arXiv subjects

S. A. Maier

Publications and source records attributed to S. A. Maier.

17 recordsLinked to original sources

arXiv2026

Programmable Synthetic Motion at a Time-Varying Interface

Space-time metamaterials that exhibit synthetic motion promise arbitrary control over the momentum, frequency and energy of scattered light, but realising the required space-time modulation in a programmable way remains a challenge. Here we program synthetic motion using a single spatial light modulator in a 4f geometry which imprints a continuously tunable pulse-front tilt onto a high-intensity pump pulse, inducing reflectivity modulations at a sub-wavelength indium tin oxide thin film with synthetic velocities spanning the sub- and superluminal regimes. The angle-resolved spectrum of a scattered probe pulse reveals space-time diffraction patterns whose gradient and bandwidth vary continuously with synthetic velocity, in excellent agreement with theory. Splitting the shaped pump into two independently controlled pulses yields space-time double-slit diffraction with tunable fringe separation and frequency-momentum gradient. This programmable platform opens a path towards non-linear and periodic space-time trajectories for tabletop analogue studies of relativistic phenomena and space-time metasurfaces.

physics.optics↗

arXiv2025

Tunable negative permeability in a quantum plasmonic metamaterial

We consider the integration of quantum emitters into a negative permeability metamaterial design in order to introduce tunability as well as nonlinear behavior. The unit cell of our metamaterial is a ring of metamolecules, each consisting of a metal nanoparticle and a two-level semiconductor quantum dot (QD). Without the QDs, the ring of the unit cell is known to act as an artificial optical magnetic resonator. By adding the QDs we show that a Fano interference profile is introduced into the magnetic field scattered from the ring. This induced interference is shown to cause an appreciable effect in the collective magnetic resonance of the unit cell. We find that the interference provides a means to tune the response of the negative permeability metamaterial. The exploitation of the QD's inherent nonlinearity is proposed to modulate the metamaterial's magnetic response with a separate control field.

quant-ph↗

arXiv2025

Space-Time Optical Diffraction from Synthetic Motion

The interaction of light with objects and media moving at relativistic and superluminal speeds enables unconventional phenomena such as Fresnel drag, Hawking radiation, and light amplification. Synthetic motion, facilitated by modulated internal degrees of freedom, enables the study of relativistic phenomena unrestricted by the speed of light. In this study, we investigate synthetically moving apertures created by high-contrast reflectivity modulations, which are generated by ultrafast laser pulses on a subwavelength thin film of indium tin oxide. The space-time diffraction of a weaker probe beam reveals a complex, non-separable spatio-temporal transformation, where changes in the frequency of the wave are correlated to changes in its momentum. By using schemes of continuous or discrete modulation we demonstrate tunable frequency-momentum diffraction patterns with gradients that depend upon the relative velocity between the modulation and the probe wave. The diffraction patterns are matched by operator-based theory and the gradients are analytically predicted using a super-relativistic Doppler model, where the modulation is described as a superluminally moving scattering particle. Our experiments open a path towards mimicking relativistic mechanics and developing complex and programmable spatio-temporal transformations of light.

physics.optics↗

arXiv2019

Enhanced light-matter interaction in an atomically thin semiconductor coupled with dielectric nano-antennas

Unique structural and optical properties of atomically thin two-dimensional semiconducting transition metal dichalcogenides enable in principle their efficient coupling to photonic cavities with optical modes volumes close to or below the diffraction limit. Recently, it has become possible to make all-dielectric nano-cavities with reduced mode volumes and negligible non-radiative losses. Here, we realise low-loss high-refractive-index dielectric gallium phosphide (GaP) nano-antennas with small mode volumes coupled to atomic mono- and bilayers of WSe$_2$. We observe a photoluminescence enhancement exceeding 10$^4$ compared with WSe$_2$ placed on planar GaP, and trace its origin to a combination of enhancement of the spontaneous emission rate, favourable modification of the photoluminescence directionality and enhanced optical excitation efficiency. A further effect of the coupling is observed in the photoluminescence polarisation dependence and in the Raman scattering signal enhancement exceeding 10$^3$. Our findings reveal dielectric nano-antennas as a promising platform for engineering light-matter coupling in two-dimensional semiconductors.

physics.app-ph↗

arXiv2019

Negative refraction in time-varying, strongly-coupled plasmonic antenna-ENZ systems

