arXiv subjects

S. A. Tarasenko

Publications and source records attributed to S. A. Tarasenko.

At least 19 recordsLinked to original sources

arXiv2025

Electric and spin-valley currents induced by structured light in 2D Dirac materials

Structured optical fields can be used for the injection and control of charge and spin-valley currents. Here, we present a systematical study of these phenomena for interband absorption of structured light in 2D Dirac materials. We derive general expressions for the current density and the quasi-classical generation rate of photoelectrons in the momentum, coordinate, and spin-valley spaces. We reveal mechanisms of the current formation determined by the local and non-local contributions to the optical generation, including the mechanisms related to optical alignment of electron momenta by linearly polarized light, optical orientation by circularly polarized light, and the class of charge and spin-valley photon drags sensitive to the phase and polarization profiles of the optical field. We develop a kinetic theory of electric and spin-valley currents driven by the optical field with spatially inhomogeneous intensity, polarization, and phase and obtain analytical expressions for the current contributions. The theory is applied to analyze the photocurrents emerging in TMDC layers and graphene excited by polarization gratings.

cond-mat.mes-hall↗

arXiv2025

Trembling motion of electrons driven by Larmor spin precession

We show that the initialization of an ensemble of electrons in the same spin state in strained n-InGaAs subject to a perpendicular magnetic field triggers an AC electric current at GHz frequencies. The AC current emerges in the absence of any driving force and survives until the coherent precession of the electron spins is lost. The current amplitude increases linearly with both the spin-orbit coupling strength and the external magnetic field. The generation mechanism of the observed oscillatory charge motion can be fruitfully described in terms of the periodic trembling motion of spin-polarized electrons, which is a solid-state analog to the Zitterbewegung of free Dirac electrons. Our results demonstrate that the hidden consequence of relativistic quantum mechanics is realized and can be studied in a rather simple solid-state system at moderate temperatures. Furthermore, the large amplitude of the AC current at high magnetic fields enables ultra-fast spin sensitive electric read-out in solids.

cond-mat.mes-hall↗

arXiv2025

Second harmonic generation due to spatial structure of radiation beam

We show that spatially structured radiation generates second harmonic in a two-dimensional system even if the system is homogeneous and isotropic. The effect originates from non-locality of electric response to structured electromagnetic field. We develop an analytical theory of such a second harmonic generation in conducting two-dimensional systems. For the general type of structured radiation, we calculate the emerging electric currents at the double frequency and the emitted second harmonic radiation. The theory applied to twisted light reveals that the angular momentum of light doubles in the second harmonic emission. Our results pave the way for second harmonic generation and structuring in two-dimensional materials beyond the constraints imposed by crystal symmetry.

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arXiv2024

Photocurrents induced by structured light

Advances in manipulating the structure of optical beams enable the study of interaction between structured light and low-dimensional semiconductor systems. We explore the photocurrents in two-dimensional systems excited by such inhomogeneous radiation with structured field. Besides the contribition associated with the intensity gradient, the photocurrent contains contributions driven by the gradients of the Stokes polarization parameters and the phase of the electromagnetic field. We develop a microscopic theory of the photocurrents induced by structured light and derive analytical expressions for all the photocurrent contributions at intraband transport of electrons. The theory is applied to analyze the radial and azimuthal photocurrents excited by twisted light beams carrying orbital angular momentum, and possible experiments to detect the photocurrents are discussed.

cond-mat.mes-hall↗

arXiv2022

Splitting of Dirac cones in HgTe quantum wells: Effects of crystallographic orientation, interface-, bulk-, and structure-inversion asymmetry

We develop a microscopic theory of the fine structure of Dirac states in $(0lh)$-grown HgTe/CdHgTe quantum wells (QWs), where $l$ and $h$ are the Miller indices. It is shown that bulk, interface, and structure inversion asymmetry causes the anticrossing of levels even at zero in-plane wave vector and lifts the Dirac state degeneracy. In the QWs of critical thickness, the two-fold degenerate Dirac cone gets split into non-degenerate Weyl cones. The splitting and the Weyl point positions dramatically depend on the QW crystallographic orientation. We calculate the splitting parameters related to bulk, interface, and structure inversion asymmetry and derive the effective Hamiltonian of the Dirac states. Further, we obtain an analytical expression for the energy spectrum and discuss the spectrum for (001)-, (013)- and (011)-grown QWs.

