arXiv subjects

S. A. Pozzi

Publications and source records attributed to S. A. Pozzi.

8 recordsLinked to original sources

arXiv2026

Improving the Predictive Capability of the Fission Reaction Event Yield Algorithm ($\mathtt{FREYA}$)

We determine the optimal parameters for thermal neutron-induced fission of $^{233,235}$U and $^{239,241}$Pu in the complete event fission model $\mathtt{FREYA}$. First, we revisit and, in most cases, improve the prior values determined for spontaneous fission using a genetic algorithm. Our optimization procedure is then applied to thermal neutron-induced fission, replacing the empirically-chosen parameters previously employed in $\mathtt{FREYA}$. Finally, the optimized parameter values are used to make predictions for spontaneous and thermal neutron-induced fission observables not included in the fits. This work represents the first step in a broader program to study neutron-induced fission as a function of incident neutron energy, to systematically improve the performance of $\mathtt{FREYA}$, capturing any energy-dependent trends of the physics-based $\mathtt{FREYA}$ parameters.

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arXiv2024

Meaurement of spin vs. TKE of $^{144}$Ba produced in spontaneous fission of $^{252}$Cf

We measure the average spin of $^{144}$Ba, a common fragment produced in $^{252}$Cf(sf), as a function of the total kinetic energy (TKE). We combined for the first time a twin Frisch-gridded ionization chamber with a world-class $\gamma$-ray spectrometer that was designed to measure high-multiplicity $\gamma$-ray events, Gammasphere. The chamber, loaded with a $^{252}$Cf(sf) source, provides a fission trigger, the TKE of the fragments, the approximate fragment masses, and the polar angle of the fission axis. Gammasphere provides the total $\gamma$-ray yield, fragment identification through the tagging of decay $\gamma$ rays, and the feeding of rotational bands in the fragments. We determine the dependence of the average spin of $^{144}$Ba on the fragments' TKE by correlating the fragment properties with the distribution of discrete levels that are fed. We find that the average spin only changes by about $0.5$ $\hbar$ across the TKE range of 158-203 MeV. The virtual independence of the spin on TKE suggests that spin is not solely generated through the statistical excitation of rotational modes, and more complex mechanisms are required.

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arXiv2022

Instrumentation for correlated prompt $n$-$γ$ emission studies in coincidence with fission fragments

Recent theoretical and experimental results have brought renewed interest and focus on the topic of fission fragment angular momentum. Measurements of neutrons and $γ$ rays in coincidence with fission fragments remain the most valuable tool in the exploration of fission physics. To achieve these scientific goals, we have developed a system that combines a state-of-the-art fission fragment detector and $n$-$γ$ radiation detectors. A new twin Frisch-gridded ionization chamber has been designed and constructed for use with a spontaneous fission source and an array of forty \textit{trans}-stilbene organic scintillators (FS-3) at Argonne National Laboratory. The new ionization chamber design we present in this work aims at minimizing particle attenuation in the chamber walls, and provides a compact apparatus that can be fit inside existing experimental systems. The ionization chamber is capable of measuring fission fragment masses and kinetic energies, whereas the FS-3 provides neutron and gamma-ray multiplicities and spectra. The details of both detector assembly are presented along with the first experimental results of this setup. Planned event-by-event analysis and future experiments are briefly discussed.

physics.ins-det↗

arXiv2021

Angular momentum removal by neutron and $γ$-ray emissions during fission fragment decays

We investigate the angular momentum removal from fission fragments (FFs) through neutron and $γ$-ray emission, where we find that about half the neutrons are emitted with angular momenta $\ge 1.5\hbar$ and that the change in angular momentum after the emission of neutrons and statistical $γ$ rays is significant, contradicting usual assumptions. Per fission event, in our simulations, the neutron and statistical $γ$-ray emissions change the spin of the fragment by 3.5 -- 5~$\hbar$, with a large standard deviation comparable to the average value. Such wide angular momentum removal distributions can hide any underlying correlations in the fission fragment initial spin values. Within our model, we reproduce data on spin measurements from discrete transitions after neutron emissions, especially in the case of light FFs. The agreement further improves for the heavy fragments if one removes from the analysis the events that would produce isomeric states. Finally, we show that while in our model the initial FF spins do not follow a saw-tooth like behavior observed in recent measurements, the average FF spin computed after neutron and statistical $γ$ emissions exhibits a shape that resembles a saw tooth. This suggests that the average FF spin measured after statistical emissions is not necessarily connected with the scission mechanism as previously implied.

