arXiv subjects

S. Datta

Publications and source records attributed to S. Datta.

At least 37 records · Page 2Linked to original sources

arXiv2010

Voltage controlled spin precession

A recent experiment reports a non-local spin-signal that shows oscillatory behavior as a function of gate voltage when the contacts are magnetized along the direction of current flow, but not when they are magnetized perpendicular to the current, in agreement with the predictions from a simple theory. In this paper we first present a straightforward extension of this theory to include the angular spectrum of electrons and the extended injecting and detecting contacts. The results are in good agreement with those from a non-equilibrium Green function (NEGF)- based model with contact parameters adjusted to fit the experimental contact conductances. They also describe certain aspects of the experiment fairly well, but other aspects deserve further investigation.

cond-mat.mes-hall↗

arXiv2009

Crystal lattice desolvation effects on the magnetic quantum tunneling of single-molecule magnets

High-frequency electron paramagnetic resonance (HFEPR) and AC susceptibility measurements are reported for a new high-symmetry Mn12 complex, [Mn12O12(O2CCH3)16(CH3OH)4].CH3OH. The results are compared with those of other high-symmetry spin S = 10 Mn12 single-molecule magnets (SMMs), including the original acetate, [Mn12(O2CCH3)16(H2O)4].2CH3CO2H.4H2O, and the [Mn12O12(O2CCH2Br)16(H2O)4].4CH2Cl2 & [Mn12O12(O2CCH2But)16(CH3OH)4].CH3OH complexes. These comparisons reveal important insights into the factors that influence the values of the effective barrier to magnetization reversal, Ueff, deduced on the basis of AC susceptibility measurements. In particular, we find that variations in Ueff can be correlated with the degree of disorder in a crystal which can be controlled by desolvating (drying) samples. This highlights the importance of careful sample handling when making measurements on SMM crystals containing volatile lattice solvents. The HFEPR data additionally provide important spectroscopic evidence suggesting that the relatively weak disorder induced by desolvation strongly influences the quantum tunneling interactions, and that it is under-barrier tunneling that is responsible for a consistent reduction in Ueff that is found upon drying samples. Meanwhile, the axial anisotropy deduced from HFEPR is found to be virtually identical for all four Mn12 complexes, with essentially no measurable reduction upon desolvation.

cond-mat.mes-hall↗

arXiv2008

Electronic transport driven spin-dynamics

We propose a model to explore the dynamics of spin-systems coupled by exchange interaction to the conduction band electrons of a semiconductor material that forms the channel in a ferromagnet/semiconductor/ferromagnet spin-valve structure. We show that recent observation of the novel transient transport signature in a MnAs/GaAs/MnAs spin-valve structure with paramagnetic Mn impurities [D. Saha et al., Phys. Rev. Lett., 100, 196603 (2008)] can be quantitatively understood in terms of current driven dynamical polarization of Mn spins. Using our model of spin polarized transport through Schottky barriers at the two ferromagnet/semiconductor junctions in a spin-valve structure and a dynamical equation describing the paramagnetic impurities coupled to conduction band electrons we explain the scaling behaviour of observed transient features such as the magnitude and time-scale with temperature.

cond-mat.mes-hall↗

arXiv2008

The Spatial String Tension and Dimensional Reduction in QCD

We calculate the spatial string tension in (2+1) flavor QCD with physical strange quark mass and almost physical light quark masses using lattices with temporal extent N_tau=4,6 and 8. We compare our results on the spatial string tension with predictions of dimensionally reduced QCD. This suggests that also in the presence of light dynamical quarks dimensional reduction works well down to temperatures 1.5T_c.

hep-lat↗

arXiv2008

The QCD Equation of State with almost Physical Quark Masses

We present results on the equation of state in QCD with two light quark flavors and a heavier strange quark. Calculations with improved staggered fermions have been performed on lattices with temporal extent Nt =4 and 6 on a line of constant physics with almost physical quark mass values; the pion mass is about 220 MeV, and the strange quark mass is adjusted to its physical value. High statistics results on large lattices are obtained for bulk thermodynamic observables, i.e. pressure, energy and entropy density, at vanishing quark chemical potential for a wide range of temperatures, 140 MeV < T < 800 MeV. We present a detailed discussion of finite cut-off effects which become particularly significant for temperatures larger than about twice the transition temperature. At these high temperatures we also performed calculations of the trace anomaly on lattices with temporal extent Nt=8. Furthermore, we have performed an extensive analysis of zero temperature observables including the light and strange quark condensates and the static quark potential at zero temperature. These are used to set the temperature scale for thermodynamic observables and to calculate renormalized observables that are sensitive to deconfinement and chiral symmetry restoration and become order parameters in the infinite and zero quark mass limits, respectively.

