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S. Chiba

Publications and source records attributed to S. Chiba.

At least 19 recordsLinked to original sources

Shell effects and the neutron emission within the multi-dimensional Langevin model for nuclear fission

We solve the Langevin equations for the time evolution of parameters that describe the shape of fissioning system. On each integration step, we calculate the probability of neutron emission and estimate whether a neutron would be emitted or not. If yes, we decrease the excitation energy of the nucleus by the neutron separation energy plus the average energy of the emitted neutron, switch to the layer of potential energy surface with a smaller number of neutrons and continue the process of integration. If the trajectory reaches the scission point, we check how many neutrons were emitted along this trajectory. The pre-scission neutron multiplicity $M_{pre}$ is defined by the ratio of the total number of emitted neutrons to the total number of fission trajectories. Besides $M_{pre}$, the mass distribution of fission fragments, the distribution of emitted neutrons with respect to the fission stage (deformation of system) and the distribution of emitted neutrons with respect to their energies are calculated. The calculated quantities are compared with the available experimental data.

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Shell effects and multi-chance fission in the sub-lead region

Within the recently developed five-dimensional Langevin approach for the description of fission of heavy nuclei, we have calculated the fission fragments mass and kinetic energy distributions for the fission of $^{180}$Hg and $^{190}$Hg formed in the reactions $^{36}$Ar +$^{144}$Sm $\Rightarrow$ $^{180}$Hg and $^{36}$Ar +$^{154}$Sm $\Rightarrow$ $^{190}$Hg at few excitation energies and found very good agreement between the calculated and experimental results. Special attention was paid to the accurate description of the dependence of shell effects on the excitation energy. It was shown that the effect of multi-chance fission on the mass distribution is noticeable only at small excitation energies. The kinetic energy distributions are more sensitive to pre-scission neutron emission.

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The 5-dimensional Langevin approach to fission of atomic nuclei

We have generalized the four-dimensional Langevin approach used in our previous works for the description of fission process to the five-dimensional by considering the neck parameter $\eps$ in the two-center shell model shape parametrization as an independent dynamical variable. The calculated results for the mass distribution of fission fragments are in better agreement with the available experimental data. In particular, the transition from the mass-symmetric to mass-asymmetric fission via the triple-humped distribution in fission of Thorium isotopes is well reproduced.

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The Langevin approach for fission of heavy and super-heavy nuclei

In this contribution, we present the main relations of the Langevin approach to the description of fission or fusion-fission reactions. The results of Langevin calculations are shown for the mass distributions of fission fragments of super-heavy elements and used for the investigation of memory effects in nuclear fission.

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Memory effects in Langevin approach to the nuclear fission process

We present the schematic calculations within the Langevin approach in order to investigate the dependence of fission width on the memory time and the excitation energy at low temperatures where the quantum fluctuations play an important role. For this we consider the simple one-dimensional case with the potential energy given by two parabolic potentials (Kramers potential). For friction and the mass parameters we use the deformation independent values fitted to the results obtained earlier within the microscopic linear response theory. We have found out that at small excitation energies (comparable with the fission barrier height) the memory effects in the friction and random force acts on the fission width in opposite direction. The total effect is not so large, but still quite noticeable (depending on the value of the relaxation time). The use of effective temperature in the diffusion coefficient turns out to be much more important compared with the memory effects. The calculated fission width at very low excitation energies is unrealistically too big.

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Development of a Reference Database for Beta-Delayed Neutron Emission

Beta-delayed neutron emission is important for nuclear structure and astrophysics as well as for reactor applications. Significant advances in nuclear experimental techniques in the past two decades have led to a wealth of new measurements that remain to be incorporated in the databases. We report on a coordinated effort to compile and evaluate all the available beta-delayed neutron emission data. The different measurement techniques have been assessed and the data have been compared with semi-microscopic and microscopic-macroscopic models. The new microscopic database has been tested against aggregate total delayed neutron yields, time-dependent group parameters in 6-and 8-group re-presentation, and aggregate delayed neutron spectra. New recommendations of macroscopic delayed-neutron data for fissile materials of interest to applications are also presented. The new Reference Database for Beta-Delayed Neutron Emission Data is available online at: http://www-nds.iaea.org/beta-delayed-neutron/database.html.

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Description of the reactions 36S + 238U and 64Ni + 238U within the two-stage fusion-fission model

We describe the capture, fusion, fission and evaporation residue formation cross sections of superheavy nuclei within the proposed earlier two stages dynamical model. The approaching of the projectile nucleus to the target nucleus is described in the first stage of the model. On the second stage, the evolution of the system formed after the touching of the projectile and target nuclei is considered. The evolution of the system on both stages is described by Langevin equations. The transport coefficients of these equations are calculated within the microscopic linear response theory. The mutual orientation of the colliding ions, the tunneling through the Coulomb barrier in the entrance channel and the shell effects in the potential energy on both stages of the calculations are taking into account. The obtained results are compared with the available experimental data and other theoretical predictions.

