arXiv subjects

S. Florens

Publications and source records attributed to S. Florens.

At least 19 recordsLinked to original sources

arXiv2019

Magnetic-Field-Induced Transition in a Quantum Dot Coupled to a Superconductor

The magnetic moment of a quantum dot can be screened by its coupling to a superconducting reservoir, depending on the hierarchy of the superconducting gap and the relevant Kondo scale. This screening-unscreening transition can be driven by electrostatic gating, tunnel coupling, and, as we demonstrate here, magnetic field. We perform high-resolution spectroscopy of subgap excitations near the screening-unscreening transition of asymmetric superconductor - quantum dot - superconductor (S-QD-S) junctions formed by the electromigration technique. Our measurements reveal a re-entrant phase boundary determined by the competition between Zeeman energy and gap reduction with magnetic field. We further track the evolution of the phase transition with increasing temperature, which is also evidenced by thermal replicas of subgap states.

cond-mat.mes-hall↗

arXiv2018

Direct measurement of the Seebeck coefficient in a Kondo-correlated single-quantum-dot transistor

We report on the first measurement of the Seebeck coefficient in a tunnel-contacted and gate-tunable individual single-quantum dot junction in the Kondo regime, fabricated using the electromigration technique. This fundamental thermoelectric parameter is obtained by directly monitoring the magnitude of the voltage induced in response to a temperature difference across the junction, while keeping a zero net tunneling current through the device. In contrast to bulk materials and single molecules probed in a scanning tunneling microscopy (STM) configuration, investigating the thermopower in nanoscale electronic transistors benefits from the electric tunability to showcase prominent quantum effects. Here, striking sign changes of the Seebeck coefficient are induced by varying the temperature, depending on the spin configuration in the quantum dot. The comparison with Numerical Renormalization Group (NRG) calculations demonstrate that the tunneling density of states is generically asymmetric around the Fermi level in the leads, both in the cotunneling and Kondo regimes.

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arXiv2016

Topologically-protected entanglement of electron pair cyclotron motions

Considering two-dimensional electron gases under a perpendicular magnetic field, we pinpoint a specific kind of long-range bipartite entanglement of the electronic motions. This entanglement is achieved through the introduction of bicomplex spinorial eigenfunctions admitting a polar decomposition in terms of a real modulus and three real phases. Within this bicomplex geometry the cyclotron motions of two electrons are intrinsically tied, so that the highlighted eigenstates of the kinetic energy operator actually describe the free motion of a genuine electron pair. Most remarkably, these states embody phase singularities in the four-dimensional (4D) space, with singular points corresponding to the simultaneous undetermination of the three phases. Because the entanglement between the two electrons forming a pair, as well as the winding and parity quantum numbers characterizing the 4D phase singularity, are topological in nature, we expect them to manifest some robustness in the presence of a smooth disorder potential and an electron-electron interaction potential. The relevance of this effective approach in terms of 4D vortices of electron pairs is discussed in the context of the fractional quantum Hall effect.

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arXiv2015

Impact of capacitance and tunneling asymmetries on Coulomb blockade edges and Kondo peaks in non-equilibrium transport through molecular quantum dots

We investigate theorerically the non-equilibrium transport through a molecular quantum dot as a function of gate and bias voltage, taking into account the typical situation in molecular electronics. In this respect, our study includes asymmetries both in the capacitances and tunneling rates to the source and drain electrodes, as well as an infinitely large charging energy on the molecule. Our calculations are based on the out-of-equilibrium Non-Crossing-Approximation (NCA), which is a reliable technique in the regime under consideration. We find that Coulomb blockade edges and Kondo peaks display strong renormalization in their width and intensity as a function of these asymmetries, and that basic expectations from Coulomb blockade theory must be taken with care in general, expecially when Kondo physics is at play. In order to help comparison of theory to experiments, we also propose a simple phenomenological model which reproduces semi-quantitatively the Coulomb blockade edges that were numerically computed from the NCA in all regimes of parameters.

cond-mat.mes-hall↗

arXiv2013

Interplay of Kondo effect and strong spin-orbit coupling in multi-hole ultraclean carbon nanotubes

We report on cotunneling spectroscopy magnetoconductance measurements of multi-hole ultraclean carbon nanotube quantum dots in the SU(4) Kondo regime with strong spin-orbit coupling. Successive shells show a gradual weakening of the Kondo effect with respect to the spin-orbital splittings, leading to an evolution from SU(4) to SU(2) symmetry with a suppressed conductance at half shell filling. The extracted energy level spectrum, overally consistent with negligible disorder in the nanotube, shows in the half filled case large renormalizations due to Coulombian effects.

cond-mat.mes-hall↗

arXiv2013

Classical percolation fingerprints in the high-temperature regime of the integer quantum Hall effect

We have performed magnetotransport experiments in the high-temperature regime (up to 50 K) of the integer quantum Hall effect for two-dimensional electron gases in semiconducting heterostructures. While the magnetic field dependence of the classical Hall law presents no anomaly at high temperatures, we find a breakdown of the Drude-Lorentz law for the longitudinal conductance beyond a crossover magnetic field B_c ~ 1 T, which turns out to be correlated with the onset of the integer quantum Hall effect at low temperatures. We show that the high magnetic field regime at B > B_c can be understood in terms of classical percolative transport in a smooth disordered potential. From the temperature dependence of the peak longitudinal conductance, we extract scaling exponents which are in good agreement with the theoretically expected values. We also prove that inelastic scattering on phonons is responsible for dissipation in a wide temperature range going from 1 to 50 K at high magnetic fields.

