arXiv subjects

Síle Nic Chormaic

Publications and source records attributed to Síle Nic Chormaic.

At least 37 records · Page 2Linked to original sources

arXiv2020

In-situ analysis of small microplastics in coastal surface water samples of the subtropical island of Okinawa, Japan

Marine plastic debris is widely recognized as a global environmental issue. Sun-micron plastic particles, with an upper size limit of 20 um, have been identified as having the highest potential for causing damage to marine ecosystems. Having accurate methods for quantifying the abundance of such particles in a natural environment is essential for defining the extent of the problem they pose. Using an optical micro-Raman tweezers setup, we have identified the composition of particles trapped in marine aggregates collected from the coastal surface waters around the subtropical island of Okinawa. Chemical composition analysis at the single-particle level indicates dominance by low-density polyethylene, which accounted for 75% of the total sub-micron plastics analyzed. Our results show the occurrence of plastics at all test sites, with the highest concentration in areas with high human activities. The average, smallest sub-micron plastics size is (2.53 +/- 0.85)um for polystyrene. We also observed additional Raman peaks on the plastics spectrum with decreasing debris size which could be related to structural modification due to weathering or embedding in organic matter. By single-particle level sub-micron plastics identification, we can begin to understand their dispersion in the ocean and define their toxicity and impacts on marine biodiversity and food chain.

physics.app-ph↗

arXiv2020

Spin selection rule for {\it S} level transitions in atomic rubidium under paraxial and nonparaxial two-photon excitation

We report on an experimental test of the spin selection rule for two-photon transitions in atoms. In particular, we demonstrate that the $5S_{1/2}\to 6S_{1/2}$ transition rate in a rubidium gas follows a quadratic dependency on the helicity parameter linked to the polarization of the excitation light. For excitation via a single Gaussian beam or two counterpropagating beams in a hot vapor cell, the transition rate scales as the squared degree of linear polarization. The rate reaches zero when the light is circularly polarized. In contrast, when the excitation is realized via an evanescent field near an optical nanofiber, the two-photon transition cannot be completely extinguished (theoretically, not lower than 13\% of the maximum rate, under our experimental conditions) by only varying the polarization of the fiber-guided light. Our findings lead to a deeper understanding of the physics of multiphoton processes in atoms in strongly nonparaxial light.

physics.atom-ph↗

arXiv2020

Polarization-Controlled Cavity Input-Output Relations

Cavity input-output relations (CIORs) describe a universal formalism relating each of the far-field amplitudes outside the cavity to the internal cavity fields. Conventionally, they are derived based on a weak-scattering approximation. In this context, the amplitude of the off-resonant field remains nearly unaffected by the cavity, with the high coupling efficiency into cavity modes being attributed to destructive interference between the transmitted (or reflected) field and the output field from the cavity. In this Letter, we show that, in a whispering gallery resonator-waveguide coupled system, in the strong-scattering regime, the off-resonant field approaches to zero, but more than 90% coupling efficiency can still be achieved due to the Purcell-enhanced channeling. As a result, the CIORs turn out to be essentially different than in the weak-scattering regime. With this fact, we propose that the CIOR can be tailored by controlling the scattering strength. This is experimentally demonstrated by the transmission spectra exhibiting either bandstop or bandpass-type behavior according to the polarization of the input light field.

physics.optics↗

arXiv2020

Generation of cold Rydberg atoms at submicron distances from an optical nanofiber

We report on a controllable, hybrid quantum system consisting of cold Rydberg atoms and an optical nanofiber interface. Using a two-photon ladder-type excitation in $^{87}$Rb, we demonstrate both coherent and incoherent Rydberg excitation at submicron distances from the nanofiber surface. The 780 nm photon, near resonant to the $5S \rightarrow 5P$ transition, is mediated by the cooling laser, while the 482 nm light, near resonant to the $5P \rightarrow 29D$ transition, is mediated by the guided mode of the nanofiber. The population loss rate of the cold atom ensemble is used to measure the Rydberg population rate. A theoretical model is developed to interpret the results and link the population rate to the experimentally measured, effective Rabi frequency of the process. This work makes headway in the study of atom-surface interactions at submicron scales and the use of cold Rydberg atoms for all-fibered quantum networks and quantum simulations.

physics.atom-ph↗

arXiv2020

Observation of the $^{87}$Rb $5S_{1/2}$ to $4D_{3/2}$ electric quadrupole transition at 516.6 nm mediated via an optical nanofibre

Light guided by an optical nanofibre can have a very steep evanescent field gradient extending from the fibre surface. This can be exploited to drive electric quadrupole transitions in nearby quantum emitters. In this paper, we report on the observation of the $5S_{1/2}$ $\rightarrow$ $4D_{3/2}$ electric quadrupole transition at 516.6 nm (in vacuum) in laser-cooled $^{87}$Rb atoms using only a few $μ$W of laser power propagating through an optical nanofibre embedded in the atom cloud. This work extends the range of applications for optical nanofibres in atomic physics to include more fundamental tests.

