arXiv subjects

S. E. Agbemava

Publications and source records attributed to S. E. Agbemava.

At least 19 recordsLinked to original sources

arXiv2023

Hexadecapole strength in the rare isotopes $^{74,76}$Kr

In the Ge-Sr mass region, isotopes with neutron number $N \leq 40$ are known to feature rapid shape changes with both nucleon number and angular momentum. To gain new insights into their structure, inelastic proton scattering experiments in inverse kinematics were performed on the rare isotopes $^{74,76}$Kr. This work focuses on observables related to the $J^π = 4^+_1$ states of the Kr isotopes and, in particular, on the hexadecapole degree of freedom. By performing coupled-channels calculations, hexadecapole deformation parameters $β_4$ were determined for the $J^π = 4^+_1$ states of $^{74,76}$Kr from inelastic proton scattering cross sections. Two possible coupled-channels solutions were found. A comparison to predictions from nuclear energy density functional theory, employing both non-relativistic and relativistic functionals, clearly favors the large, positive $β_4$ solutions. These $β_4$ values are unambiguously linked to the well deformed prolate configuration. Given the $β_2 - β_4$ trend, established in this work, it appears that $β_4$ values could provide a sensitive measure of the nuclear shell structure.

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arXiv2020

Hyperheavy spherical and toroidal nuclei: the role of shell structure

The properties of toroidal hyperheavy even-even nuclei and the role of toroidal shell structure are extensively studied within covariant density functional theory. The general trends in the evolution of toroidal shapes in the $Z\approx 130-180$ region of nuclear chart are established for the first time. These nuclei are stable with respect of breathing deformations. The most compact fat toroidal nuclei are located in the $Z\approx 136, N\approx 206$ region of nuclear chart, but thin toroidal nuclei become dominant with increasing proton number and on moving towards proton and neutron drip lines. The role of toroidal shell structure, its regularity, supershell structure, shell gaps as well as the role of different groups of the pairs of the orbitals in its formation are investigated in detail. The lowest in energy solutions at axial symmetry are characterized either by large shell gaps or low density of the single-particle states in the vicinity of the Fermi level in at least one of the subsystems (proton or neutron). Related quantum shell effects are expected to act against the instabilities in breathing and sausage deformations for these subsystems. The investigation with large set of covariant energy density functionals reveals that substantial proton $Z=154$ and 186 and neutron $N=228$, 308 and 406 spherical shell gaps exist in all functionals. The nuclei in the vicinity of the combination of these particle numbers form the islands of stability of spherical hyperheavy nuclei. The study suggests that the $N=210$ toroidal shell gap plays a substantial role in the stabilization of fat toroidal nuclei.

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arXiv2020

Covariant density functional theory input for r-process simulations in actinides and superheavy nuclei: the ground state and fission properties

The systematic investigation of the ground state and fission properties of even-even actinides and superheavy nuclei with $Z=90-120$ from the two-proton up to two-neutron drip lines with proper assessment of systematic theoretical uncertainties has been performed for the first time in the framework of covariant density functional theory (CDFT). These results provide a necessary theoretical input for the r-process modeling in heavy nuclei and, in particular, for the study of fission recycling. Four state-of-the-art globally tested covariant energy density functionals (CEDFs), namely, DD-PC1, DD-ME2, NL3* and PC-PK1, representing the major classes of the CDFT models are employed in the present study. Ground state deformations, binding energies, two neutron separation energies, $α$-decay $Q_α$ values and half-lives and the heights of fission barriers have been calculated for all these nuclei. Theoretical uncertainties in these physical observables and their evolution as a function of proton and neutron numbers have been quantified and their major sources have been identified. Spherical shell closures at $Z=120$, $N=184$ and $N=258$ and the structure of the single-particle (especially, high-$j$) states in their vicinities as well as nuclear matter properties of employed CEDFs are two major factors contributing into theoretical uncertainties. However, different physical observables are affected in a different way by these two factors. For example, theoretical uncertainties in calculated ground state deformations are affected mostly by former factor, while theoretical uncertainties in fission barriers depend on both of these factors.

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arXiv2020

Exploring nuclear exotica at the limits

The study of nuclear limits has been performed and new physical mechanisms and exotic shapes allowing the extension of nuclear landscape beyond the commonly accepted boundaries have been established. The transition from ellipsoidal to toroidal shapes plays a critical role in potential extension of nuclear landscape to hyperheavy nuclei. Rotational excitations leading to the birth of particle (proton or neutron) bound rotational bands provide a mechanism for an extension of nuclear landscape beyond spin zero proton and neutron drip lines.

