arXiv subjects

S. A. Gillespie

Publications and source records attributed to S. A. Gillespie.

14 recordsLinked to original sources

arXiv2026

Rapid structural evolution of neutron-rich silicon isotopes toward N = 28

Neutron-rich Si isotopes represent a unique case of shell evolution, exhibiting a robust shell closure at $N=20$ and pronounced quadrupole collectivity at $N = 28$. We report lifetime measurements of excited states in $^{40}$Si and the first simultaneous lifetime and heavy-ion inelastic-scattering measurements in $^{41}$Si. In $^{40}$Si, the extracted lifetimes for the $2_1^+$ and $(2_2^+)$ states indicate moderate quadrupole collectivity at $N=26$, together with signatures of triaxiality. In $^{41}$Si, two near-degenerate states at 570 and 658~keV exhibit comparable $B(E2)$ strengths as extracted from inelastic scattering, while the measured lifetimes indicate dominant $M1$ decays. The combined lifetime and inelastic-scattering results suggest an evolution toward oblate shape, consistent with large-scale shell-model predictions.

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arXiv2025

Determination of proton and neutron contributions to the $0_{g.s.}^+ \rightarrow 2_1^+$ excitations in $^{42}$Si and $^{44}$S using inelastic proton scattering in inverse kinematics and intermediate energy Coulomb excitation

We have measured the $0_{g.s.}^+ \rightarrow 2_1^+$ transition in the neutron rich $N=28$ isotope $^{42}$Si using the probes of intermediate energy Coulomb excitation and inelastic proton scattering in inverse kinematics at the Facility for Rare Isotope Beams with beam particle rates of $\approx 5$ particles/s. The results of these two measurements allowed us to determine $M_n/M_p$, the ratio of the neutron and proton transition matrix elements for the $0_{g.s.}^+ \rightarrow 2_1^+$ transition. In addition, we have measured the $0_{\mathrm{g.s.}}^+ \rightarrow 2_1^+$ transition in the isotone $^{44}$S using inverse kinematics inelastic proton scattering. By comparing the $^{44}$S proton scattering result with a recent intermediate energy Coulomb excitation result on the same transition, we were able to determine $M_n/M_p$ for the $0_{g.s.}^+ \rightarrow 2_1^+$ transition in this nucleus as well. This work strengthens the evidence that $^{42}$Si has a stable quadrupole deformation in its ground state and that $^{44}$S does not. Both conclusions are further supported by shell model calculations carried out with the FSU interaction.

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arXiv2024

In-beam $γ$-ray spectroscopy towards the proton dripline: The curious case of $^{32}$Ar

High-resolution in-beam $γ$-ray spectroscopy was used to study excited states of the neutron-deficient nucleus $^{32}$Ar populated in fast-beam induced four- and six-nucleon removal reactions from $^{36,38}$Ca. One new $γ$-ray transition and indications for an additional two were found, allowing for a glimpse at the level scheme beyond the known $2^+_1$ state. The nature of the new $1900(4)$-keV transition is discussed in the context of the known energy spectrum of the mirror nucleus $^{32}$Si and shell-model calculations using the FSU and SDPF-M cross-shell effective interactions. Its resulting parent state at $3767(5)$ keV, more than $1.3$ MeV above the proton separation energy, is tentatively assigned to have mixed sd-shell and $2p$-$2h$ character. It might either be the mirror of the $J^π=2^+_2$ state of $^{32}$Si at $4230.8(8)$ keV, but with a decay branch favoring a transition to the $2^+_1$ over the ground state, or the mirror of the $4983.9(11)$-keV state with quantum numbers $0^+$. The resulting mirror-energy differences of $-473(5)$ and $-1218(5)$ keV are both sizable when compared to systematics; in the latter case it would, in fact, be among the largest reported to date in the entire nuclear chart or suggest the potential existence of an additional, hitherto unidentified, low-lying $0^+$ state of $^{32}$Si.

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arXiv2024

In-beam $γ$-ray spectroscopy of negative-parity states of $^{37}$K populated in dissipative reactions

In-beam $γ$-ray spectroscopy was used to study excited states of the neutron-deficient nucleus $^{37}$K populated in fast-beam inelastic-scattering and proton-removal reactions at high-momentum loss. New $γ$-ray transitions and $γγ$ coincidence relationships were established using the $γ$-ray tracking array GRETINA. The extension of the level scheme up to the first $(13/2^-)$ state highlights the potential of this recently demonstrated population pathway for studies of isospin symmetry involving mirror-energy differences. The nature of the newly identified states is discussed in comparison to shell-model calculations with the FSU cross-shell effective interaction. The calculated occupation numbers of individual orbitals are shown to offer a consistent explanation of the measured mirror-energy differences between $^{37}$K and $^{37}$Ar.

