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S. Blatt

Publications and source records attributed to S. Blatt.

17 recordsLinked to original sources

Fine-Structure Qubit Encoded in Metastable Strontium Trapped in an Optical Lattice

We demonstrate coherent control of the fine-structure qubit in neutral strontium atoms. This qubit is encoded in the metastable $^3\mathrm{P}_2$ and $^3\mathrm{P}_0$ states, coupled by a Raman transition. Using a magnetic quadrupole transition, we demonstrate coherent state-initialization of this THz qubit. We show Rabi oscillations with more than 60 coherent cycles and single-qubit rotations on the $\mu$s scale. With spin-echo, we demonstrate coherence times of tens of ms. Our results pave the way for fast quantum information processors and highly tunable quantum simulators with two-electron atoms.

quant-ph

Coherent excitation of a $\mu$Hz scale optical magnetic quadrupole transition

We report on the coherent excitation of the ultranarrow $^{1}\mathrm{S}_0$-$^{3}\mathrm{P}_2$ magnetic quadrupole transition in $^{88}\mathrm{Sr}$. By confining atoms in a state insensitive optical lattice, we achieve excitation fractions of 97(1)% and observe linewidths as narrow as 58(1) Hz. With Ramsey spectroscopy, we find coherence times of 14(1) ms, which can be extended to 266(36) ms using a spin-echo sequence. We determine the linewidth of the M2 transition to 24(7) $\mu$Hz, confirming longstanding theoretical predictions. These results establish an additional clock transition in strontium and pave the way for applications of the metastable $^{3}\mathrm{P}_2$ state in quantum computing and quantum simulations.

physics.atom-ph

The $^{1}\mathrm{S}_0$-$^{3}\mathrm{P}_2$ magnetic quadrupole transition in neutral strontium

We present a detailed investigation of the ultranarrow magnetic-quadrupole $^{1}\mathrm{S}_0$-$^{3}\mathrm{P}_2$ transition in neutral strontium and show how it can be made accessible for quantum simulation and quantum computation. By engineering the light shift in a one-dimensional optical lattice, we perform high-resolution spectroscopy and observe the characteristic absorption patterns for a magnetic quadrupole transition. We measure an absolute transition frequency of 446,647,242,704(2) kHz in $^{88}\mathrm{Sr}$ and an $^{88}\mathrm{Sr}$-$^{87}\mathrm{Sr}$ isotope shift of +62.91(4) MHz. In a proof-of-principle experiment, we use this transition to demonstrate local addressing in an optical lattice with 532 nm spacing with a Rayleigh-criterion resolution of 494(45) nm. Our results pave the way for applications of the magnetic quadrupole transition as an optical qubit and for single-site addressing in optical lattices.

physics.atom-ph

Cavity-enhanced optical lattices for scaling neutral atom quantum technologies to higher qubit numbers

We demonstrate a cavity-based solution to scale up experiments with ultracold atoms in optical lattices by an order of magnitude over state-of-the-art free space lattices. Our two-dimensional optical lattices are created by power enhancement cavities with large mode waists of 489(8) $\mu$m and allow us to trap ultracold strontium atoms at a lattice depth of 60 $\mu$K by using only 80 mW of input light per cavity axis. We characterize these lattices using high-resolution clock spectroscopy and resolve carrier transitions between different vibrational levels. With these spectral features, we locally measure the lattice potential envelope and the sample temperature with a spatial resolution limited only by the optical resolution of the imaging system. The measured ground-band and trap lifetimes are 18(3) s and 59(2) s, respectively, and the lattice frequency (depth) is long-term stable on the MHz (0.1\%) level. Our results show that large, deep, and stable two-dimensional cavity-enhanced lattices can be created at any wavelength and can be used to scale up neutral-atom-based quantum simulators, quantum computers, sensors, and optical lattice clocks.

cond-mat.quant-gas

Crossed optical cavities with large mode diameters

We report on a compact, ultrahigh-vacuum compatible optical assembly to create large-scale, two-dimensional optical lattices for use in experiments with ultracold atoms. The assembly consists of an octagon-shaped spacer made from ultra-low-expansion glass, to which we optically contact four fused-silica cavity mirrors, making it highly mechanically and thermally stable. The mirror surfaces are nearly plane-parallel which allows us to create two perpendicular cavity modes with diameters $\sim$1 mm. Such large mode diameters are desirable to increase the optical lattice homogeneity, but lead to strong angular sensitivities of the coplanarity between the two cavity modes. We demonstrate a procedure to precisely position each mirror substrate that achieves a deviation from coplanarity of $d = 1(5)$ $μ$m. Creating large optical lattices at arbitrary visible and near infrared wavelengths requires significant power enhancements to overcome limitations in the available laser power. The cavity mirrors have a customized low-loss mirror coating that enhances the power at a set of relevant wavelengths from the visible to the near infrared by up to three orders of magnitude.