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Fission of super-heavy elements: $^{132}$Sn-plus-the-rest, or $^{208}$Pb-plus-the-rest ?

In this work we try to settle down the controversial predictions on the effect of doubly magic nuclei $^{132}$Sn and $^{208}$Pb on the mass distributions of fission fragments of super-heavy nuclei. For this we have calculated the mass distribution of super-heavy nuclei from $^{286}$Cn to $^{306}$122 within the dynamical 4-dimensional Langevin approach. We have found that in "light" super-heavies the influence of $^{208}$Pb on the mass distributions is present but negligible small. In "heavy" super-heavies, Z=120-122, the (quasi)symmetric peaks and strongly asymmetric peaks at fragment mass $A_F$ close to $A_F$=208 are of comparable magnitude.

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Neutrino-13C Cross Sections at Supernova Neutrino Energies

We present neutrino capture cross sections on 13C at supernova neutrino energies, up to 50 MeV. For both charged-current and neutral-current reactions partial cross sections are calculated using statistical Hauser-Feschbach method. Coherent elastic neutrino scattering cross section for a 13C target is also provided.

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Description of the mass-asymmetric fission of the Pt isotopes, obtained in the reaction $^{36}$Ar + $^{142}$Nd within the two-stage fusion-fission model

The two stages dynamical stochastic model developed earlier for description of fusion-fission reactions is applied to the calculation of mass- and energy-distributions of fission fragments of platinum isotopes in reaction ${\rm ^{36}Ar + ^{142}Nd \to ^{178-x}Pt + xn}$. The first stage of this model is the calculation of the approaching of projectile nucleus to the target nucleus. On the second stage of the model, the evolution of the system formed after the touching of the projectile and target nuclei is considered. The evolution of the system on both stages is described by three-dimensional Langevin equations for the shape parameters of the system. The mutual orientation of the colliding ions and tunneling through the Coulomb barrier in the entrance channel are also taken into account. The potential energy of the system is calculated within the macroscopic-microscopic approach. The calculated mass-energy distributions of fission fragments are compared with the available experimental data. The impact of shell effects, rotation of the system and neutron evaporation on the calculated results is discussed.

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Correlated transitions in TKE and mass distributions of fission fragments described by 4-D Langevin equation

We have decomposed to symmetric and asymmetric modes the mass-TKE fission fragment distributions calculated by 4-dimensional Langevin approach and observed how the dominant fission mode and symmetric mode change as functions of $Z^2/\sqrt[3]{A}$ of the fissioning system in the actinides and trans-actinide region. As a result, we found that the symmetric mode makes a sudden transition from super-long to super short fission mode around $^{254}$Es. The dominant fission modes on the other hand, are persistently asymmetric except for $^{258}$Fm, $^{259}$Fm and $^{260}$Md when the dominant fission mode suddenly becomes symmetric although it returns to the asymmetric mode around $^{256}$No. These correlated "twin transitions" have been known empirically by Darleane Hoffman and her group back in 1989, but for the first time we have given a clear explanation in terms of a dynamical model of nuclear fission. More specifically, since we kept the shape model parameters unchanged over the entire mass region, we conclude that the correlated twin transition emerge naturally from the dynamics in 4-D potential energy surface.

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The temperature dependence of the shell corrections

We have examined the dependence of the shell correction to the nuclear liquid drop energy at finite excitations on the excitation energy (temperature). For this we have calculated the shell correction to the energy and free energy in very broad region of nuclei and deformations starting directly from their formal definitions. We have found out that the dependence of the shell corrections on the excitation energy differ substantially from the widely used approximation $δE(E^*)=δE(0)\exp(-E^*/E_d)$ both at small and large excitations. In particular, below the critical temperature at which the pairing effects vanish, the shell correction to the free energy is rather insensitive to the excitation energy. We suggest a more accurate approximation for the temperature dependence of the shell correction to the energy and free energy that is expressed in terms of the shell correction to the energy of independent particles and the shell correction to the pairing energy at T=0 and few fitted constants.

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A degree sum condition on the order, the connectivity and the independence number for Hamiltonicity

In [Graphs Combin.~24 (2008) 469--483.], the third author and the fifth author conjectured that if $G$ is a $k$-connected graph such that $σ_{k+1}(G) \ge |V(G)|+κ(G)+(k-2)(α(G)-1)$, then $G$ contains a Hamiltonian cycle, where $σ_{k+1}(G)$, $κ(G)$ and $α(G)$ are the minimum degree sum of $k+1$ independent vertices, the connectivity and the independence number of $G$, respectively. In this paper, we settle this conjecture. This is an improvement of the result obtained by Li: If $G$ is a $k$-connected graph such that $σ_{k+1}(G) \ge |V(G)|+(k-1)(α(G)-1)$, then $G$ is Hamiltonian. The degree sum condition is best possible.