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arXiv2012

Observation of Majorana Quantum Critical Behavior in a Resonant Level Coupled to a Dissipative Environment

We investigate experimentally an exotic state of electronic matter obtained by fine-tuning to a quantum critical point (QCP), realized in a spin-polarized resonant level coupled to strongly dissipative electrodes. Several transport scaling laws near and far from equilibrium are measured, and then accounted for theoretically. Our analysis reveals a splitting of the resonant level into two quasi-independent Majorana modes, one strongly hybridized to the leads, and the other tightly bound to the quantum dot. Residual interactions involving these Majorana fermions result in the observation of a striking quasi-linear non-Fermi liquid scattering rate at the QCP. Our devices constitute a viable alternative to topological superconductors as a platform for studying strong correlation effects within Majorana physics.

cond-mat.mes-hall↗

arXiv2012

Robust Nodal Structure of Landau Level Wave Functions Revealed by Fourier Transform Scanning Tunneling Spectroscopy

Scanning tunneling spectroscopy is used to study the real-space local density of states (LDOS) of a two-dimensional electron system in magnetic field, in particular within higher Landau levels (LL). By Fourier transforming the LDOS, we find a set of n radial minima at fixed momenta for the nth LL. The momenta of the minima depend only on the inverse magnetic length. By comparison with analytical theory and numerical simulations, we attribute the minima to the nodes of the quantum cyclotron orbits, which decouple in Fourier representation from the random guiding center motion due to the disorder. This robustness of the nodal structure of LL wave functions should be viewed as a key property of quantum Hall states.

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arXiv2011

Quantum phase transition in the spin boson model

In this paper we give a general introduction to quantum critical phenomena, which we practically illustrate by a detailed study of the low energy properties of the spin boson model (SBM), describing the dynamics of a spin 1/2 impurity (or more generically a two-level system) coupled to a bath of independent harmonic oscillators. We show that the behavior of the model is very sensitive to the bath spectrum, in particular how the properties of the quantum critical point in the SBM are affected by the functional form of the bath Density of States (DoS). To this effect, we review the renormalization group (RG) treatment of the SBM for various bath DoS, based on an unconventional Majorana representation of the spin 1/2 degree of freedom. We also discuss the derivation of Shiba's relation for the sub-ohmic SBM, and explicitely derive an effective action vindicating the quantum to classical mapping.

cond-mat.str-el↗

arXiv2011

Nonlocal correlations of the local density of states in disordered quantum Hall systems

Motivated by recent high-resolution scanning tunneling microscopy (STM) experiments in the quantum Hall regime both on massive two-dimensional electron gas and on graphene, we consider theoretically the disorder averaged nonlocal correlations of the local density of states (LDoS) for electrons moving in a smooth disordered potential in the presence of a high magnetic field. The intersection of two quantum cyclotron rings around the two different positions of the STM tip, correlated by the local disorder, provides peaks in the spatial dispersion of the LDoS-LDoS correlations when the intertip distance matches the sum of the two quantum Larmor radii. The energy dependence displays also complex behavior: for the local LDoS-LDoS average (i.e., at coinciding tip positions), sharp positive correlations are obtained for tip voltages near Landau level, and weak anticorrelations otherwise.

cond-mat.mes-hall↗

arXiv2009

Electron quantum dynamics in closed and open potentials at high magnetic fields: Quantization and lifetime effects unified by semicoherent states

We have developed a Green's function formalism based on the use of an overcomplete semicoherent basis of vortex states, specially devoted to the study of the Hamiltonian quantum dynamics of electrons at high magnetic fields and in an arbitrary potential landscape smooth on the scale of the magnetic length. This formalism is used here to derive the exact Green's function for an arbitrary quadratic potential in the special limit where Landau level mixing becomes negligible. This solution remarkably embraces under a unified form the cases of confining and unconfining quadratic potentials. This property results from the fact that the overcomplete vortex representation provides a more general type of spectral decomposition of the Hamiltonian operator than usually considered. Whereas confining potentials are naturally characterized by quantization effects, lifetime effects emerge instead in the case of saddle-point potentials. Our derivation proves that the appearance of lifetimes has for origin the instability of the dynamics due to quantum tunneling at saddle points of the potential landscape. In fact, the overcompleteness of the vortex representation reveals an intrinsic microscopic irreversibility of the states synonymous with a spontaneous breaking of the time symmetry exhibited by the Hamiltonian dynamics.