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arXiv2024

Coulomb Excitation of $^{80}$Sr and the limits of the $N = Z = 40$ island of deformation

The region of $N\approx Z\approx 40$ has long been associated with strongly deformed nuclear configurations. The presence of this strong deformation was recently confirmed through lifetime measurements in $N\approx Z$ Sr and Zr nuclei. Theoretically, however, these nuclei present a challenge due to the vast valence space required to incorporate all deformation driving interactions. Recent state-of-the-art predictions indicate a near axial prolate deformation for $N=Z$ and $N=Z+2$ nuclei between $N=Z=36$ and $N=Z=40$. In this work we investigate the shores of this island of deformation through a sub-barrier Coulomb excitation study of the $N=Z+4$ nucleus, \textsuperscript{80}Sr. Extracting a spectroscopic quadrupole moment of $Q_s(2^+_1) = 0.45^{+0.83}_{-0.88}$~eb, we find that \textsuperscript{80}Sr is inconsistent with significant axial prolate deformation. This indicates that the predicted region of strong prolate deformation around $N=Z=40$ is tightly constrained to the quartet of nuclei: \textsuperscript{76,78}Sr and \textsuperscript{78,80}Zr.

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arXiv2024

Probing proton cross-shell excitations through the two-neutron removal from 38Ca

Bound states of the neutron-deficient, near-dripline nucleus $^{36}$Ca were populated in two-neutron removal from the ground state of $^{38}$Ca, a direct reaction sensitive to the single-particle configurations and couplings of the removed neutrons in the projectile wave function. Final-state exclusive cross sections for the formation of $^{36}$Ca and the corresponding longitudinal momentum distributions, both determined through the combination of particle and $γ$-ray spectroscopy, are compared to predictions combining eikonal reaction theory and shell-model two-nucleon amplitudes from the USDB, USDC, and ZBM2 effective interactions. The final-state cross-section ratio $σ(2^+_1)/σ(0^+)$ shows particular sensitivity and is approximately reproduced only with the two-nucleon amplitudes from the ZBM2 effective interaction that includes proton cross-shell excitations into the $pf$ shell. Characterizing the proton $pf$-shell occupancy locally and schematically, an increase of the $sd$-$pf$ shell gap by $250$ keV yields an improved description of this cross-section ratio and simultaneously enables a reproduction of the $B(E2;0^+_1\to2^+_1)$ excitation strength of $^{36}$Ca. This highlights an important aspect if a new shell-model effective interaction for the region was to be developed on the quest to model the neutron-deficient Ca isotopes and surrounding nuclei whose structure is impacted by proton cross-shell excitations.

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arXiv2024

Cross-shell excited configurations in the structure of 34Si

The cross-shell excited states of $^{34}$Si have been investigated via $β$-decays of the $4^-$ ground state and the $1^+$ isomeric state of $^{34}$Al. Since the valence protons and valence neutrons occupy different major shells in the ground state as well as the intruder $1^+$ isomeric state of $^{34}$Al, intruder levels of $^{34}$Si are populated via allowed $β$ decays. Spin assignments to such intruder levels of $^{34}$Si were established through $γ$-$γ$ angular correlation analysis for the negative parity states with dominant configurations $(νd_{3/2})^{-1} \otimes (νf_{7/2})^{1}$ as well as the positive parity states with dominant configurations $(νsd)^{-2} \otimes (νf_{7/2}p_{3/2})^2$. The configurations of such intruder states play crucial roles in our understanding of the $N=20$ shell gap evolution. A configuration interaction model derived from the FSU Hamiltonian was utilized in order to interpret the intruder states in $^{34}$Si. Shell model interaction derived from a more fundamental theory with the Valence Space In Medium Similarity Renormalization Group (VS-IMSRG) method was also employed to interpret the structure of $^{34}$Si.

