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S. E. A. Orrigo

Publications and source records attributed to S. E. A. Orrigo.

At least 19 recordsLinked to original sources

Measurement of the ambient neutron flux and spectral distribution at the Canfranc Underground Laboratory

We report on the measurement of the ambient neutron flux and its energy distribution over a broad range of neutron energies, conducted in Hall A of the Canfranc Underground Laboratory using the High Efficiency Neutron Spectrometry Array (HENSA), with a total livetime of 248 days. In particular, we obtained a thermal neutron flux of $3.4(2) \times 10^{-6}$ cm$^{-2}$ s$^{-1}$ and a total energy-integrated flux of $14.8(2) \times 10^{-6}$ cm$^{-2}$ s$^{-1}$. This work represents the first long-term measurement of the ambient neutron flux that includes a full spectral characterization across a wide energy interval (from $10^{-4}$ eV to 20 MeV), performed in an underground laboratory to date. The results are relevant for rare-event search experiments located underground, ranging from nuclear astrophysics to astroparticle physics.

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Status of the HENSA collaboration at the Canfranc Underground Laboratory: results from two years of measurement of the neutron flux in hall B

Thiswork deals with the characterization of the neutron flux in hall B of the CanfrancUnderground Laboratory (LSC) employing the High Efficiency Neutron Spectrometry Array (HENSA). The ultimate goal of this measurement is to set a limit on the corresponding effects of the neutron flux in the background of the ANAIS-112 experiment. The preliminary neutron counting rates of two years of measurement are reported. Various data analysis techniques, including pulse shape discrimination, are discussed. The first results on the spectral reconstruction of the neutron flux are also presented.

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The beta decay of Tz=-2 64Se and its descendants: the T=2 isobaric multiplet

In this paper we present our results on the decay of 64Se. It is the heaviest Tz=-2 nucleus that both beta decays and has a stable mirror partner Tz=+2, thus allowing comparison with charge exchange reaction studies. The beta decays of 64Se and its descendants were studied at the RIKEN Nishina Center (Tokyo, Japan) following their production in the fragmentation of 78Kr on a beryllium target. Beta-delayed gamma-ray and particle radiation was identified for each of the nuclei in the decay chain allowing us to obtain decay schemes for 64Se, 64As, and 63Ge. Thus new excited states could be found for the descendant nuclei, including the interesting case of the N=Z nucleus 64Ge. Furthermore we observed for the first time the beta-delayed proton emission of 64Se and 64As. Based on these results we obtained proton branching ratios of 48.0(9)% in 64Se decay and 4.4(1)% in 64As decay. We obtained a half-life value of 22.5(6) ms for 64Se decay and half-lives slightly more precise than those in the literature for each nucleus involved in the decay chain. Using our results on the excited levels of 64As and the mass excess in the literature for 63Ge we obtained -39588(50) keV for the mass excess of 64As. Then based on the IMME we obtained the mass excess of -27429(88) keV for 64Se by extrapolation. The mirror process of 64Se beta decay, the charge exchange reaction 64Zn(3He,t)64Ga, has already been measured allowing us to study the mirror symmetry through the comparison of the weak force (beta decay) and strong force (charge exchange reaction). An interpretation of the decay schemes based on the idea of the Anti Analogue State is proposed.

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Isospin breaking in the $^{71}$Kr and $^{71}$Br mirror system

Isospin symmetry is a fundamental concept in nuclear physics. Even though isospin symmetry is partially broken, it holds approximately for most nuclear systems, which makes exceptions very interesting from the nuclear structure perspective. In this framework, it is expected that the spins and parities of the ground states of mirror nuclei should be the same, in particular for the simplest systems where a proton is exchanged with a neutron or vice versa. In this work, we present evidence that this assumption is broken in the mirror pair $^{71}$Br and $^{71}$Kr system. Our conclusions are based on a high-statistics $β$ decay study of $^{71}$Kr and on state-of-the-art shell model calculations. In our work, we also found evidence of a new state in $^{70}$Se, populated in the $β$-delayed proton emission process which can be interpreted as the long sought coexisting 0$^+$ state.

