arXiv subjects

S. A. van den Berg

Publications and source records attributed to S. A. van den Berg.

4 recordsLinked to original sources

arXiv2008

Direct frequency comb spectroscopy of trapped ions

Direct frequency comb spectroscopy of trapped ions is demonstated for the first time. It is shown that the 4s^2S_(1/2)-4p^2P_(3/2) transition in calcium ions can be excited directly with a frequency comb laser that is upconverted to 393 nm. Detection of the transition is performed using a shelving scheme to suppress background signal from non-resonant comb modes. The measured transition frequency of f=761 905 012.7(0.5) MHz presents an improvement in accuracy of more than two orders of magnitude.

physics.atom-ph↗

arXiv2008

Frequency metrology on the 4s 2S1/2 - 4p 2P1/2 transition in the calcium ion for a comparison with quasar data

High accuracy frequency metrology on the 4s 2S1/2 - 4p 2P1/2 transition in calcium ions is performed using laser cooled and crystallized ions in a linear Paul trap. Calibration is performed with a frequency comb laser, resulting in a transition frequency of f=755222766.2(1.7) MHz. The accuracy presents an improvement of more than one order of magnitude, and will facilitate a comparison with quasar data in a search for a possible change of the fine structure constant on a cosmological time scale.

physics.atom-ph↗

arXiv2004

Photoluminescence studies study of a phenyl-substituted PPV

We report on the photophysics of a phenyl-substituted PPV both in solution and as a film. For both systems we have studied the decay of the photoluminescence and of the emission anisotropy for a large set of wavelengths spanning the entire photoluminescence spectrum. At long wavelengths the decay behavior is that of an interchain species. At the shortest wavelengths the decay of the photoluminescence from the film is observed to have a long-lived component, in addition to the rapidly decaying component usually associated with energy transfer. We attribute this slow component to emission by isolated intrachain excitons with reduced nonradiative relaxation.

physics.chem-ph↗

arXiv2004

Measuring the gain dynamics in a conjugated polymer film

We present a simple method for measuring the gain decay time in a conjugated polymer film by optically exciting the film with two mutually delayed ultrashort pump pulses. When the pump is set at such a power level that amplified spontaneous emission marginally develops along the polymer waveguide, the total output emitted from its edge decays exponentially as a function of the interpulse delay. The corresponding decay time represents the decay time of the gain of the polymer material.

physics.chem-ph↗