry, Rashba, and Dzyaloshinskii-Moriya interactions (DMI). The widely used magnetic materials, based on 3d metals such as Fe and Co, possess a small SOC. To circumvent this shortcoming, the common practice has been to utilize the large SOC of nonmagnetic layers of 5d heavy metals (HMs), such as Pt, to generate spin currents by Spin Hall Effect (SHE) and, in turn, exert spin torques on the magnetic layers. Here, we introduce a new class of material architectures, excluding nonmagnetic 5d HMs, for high-performance spintronics operations. We demonstrate very strong current-induced torques exerted on single GdFeCo layers due to the combination of large SOC of the Gd 5d states, and inversion symmetry breaking mainly engineered by interfaces. These "self-torques" are enhanced around the magnetization compensation temperature (close to room temperature) and can be tuned by adjusting the spin absorption outside the GdFeCo layer. In other measurements, we determine the very large emission of spin current from GdFeCo. This material platform opens new perspectives to exert "self-torques" on single magnetic layers as well as to generate spin currents from a magnetic layer.

cond-mat.mes-hall↗

arXiv2019

Modulation and phase-locking in nanocontact vortex oscillators

We have conducted experiments to probe how the dynamics of nanocontact vortex oscillators can be modulated by an external signal. We explore the phase-locking properties in both the commensurate and chaotic regimes, where chaos appears to impede phase-locking while a more standard behavior is seen in the commensurate phase. These different regimes correspond to how the periodicity of the vortex core reversal relates to the frequency of core gyration around the nanocontact; a commensurate phase appears when the reversal rate is an integer fraction of the gyration frequency, while a chaotic state appears when this ratio is irrational. External modulation where the power spectral density exhibits rich features, appears due to the modulation between the external source frequency, gyration frequency, and core reversal frequency. We explain these features with first- or second-order modulation between the three frequencies. Phase-locking is also visible between the external source frequency and internal vortex modes (gyration and core reversal modes).

cond-mat.mes-hall↗

arXiv2019

Chaos in Magnetic Nanocontact Vortex Oscillators

We present an experimental study of spin-torque driven vortex self-oscillations in magnetic nanocontacts. We find that above a certain threshold in applied currents, the vortex gyration around the nanocontact is modulated by relaxation oscillations, which involve periodic reversals of the vortex core. This modulation leads to the appearance of commensurate but also more interestingly here, incommensurate states, which are characterized by devil's staircases in the modulation frequency. We use frequency- and time-domain measurements together with advanced time-series analyses to provide experimental evidence of chaos in incommensurate states of vortex oscillations, in agreement with theoretical predictions.

cond-mat.mes-hall↗

arXiv2019

Pattern generation and symbolic dynamics in a nanocontact vortex oscillator

Harnessing chaos or intrinsic nonlinear behaviours from dynamical systems is a promising avenue for the development of unconventional information processing technologies. However, the exploitation of such features in spintronic devices has not been attempted despite the many theoretical and experimental evidence of nonlinear behaviour of the magnetization dynamics in nanomagnetic systems. Here, we propose a first step in that direction by unveiling and characterizing the patterns and symbolic dynamics originating from the nonlinear chaotic time-resolved electrical signals generated experimentally by a nanocontact vortex oscillator (NCVO). We use advanced filtering methods to dissociate nonlinear deterministic patterns from thermal fluctuations and show that the emergence of chaos results in the unpredictable alternation of simple oscillatory patterns controlled by the NCVO's core-polarity switching. With phase-space reconstruction techniques, we perform a symbolic analysis of the time series to assess the level of complexity and entropy generated in the chaotic regime. We find that at the centre of its incommensurate region, it can exhibit maximal entropy and complexity. This suggests that NCVOs are promising nonlinear nanoscale source of entropy that could be harnessed for information processing.

cond-mat.mes-hall↗