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arXiv2020

Using isotope shift for testing nuclear theory: the case of nobelium isotopes

We calculate field isotope shifts for nobelium atoms using nuclear charge distributions which come from different nuclear models. We demonstrate that comparing calculated isotope shifts with experiment can serve as a testing ground for nuclear theories. It also provides a way of extracting parameters of nuclear charge distribution beyond nuclear RMS radius, e.g. parameter of quadrupole deformation $β$. We argue that previous interpretation of the isotope measurements in terms of $δ\langle r^2 \rangle$ between $^{252,254}$No isotopes should be amended when nuclear deformation is taken into account. We calculate isotope shifts for other known isotopes and for hypothetically metastable isotope $^{286}$No for which the predictions of nuclear models differ substantially.

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arXiv2019

Parametric correlations in energy density functionals

Parametric correlations are studied in several classes of covariant density functional theories (CDFTs) using a statistical analysis in a large parameter hyperspace. In the present manuscript, we investigate such correlations for two specific types of models, namely, for models with density dependent meson exchange and for point coupling models. Combined with the results obtained previously in Ref. [1] for a non-linear meson exchange model, these results indicate that parametric correlations exist in all major classes of CDFTs when the functionals are fitted to the ground state properties of finite nuclei and to nuclear matter properties. In particular, for the density dependence in the isoscalar channel only one parameter is really independent. Accounting for these facts potentially allows one to reduce the number of free parameters considerably.

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arXiv2019

Extension of nuclear landscape to hyperheavy nuclei

The properties of hyperheavy nuclei and the extension of nuclear landscape to hyperheavy nuclei are extensively studied within covariant density functional theory. Axial reflection symmetric and reflection asymmetric relativistic Hartree-Bogoliubov (RHB) calculations are carried out. The role of triaxiality is studied within triaxial RHB and triaxial relativistic mean field + BCS frameworks. With increasing proton number beyond Z~130 the transition from ellipsoidal-like nuclear shapes to toroidal ones takes place. The description of latter shapes requires the basis which is typically significantly larger than the one employed for the description of ellipsoidal-like shapes. Many hyperheavy nuclei with toroidal shapes are expected to be unstable towards multifragmentation. However, three islands of stability of spherical hyperheavy nuclei have been predicted for the first time in Ref. [1]. Proton and neutron densities, charge radii, neutron skins and underlying shell structure of the nuclei located in the centers of these islands have been investigated in detail. Large neutron shell gaps at N=228, 308 and 406 define approximate centers of these islands in neutron number. On the contrary, large proton gap appear only at Z=154 in the (Z~156, N~310) island. As a result, this is the largest island of stability of spherical hyperheavy nuclei found in the calculations. The calculations indicate the stability of the nuclei in these islands with respect of octupole and triaxial distortions. Fission barriers in neutron-rich superheavy nuclei are studied in triaxial RHB framework; the impact of triaxiality on the heights of fission barriers is substantial in some parts of this region. Based on the results obtained in the present work, the extension of nuclear landscape to hyperheavy nuclei is provided.

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arXiv2018

Hyperheavy nuclei: existence and stability

What are the limits of the existence of nuclei? What are the highest proton numbers $Z$ at which the nuclear landscape and periodic table of chemical elements cease to exist? These deceivably simple questions are difficult to answer especially in the region of hyperheavy ($Z\geq 126$) nuclei. We present the covariant density functional study of different aspects of the existence and stability of hyperheavy nuclei. For the first time, we demonstrate the existence of three regions of spherical hyperheavy nuclei centered around ($Z\sim 138, N\sim 230$), ($Z\sim 156, N\sim 310$) and ($Z\sim 174, N\sim 410$) which are expected to be reasonably stable against spontaneous fission. The triaxiality of the nuclei plays an extremely important role in the reduction of the stability of hyperheavy nuclei against fission. As a result, the boundaries of nuclear landscape in hyperheavy nuclei are defined by spontaneous fission and not by the particle emission as in lower $Z$ nuclei. Moreover, the current study suggests that only localized islands of stability can exist in hyperheavy nuclei.