Time-varying metasurfaces are emerging as a powerful instrument for the dynamical control of the electromagnetic properties of a propagating wave. Here we demonstrate an efficient time-varying metasurface based on plasmonic nano-antennas strongly coupled to an epsilon-near-zero (ENZ) deeply sub-wavelength film. The plasmonic resonance of the metal resonators strongly interacts with the optical ENZ modes, providing a Rabi level spitting of ~30%. Optical pumping at frequency ω induces a nonlinear polarisation oscillating at 2ω responsible for an efficient generation of a phase conjugate and a negative refracted beam with a conversion efficiency that is more than four orders of magnitude greater compared to the bare ENZ film. The introduction of a strongly coupled plasmonic system therefore provides a simple and effective route towards the implementation of ENZ physics at the nanoscale

physics.optics↗

arXiv2017

Experimental verification of entanglement generated in a plasmonic system

A core process in many quantum tasks is the generation of entanglement. It is being actively studied in a variety of physical settings - from simple bipartite systems to complex multipartite systems. In this work we experimentally study the generation of bipartite entanglement in a nanophotonic system. Entanglement is generated via the quantum interference of two surface plasmon polaritons in a beamsplitter structure, i.e. utilising the Hong-Ou-Mandel (HOM) effect, and its presence is verified using quantum state tomography. The amount of entanglement is quantified by the concurrence and we find values of up to 0.77 +/- 0.04. Verifying entanglement in the output state from HOM interference is a nontrivial task and cannot be inferred from the visibility alone. The techniques we use to verify entanglement could be applied to other types of photonic system and therefore may be useful for the characterisation of a range of different nanophotonic quantum devices.

quant-ph↗

arXiv2016

High-performance functional renormalization group calculations for interacting fermions

We derive a novel computational scheme for functional Renormalization Group (fRG) calculations for interacting fermions on 2D lattices. The scheme is based on the exchange parametrization fRG for the two-fermion interaction, with additional insertions of truncated partitions of unity. These insertions decouple the fermionic propagators from the exchange propagators and lead to a separation of the underlying equations. We demonstrate that this separation is numerically advantageous and may pave the way for refined, large-scale computational investigations even in the case of complex multiband systems. Furthermore, on the basis of speedup data gained from our implementation, it is shown that this new variant facilitates efficient calculations on a large number of multi-core CPUs. We apply the scheme to the $t$,$t'$ Hubbard model on a square lattice to analyze the convergence of the results with the bond length of the truncation of the partition of unity. In most parameter areas, a fast convergence can be observed. Finally, we compare to previous results in order to relate our approach to other fRG studies.

cond-mat.str-el↗

arXiv2016

Attosecond physics at the nanoscale

Recently two emerging areas of research, attosecond and nanoscale physics, have started to come together. Attosecond physics deals with phenomena occurring when ultrashort laser pulses, with duration on the femto- and sub-femtosecond time scales, interact with atoms, molecules or solids. The laser-induced electron dynamics occurs natively on a timescale down to a few hundred or even tens of attoseconds, which is comparable with the optical field. On the other hand, the second branch involves the manipulation and engineering of mesoscopic systems, such as solids, metals and dielectrics, with nanometric precision. Although nano-engineering is a vast and well-established research field on its own, the merger with intense laser physics is relatively recent. In this article we present a comprehensive experimental and theoretical overview of physics that takes place when short and intense laser pulses interact with nanosystems, such as metallic and dielectric nanostructures. In particular we elucidate how the spatially inhomogeneous laser induced fields at a nanometer scale modify the laser-driven electron dynamics. Consequently, this has important impact on pivotal processes such as ATI and HHG. The deep understanding of the coupled dynamics between these spatially inhomogeneous fields and matter configures a promising way to new avenues of research and applications. Thanks to the maturity that attosecond physics has reached, together with the tremendous advance in material engineering and manipulation techniques, the age of atto-nano physics has begun, but it is in the initial stage. We present thus some of the open questions, challenges and prospects for experimental confirmation of theoretical predictions, as well as experiments aimed at characterizing the induced fields and the unique electron dynamics initiated by them with high temporal and spatial resolution.

physics.atom-ph↗

arXiv2016

Bianisotropy and magnetism in plasmonic gratings

We present a simple design to achieve bianisotropy at visible wavelengths: an ultrathin plasmonic grating made of a gold grating covered by a thin flat layer of gold. We show experimentally and through simulations that the grating exhibits magneto-electric coupling and features asymmetric reflection and absorption, all that with a device thickness of a tenth of the operating wavelength. We compared the spectral results and retrieved the effective material parameters of different polarizations and devices. We show that both asymmetry and strong coupling between the incoming light and the optically interacting surfaces are required for obtaining asymmetric optical behavior in metasurfaces.

cond-mat.mes-hall↗

arXiv2015

Signatures of the $A^2$ term in ultrastrongly-coupled oscillators

We study a bosonic matter excitation coupled to a single-mode cavity field via electric dipole. Counter-rotating and $A^2$ terms are included in the interaction model, ${\mathbf A}$ being the vector potential of the cavity field. In the ultrastrong coupling regime the vacuum of the bare modes is no longer the ground state of the Hamiltonian and contains a nonzero population of polaritons, the true normal modes of the system. If the parameters of the model satisfy the Thomas-Reiche-Kuhn sum rule, we find that the two polaritons are always equally populated. We show how this prediction could be tested in a quenching experiment, by rapidly switching on the coupling and analyzing the radiation emitted by the cavity. A refinement of the model based on a microscopic minimal coupling Hamiltonian is also provided, and its consequences on our results are characterized analytically.

