arXiv subjects

S. -I. Lee

Publications and source records attributed to S. -I. Lee.

At least 19 recordsLinked to original sources

arXiv2014

Small-Angle Neutron Scattering and Magnetization Study of HoNi2B2C

The superconducting and magnetic properties of HoNi2B2C single crystals are investigated through transport, magnetometry and small-angle neutron scattering measurements. In the magnetic phases that enter below the superconducting critical temperature, the small-angle neutron scattering data uncover networks of magnetic surfaces. These likely originate from uncompensated moments e.g. at domain walls pinned to crystallographic grain boundaries. The field and temperature dependent behaviour appears consistent with the metamagnetic transitions reported in earlier works.

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arXiv2011

Momentum-space electronic structures and charge orders of high-temperature superconductors Ca2-xNaxCuO2Cl2 and Bi2Sr2CaCu2O8+delta

We study the electronic structure of Ca2-xNaxCuO2Cl2 and Bi2Sr2CaCu2O8+d samples in a wide range of doping, using angle-resolved photoemission spectroscopy, with emphasis on on the Fermi surface (FS) in the near anti-nodal region. The "nesting wave vector", i.e., the wave vector that connects two nearly flat pieces of the Fermi surface in the anti-nodal region, reveals a universal monotonic decrease in magnitude as a function of doping. Comparing our results to the charge order recently observed by scanning tunneling spectroscopy (STS), we conclude that the FS nesting and the charge order pattern seen in STS do not have a direct relationship. Therefore,the charge order likely arises due to strong correlation physics rather than FS nesting physics.

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arXiv2011

Superconducting energy gap in MgCNi3 single crystals: Point-contact spectroscopy and specific-heat measurements

Specific heat has been measured down to 600 mK and up to 8 Tesla by the highly sensitive AC microcalorimetry on the MgCNi3 single crystals with Tc ~ 7 K. Exponential decay of the electronic specific heat at low temperatures proved that a superconducting energy gap is fully open on the whole Fermi surface, in agreement with our previous magnetic penetration depth measurements on the same crystals. The specific-heat data analysis shows consistently the strong coupling strength 2D/kTc ~ 4. This scenario is supported by the direct gap measurements via the point-contact spectroscopy. Moreover, the spectroscopy measurements show a decrease in the critical temperature at the sample surface accounting for the observed differences of the superfluid density deduced from the measurements by different techniques.

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arXiv2010

Superconducting order parameter in nonmagnetic borocarbides RNi$_{2}$B$_{2}$C (R=Y, Lu) probed by point-contact Andreev reflection spectroscopy

We report on the measurements of the superconducting order parameter in the nonmagnetic borocarbides LuNi$_2$B$_2$C and YNi$_2$B$_2$C. Andreev conductance spectra are obtained from nanoscale metallic junctions on single crystal surfaces prepared along three major crystallographic orientations: [001], [110], and [100]. The gap values extracted by the single-gap Blonder-Tinkham-Klapwijk model follow the BCS predictions as a function of temperature and magnetic field and exhibit a small anisotropy. These observations are robust and reproducible among all the measurements on two different sets of LuNi$_2$B$_2$C crystals and one set of YNi$_2$B$_2$C crystals. We suggest possible explanations for the small gap anisotropy based on the recent detailed gap measurements by angle-resolved photoemission spectroscopy and the tunneling cone effect. Our results provide a consistent picture of the superconducting gap structure in these materials, addressing the controversy particularly in the reported results of point-contact Andreev reflection spectroscopy.

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arXiv2010

Comparative study of the pressure effects on the magnetic penetration depth in electron- and hole-doped cuprate superconductors

The effect of pressure on the magnetic penetration depth $λ$ was tested in the hole-doped superconductor YBa2Cu3O(7-d) and in the electron-doped one Sr0.9La0.1CuO2 by means of magnetization measurements. Whereas a large change of $λ$ was found in YBa2Cu3O(7-d), confirming the non-adiabatic character of the electron-phonon coupling in hole-doped superconductors, the same quantity is not affected by pressure in the electron-doped Sr0.9La0.1CuO2, suggesting a close similarity of the latter to conventional adiabatic BCS superconductors. The present results imply a remarkable difference between the electronic properties of hole-doped cuprates and the electron-doped Sr0.9La0.1CuO2, giving a strong contribution to the long debated asymmetric consequences of hole- and electron-doping in cuprate superconductors.

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arXiv2010

Different Evolution of Intrinsic Gap in Kondo Semiconductors SmB6 and YbB12

Dependence of the spectral functions on temperature and rare-earth substitution was examined in detail for Kondo semiconductor alloys Sm1-xEuxB6 and Yb1-xLuxB12 by bulk-sensitive photoemission. It is found that the 4f lattice coherence and intrinsic (small) energy gap are robust for SmB6 against the Eu substitution up to x = 0.15 while both collapse by Lu substitution already at x = 0.125 for YbB12. Our results suggest that the mechanism of the intrinsic gap formation is different between SmB6 and YbB12 although they were so far categorized in the same kind of Kondo semiconductors.

