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Søren V. Hoffmann

Publications and source records attributed to Søren V. Hoffmann.

2 recordsLinked to original sources

Micro- and nanoscale focusing across the XUV range of the ASTRID2 light source with a capillary optic

Focusing of synchrotron light across extreme ultraviolet (XUV) and soft X-ray regimes is increasingly desired for photoemission-based techniques where reduced beam width gives access to smaller samples such as microscopic single crystals and functioning two-dimensional (2D) heterostructures and devices. Many existing focusing methods, however, are not able to take full advantage of the synchrotron beam due to limited photon energy range or low transmission. Modern capillary optics have enabled achromatic, high transmission focusing of XUV and X-ray light. Here, we present a detailed characterisation of such an achromatic capillary optic installed at the AU-SGM4 beamline for spatial- and angle-resolved photoemission spectroscopy (ARPES) experiments at the ASTRID2 light source. The transmission of the capillary as a function of photon energy is given, and the dependence of the beam width, position, and transmission are measured against the source size. Analysis of the far-field image of the beam allows for slope errors on the inner surface of the capillary to be overcome by selectively aperturing the beam, resulting in a minimum beam width of 900 nm measured in a photoemission geometry.

physics.optics↗

A new endstation for extreme-ultraviolet spectroscopy of free clusters and nanodroplets

We present a new endstation for the AMOLine of the ASTRID2 synchrotron at Aarhus University, which combines a cluster and nanodroplet beam source with a velocity map imaging and time-of-flight spectrometer for coincidence imaging spectroscopy. Extreme-ultraviolet spectroscopy of free nanoparticles is a powerful tool for studying the photophysics and photochemistry of resonantly excited or ionized nanometer-sized condensed-phase systems. Here we demonstrate this capability by performing photoelectron-photoion coincidence (PEPICO) experiments with pure and doped superfluid helium nanodroplets. Different doping options and beam sources provide a versatile platform to generate various van der Waals clusters as well as He nanodroplets. We present a detailed characterization of the new setup and present examples of its use for measuring high-resolution yield spectra of charged particles, time-of-flight ion mass spectra, anion-cation coincidence spectra, multi-coincidence electron spectra and angular distributions. A particular focus of the research with this new endstation is on intermolecular charge and energy-transfer processes in heterogeneous nanosystems induced by valence-shell excitation and ionization.

physics.atm-clus↗