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arXiv2022

Second harmonic generation at the edge of a two-dimensional electron gas

We show that driving a two-dimensional electron gas by an in-plane electric field oscillating at the frequency $ω$ gives rise to an electric current at $2ω$ flowing near the edge of the system. This current has both parallel and perpendicular to the edge components, which emit electromagnetic waves at $2ω$ with different polarizations. We develop a microscopic theory of such an edge second harmonic generation and calculate the edge current at $2ω$ in different regimes of electron transport and electric field screening. We also show that at high frequencies the spatial profile of the edge current contains oscillations caused by excitation of plasma waves.

cond-mat.mes-hall↗

arXiv2022

Spin splitting in low-symmetry quantum wells beyond Rashba and Dresselhaus terms

Spin-orbit interaction in semiconductor structures with broken space inversion symmetry leads to spin splitting of electron and hole states even in the absence of magnetic field. We discover that, beyond the Rashba and Dresselhaus contributions, there is an additional type of the zero-field spin splitting which is caused by the interplay of the cubic shape of crystal unit cell and macroscopic structure asymmetry. In quantum wells grown along low-symmetry crystallographic axes, this type of spin-orbit interaction couples the out-of-plane component of carrier's spin with the in-plane momentum while the coupling strength is controlled by structure inversion asymmetry. We carry out numerical calculations and develop an analytical theory, which demonstrate that this interaction can dominate $\boldsymbol{k}$-linear spin splitting of heavy-hole subbands.

cond-mat.mes-hall↗

arXiv2021

Inverted fine structure of a 6H-SiC qubit enabling robust spin-photon interface

Optically controllable solid-state spin qubits are one of the basic building blocks for applied quantum technology. Efficient extraction of emitted photons and a robust spin-photon interface are crucial for the realization of quantum sensing protocols and essential for the implementation of quantum repeaters. Though silicon carbide (SiC) is a very promising material platform hosting highly-coherent silicon vacancy spin qubits, a drawback for their practical application is the unfavorable ordering of the electronic levels in the optically excited state. Here, we demonstrate that due to polytypism of SiC, a particular type of silicon vacancy qubits in 6H-SiC possesses an unusual inverted fine structure. This results in the directional emission of light along the hexagonal crystallographic axis, making photon extraction more efficient and integration into photonic structures technologically straightforward. From the angular polarization dependencies of the emission, we reconstruct the spatial symmetry and determine the optical selection rules depending on the local deformation and spin-orbit interaction, enabling direct implementation of robust spin-photon entanglement schemes. Furthermore, the inverted fine structure leads to unexpected behavior of the spin readout contrast. It vanishes and recovers with lattice cooling due to two competing optical spin pumping mechanisms. Our experimental and theoretical approaches provide a deep insight into the optical and spin properties of atomic-scale qubits in SiC required for quantum communication and distributed quantum information processing.

quant-ph↗

arXiv2021

Intrinsic circularly-polarized exciton emission in a twisted van-der-Waals heterostructure

The investigation of excitons in van-der-Waals heterostructures has led to profound insights into the interplay of crystal symmetries and fundamental effects of light-matter coupling. In particular, the polarization selection rules in undistorted, slightly twisted heterostructures of MoSe$_2$/WSe$_2$ were found to be connected with the Moiré superlattice. Here, we report the emergence of a significant degree of circular polarization of excitons in such a hetero-structure upon non-resonant driving with a linearly polarized laser. The effect is present at zero magnetic field, and sensibly reacts on perpendicularly applied magnetic field. The giant magnitude of polarization, which cannot be explained by conventional birefringence or optical activity of the twisted lattice, suggests a kinematic origin arising from an emergent pyromagnetic symmetry in our structure, which we exploit to gain insight into the microscopic processes of our device.