cond-mat.quant-gas

State-dependent optical lattices for the strontium optical qubit

We demonstrate state-dependent optical lattices for the Sr optical qubit at the tune-out wavelength for its ground state. We tightly trap excited state atoms while suppressing the effect of the lattice on ground state atoms by more than four orders of magnitude. This highly independent control over the qubit states removes inelastic excited state collisions as the main obstacle for quantum simulation and computation schemes based on the Sr optical qubit. Our results also reveal large discrepancies in the atomic data used to calibrate the largest systematic effect of Sr optical lattice clocks.

physics.atom-ph

Fast and dense magneto-optical traps for Strontium

We improve the efficiency of sawtooth-wave-adiabatic-passage (SWAP) cooling for strontium atoms in three dimensions and combine it with standard narrow-line laser cooling. With this technique, we create strontium magneto-optical traps with $6\times 10^7$ bosonic $^{88}$Sr ($1\times 10^7$ fermionic $^{87}$Sr) atoms at phase-space densities of $2\times 10^{-3}$ ($1.4\times 10^{-4}$). Our method is simple to implement and is faster and more robust than traditional cooling methods.

physics.atom-ph

Implementation of a stable, high-power optical lattice for quantum gas microscopy

We describe the design and implementation of a stable high-power 1064 nm laser system to generate optical lattices for experiments with ultracold quantum gases. The system is based on a low-noise laser amplified by an array of four heavily modified, high-power fiber amplifiers. The beam intensity is stabilized and controlled with a nonlinear feedback loop. Using real-time monitoring of the resulting optical lattice, we find the stability of the lattice site positions to be well below the lattice spacing over the course of hours. The position of the harmonic trap produced by the Gaussian envelope of the lattice beams is stable to about one lattice spacing and the long-term (six-month) relative RMS stability of the lattice spacing itself is 0.5%.

cond-mat.quant-gas

Optical Feshbach resonances: Field-dressed theory and comparison with experiments

Optical Feshbach resonances (OFRs) have generated significant experimental interest in recent years. These resonances are promising for many-body physics experiments, yet the practical application of OFRs has been limited. The theory of OFRs has been based on an approximate model that fails in important detuning regimes, and the incomplete theoretical understanding of this effect has hindered OFR experiments. We present the most complete theoretical treatment of OFRs to date, demonstrating important characteristics that must be considered in OFR experiments and comparing OFRs to the well-studied case of magnetic Feshbach resonances. We also present a comprehensive treatment of the approximate OFR model, including a study of the range of validity for this model. Finally, we derive experimentally useful expressions that can be applied to real experimental data to extract important information about the resonance structure of colliding atoms.

physics.atom-ph

Low-noise optical lattices for ultracold $^6$Li

We demonstrate stable, long-term trapping of fermionic $^6$Li atoms in an optical lattice with MHz trap frequencies for use in a quantum gas microscope. Adiabatic release from the optical lattice in the object plane of a high-numerical-aperture imaging system allows a measurement of the population distribution among the lowest three bands in both radial directions with atom numbers as low as $7\times 10^2$. We measure exponential ground band heating rates as low as 0.014(1) s$^{-1}$ corresponding to a radial ground state $1/e$ lifetime of 71(5) s, fundamentally limited by scattering of lattice photons. For all lattice depths above 2 recoil, we find radial ground state lifetimes $\ge 1.6 \times 10^6$ recoil times.

physics.atom-ph

Systematic study of Optical Feshbach Resonances in an ideal gas

Using a narrow intercombination line in alkaline earth atoms to mitigate large inelastic losses, we explore the Optical Feshbach Resonance (OFR) effect in an ultracold gas of bosonic $^{88}$Sr. A systematic measurement of three resonances allows precise determinations of the OFR strength and scaling law, in agreement with coupled-channels theory. Resonant enhancement of the complex scattering length leads to thermalization mediated by elastic and inelastic collisions in an otherwise ideal gas. OFR could be used to control atomic interactions with high spatial and temporal resolution.