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arXiv2020

Rossi-alpha Uncertainty Quantification by Analytic, Bootstrap, and Sample Methods to Inform Fitting Best Practices

The prompt neutron period (the negative reciprocal of the prompt neutron decay constant) can be estimated using the Rossi-alpha technique that is predicated on fitting Rossi-alpha histograms and of interest in nuclear criticality safety and nonproliferation [1, 2, 3]. The histograms are traditionally fit with a one-exponential model; however, recent work has proposed a two-exponential model to account for reflector-induced phenomenon [4, 5, 6]. Until recently, the uncertainty quantification for either model was inadequate (inaccurate and demanded large measurement times). Measurement uncertainty quantification by sample and analytic methods was developed and validated in Ref. [7]. The purpose of this transaction is to (i) validate a new bootstrap method by comparing bin-by-bin error bar estimates and (ii) demonstrate how to choose bin widths and reset times to optimize precision and accuracy.

physics.data-an↗

arXiv2020

Fast Rossi-alpha Measurements of Plutonium using Organic Scintillators

In this work, Rossi-alpha measurements were simultaneously performed with a $^3$He-based detection system and an organic scintillator-based detection system. The assembly is 15 kg of plutonium (93 wt$\%$ $^{239}$Pu) reflected by copper and moderated by lead. The goal of Rossi-alpha measurements is to estimate the prompt neutron decay constant, alpha. Simulations estimate $k_\text{eff}$ = 0.624 and $α$ = 52.3 $\pm$ 2.5 ns for the measured assembly. The organic scintillator system estimated $α$ = 47.4 $\pm$ 2.0 ns, having a 9.37$\%$ error (though the 1.09 standard deviation confidence intervals overlapped). The $^3$He system estimated $α$ = 37 $μ$s. The known slowing down time of the $^3$He system is 35-40 $μ$s, which means the slowing down time dominates and obscures the prompt neutron decay constant. Subsequently, the organic scintillator system should be used for assemblies with alpha much less than 35 $μ$s.

physics.ins-det↗

arXiv2018

High resolution measurement of tagged two-neutron energy and angle correlations in Cf-252(sf)

Background: Spontaneous fission events emit prompt neutrons correlated with one another in emission angle and energy. Purpose: We explore the relationship in energy and angle between correlated prompt neutrons emitted from 252Cf spontaneous fission. Methods: Measurements with the Chi-Nu array provide experimental data for coincident neutrons tagged with a fission chamber signal with 10 degree angular resolution and 1 ns timing resolution for time-of-flight energy calculations. The experimental results are compared to simulations produced by the fission event generators CGMF, FREYA, and MCNPX-POLIMI IPOL(1)=1. Results: We find that the measurements and the simulations all exhibit anisotropic neutron emission, though differences exist between fission event generators. Conclusions: This work shows that the dependence of detected neutron energy on the energy of a neutron detected in coincidence, although weak, is non-negligible, indicating that there may be correlations in energy between two neutrons emitted in the same fission event.

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arXiv2018

Correlated Prompt Fission Data in Transport Simulations

Detailed information on the fission process can be inferred from the observation, modeling and theoretical understanding of prompt fission neutron and $γ$-ray~observables. Beyond simple average quantities, the study of distributions and correlations in prompt data, e.g., multiplicity-dependent neutron and \gray~spectra, angular distributions of the emitted particles, $n$-$n$, $n$-$γ$, and $γ$-$γ$~correlations, can place stringent constraints on fission models and parameters that would otherwise be free to be tuned separately to represent individual fission observables. The FREYA~and CGMF~codes have been developed to follow the sequential emissions of prompt neutrons and $γ$-rays~from the initial excited fission fragments produced right after scission. Both codes implement Monte Carlo techniques to sample initial fission fragment configurations in mass, charge and kinetic energy and sample probabilities of neutron and $γ$~emission at each stage of the decay. This approach naturally leads to using simple but powerful statistical techniques to infer distributions and correlations among many observables and model parameters. The comparison of model calculations with experimental data provides a rich arena for testing various nuclear physics models such as those related to the nuclear structure and level densities of neutron-rich nuclei, the $γ$-ray~strength functions of dipole and quadrupole transitions, the mechanism for dividing the excitation energy between the two nascent fragments near scission, and the mechanisms behind the production of angular momentum in the fragments, etc. Beyond the obvious interest from a fundamental physics point of view, such studies are also important for addressing data needs in various nuclear applications. (See text for full abstract.)

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