hep-lat↗

arXiv2007

Direct observation of mixing of spin-multiplets in an antiferromagnetic molecular nanomagnet by electron paramagnetic resonance

High-frequency electron paramagnetic resonance (EPR) studies of the antiferromagnetic Mn-$[3\times 3]$ molecular grid clearly reveal a breaking of the $ΔS = 0$ selection rule, providing direct evidence for the mixing of spin wavefunctions ($S$-mixing) induced by the comparable exchange and magneto-anisotropy energy scales within the grid. This finding highlights the potential utility of EPR for studies of exchange splittings in molecular nanomagnets, which is normally considered the sole domain of inelastic neutron scattering, thereby offering improved sensitivity and energy resolution.

cond-mat.other↗

arXiv2007

Structure, bonding and magnetism in cobalt clusters

The structural, electronic and magnetic properties of Co$_n$ clusters ($n=2-$20) have been investigated using density functional theory within the pseudopotential plane wave method. An unusual hexagonal growth pattern has been observed in the intermediate size range, $n=15-$20. The cobalt atoms are ferromagnetically ordered and the calculated magnetic moments are found to be higher than that of corresponding hcp bulk value, which are in good agreement with the recent Stern-Gerlach experiments. The average coordination number is found to dominate over the average bond length to determine the effective hybridization and consequently the cluster magnetic moment.

physics.atm-clus↗

arXiv2006

The transition temperature in QCD

We present a detailed calculation of the transition temperature in QCD with two light and one heavier (strange) quark mass on lattices with temporal extent N_t =4 and 6. Calculations with improved staggered fermions have been performed for various light to strange quark mass ratios in the range, 0.05 <= m_l/m_s <= 0.5, and with a strange quark mass fixed close to its physical value. From a combined extrapolation to the chiral (m_l -> 0) and continuum (aT = 1/N_t -> 0) limits we find for the transition temperature at the physical point T_c r_0 = 0.457(7) where the scale is set by the Sommer-scale parameter r_0 defined as the distance in the static quark potential at which the slope takes on the value, (dV_qq(r)/dr)_r=r_0 = 1.65/r_0^2. Using the currently best known value for r_0 this translates to a transition temperature T_c = 192(7)(4)MeV. The transition temperature in the chiral limit is about 3% smaller. We discuss current ambiguities in the determination of T_c in physical units and also comment on the universal scaling behavior of thermodynamic quantities in the chiral limit.

hep-lat↗

arXiv2006

Phonon runaway in nanotube quantum dots

We explore electronic transport in a nanotube quantum dot strongly coupled with vibrations and weakly with leads and the thermal environment. We show that the recent observation of anomalous conductance signatures in single-walled carbon nanotube (SWCNT) quantum dots can be understood quantitatively in terms of current driven `hot phonons' that are strongly correlated with electrons. Using rate equations in the many-body configuration space for the joint electron-phonon distribution, we argue that the variations are indicative of strong electron-phonon coupling requiring an analysis beyond the traditional uncorrelated phonon-assisted transport (Tien-Gordon) approach.

cond-mat.mes-hall↗

arXiv2006

Meson correlation functions at high temperatures

We present preliminary results for the correlation- and spectral functions of different meson channels on the lattice. The main focus lies on gaining control over cut-off as well as on the finite-volume effects. Extrapolations of screening masses above the deconfining temperature are guided by the result of the free ($T=\infty$) case on the lattice and in the continuum. We study the quenched non-perturbatively improved Wilson-clover fermion as well as the hypercube fermion action which might show less cut-off effects.

hep-lat↗

arXiv2006

Quarkonia in a deconfined gluonic plasma

We discuss lattice results on the properties of finite momentum charmonium states in a gluonic plasma. We also present preliminary results for bottomonium correlators and spectral functions in the plasma. Significant modifications of chi_b states are seen at temperatures of 1.5 Tc.