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arXiv2018

Octupole deformation in neutron-rich actinides and superheavy nuclei and the role of nodal structure of single-particle wavefunctions in extremely deformed structures of light nuclei

Octupole deformed shapes in neutron-rich actinides and superheavy nuclei as well as extremely deformed shapes of the N~Z light nuclei have been investigated within the framework of covariant density functional theory. We confirmed the presence of new region of octupole deformation in neutron-rich actinides with the center around Z~96, N~196 but our calculations do not predict octupole deformation in the ground states of superheavy Z~108 nuclei. As exemplified by the study of 36Ar, the nodal structure of the wavefunction of occupied single-particle orbitals in extremely deformed structures allows to understand the formation of the alpha-clusters in very light nuclei, the suppression of the alpha-clusterization with the increase of mass number, the formation of ellipsoidal mean-field type structures and nuclear molecules.

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arXiv2017

Recent progress in the studies of neutron rich and high-$Z$ systems within the covariant density functional theory

The analysis of statistical and systematic uncertainties and their propogation to nuclear extremes has been performed. Two extremes of nuclear landscape (neutron-rich nuclei and superheavy nuclei) have been investigated. For the first extreme, we focus on the ground state properties. For the second extreme, we pay a particular attention to theoretical uncertainties in the description of fission barriers of superheavy nuclei and their evolution on going to neutron-rich nuclei.

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arXiv2017

Octupole deformation in the ground states of even-even $Z\sim 96, N\sim 196$ actinides and superheavy nuclei

A systematic search for axial octupole deformation in the actinides and superheavy nuclei with proton numbers $Z=88-126$ and neutron numbers from two-proton drip line up to $N=210$ has been performed in covariant density functional theory (DFT) using four state-of-the-art covariant energy density functionals representing different model classes. The nuclei in the $Z\sim 96, N\sim 196$ region of octupole deformation have been investigated in detail and the systematic uncertainties in the description of their observables have been quantified. Similar region of octupole deformation exists also in Skyrme DFT and microscopic+macroscopic approach but it is centered at somewhat different particle numbers. Theoretical uncertainties in the predictions of the regions of octupole deformation are increasing on going to superheavy nuclei with $Z\sim 120, N\sim 190$. There are no octupole deformed nuclei for $Z=112-126$ in covariant DFT calculations. This agrees with Skyrme DFT calculations, but disagrees with Gogny DFT and microscopic+macroscopic calculations which predict extended $Z\sim 120, N\sim 190$ region of octupole deformation.

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arXiv2017

Assessing theoretical uncertainties in fission barriers of superheavy nuclei

Theoretical uncertainties in the predictions of inner fission barrier heights in superheavy elements have been investigated in a systematic way for a set of state-of-the-art covariant energy density functionals which represent major classes of the functionals used in covariant density functional theory. They differ in basic model assumptions and fitting protocols. Both systematic and statistical uncertainties have been quantified where the former turn out to be larger. Systematic uncertainties are substantial in superheavy elements and their behavior as a function of proton and neutron numbers contains a large random component. The benchmarking of the functionals to the experimental data on fission barriers in the actinides allows to reduce the systematic theoretical uncertainties for the inner fission barriers of unknown superheavy elements. However, even then they on average increase on moving away from the region where benchmarking has been performed. In addition, a comparison with the results of non-relativistic approaches is performed in order to define full systematic theoretical uncertainties over the state-of-the-art models. Even for the models benchmarked in the actinides, the difference in the inner fission barrier height of some superheavy elements reaches $5-6$ MeV. This uncertainty in the fission barrier heights will translate into huge (many tens of the orders of magnitude) uncertainties in the spontaneous fission half-lives.

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arXiv2016

Covariant energy density functionals: nuclear matter constraints and global ground state properties

The correlations between global description of the ground state properties (binding energies, charge radii) and nuclear matter properties of the state-of-the-art covariant energy density functionals have been studied. It was concluded that the strict enforcement of the constraints on the nuclear matter properties (NMP) defined in Ref.\ \cite{RMF-nm} will not necessary lead to the functionals with good description of the binding energies and other ground and excited state properties. In addition, it will not substantially reduce the uncertainties in the predictions of the binding energies in neutron-rich systems. It turns out that the functionals, which come close to satisfying these NMP constraints, have some problems in the description of existing data. On the other hand, these problems are either absent or much smaller in the functionals which are carefully fitted to finite nuclei but which violate some NMP constraints. This is a consequence of the fact that the properties of finite nuclei are defined not only by nuclear matter properties but also by underlying shell effects. The mismatch of phenomenological content, existing in all modern functionals, related to nuclear matter physics and the physics of finite nuclei could also be responsible.