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First Exploration of Monopole-Driven Shell Evolution above the N = 126 shell closure: new Millisecond Isomers in 213Tl and 215Tl

Isomer spectroscopy of heavy neutron-rich nuclei beyond the N=126 closed shell has been performed for the first time at the Radioactive Isotope Beam Factory of the RIKEN Nishina Center. New millisecond isomers have been identified at low excitation energies, 985.3(19) keV in 213Tl and 874(5) keV in 215Tl. The measured half-lives of 1.34(5) ms in 213Tl and 3.0(3) ms in 215Tl suggest spins and parities 11/2- with the single proton-hole configuration h11/2 as leading component. They are populated via E1 transitions by the decay of higher-lying isomeric states with proposed spin and parity 17/2+, interpreted as arising from a single s1/2 proton hole coupled to the 8+ seniority isomer in the (A+1)Pb cores. The lowering of the 11/2- states is ascribed to an increase of the h11/2 proton effective single-particle energy as the second g9/2 orbital is filled by neutrons, owing to a significant reduction of the proton-neutron monopole interaction between the h11/2 and g9/2 orbitals. The new ms-isomers provide the first experimental observation of shell evolution in the almost unexplored N>126 nuclear region below doubly-magic 208Pb.

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A walk along the proton drip-line by $β$-decay spectroscopy

During the last decade we have carried out a systematic study of the $β$ decay of neutron-deficient nuclei, providing rich spectroscopic information of importance for both nuclear structure and nuclear astrophysics. We present an overview of the most relevant achievements, including the discovery of a new exotic decay mode in the fp-shell, the $β$-delayed $γ$-proton decay in $^{56}$Zn, the first observation of the 2$^+$ isomer in $^{52}$Co and the latest results on the heavier systems $^{60}$Ge and $^{62}$Ge. We also report on our deduced mass excesses in comparison with systematics and a recent measurement. Finally, we summarise our results on the half-lives of $T_z=$ -1/2, -1 and -2 neutron-deficient nuclides, and analyse their trend.

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$β$-decay spectroscopy of neutron-deficient nuclei

A systematic study of the $β$-decay of neutron-deficient nuclei has been carried out and has provided spectroscopic information of importance for both nuclear structure and nuclear astrophysics. Following an overview of the most relevant achievements, we focus on the latest results on the $β$ decay of $^{60}$Ge and $^{62}$Ge. We also summarise our results on the mass excesses in comparison with systematics and a recent measurement. Finally, we present updated half-life trends for $T_z=$ -1/2, -1 and -2 neutron-deficient nuclides.

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Bulk and decay properties of neutron-deficient odd-mass Hg isotopes around A = 185

Ground and isomeric states of the neutron-deficient odd-$A$ isotopes $^{183}$Hg, $^{185}$Hg, and $^{187}$Hg are described from a microscopic calculation based on a self-consistent, axially-deformed Hartree-Fock mean field with the Skyrme functional and pairing within BCS approximation. For each equilibrium shape and different odd-neutron states, results on mean square charge radii and magnetic dipole moments are given and analyzed in the context of their sensitivity to the nuclear deformation and to the spin and parity. Spin-isospin correlations within proton-neutron quasiparticle random phase approximation are then introduced in the nuclear states to obtain the distributions of Gamow-Teller strength and the $β^+/EC$ half-lives of these isotopes, whose measurements are planned at ISOLDE-CERN using total absorption gamma-ray spectroscopy techniques.

