SearcharxivSearch

arXiv subjects

S. C. Chen

Publications and source records attributed to S. C. Chen.

3 recordsLinked to original sources

Electronic properties of germanene nanoribbons in external fields

Germanene nanoribbons, with buckled structures, exhibit unique electronic properties. The complicated relations among the quantum confinement, the spin-orbital coupling, the magnetic quantization, the electric-field dominated quantum numbers, energy dispersions, energy gap, state degeneracy, and wave functions. Such mechanisms can diversify spatial charge distributions and spin configurations on distinct sublattices. There exist the spin-split quasi-Landau levels and the valley-dependent asymmetric energy spectrum in a composite electric and magnetic field, manly owing to the destruction of z=0 mirror symmetry. The rich electronic structures are revealed in density of states as a lot of special structures. The predicted results could be directly verified by the scanning tunneling spectroscopy.

cond-mat.mtrl-sci

Quantization Phenomena of critical Hamiltonians in 2D systems

This review work addresses the recent advances in solving more comprehensive Hamiltonians. The generalized tight-binding model is developed to investigate the feature-rich quantization phenomena in emergent 2D materials. The mutli-orbital bondings, the spin-orbital interactions, the various geometric structures, and the external fields are taken into consideration simultaneously. Specifically, the IV-group layered systems, black phosphorus and MoS$_{2}$ exhibit the unique magnetic quantization. This is clearly indicated in three kinds of Landau levels (LLs), the orbital-, spin- and valley-dependent LL groups, the abnormal LL energy spectra, and the splitting, crossing and anticrossing behaviors. A detailed comparison with the effective-mass model is made. Some theoretical predictions have been confirmed by the experimental measurements.

cond-mat.mtrl-sci

Nitrogen-Functionalized Graphene Nanoflakes (GNFs:N): Tunable Photoluminescence and Electronic Structures

This study investigates the strong photoluminescence (PL) and X-ray excited optical luminescence observed in nitrogen-functionalized 2D graphene nanoflakes (GNFs:N), which arise from the significantly enhanced density of states in the region of π states and the gap between π and π* states. The increase in the number of the sp2 clusters in the form of pyridine-like N-C, graphite-N-like, and the C=O bonding and the resonant energy transfer from the N and O atoms to the sp2 clusters were found to be responsible for the blue shift and the enhancement of the main PL emission feature. The enhanced PL is strongly related to the induced changes of the electronic structures and bonding properties, which were revealed by the X-ray absorption near-edge structure, X-ray emission spectroscopy, and resonance inelastic X-ray scattering. The study demonstrates that PL emission can be tailored through appropriate tuning of the nitrogen and oxygen contents in GNFs and pave the way for new optoelectronic devices.

cond-mat.mtrl-sci