cond-mat.mes-hall↗

arXiv2020

Edge photogalvanic effect caused by optical alignment of carrier momenta in 2D Dirac materials

We show that the inter-band absorption of radiation in a 2D Dirac material leads to a direct electric current flowing at sample edges. The photocurrent originates from the momentum alignment of electrons and holes and is controlled by the radiation polarization. We develop a microscopic theory of such an edge photogalvanic effect and calculate the photocurrent for gapped and gapless 2D Dirac materials, also in the presence of a static magnetic field which introduces additional imbalance between the electron and hole currents. Further, we show that the photocurrent can be considerably multiplied in a ratchet-like structure with an array of narrow strips.

cond-mat.mes-hall↗

arXiv2020

Edge photocurrent driven by THz electric field in bi-layer graphene

We report on the observation of edge electric currents excited in bi-layer graphene by terahertz laser radiation. We show that the current generation belongs to the class of second order in electric field phenomena and is controlled by the orientation of the THz electric field polarization plane. Additionally, applying a small magnetic field normal to the graphene plane leads to a phase shift in the polarization dependence. Increasing the magnetic field strength, the current starts to exhibit 1/B-magnetooscillations with a period consistent with that of the Shubnikov-de-Haas effect and amplitude by an order of magnitude larger as compared to the current at zero magnetic field measured under the same conditions. The microscopic theory developed shows that the current is formed in the edges vicinity limited by the mean-free path of carriers and the screening length of the high-frequency electric field. The current originates from the alignment of the free carrier momenta and dynamic accumulation of charge at the edges, where the P-symmetry is naturally broken. The observed magnetooscillations of the photocurrent are attributed to the formation of Landau levels.

cond-mat.mes-hall↗

arXiv2020

Terahertz Magnetospectroscopy of Cyclotron Resonances from Topological Surface States in Thick Films of Cd$_x$Hg$_{1-x}$Te

We present studies of the cyclotron resonance (CR) in thick Cd$_x$Hg$_{1-x}$Te films with different cadmium concentrations corresponding to inverted and normal band order, as well as to an almost linear energy dispersion. Our results demonstrate that formation of two-dimensional topological surface states requires sharp interfaces between layers with inverted and normal band order, in which case the corresponding CR is clearly observed for the out-of-plane orientation of magnetic field, but does not show up for an in-plane orientation. By contrast, all samples having more conventional technological design with smooth interfaces (i.e., containing regions of Cd$_x$Hg$_{1-x}$Te with gradually changing Cd content $x$) show equally pronounced CR in both in-plane and out-of-plane magnetic field revealing that CR is excited in three-dimensional states. Modeling of the surface states for different film designs supports our main observations. In all samples, we observe additional broad helicity-independent resonances which are attributed to photo-ionization and magnetic freeze-out of impurity states.

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arXiv2019

Symmetry breaking and circular photogalvanic effect in epitaxial Cd$_x$Hg$_{1-x}$Te films

We report on the observation of symmetry breaking and the circular photogalvanic effect in Cd$_x$Hg$_{1-x}$Te alloys. We demonstrate that irradiation of bulk epitaxial films with circularly polarized terahertz radiation leads to the circular photogalvanic effect (CPGE) yielding a photocurrent whose direction reverses upon switching the photon helicity. This effect is forbidden in bulk zinc-blende crystals by symmetry arguments, therefore, its observation indicates either the symmetry reduction of bulk material or that the photocurrent is excited in the topological surface states formed in a material with low Cadmium concentration. We show that the bulk states play a crucial role because the CPGE was also clearly detected in samples with non-inverted band structure. We suggest that strain is a reason of the symmetry reduction. We develop a theory of the CPGE showing that the photocurrent results from the quantum interference of different pathways contributing to the free-carrier absorption (Drude-like) of monochromatic radiation.