hep-lat↗

arXiv2005

Probing electronic excitations in molecular conduction

We identify experimental signatures in the current-voltage (I-V) characteristics of weakly contacted molecules directly arising from excitations in their many electron spectrum. The current is calculated using a multielectron master equation in the Fock space of an exact diagonalized model many-body Hamiltonian for a prototypical molecule. Using this approach, we explain several nontrivial features in frequently observed I-Vs in terms of a rich spectrum of excitations that may be hard to describe adequately with standard one-electron self-consistent field (SCF) theories.

cond-mat.mes-hall↗

arXiv2005

Heavy Quarkonium Physics

This report is the result of the collaboration and research effort of the Quarkonium Working Group over the last three years. It provides a comprehensive overview of the state of the art in heavy-quarkonium theory and experiment, covering quarkonium spectroscopy, decay, and production, the determination of QCD parameters from quarkonium observables, quarkonia in media, and the effects on quarkonia of physics beyond the Standard Model. An introduction to common theoretical and experimental tools is included. Future opportunities for research in quarkonium physics are also discussed.

hep-ph↗

arXiv2004

Meson correlators above deconfinement

We review recent progress in studying spectral functions for mesonic observables at finite temperatures, by analysis of imaginary time correlators directly calculated on isotropic lattices. Special attention is paid to the lattice artifacts present in such calculations.

hep-lat↗

arXiv2004

Heavy-light decay constants using clover valence quarks and three flavors of dynamical improved staggered quarks

Starting in 2001, the MILC Collaboration began a large scale calculation of heavy-light meson decay constants using clover valence quarks on ensembles of three flavor configurations. For the coarse configurations, with a=0.12 fm, eight combinations of dynamical light and strange quarks have been analyzed. For the fine configurations, with a=0.09 fm, three combinations of quark masses are studied. Since we last reported on this calculation, statistics have been increased on the fine ensembles, and, more importantly, a preliminary value for the perturbative renormalization of the axial-vector current has become available. Thus, results for f_B, f_{B_s}, f_D and f_{D_s} can, in principle, be calculated in MeV, in addition to decay-constant ratios that were calculated previously.

hep-lat↗

arXiv2004

Charging induced asymmetry in molecular conductors

We investigate the origin of asymmetry in various measured current-voltage (I-V) characteristics of molecules with no inherent spatial asymmetry, with particular focus on a recent break junction measurement. We argue that such asymmetry arises due to unequal coupling with the contacts and a consequent difference in charging effects, which can only be captured in a self-consistent model for molecular conduction. The direction of the asymmetry depends on the sign of the majority carriers in the molecule. For conduction through highest occupied molecular orbitals (i.e. HOMO or p-type conduction), the current is smaller for positive voltage on the stronger contact, while for conduction through lowest unoccupied molecular orbitals (i.e. LUMO or n-type conduction), the sense of the asymmetry is reversed. Within an extended Huckel description of the molecular chemistry and the contact microstructure (with two adjustable parameters, the position of the Fermi energy and the sulphur-gold bond length), an appropriate description of Poisson's equation, and a self-consistently coupled non-equilibrium Green's function (NEGF) description of transport, we achieve good agreement between theoretical and experimental I-V characteristics, both in shape as well as overall magnitude.

cond-mat.mes-hall↗

arXiv2003

Charmonium at finite temperature

We study charmoinum correlators and spectral functions at finite temperature within the quenched approximation using isotropic lattices with lattice spacing a^-1=4.86 GeV and 9.72 GeV. Although we observe some medium modifications of the ground state charmonium spectral function above deconfinement, we find that ground state charmonia (J/psi and eta_c) exist in the deconfined phase at least up to temperatures as high as 1.5Tc. P-wave charmonia (chi_c) on the other hand are dissociated already at 1.12Tc.

hep-lat↗

arXiv2003

Silicon-based molecular electronics

Molecular electronics on silicon has distinct advantages over its metallic counterpart. We describe a theoretical formalism for transport through semiconductor-molecule heterostructures, combining a semi-empirical treatment of the bulk silicon bandstructure with a first-principles description of the molecular chemistry and its bonding with silicon. Using this method, we demonstrate that the presence of a semiconducting band-edge can lead to a novel molecular resonant tunneling diode (RTD) that shows negative differential resistance (NDR) when the molecular levels are driven by an STM potential into the semiconducting band-gap. The peaks appear for positive bias on a p-doped and negative for an n-doped substrate. Charging in these devices is compromised by the RTD action, allowing possible identification of several molecular highest occupied (HOMO) and lowest unoccupied (LUMO) levels. Recent experiments by Hersam et al. [1] support our theoretical predictions.

cond-mat.mes-hall↗