math.CO

Predicting the optical observables for nucleon scattering on even-even actinides

Previously derived Lane consistent dispersive coupled-channel optical model for nucleon scattering on $^{232}$Th and $^{238}$U nuclei is extended to describe scattering on even-even actinides with $Z=$90--98. A soft-rotator-model (SRM) description of the low-lying nuclear structure is used, where SRM Hamiltonian parameters are adjusted to the observed collective levels of the target nucleus. SRM nuclear wave functions (mixed in $K$ quantum number) have been used to calculate coupling matrix elements of the generalized optical model. The "effective" deformations that define inter-band couplings are derived from SRM Hamiltonian parameters. Conservation of nuclear volume is enforced by introducing a dynamic monopolar term to the deformed potential leading to additional couplings between rotational bands. Fitted static deformation parameters are in very good agreement with those derived by Wang and collaborators using the Weizsäcker-Skyrme global mass model (WS4), allowing to use the latter to predict cross section for nuclei without experimental data. A good description of scarce "optical" experimental database is achieved. SRM couplings and volume conservation allow a precise calculation of the compound-nucleus formation cross sections, which is significantly different from the one calculated with rigid-rotor potentials coupling the ground-state rotational band. Derived parameters can be used to describe both neutron and proton induced reactions.

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Nucleon scattering on actinides using a dispersive optical model with extended couplings

Tamura coupling model has been extended to consider the coupling of additional low-lying rotational bands to the ground state band. Rotational bands are built on vibrational bandheads (even-even targets) or single particle bandheads (odd-$A$ targets) including both axial and non-axial deformations. These additional excitations are introduced as a perturbation to the underlying axially-symmetric rigid rotor structure of the ground state rotational band. Coupling matrix elements of the generalized optical model are derived for extended multi-band transitions in even-even and odd-$A$ nuclei. Isospin symmetric formulation of the optical model is employed. A coupled-channels optical model potential (OMP) containing a dispersive contribution is used to fit simultaneously all available optical experimental databases including neutron strength functions for nucleon scattering on $^{232}$Th, $^{233,235,238}$U and $^{239}$Pu nuclei and quasi-elastic ($p$,$n$) scattering data on $^{232}$Th and $^{238}$U. Lane consistent OMP is derived for all actinides if corresponding multi-band coupling schemes are defined. Calculations using the derived OMP potential reproduce measured total cross-section differences between several actinide pairs within experimental uncertainty for incident neutron energies from 50 keV up to 150MeV. Multi-band coupling is stronger in even-even targets due to the collective nature of the coupling; the impact of extended coupling on predicted compound-nucleus formation cross section reaches 5% below 3 MeV of incident neutron energy. Coupling of ground-state rotational band levels in odd-$A$ nuclei is sufficient for a good description of the compound-nucleus formation cross sections as long as the coupling is saturated (a minimum of 7 coupled levels are typically needed).

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Relative contributions of the weak, main and fission-recycling r-process

There has been a persistent conundrum in attempts to model the nucleosynthesis of heavy elements by rapid neutron capture (the $r$-process). Although the location of the abundance peaks near nuclear mass numbers 130 and 195 identify an environment of rapid neutron capture near closed nuclear shells, the abundances of elements just above and below those peaks are often underproduced by more than an order of magnitude in model calculations. At the same time there is a debate in the literature as to what degree the $r$-process elements are produced in supernovae or the mergers of binary neutron stars. In this paper we propose a novel solution to both problems. We demonstrate that the underproduction of elements above and below the $r$-process peaks characteristic in the main or weak $r$-process events (like magnetohydrodynamic jets or neutrino-driven winds in core-collapse supernovae) can be supplemented via fission fragment distributions from the recycling of material in a neutron-rich environment such as that encountered in neutron star mergers. In this paradigm, the abundance peaks themselves are well reproduced by a moderately neutron rich, main $r$-process environment such as that encountered in the magnetohydrodynamical jets in supernovae supplemented with a high-entropy, weakly neutron rich environment such as that encountered in the neutrino-driven-wind model to produce the lighter $r$-process isotopes. Moreover, we show that the relative contributions to the $r$-process abundances in both the solar-system and metal-poor stars from the weak, main, and fission-recycling environments required by this proposal are consistent with estimates of the relative Galactic event rates of core-collapse supernovae for the weak and main $r$-process and neutron star mergers for the fission-recycling $r$-process.

astro-ph.SR

Fission dynamics at low excitation energy. 2

The mass asymmetry in the fission of U-236 at low excitation energy is clarified by the analysis of the trajectories obtained by solving the Langevin equations for the shape degrees of freedom. It is demonstrated that the position of the peaks in the mass distribution of fission fragments is determined mainly by the saddle point configuration originating from the shell correction energy. The width of the peaks, on the other hand, results from the shape fluctuations close to the scission point caused by the random force in the Langevin equation. We have found out that the fluctuations between elongated and compact shapes are essential for the fission process. According to our results the fission does not occur with continuous stretching in the prolate direction, similarly to that observed in starch syrup, but is accompanied by the fluctuations between elongated and compact shapes. This picture presents a new viewpoint of fission dynamics and the splitting mechanism.

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