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arXiv2016

Octupole deformation in the ground states of even-even nuclei: a global analysis within the covariant density functional theory

A systematic investigation of octupole deformed nuclei is presented for even-even systems with $Z\leq 106$ located between the two-proton and two-neutron drip lines. For this study we use five most up-to-date covariant energy density functionals of different types, with a non-linear meson coupling, with density dependent meson couplings, and with density-dependent zero-range interactions. Pairing correlations are treated within relativistic Hartree-Bogoliubov (RHB) theory based on an effective separable particle-particle interaction of finite range. This allows us to assess theoretical uncertainties within the present covariant models for the prediction of physical observables relevant for octupole deformed nuclei. In addition, a detailed comparison with the predictions of non-relativistic models is performed. A new region of octupole deformation, centered around $Z\sim 98, N\sim 196$ is predicted for the first time. In terms of its size in the $(Z,N)$ plane and the impact of octupole deformation on binding energies this region is similar to the best known region of octupole deformed nuclei centered at $Z\sim 90, N\sim 136$. For the later island of octupole deformed nuclei, the calculations suggest substantial increase of its size as compared with available experimental data.

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arXiv2016

Nuclear structure theory of the heaviest nuclei

The current status of the application of covariant density functional theory to the description of actinides and superheavy nuclei is reviewed. The achievements and open problems are discussed.

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arXiv2015

Covariant density functional theory: Reexamining the structure of superheavy nuclei

A systematic investigation of even-even superheavy elements in the region of proton numbers $100 \leq Z \leq 130$ and in the region of neutron numbers from the proton-drip line up to neutron number $N=196$ is presented. For this study we use five most up-to-date covariant energy density functionals of different types, with a non-linear meson coupling, with density dependent meson couplings, and with density-dependent zero-range interactions. Pairing correlations are treated within relativistic Hartree-Bogoliubov (RHB) theory based on an effective separable particle-particle interaction of finite range and deformation effects are taken into account. This allows us to assess the spread of theoretical predictions within the present covariant models for the binding energies, deformation parameters, shell structures and $α$-decay half-lives. Contrary to the previous studies in covariant density functional theory, it was found that the impact of $N=172$ spherical shell gap on the structure of superheavy elements is very limited. Similar to non-relativistic functionals some covariant functionals predict the important role played by the spherical $N=184$ gap. For these functionals (NL3*, DD-ME2 and PC-PK1), there is a band of spherical nuclei along and near the $Z=120$ and $N=184$ lines. However, for other functionals (DD-PC1 and DD-ME$δ$) oblate shapes dominate at and in the vicinity of these lines. Available experimental data are in general described with comparable accuracy and do not allow to discriminate these predictions.

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arXiv2015

The neutron drip line: single-particle degrees of freedom and pairing properties as sources of theoretical uncertainties

The sources of theoretical uncertainties in the prediction of the two-neutron drip line are analyzed in the framework of covariant density functional theory. We concentrate on single-particle and pairing properties as potential sources of these uncertainties. The major source of these uncertainties can be traced back to the differences in the underlying single-particle structure of the various covariant energy density functionals (CEDF). It is found that the uncertainties in the description of single-particle energies at the two-neutron drip line are dominated by those existing already in known nuclei. Only approximately one third of these uncertainties are due to the uncertainties in the isovector channel of CEDF's. Thus, improving the CEDF description of single-particle energies in known nuclei will also reduce the uncertainties in the prediction of the position of two-neutron drip line. The predictions of pairing properties in neutron rich nuclei depend on the CEDF. Although pairing properties affect moderately the position of the two-neutron drip line they represent only a secondary source for the uncertainties in the definition of the position of the two-neutron drip line.

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arXiv2015

Nuclear energy density functionals: what we can learn about/from their global performance?

A short review of recent results on the global performance of covariant energy density functionals is presented. It is focused on the analysis of the accuracy of the description of physical observables of ground and excited states as well as to related theoretical uncertainties. In addition, a global analysis of pairing properties is presented and the impact of pairing on the position of two-neutron drip line is discussed.

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