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Long-term evolution of the neutron rate at the Canfranc Underground Laboratory

We report results on the long-term variation of the neutron counting rate at the Canfranc Underground Laboratory, of importance for several low-background experiments installed there, including rare-event searches. The measurement campaign was performed employing the High Efficiency Neutron Spectrometry Array (HENSA) mounted in Hall A and lasted 412 live days. The present study is the first long-term measurement of the neutron rate with sensitivity over a wide range of neutron energies (from thermal up to 0.1 GeV and beyond) performed in any underground laboratory so far. Data on the environmental variables inside the experimental hall (radon concentration, air temperature, air pressure and humidity) were also acquired during all the measurement campaign. We have investigated for the first time the evolution of the neutron rate for different energies of the neutrons and its correlation with the ambient variables.

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Total absorption $γ$-ray spectroscopy of the $β$ decays of $^{96\text{gs,m}}$Y

The $β$ decays of the ground state (gs) and isomeric state (m) of $^{96}$Y have been studied with the total absorption $γ$-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility. The separation of the 8$^{+}$ isomeric state from the 0$^{-}$ ground state was achieved thanks to the purification capabilities of the JYFLTRAP double Penning trap system. The $β$-intensity distributions of both decays have been independently determined. In the analyses the de-excitation of the 1581.6 keV level in $^{96}$Zr, in which conversion electron emission competes with pair production, has been carefully considered and found to have significant impact on the $β$-detector efficiency, influencing the $β$-intensity distribution obtained. Our results for $^{96\text{gs}}$Y (0$^+$) confirm the large ground state to ground state $β$-intensity probability, although a slightly larger value than reported in previous studies was obtained, amounting to $96.6_{-2.1}^{+0.3}\%$ of the total $β$ intensity. Given that the decay of $^{96\text{gs}}$Y is the second most important contributor to the reactor antineutrino spectrum between 5 and 7 MeV, the impact of the present results on reactor antineutrino summation calculations has been evaluated. In the decay of $^{96\text{m}}$Y (8$^{+}$), previously undetected $β$ intensity in transitions to states above 6 MeV has been observed. This shows the importance of total absorption $γ$-ray spectroscopy measurements of $β$ decays with highly fragmented de-excitation patterns. $^{96\text{m}}$Y (8$^{+}$) is a major contributor to reactor decay heat in uranium-plutonium and thorium-uranium fuels around 10 s after fission pulses, and the newly measured average $β$ and $γ$ energies differ significantly from the previous values in evaluated databases (...)

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Beta decay of the very neutron-deficient $^{60}$Ge and $^{62}$Ge nuclei

We report here the results of a study of the $β$ decay of the proton-rich Ge isotopes, $^{60}$Ge and $^{62}$Ge, produced in an experiment at the RIKEN Nishina Center. We have improved our knowledge of the half-lives of $^{62}$Ge (73.5(1) ms), $^{60}$Ge (25.0(3) ms) and its daughter nucleus, $^{60}$Ga (69.4(2) ms). We measured individual $β$-delayed proton and $γ$ emissions and their related branching ratios. Decay schemes and absolute Fermi and Gamow-Teller transition strengths have been determined. The mass excesses of the nuclei under study have been deduced. A total $β$-delayed proton-emission branching ratio of 67(3)% has been obtained for $^{60}$Ge. New information has been obtained on the energy levels populated in $^{60}$Ga and on the 1/2$^-$ excited state in the $βp$ daughter $^{59}$Zn. We extracted a ground state to ground state feeding of 85.3(3)% for the decay of $^{62}$Ge. Eight new $γ$ lines have been added to the de-excitation of levels populated in the $^{62}$Ga daughter.

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Measurement of the neutron flux at the Canfranc Underground Laboratory with HENSA

We have performed a long-term measurement of the neutron flux with the High Efficiency Neutron Spectrometry Array HENSA in the Hall A of the Canfranc Underground Laboratory. The Hall A measurement campaign lasted from October 2019 to March 2021, demonstrating an excellent stability of the HENSA setup. Preliminary results on the neutron flux from this campaign are presented for the first time. In Phase 1 (113 live days) a total neutron flux of 1.66(2) $\times$10$^{-5}$ cm$^{-2}$ s$^{-1}$ is obtained. Our results are in good agreement with those from our previous shorter measurement where a reduced experimental setup was employed.