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arXiv2008

Observation of vortices and hidden pseudogap from scanning tunneling spectroscopic studies of electron-doped cuprate superconductor $Sr_{0.9}La_{0.1}CuO_2$

We present the first demonstration of vortices in an electron-type cuprate superconductor, the highest $T_c$ (= 43 K) electron-type cuprate $Sr_{0.9}La_{0.1}CuO_2$. Our spatially resolved quasiparticle tunneling spectra reveal a hidden low-energy pseudogap inside the vortex core and unconventional spectral evolution with temperature and magnetic field. These results cannot be easily explained by the scenario of pure superconductivity in the ground state of high-$T_c$ superconductivity.

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arXiv2008

Role of bosonic modes in the mechanism of high temperature Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$ superconductors using ultrafast optical techniques

Using ultrafast optical techniques, we probe the hole-doping dependence of the electron-boson coupling constant $λ$ in Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$. In the overdoped region, we observe a correlation between ($λ$) and the superconducting transition temperature $T_{c}$. Upon performing the McMillan analysis, however, we find that $λ$ is too small to explain the high $T_{c}$'s, and that the Coulomb pseudopotential $μ^{\ast}$ is negative. Our analysis therefore reveals two components in the mechanism of high-$T_{c}$ superconductivity -- a dominant pre-existing pairing interaction, together with a weaker electron-phonon interaction that fine-tunes $T_{c}$.

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arXiv2008

Nodeless superconductivity in the infinite-layer electron-doped Sr_0.9La_0.1CuO_2 cuprate superconductor

We report on measurements of the in-plane magnetic penetration depth λ_{ab} in the infinite-layer electron-doped high-temperature cuprate superconductor Sr_0.9La_0.1CuO_2 by means of muon-spin rotation. The observed temperature and magnetic field dependences of λ_{ab} are consistent with the presence of a substantial s-wave component in the superconducting order parameter in good agreement with the results of tunneling, specific heat, and small-angle neutron scattering experiments.

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arXiv2007

Torque magnetometry studies of new low temperature metamagnetic states in ErNi_{2}B_{2}C

The metamagnetic transitions in single-crystal ErNi$_2$B$_2$C have been studied at 1.9 K with a Quantum Design torque magnetometer. The critical fields of the transitions depend crucially on the angle between applied field and the easy axis [100]. Torque measurements have been made while changing angular direction of the magnetic field (parallel to basal tetragonal $ab$-planes) in a wide angular range (more than two quadrants). Sequences of metamagnetic transitions with increasing field are found to be different for the magnetic field along (or close enough to) the easy [100] axis from that near the hard [110] axis. The study have revealed new metamagnetic states in ErNi$_{2}$B$_2$C which were not apparent in previous longitudinal-magnetization and neutron studies.

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arXiv2007

Macroscopic evidence for quantum criticality and field-induced quantum fluctuations in cuprate superconductors

We present macroscopic experimental evidence for field-induced microscopic quantum fluctuations in different hole- and electron-type cuprate superconductors with varying doping levels and numbers of CuO$_2$ layers per unit cell. The significant suppression of the zero-temperature in-plane magnetic irreversibility field relative to the paramagnetic field in all cuprate superconductors suggests strong quantum fluctuations due to the proximity of the cuprates to quantum criticality.

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arXiv2007

Observation of Competing Order in a High-$T_{c}$ Superconductor with Femtosecond Optical Pulses

We present studies of the photoexcited quasiparticle dynamics in Tl$_{2}$Ba$_{2}$Ca$_{2}$Cu$_{3}$O$_{y}$ (Tl-2223) using femtosecond optical techniques. Deep into the superconducting state (below 40 K), a dramatic change occurs in the temporal dynamics associated with photoexcited quasiparticles rejoining the condensate. This is suggestive of entry into a coexistence phase which, as our analysis reveals, opens a gap in the density of states (in addition to the superconducting gap), and furthermore, competes with superconductivity resulting in a depression of the superconducting gap.

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arXiv2006

Investigating the Physical Origin of Unconventional Low-Energy Excitations and Pseudogap Phenomena in Cuprate Superconductors

We investigate the physical origin of unconventional low-energy excitations in cuprate superconductors by considering the effect of coexisting competing orders (CO) and superconductivity (SC) and of quantum fluctuations and other bosonic modes on the low-energy charge excitation spectra. By incorporating both SC and CO in the bare Green's function and quantum phase fluctuations in the self-energy, we can consistently account for various empirical findings in both the hole- and electron-type cuprates, including the excess subgap quasiparticle density of states, ``dichotomy'' in the fluctuation-renormalized quasiparticle spectral density in momentum space, and the occurrence and magnitude of a low-energy pseudogap being dependent on the relative gap strength of CO and SC. Comparing these calculated results with experiments of ours and others, we suggest that there are two energy scales associated with the pseudogap phenomena, with the high-energy pseudogap probably of magnetic origin and the low-energy pseudogap associated with competing orders.