physics.atom-ph

Rabi Spectroscopy and Excitation Inhomogeneity in a 1D Optical Lattice Clock

We investigate the influence of atomic motion on precision Rabi spectroscopy of ultracold fermionic atoms confined in a deep, one dimensional (1D) optical lattice. We analyze the spectral components of longitudinal sideband spectra and present a model to extract information about the transverse motion and sample temperature from their structure. Rabi spectroscopy of the clock transition itself is also influenced by atomic motion in the weakly confined transverse directions of the optical lattice. By deriving Rabi flopping and Rabi lineshapes of the carrier transition, we obtain a model to quantify trap state dependent excitation inhomogeneities. The inhomogeneously excited ultracold fermions become distinguishable, which allows s-wave collisions. We derive a detailed model of this process and explain observed density shift data in terms of a dynamic mean field shift of the clock transition.

physics.atom-ph

Probing Interactions between Ultracold Fermions

At ultracold temperatures, the Pauli exclusion principle suppresses collisions between identical fermions. This has motivated the development of atomic clocks using fermionic isotopes. However, by probing an optical clock transition with thousands of lattice-confined, ultracold fermionic Sr atoms, we have observed density-dependent collisional frequency shifts. These collision effects have been measured systematically and are supported by a theoretical description attributing them to inhomogeneities in the probe excitation process that render the atoms distinguishable. This work has also yielded insights for zeroing the clock density shift.

physics.atom-ph

New Limits on Coupling of Fundamental Constants to Gravity Using $^{87}$Sr Optical Lattice Clocks

The $^1\mathrm{S}_0$-$^3\mathrm{P}_0$ clock transition frequency $ν_\text{Sr}$ in neutral $^{87}$Sr has been measured relative to the Cs standard by three independent laboratories in Boulder, Paris, and Tokyo over the last three years. The agreement on the $1\times 10^{-15}$ level makes $ν_\text{Sr}$ the best agreed-upon optical atomic frequency. We combine periodic variations in the $^{87}$Sr clock frequency with $^{199}$Hg$^+$ and H-maser data to test Local Position Invariance by obtaining the strongest limits to date on gravitational-coupling coefficients for the fine-structure constant $α$, electron-proton mass ratio $μ$ and light quark mass. Furthermore, after $^{199}$Hg$^+$, $^{171}$Yb$^+$ and H, we add $^{87}$Sr as the fourth optical atomic clock species to enhance constraints on yearly drifts of $α$ and $μ$.

physics.atom-ph

Sr lattice clock at 1x10^{-16} fractional uncertainty by remote optical evaluation with a Ca clock

Optical atomic clocks promise timekeeping at the highest precision and accuracy, owing to their high operating frequencies. Rigorous evaluations of these clocks require direct comparisons between them. We have realized a high-performance remote comparison of optical clocks over km-scale urban distances, a key step for development, dissemination, and application of these optical standards. Through this remote comparison and a proper design of lattice-confined neutral atoms for clock operation, we evaluate the uncertainty of a strontium (Sr) optical lattice clock at the 1x10-16 fractional level, surpassing the best current evaluations of cesium (Cs) primary standards. We also report on the observation of density-dependent effects in the spin-polarized fermionic sample and discuss the current limiting effect of blackbody radiation-induced frequency shifts.

physics.atom-ph

Compact, thermal-noise-limited optical cavity for diode laser stabilization at 1 x 10-15

We demonstrate phase and frequency stabilization of a diode laser at the thermal noise limit of a passive optical cavity. The system is compact and exploits a cavity design that reduces vibration sensitivity. The sub-Hz laser is characterized by comparison to a second independent system with similar fractional frequency stability (1 x 10-15 at 1 s). The laser is further characterized by resolving a 2 Hz wide, ultranarrow optical clock transition in ultracold strontium.

physics.optics

Dynamic cancellation of ac Stark shift for pulsed EIT/Raman optical lattice clocks

We propose a combination of Electromagnetically Induced Transparency (EIT)/Raman and pulsed spectroscopy techniques to accurately cancel frequency shifts arising from EIT fields in forbidden optical lattice clock transitions of alkaline earth atoms. Time-separated laser pulses are designed to trap atoms in coherent superpositions while eliminating off-resonance ac Stark contributions at particular laser detunings from the intermediate excited state. The scheme achieves efficient population transfer up to 60% with potential inaccuracy $<$ $10^{-17}$. Cancellation of external light shifts determined by a density matrix approach is confirmed by a complex wave-function formalism, sufficient at the mHz accuracy, under low field strengths or short interaction times.

physics.atom-ph