quant-ph↗

arXiv2014

Attosecond streaking of photoelectron emission from disordered solids

Attosecond streaking of photoelectrons emitted by extreme ultraviolet light has begun to reveal how electrons behave during their transport within simple crystalline solids. Many sample types within nanoplasmonics, thin-film physics, and semiconductor physics, however, do not have a simple single crystal structure. The electron dynamics which underpin the optical response of plasmonic nanostructures and wide-bandgap semiconductors happen on an attosecond timescale. Measuring these dynamics using attosecond streaking will enable such systems to be specially tailored for applications in areas such as ultrafast opto-electronics. We show that streaking can be extended to this very general type of sample by presenting streaking measurements on an amorphous film of the wide-bandgap semiconductor tungsten trioxide, and on polycrystalline gold, a material that forms the basis of many nanoplasmonic devices. Our measurements reveal the near-field temporal structure at the sample surface, and photoelectron wavepacket temporal broadening consistent with a spread of electron transport times to the surface.

physics.optics↗

arXiv2014

Functional renormalization group study of an eight-band model for the iron arsenides

We investigate the superconducting pairing instabilities of eight-band models for the iron arsenides. Using a functional renormalization group treatment, we determine how the critical energy scale for superconductivity depends on the electronic band structure. Most importantly, if we vary the parameters from values corresponding to LaFeAsO to SmFeAsO, the pairing scale is strongly enhanced, in accordance with the experimental observation. We analyze the reasons for this trend and compare the results of the eight-band approach to those found using five-band models.

cond-mat.supr-con↗

arXiv2014

Observation of quantum interference in the plasmonic Hong-Ou-Mandel effect

We report direct evidence of the bosonic nature of surface plasmon polaritons (SPPs) in a scattering-based beamsplitter. A parametric down-conversion source is used to produce two indistinguishable photons, each of which is converted into a SPP on a metal-stripe waveguide and then made to interact through a semi-transparent Bragg mirror. In this plasmonic analog of the Hong-Ou-Mandel experiment, we measure a coincidence dip with a visibility of 72%, a key signature that SPPs are bosons and that quantum interference is clearly involved.

quant-ph↗

arXiv2013

Quantum Plasmonics

Quantum plasmonics is a rapidly growing field of research that involves the study of the quantum properties of light and its interaction with matter at the nanoscale. Here, surface plasmons - electromagnetic excitations coupled to electron charge density waves on metal-dielectric interfaces or localized on metallic nanostructures - enable the confinement of light to scales far below that of conventional optics. In this article we review recent progress in the experimental and theoretical investigation of the quantum properties of surface plasmons, their role in controlling light-matter interactions at the quantum level and potential applications. Quantum plasmonics opens up a new frontier in the study of the fundamental physics of surface plasmons and the realization of quantum-controlled devices, including single-photon sources, transistors and ultra-compact circuitry at the nanoscale.

quant-ph↗

arXiv2013

Surface Plasmons and Nonlocality: a Simple Model

Surface plasmons on metals can concentrate light into sub-nanometric volumes and on these near atomic length scales the electronic response at the metal interface is smeared out over a Thomas-Fermi screening length. This nonlocality is a barrier to a good understanding of atomic scale response to light and complicates the practical matter of computing the fields. In this letter, we present a local analogue model and show that spatial nonlocality can be represented by replacing the nonlocal metal with a composite material, comprising a thin dielectric layer on top of a local metal. This method not only makes possible the quantitative analysis of nonlocal effects in complex plasmonic phenomena with unprecedented simplicity and physical insight, but also offers great practical advantages in their numerical treatment.

cond-mat.mes-hall↗

arXiv2012

Near-field optical imaging with a CdSe single nanocrystal-based active tip

We report near-field scanning optical imaging with an active tip made of a single fluorescent CdSe nanocrystal attached at the apex of an optical tip. Although the images are acquired only partially because of the random blinking of the semiconductor particle, our work validates the use of such tips in ultra-high spatial resolution optical microscopy.

physics.optics↗

arXiv2010

Optical properties of carbon nanofiber photonic crystals

Carbon nanofibers (CNF) are used as components of planar photonic crystals. Square and rectangular lattices and random patterns of vertically aligned CNF were fabricated and their properties studied using ellipsometry. We show that detailed information such as symmetry directions and the band structure of these novel materials can be extracted from considerations of the polarization state in the specular beam. The refractive index of the individual nanofibers was found to be n_CNF = 4.1.

physics.optics↗