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arXiv2005

Torque magnetometry studies of metamagnetic transitions in single-crystal HoNi_{2}B_{2}C and ErNi_{2}B_{2}C at T\approx 1.9 K

The metamagnetic transitions in single-crystal rare-earth nickel borocarbide HoNi_{2}B_{2}C and ErNi_{2}B_{2}C have been studied at 1.9 K with a Quantum Design torque magnetometer. The critical fields of the transitions depend crucially on the angle between applied field and the easy axis [110] for HoNi_2B_2C and [100] for ErNi_2B_2C. Torque measurements have been made while changing angular direction of the magnetic field (parallel to basal tetragonal ab-planes) in a wide angular range (more than two quadrants). The results are used not only to check and refine the angular diagram for metamagnetic transitions in these compounnds, but also to find new features of the metamagnetic states. Among new results for the Ho borocarbide are the influence of a multidomain antiferromagnetic state, and ``frustrated'' behavior of the magnetic system for field directions close to the hard axis [100]. Torque measurements of the Er borocarbide clearly show that the sequence of metamagnetic transitions with increasing field (and the corresponding number of metamagnetic states) depends on the angular direction of the magnetic field relative to the easy axis.

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arXiv2004

Elastic anomalies in HoNi2B2C single crystals

We have measured temperature and magnetic field dependencies of the sound velocities and the sound attenuation in HoNi2B2C single crystals. The main result is a huge softening the velocity of C66 mode due to a cooperative Jahn-Teller effect, resulting in a tetragonal-orthorhombic structural phase transition. Anomalies in the behavior of the C66 mode through various magnetic phase transitions permit us to revise the low temperature H-T phase diagrams of this compound.

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arXiv2004

Experimental Investigation of the Competing Orders and Quantum Criticality in Hole- and Electron-Doped Cuprate Superconductors

We investigate the issues of competing orders and quantum criticality in cuprate superconductors via experimental studies of the high-field thermodynamic phase diagrams and the quasiparticle tunneling spectroscopy. Our results suggest substantial field-induced quantum fluctuations in all cuprates investigated, and their correlation with quasiparticle spectra implies that both electron- (n-type) and hole-doped (p-type) cuprate superconductors are in close proximity to a quantum critical point that separates a pure superconducting (SC) phase from a phase consisting of coexisting SC and a competing order. We further suggests that the relevant competing order is likely a spin-density wave (SDW) or a charge density wave (CDW), which can couple to an in-plane Cu-O bond stretching longitudinal optical (LO) phonon mode in the p-type cuprates but not in the n-type cuprates. This cooperative interaction may account for the pseudogap phenomenon above Tc only in the p-type cuprate superconductors.

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arXiv2004

Quasiparticle spectroscopy and high-field phase diagrams of cuprate superconductors -- An investigation of competing orders and quantum criticality

We present scanning tunneling spectroscopic and high-field thermodynamic studies of hole- and electron-doped (p- and n-type) cuprate superconductors. Our experimental results are consistent with the notion that the ground state of cuprates is in proximity to a quantum critical point (QCP) that separates a pure superconducting (SC) phase from a phase comprised of coexisting SC and a competing order, and the competing order is likely a spin-density wave (SDW). The effect of applied magnetic field, tunneling current, and disorder on the revelation of competing orders and on the low-energy excitations of the cuprates is discussed.

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arXiv2004

Dimensionality of superconductivity in the infinite-layer high-temperature cuprate Sr0.9M0.1CuO2 (M = La, Gd)

The high magnetic field phase diagram of the electron-doped infinite layer high-temperature superconducting (high-T_c) compound Sr_{0.9}La_{0.1}CuO_2 was probed by means of penetration depth and magnetization measurements in pulsed fields to 60 T. An anisotropy ratio of 8 was detected for the upper critical fields with H parallel (H_{c2}^{ab}) and perpendicular (H_{c2}^c) to the CuO_2 planes, with H_{c2}^{ab} extrapolating to near the Pauli paramagnetic limit of 160 T. The longer superconducting coherence length than the lattice constant along the c-axis indicates that the orbital degrees of freedom of the pairing wavefunction are three dimensional. By contrast, low-field magnetization and specific heat measurements of Sr_{0.9}Gd_{0.1}CuO_2 indicate a coexistence of bulk s-wave superconductivity with large moment Gd paramagnetism close to the CuO_2 planes, suggesting a strong confinement of the spin degrees of freedom of the Cooper pair to the CuO_2 planes. The region between H_{c2}^{ab} and the irreversibility line in the magnetization, H_{irr}^{ab}, is anomalously large for an electron-doped high-T_c cuprate, suggesting the existence of additional quantum fluctuations perhaps due to a competing spin-density wave order.

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