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arXiv2023

Decay Spectroscopy of $^{160}$Eu: Quasiparticle Configurations of Excited States and Structure of $K^π$=$4^+$ Band-heads in $^{160}$Gd

\noindent \textbf{Background:} Detailed spectroscopy of neutron-rich, heavy, deformed nuclei is of broad interest for nuclear astrophysics and nuclear structure. Nuclei in the r-process path and following freeze-out region impact the resulting r-process abundance distribution, and the structure of nuclei midshell in both proton and neutron number helps to understand the evolution of subshell gaps and large deformation in these nuclei. \noindent \textbf{Purpose:} To improve the understanding of the nuclear structure of $^{160}$Gd, specifically the $K^π$=$4^+$ bands, as well as study the $β$-decay of $^{160}$Eu into $^{160}$Gd. \noindent \textbf{Methods:} High-statistics decay spectroscopy of $^{160}$Gd resulting from the $β$-decay of $^{160}$Eu was collected using the GRIFFIN spectrometer at the TRIUMF-ISAC facility. \noindent \textbf{Results:} Two new excited states and ten new transitions were observed in $^{160}$Gd. The $β$-decaying half-lives of the low- and high-spin isomer in $^{160}$Eu were determined, and the low-spin state's half-life was measured to be $t_{1/2}=26.0(8)$~s, $\sim$16\% shorter than previous measurements. Lifetimes of the two $K^π$=$4^+$ band-heads in $^{160}$Gd were measured for the first time, as well as $γ$-$γ$ angular correlations and mixing ratios of intense transitions out of those band-heads. \noindent \textbf{Conclusions:} Lifetimes and mixing ratios suggest that the hexadecapole phonon model of the $K^π$=$4^+$ band-heads in $^{160}$Gd is preferred over a simple two-state strong mixing scenario, although further theoretical calculations are needed to fully understand these states. Additionally, the 1999.0 keV state in $^{160}$Gd heavily populated in $β$-decay is shown to have positive parity, which raises questions regarding the structure of the high-spin $β$-decaying state in $^{160}$Eu.

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arXiv2023

Cross Sections of the $^{83}$Rb(p,$γ)^{84}$Sr and $^{84}$Kr(p,$γ)^{85}$Rb Reactions at Energies Characteristic of the Astrophysical $γ$ Process

We have measured the cross section of the $^{83}$Rb(p,$γ)^{84}$Sr radiative capture reaction in inverse kinematics using a radioactive beam of $^{83}$Rb at incident energies of 2.4 and $2.7 A$ MeV. Prior to the radioactive beam measurement, the $^{84}$Kr(p,$γ)^{85}$Rb radiative capture reaction was measured in inverse kinematics using a stable beam of $^{84}$Kr at an incident energy of $2.7 A$ MeV. The effective relative kinetic energies of these measurements lie within the relevant energy window for the $γ$ process in supernovae. The central values of the measured partial cross sections of both reactions were found to be $0.17-0.42$ times the predictions of statistical model calculations. Assuming the predicted cross section at other energies is reduced by the same factor leads to a slightly higher calculated abundance of the $p$ nucleus $^{84}$Sr, caused by the reduced rate of the $^{84}$Sr($γ$,p)$^{83}$Rb reaction derived from the present measurement.

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arXiv2022

Single neutron transfer on 23Ne and its relevance forthepathway ofnucleosynthesis in astrophysical X-ray bursts

We present new experimental measurements of resonance strengths in the astrophysical 23Al(p, γ)24Si reaction, constraining the pathway of nucleosynthesis beyond 22Mg in X-ray burster scenarios. Specifically, we have performed the first measurement of the (d, p) reaction using a radioactive beam of 23Ne to explore levels in 24Ne, the mirror analog of 24Si. Four strong single-particle states were observed and corresponding neutron spectroscopic factors were extracted with a precision of {\sim}20{\%}. Using these spectroscopic factors, together with mirror state identifications, we have reduced uncertainties in the strength of the key {\ell} = 0 resonance at Er= 157 keV, in the astrophysical 23Al(p, γ) reaction, by a factor of 4. Our results show that the 22Mg(p, γ)23Al(p, γ) pathway dominates over the competing 22Mg(α, p) reaction in all but the most energetic X-ray burster events (T>0.85GK), significantly affecting energy production and the preservation of hydrogen fuel.

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arXiv2022

Improved measurement of the $0_2^+\rightarrow0_1^+$ E0 transition strength for $^{72}$Se using the SPICE spectrometer

The selenium isotopes lie at the heart of a tumultuous region of the nuclear chart where shape coexistence effects grapple with neutron-proton pairing correlations, triaxiality, and the impending proton dripline. In this work a study of $^{72}$Se by internal conversion electron and $γ$-ray spectroscopy was undertaken with the SPICE and TIGRESS arrays. New measurements of the branching ratio and lifetime of the $0_2^+$ state were performed yielding a determination of $ρ^2(E0;0_2^+{\rightarrow}0_1^+)=29(3)$ milliunits. two state mixing calculations were performed that highlighted the importance of interpretation of such $E0$ strength values in the context of shape-coexistence.