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On the $β$-decay of $^{186}$Hg

The Gamow-Teller strength distribution of the decay of $^{186}$Hg into $^{186}$Au has been determined for the first time using the total absorption gamma spectroscopy technique and has been compared with theoretical QRPA calculations using the SLy4 Skyrme force. The measured Gamow-Teller strength distribution and the half-life are described by mixing oblate and prolate configurations independently in the parent and daughter nuclei. The best description of the experimental beta strength is obtained with dominantly prolate components for both parent $^{186}$Hg and daughter $^{186}$Au. The approach also allowed us to determine an upper limit of the oblate component in the parent state. The complexity of the analysis required the development of a new approach in the analysis of the X-ray gated total absorption spectrum.

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Determination of Beta Decay Ground State Feeding of Nuclei of Importance for Reactor Applications

In $β$-decay studies the determination of the decay probability to the ground state of the daughter nucleus often suffers from large systematic errors. The difficulty of the measurement is related to the absence of associated delayed $γ$-ray emission. In this work we revisit the $4πγ-β$ method proposed by Greenwood and collaborators in the 1990s, which has the potential to overcome some of the experimental difficulties. Our interest is driven by the need to determine accurately the $β$-intensity distributions of fission products that contribute significantly to the reactor decay heat and to the antineutrinos emitted by reactors. A number of such decays have large ground state branches. The method is relevant for nuclear structure studies as well. Pertinent formulae are revised and extended to the special case of $β$-delayed neutron emitters, and the robustness of the method is demonstrated with synthetic data. We apply it to a number of measured decays that serve as test cases and discuss the features of the method. Finally, we obtain ground state feeding intensities with reduced uncertainty for four relevant decays that will allow future improvements in antineutrino spectrum and decay heat calculations using the summation method.

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Total absorption $γ$-ray spectroscopy of the $β$-delayed neutron emitters $^{137}$I and $^{95}$Rb

The decays of the $β$-delayed neutron emitters $^{137}$I and $^{95}$Rb have been studied with the total absorption $γ$-ray spectroscopy technique. The purity of the beams provided by the JYFLTRAP Penning trap at the ion guide isotope separator on-line facility in Jyväskylä allowed us to carry out a campaign of isotopically pure measurements with the decay total absorption $γ$-ray spectrometer, a segmented detector composed of eighteen NaI(Tl) modules. The contamination coming from the interaction of neutrons with the spectrometer has been carefully studied, and we have tested the use of time differences between prompt $γ$-rays and delayed neutron interactions to eliminate this source of contamination. Due to the sensitivity of our spectrometer, we have found a significant amount of $β$-intensity to states above the neutron separation energy that de-excite by $γ$-rays, comparable to the neutron emission probability. The competition between $γ$ de-excitation and neutron emission has been compared with Hauser-Feshbach calculations, and it can be understood as a nuclear structure effect. In addition, we have studied the impact of the $β$-intensity distributions determined in this work on reactor decay heat and reactor antineutrino spectrum summation calculations. The robustness of our results is demonstrated by a thorough study of uncertainties, and with the reproduction of the spectra of the individual modules and the module-multiplicity gated spectra. This work represents the state-of-the-art of our analysis methodology for segmented total absorption spectrometers.