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arXiv2008

Kondo effects in a C_60 single-molecule transistor

We have used the electromigration technique to fabricate a $\rm{C_{60}}$ single-molecule transistor (SMT). We present a full experimental study as a function of temperature, down to 35 mK, and as a function of magnetic field up to 8 T in a SMT with odd number of electrons, where the usual spin-1/2 Kondo effect occurs, with good agreement with theory. In the case of even number of electrons, a low temperature magneto-transport study is provided, which demonstrates a Zeeman splitting of the zero-bias anomaly at energies well below the Kondo scale.

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arXiv2007

Gate-tuned high frequency response of carbon nanotube Josephson junctions

Carbon nanotube (CNT) Josephson junctions in the open quantum dot limit exhibit superconducting switching currents which can be controlled with a gate electrode. Shapiro voltage steps can be observed under radiofrequency current excitations, with a damping of the phase dynamics that strongly depends on the gate voltage. These measurements are described by a standard RCSJ model showing that the switching currents from the superconducting to the normal state are close to the critical current of the junction. The effective dynamical capacitance of the nanotube junction is found to be strongly gate-dependent, suggesting a diffusive contact of the nanotube.

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arXiv2004

Climbing the Entropy Barrier: Driving the Single- towards the Multichannel Kondo Effect by a Weak Coulomb Blockade of the Leads

We study a model proposed recently in which a small quantum dot is coupled symmetrically to several large quantum dots characterized by a charging energy E_c. Even if E_c is much smaller than the Kondo temperature T_K, the long-ranged interactions destabilize the single-channel Kondo effect and induce a flow towards a multi-channel Kondo fixed point associated with a rise of the impurity entropy with decreasing temperature. Such an ``uphill flow'' implies a negative impurity specific heat, in contrast to all systems with local interactions. An exact solution found for a large number of channels allows us to capture this physics and to predict transport properties.

cond-mat.str-el↗

arXiv2004

A brief review of recent advances on the Mott transition: unconventional transport, spectral weight transfers, and critical behaviour

Strongly correlated metals close to the Mott transition display unusual transport regimes, together with large spectral weight transfers in optics and photoemission. We briefly review the theoretical understanding of these effects, based on the dynamical mean-field theory, and emphasize the key role played by the two energy scales associated with quasiparticle coherence scale and with the Mott gap. Recent experimental results on two-dimensional organic compounds and transition metal oxides are considered in this perspective. The liquid-gas critical behaviour at the Mott critical endpoint is also discussed. Transport calculations using the numerical renormalization group are presented.

cond-mat.str-el↗

arXiv2003

Coherence and Coulomb blockade in single electron devices: a unified treatment of interaction effects

We study the interplay between Coulomb blockade and the Kondo effect in quantum dots. We use a self-consistent scheme which describes mesoscopic devices in terms of a collective phase variable (slave rotor) and quasiparticle degrees of freedom. In the strong Coulomb blockade regime, we recover the description of metallic islands in terms of a phase only action. For a dot with well-separated levels, our method leads to the Kondo effect. We identify the regime where a crossover between the Coulomb blockade regime at high temperatures and the formation of a Kondo resonance at lower temperature takes place. In addition, we find that for a dot with many overlapping resonances, an {\it inverse crossover} can take place. A Kondo resonance which involves many levels within the dot is first formed, and this coherent state is suppressed by correlation effects at lower temperatures. A narrower Kondo resonance, due to a single level in the dot can emerge at even lower temperatures.

cond-mat.mes-hall↗

arXiv2003

Spectroscopic signatures of a bandwidth-controlled Mott transition at the surface of 1T-TaSe$_2$

High-resolution angle-resolved photoemission (ARPES) data show that a metal-insulator Mott transition occurs at the surface of the quasi-two dimensional compound TaSe$_2$. The transition is driven by the narrowing of the Ta $5d$ band induced by a temperature-dependent modulation of the atomic positions. A dynamical mean-field theory calculation of the spectral function of the half-filled Hubbard model captures the main qualitative feature of the data, namely the rapid transfer of spectral weight from the observed quasiparticle peak at the Fermi surface to the Hubbard bands, as the correlation gap opens up.

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arXiv2003

Mott transition and transport crossovers in the organic compound $κ-(BEDT-TTF)_2 Cu[N(CN)_2] Cl$

We have performed in-plane transport measurements on the two-dimensional organic salt $κ$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Cl. A variable (gas) pressure technique allows for a detailed study of the changes in conductivity through the insulator-to-metal transition. We identify four different transport regimes as a function of pressure and temperature (corresponding to insulating, semi-conducting, ''bad metal'', and strongly correlated Fermi liquid behaviours). Marked hysteresis is found in the transition region, which displays complex physics that we attribute to strong spatial inhomogeneities. Away from the critical region, good agreement is found with a dynamical mean-field calculation of transport properties using the numerical renormalization group technique.

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