physics.atom-ph↗

arXiv2020

Fabrication of Optical Nanofibre-Based Cavities using Focussed Ion-Beam Milling -- A Review

Nanofibre-based optical cavities are particularly useful for quantum optics application, such as the development of integrated single-photon sources, and for studying fundamental light-matter interactions in cavity quantum electrodynamics (cQED). Although several techniques have been used to produce nanofibre-based optical cavities, focussed ion beam (FIB) milling is becoming popular; it can be used for the fabrication of complex structures directly in the nanofibre. This technique uses a highly accelerated ion beam to remove atoms from the target material with high resolution. However, it is challenging to mill insulating materials with highly-curved structures and large aspect ratios, such as silica nanofibres, due to charge accumulation in the material that leads to mechanical vibrations and misalignment issues. In this article, we highlight the main features of nanofibres and briefly review cQED with nanofibre-based optical cavities. An overview of the milling process is given with a summary of different FIB milled devices and their applications. Finally, we present our technique to produce nanofibre cavities by FIB milling. To overcome the aforementioned challenges, we present a specially designed base plate with an indium tin oxide (ITO)-coated Si substrate and outline our procedure, which improves stability during milling and increases repeatability.

physics.optics↗

arXiv2020

Enhanced Directional Coupling of Light with a Whispering Gallery Microcavity

Directional coupling of light in nanophotonic circuits has recently attracted increasing interest, with numerous experimental realizations based on broken rotational or mirror symmetries of the light-matter system. The most prominent underlying effect is the spin-orbit interaction of light in subwavelength structures. Unfortunately, coupling of light to such structures is, in general, very inefficient. In this work, we experimentally demonstrate an order of magnitude enhancement of the directional coupling between two nanowaveguides by means of a whispering gallery microcavity. We also show that both transversmagnetic and transverse electric modes can be used for the enhancement.

physics.optics↗

arXiv2019

Raman Laser Switching Induced by Cascaded Light Scattering

We show that, in multimode Raman lasers, cascaded light scattering (CLS) not only extends the optical frequency range, but could also modulate the laser dynamics. The origin of this phenomenon is based on the fact that many Raman lasing modes are directly correlated through CLS. The coupled-mode equations only describe single-mode cascaded Raman lasers and are insufficient for describing the multimode case. In this work, we introduce additional terms to account for intermodal interaction and, thence, reveal the physical mechanism behind the mode-switching phenomenon. Additionally, mode-switching controlled solely by a single-mode pump in whispering gallery mode (WGM) silica Raman lasers is demonstrated. As the intracavity pump power is increased, laser switching happens between two adjacent WGMs in the same mode family.

physics.optics↗

arXiv2019

Light-induced rotation of dielectric microparticles around an optical nanofiber

We experimentally demonstrate orbiting of isotropic, dielectric microparticles around an optical nanofiber that guides elliptically polarized fundamental modes. The driving transverse radiation force appears in the evanescent electromagnetic fields due to orbital angular momentum. The force direction is opposite to that of the energy flow circulation around the nanofiber. Our results verify the theoretically predicted negative optical torque on a sufficiently large particle in the vicinity of a nanofiber.

physics.optics↗

arXiv2019

Plasmonic Optical Tweezers based on Nanostructures: fundamentals, advances and prospects

The ability of metallic nanostructures to confine light at the sub-wavelength scale enables new perspectives and opportunities in the field of nanotechnology. Making use of this unique advantage, nano-optical trapping techniques have been developed to tackle new challenges in a wide range of areas from biology to quantum optics. In this work, starting from basic theories, we present a review of research progress in near-field optical manipulation techniques based on metallic nanostructures, with an emphasis on some of the most promising advances in molecular technology, such as the precise control of single-biomolecules. We also provide an overview of possible future research directions of nano-manipulation techniques.

physics.optics↗

arXiv2019

Polarisation control for optical nanofibres by imaging through a single lens

We present a simple method for controlling the polarisation state of light at the waist of a single-mode optical nanofibre. The method consists of complete polarisation compensation based on imaging scattered light from inherent inhomogeneities both on the fibre surface and in the glass material itself. In contrast to the recently reported protocol exploiting two imaging systems oriented at 45 degrees to each other, our method requires only one lens and a video camera. It is particularly useful for nanofibre-based applications with severe geometric constraints, such as inside vacuum chambers for experiments with cold atoms. The measured fidelity of the achieved control is about 98\% using lenses with moderate numerical apertures.

physics.optics↗

arXiv2019

Excitation of whispering gallery modes with a "point-and-play", fiber-based, optical nano-antenna

We demonstrate the excitation and detection of whispering gallery modes in optical microresonators using a "point-and-play", fiber-based, optical nano-antenna. The coupling mechanism is based on cavity-enhanced Rayleigh scattering. Collected spectra exhibit Lorentzian dips, Fano shapes, or Lorentzian peaks, with a coupling efficiency around 13\%. The spectra are characterized by the coupling gap, polarization, and fiber tip position. The coupling method is simple, low-cost and, most importantly, the \textit{Q}-factor can be maintained at $10^8$ over a wide coupling range, thereby making it suitable for metrology, sensing, or cavity quantum electrodynamics (cQED) experiments.