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Total absorption $γ$-ray spectroscopy of niobium isomers

The $β$ intensity distributions of the decays of $^{100\text{gs},100\text{m}}$Nb and $^{102\text{gs},102\text{m}}$Nb have been determined using the Total Absorption $γ$-Ray Spectroscopy technique. The JYFLTRAP double Penning trap system was employed to disentangle the isomeric states involved, lying very close in energy, in a campaign of challenging measurements performed with the Decay Total Absorption $γ$-ray Spectrometer at the Ion Guide Isotope Separator On-Line facility in Jyväskylä. The low-spin isomeric state of each niobium case was populated through the decay of the zirconium parent, that was treated as a contaminant. We have applied a method to extract this contamination, and additionally we have obtained $β$ intensity distributions for these zirconium decays. The $β$-strength distributions evaluated with these results were compared with calculations in quasiparticle random-phase approximation, suggesting a prolate configuration for the ground states of $^{100,102}$Zr. The footprint of the Pandemonium effect was found when comparing our results for the analyses of the niobium isotopes with previous decay data. The $β$-intensities of the decay of $^{102\text{m}}$Nb were obtained for the first time. A careful evaluation of the uncertainties was carried out, and the consistency of our results was validated taking advantage of the segmentation of our spectrometer. The final results were used as input in reactor summation calculations. A large impact on antineutrino spectrum calculations was already reported and here we detail the significant impact on decay heat calculations.

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First determination of $β$-delayed multiple neutron emission beyond A = 100 through direct neutron measurement: The P$_{2n}$ value of $^{136}$Sb

Background: $β$-delayed multiple neutron emission has been observed for some nuclei with A$\leq$100, with $^{100}$Rb being the heaviest $β$2n emitter measured to date. So far, only 25 P$_{2n}$ values have been determined for the $\sim$300 nuclei that may decay in this way. Accordingly, it is of interest to measure P$_{2n}$ values for the other possible multiple neutron emitters throughout the chart of the nuclides. It is of particular interest to make such measurement for nuclei with A$>$100 to test the predictions of theoretical models and simulation tools for the decays of heavy nuclei in the region of very neutron-rich nuclei. In addition, the decay properties of these nuclei are fundamental for the understanding of astrophysical nucleosynthesis processes such as the $r$-process, and safety inputs for nuclear reactors. Purpose: To determine for the first time the two neutron branching ratio, P$_{2n}$ value, for $^{136}$Sb through a direct neutron measurement, and to provide precise P$_{1n}$ values for $^{136}$Sb and $^{136}$Te. Method: Pure beams were provided by the JYFLTRAP at the IGISOL facility of the University of Jyväskylä, Finland. The purified ions were implanted into a moving tape at the end of the beam line. The detection setup consisted of a plastic scintillator placed right behind the implantation point, and the BELEN detector, based on neutron counters embedded in a polyethylene matrix. The analysis was based on the study of the $β$- and neutron- growth-and-decay curves and the $β$-one-neutron and $β$-two-neutron time correlations. Results: The P$_{2n}$ value of $^{136}$Sb was found to be 0.14(3)\% and the measured P$_{1n}$ values for $^{136}$Sb and $^{136}$Te were found to be 32.2(15)\% and 1.47(6)\%, respectively. The measured P$_{2n}$ value is a factor 44 smaller than predicted by the FRDM+QRPA model used for $r$-process calculations.

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Characterization and performance of the DTAS detector

DTAS is a segmented total absorption γ-ray spectrometer developed for the DESPEC experiment at FAIR. It is composed of up to eighteen NaI(Tl) crystals. In this work we study the performance of this detector with laboratory sources and also under real experimental conditions. We present a procedure to reconstruct offline the sum of the energy deposited in all the crystals of the spectrometer, which is complicated by the effect of NaI(Tl) light-yield non-proportionality. The use of a system to correct for time variations of the gain in individual detector modules, based on a light pulse generator, is demonstrated. We describe also an event-based method to evaluate the summing-pileup electronic distortion in segmented spectrometers. All of this allows a careful characterization of the detector with Monte Carlo simulations that is needed to calculate the response function for the analysis of total absorption γ-ray spectroscopy data. Special attention was paid to the interaction of neutrons with the spectrometer, since they are a source of contamination in studies of \b{eta}-delayed neutron emitting nuclei.

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