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arXiv2019

Spin noise at electron paramagnetic resonance

We develop a microscopic theory of spin noise in solid-state systems at electron paramagnetic resonance, when the spin dynamics is driven by static and radio-frequency (RF) magnetic fields and the stochastic effective magnetic field stemming from the interaction with environment. The RF field splits the peaks in the power spectrum of spin noise into the Mollow-like triplets and also gives rise to additional spin-spin correlations which oscillate in the absolute time at the RF frequency and the double frequeqncy. Even in systems with strong inhomogeneous broadening, the spin noise spectrum contains narrow lines insensitive to the dispersion of the effective $g$-factors. Thus, the measurements of spin noise at electron paramagnetic resonance provides an access to the intrinsic spin lifetime of electrons.

cond-mat.mes-hall↗

arXiv2019

Thermal generation of shift electric current

It is shown that the dissipation of energy in an electron gas confined in a quantum well made of non-centrosymmetric crystal leads to a direct electric current. The current originates from the real-space shift of the wavepackets of Bloch electrons at the electron scattering by phonons, which tends to restore thermal equilibrium between the electron and phonon subsystems. We develop a microscopic theory of such a phonogalvanic effect for narrow band gap zinc-blende quantum wells.

cond-mat.mes-hall↗

arXiv2019

High-frequency nonlinear transport and photogalvanic effects in two-dimensional topological insulators

Excitation of a topological insulator by a high-frequency electric field of a laser radiation leads to a dc electric current in the helical edge channel whose direction and magnitude are sensitive to the radiation polarization and depend on the physical properties of the edge. We present an overview of theoretical and experimental studies of such edge photoelectric effects in two-dimensional topological insulators based on semiconductor quantum wells. First, we give a phenomenological description of edge photocurrents, which may originate from the photogalvanic effects or the photon drag effects, for edges of all possible symmetry. Then, we discuss microscopic mechanisms of photocurrent generation for different types of optical transitions involving helical edge states. They include direct and indirect optical transitions within the edge channel and edge-to-bulk optical transitions.

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arXiv2018

Excitation and coherent control of spin qudit modes with sub-MHz spectral resolution

Quantum bit or qubit is a two-level system, which builds the foundation for quantum computation, simulation, communication and sensing. Quantum states of higher dimension, i.e., qutrits (D = 3) and especially qudits (D = 4 or higher), offer significant advantages. Particularly, they can provide noise-resistant quantum cryptography, simplify quantum logic and improve quantum metrology. Flying and solid-state qudits have been implemented on the basis of photonic chips and superconducting circuits, respectively. However, there is still a lack of room-temperature qudits with long coherence time and high spectral resolution. The silicon vacancy centers in silicon carbide (SiC) with spin S = 3/2 are quite promising in this respect, but until now they were treated as a canonical qubit system. Here, we apply a two-frequency protocol to excite and image multiple qudit modes in a SiC spin ensemble under ambient conditions. Strikingly, their spectral width is about one order of magnitude narrower than the inhomogeneous broadening of the corresponding spin resonance. By applying Ramsey interferometry to these spin qudits, we achieve a spectral selectivity of 600 kHz and a spectral resolution of 30 kHz. As a practical consequence, we demonstrate absolute DC magnetometry insensitive to thermal noise and strain fluctuations.

quant-ph↗

arXiv2018

Edge currents driven by terahertz radiation in graphene in quantum Hall regime

We observe that the illumination of unbiased graphene in the quantum Hall regime with polarized terahertz laser radiation results in a direct edge current. This photocurrent is caused by an imbalance of persistent edge currents, which are driven out of thermal equilibrium by indirect transitions within the chiral edge channel. The direction of the edge photocurrent is determined by the polarity of the external magnetic field, while its magnitude depends on the radiation polarization. The microscopic theory developed in this paper describes well the experimental data.

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