physics.optics↗

arXiv2019

Complete polarization control for a nanofiber waveguide using directional coupling

Optical nanofiber waveguides are widely used for near-field delivery and measurement of light. Despite their versatility and efficiency, nanofibers have a critical drawback - their inability to maintain light's polarization state on propagation. Here, we design a directional coupler consisting of two crossed nanofibers to probe the polarization state at the waist region. Directionality of coupling occurs due to asymmetric dipolar emission or spin-locking when the evanescent field pattern breaks the mirror symmetry of the crossed-nanofiber system. We demonstrate that, by monitoring the outputs from the directional coupler, two non-orthogonal polarization states can be prepared at the nanofiber waist with a fidelity higher than 99%. Based on these states, we devise a simple and reliable method for complete control of the polarization along a nanofiber waveguide.

physics.optics↗

arXiv2018

A simple, narrow, and robust atomic frequency reference at 993 nm exploiting the rubidium (Rb) $5\mathit{S}_{1/2}$ to $6\mathit{S}_{1/2}$ transition using one-color two-photon excitation

We experimentally demonstrate a one-color two-photon transition from the $5\mathit{S}_{1/2}$ ground state to the $6\mathit{S}_{1/2}$ excited state in rubidium (Rb) vapor using a continuous wave laser at 993 nm. The Rb vapor contains both isotopes ($^{85}$Rb and $^{87}$Rb) in their natural abundances. The electric dipole allowed transitions are characterized by varying the power and polarization of the excitation laser. Since the optical setup is relatively simple, and the energies of the allowed levels are impervious to stray magnetic fields, this is an attractive choice for a frequency reference at 993 nm, with possible applications in precision measurements and quantum information processing.

physics.atom-ph↗

arXiv2018

Efficient Microparticle Trapping with Plasmonic Annular Apertures Arrays

In this work, we demonstrate trapping of microparticles using a plasmonic tweezers based on arrays of annular apertures. The transmission spectra and the E- field distribution are simulated to calibrate the arrays. Theoretically, we observe sharp peaks in the transmission spectra for dipole resonance modes and these are redshifted as the size of the annular aperture is reduced. We also expect an absorption peak at approximately 1,115 um for the localised plasmon resonance. Using a laser frequency between the two resonances, multiple plasmonic hotspots are created and used to trap and transport micron and submicron particles. Experimentally, we demonstrate trapping of individual 0.5 um and 1 um polystyrene particles and particle transportation over the surface of the annular apertures using less than 1.5 mW/um2 incident laser intensity at 980 nm.

physics.optics↗

arXiv2018

Tailoring a nanofiber for enhanced photon emission and coupling efficiency from single quantum emitters

We present a novel approach to enhance the spontaneous emission rate of single quantum emitters in an optical nanofiber-based cavity by introducing a narrow air-filled groove into the cavity. Our results show that the Purcell factor for single quantum emitters located inside the groove of the nanofiber-based cavity can be at least six times greater than that for such an emitter on the fiber surface when using an optimized cavity mode and groove width. Moreover, the coupling efficiency of single quantum emitters into the guided mode of this nanofiber-based cavity can reach up to $\sim$ 80 $\%$ with only 35 cavity-grating periods. This new system has the potential to act as an all-fiber platform to realize efficient coupling of photons from single emitters into an optical fiber for quantum information applications.

physics.optics↗

arXiv2016

Tunable erbium-doped microbubble laser fabricated by sol-gel coating

In this work, we show that the application of a sol-gel coating renders a microbubble whispering gallery resonator into an active device. During the fabrication of the resonator, a thin layer of erbium-doped sol-gel is applied to a tapered microcapillary, then a microbubble with a wall thickness of 1.3 $μ$m is formed with the rare earth diffused into its walls. The doped microbubble is pumped at 980 nm and lasing in the emission band of the Er$^{3+}$ ions with a wavelength of 1535 nm is observed. The laser wavelength can be tuned by aerostatic pressure tuning of the whispering gallery modes of the microbubble. Up to 240 pm tuning is observed with 2 bar of applied pressure. It is shown that the doped microbubble could be used as a compact, tunable laser source. The lasing microbubble can also be used to improve sensing capabilities in optofluidic sensing applications.

physics.optics↗

arXiv2016

Cavity ring-up spectroscopy for dissipative and dispersive sensing in a whispering gallery mode resonator

In whispering gallery mode resonator sensing applications, the conventional way to detect a change in the parameter to be measured is by observing the steady state transmission spectrum through the coupling waveguide. Alternatively, cavity ring-up spectroscopy (CRUS) sensing can be achieved transiently. In this work, we investigate CRUS using coupled mode equations and find analytical solutions with a large spectral broadening approximation of the input pulse. The relationships between the frequency detuning, coupling gap and ring-up peak height are determined and experimentally verified using an ultrahigh \textit{Q}-factor silica microsphere. This work shows that distinctive dispersive and dissipative transient sensing can be realised by simply measuring the peak height of the CRUS signal, which might improve the data collection rate.

physics.optics↗