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arXiv2021

First Direct Measurement of an Astrophysical p-Process Reaction Cross Section Using a Radioactive Ion Beam

We have performed the first direct measurement of the 83Rb(p,g) radiative capture reaction cross section in inverse kinematics using a radioactive beam of 83Rb at incident energies of 2.4 and 2.7 A MeV. The measured cross section at an effective relative kinetic energy of Ecm = 2.393 MeV, which lies within the relevant energy window for core collapse supernovae, is smaller than the prediction of statistical model calculations. This leads to the abundance of 84Sr produced in the astrophysical p process being higher than previously calculated. Moreover, the discrepancy of the present data with theoretical predictions indicates that further experimental investigation of p-process reactions involving unstable projectiles is clearly warranted.

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arXiv2021

Charged-particle branching ratios above the neutron threshold in $^{19}$F: constraining $^{15}$N production in core-collapse supernovae

Spatially-correlated overabundances of $^{15}$N and $^{18}$O observed in some low-density graphite meteoritic grains have been connected to nucleosynthesis taking place in the helium-burning shell during core-collapse supernovae. Two of the reactions which have been identified as important to the final abundances of $^{15}$N and $^{18}$O are $^{18}$F($n,α$)$^{15}$N and $^{18}$F($n,p$)$^{18}$O. The relative strengths of the $^{18}$F($n,α$)$^{15}$N and $^{18}$F($n,p$)$^{18}$O reactions depend on the relative $α_0$ and $p_0$ decays from states above the neutron threshold in $^{19}$F in addition to other properties. Experimental data on the charged-particle decays from these highly excited states are lacking or inconsistent. Two experiments were performed using proton inelastic scattering from LiF targets and magnetic spectrographs. The first experiment used the high-resolution Q3D spectrograph at Munich to constrain properties of levels in $^{19}$F. A second experiment using the Orsay Split-Pole spectrograph and an array of silicon detectors was performed in order to measure the charged-particle decays of neutron-unbound levels in $^{19}$F. A number of levels in $^{19}$F have been identified along with their corresponding charged-particle decays. The first state above the neutron threshold which has an observed proton-decay branch to the ground state of $^{18}$O lies 68 keV above the neutron threshold while the $α$-particle decays from the neutron-unbound levels are generally observed to be much stronger than the proton decays. Neutron-unbound levels in $^{19}$F are observed to decay predominantly by $α$-particle emission, supporting the role of $^{18}$F($n,α$)$^{15}$N in the production of $^{15}$N in the helium-burning shell of supernovae. Improved resonant-scattering reaction data are required in order to be able to determine the reaction rates accurately.

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arXiv2020

Sub-threshold states in $^{19}$Ne relevant to $^{18}$F(p,$α$)$^{15}$O

Classical novae result from thermonuclear explosions producing several $γ$-ray emitters which are prime targets for satellites observing in the MeV range. The early 511 keV gamma-ray emission depends critically on the $^{18}$F(p,$α$)$^{15}$O reaction rate which, despite many experimental and theoretical efforts, still remains uncertain. One of the main uncertainties in the $^{18}$F(p,$α$)$^{15}$O reaction rate is the contribution in the Gamow window of interference between sub-threshold $^{19}$Ne states and known broad states at higher energies. Therefore the goal of this work is to clarify the existence and the nature of these sub-threshold states. States in the $^{19}$Ne compound nucleus were studied at the Tandem-ALTO facility using the $^{19}$F($^3$He,t)$^{19}$Ne charge exchange reaction. Tritons were detected with an Enge Split-pole spectrometer while decaying protons or $α$-particles from unbound $^{19}$Ne states were collected, in coincidence, with a double-sided silicon strip detector array. Angular correlations were extracted and constraints on the spin and parity of decaying states established. The coincidence yield at $E_x$ = 6.29 MeV was observed to be high spin, supporting the conclusion that it is indeed a doublet consisting of high spin and low spin components. Evidence for a broad, low spin state was observed around 6 MeV. Branching ratios were extracted for several states above the proton threshold and were found to be consistent with the literature. R-matrix calculations show the relative contribution of sub-threshold states to the astrophysically important energy region above the proton threshold. The levels schemes of $^{19}$Ne and $^{19}$F are still not sufficiently well known and further studies of the analogue assignments are needed. The tentative broad state at 6 MeV may only play a role if the reduced proton width is large.

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