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S. Franchoo

Publications and source records attributed to S. Franchoo.

At least 19 recordsLinked to original sources

Evolution of Spectroscopic Factors in Neutron-deficient $p$-shell Nuclei in connection with Short-Range Correlations

We report an uncertainty-controlled determination of neutron-removal spectroscopic factors in the neutron-deficient $p$-shell nuclei $^{12}\mathrm{C}$, $^{10}\mathrm{C}$, $^{9}\mathrm{C}$, and $^{8}\mathrm{B}$, all measured under uniform conditions through exclusive ground-state-to-ground-state $(p,d)$ reactions at about 50 MeV/nucleon in a liquid hydrogen target at the GANIL/LISE facility. The deuterons were detected in the highly-segmented MUST2 detector placed at forward angles and the excitation energy was reconstructed by the missing mass method. Several transitions, including a new state in $^7\mathrm{B}$, were observed. Differential cross sections, which display an $L=1$ pattern for all nuclei, were fitted with 416 sets of uncertainty-quantified optical-model potential parameters and considering various single-particle bound-state wavefunctions to derive $C^2S$ values. The ratio between experimental and shell-model calculated values, $R_S$, is found to be slightly decreasing as a function of increasing proton to neutron separation energy asymmetry $\Delta S$, with a slope of $-0.0049(36)_{\rm stat}(13)_{\rm omp}(8)_{\rm s.p.}$. The observed trend is compatible with the phenomenological expectation that the short-range correlation effect on $C^2S$ increases with the degree of nucleon minority. The present data set delivers a high-precision benchmark that will tightly constrain future microscopic descriptions of short-range correlations in asymmetric nuclei.

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Probing the Size of Neutron and Proton Single-Particle Orbitals from Nucleon Knockout Reactions

The size of neutron and proton single-particle orbitals of $^{52}$Ca, $^{53}$Ca, $^{54}$Ca, and $^{55}$Sc were investigated via nucleon knockout reactions at $\sim$ 230 MeV/nucleon. The determination method is based on the measured fragment momentum distributions in $(p,pn)$ and $(p,2p)$ reactions, which are shown to be sensitive to the spatial extension of the wave function of the knocked-out nucleon, interpreted within the distorted wave impulse approximation (DWIA) framework. A systematic sensitivity study is carried out for the $(p,pn)$ recoil-momentum distribution method and is presented in this work. The experimental momentum distributions are compared to state-of-the-art mean field and $ab$ $initio$ in-medium similarity renormalization group and self-consistent Green's function calculations in combination with DWIA reaction theory calculations. Based on this work, the 1$p$ neutron orbitals are consistently found $0.48-0.78$ fm larger than the $0f_{7/2}$ neutron orbitals in $^{52-54}$Ca, while the size evolution of the valence proton orbitals remains inconclusive due to the large associated statistical uncertainties.

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A prototype gas cell for the stopping, extraction and neutralization of radioactive nuclei from the SPIRAL2 Super Separator Spectrometer (S$^3$)

We present the design and simulation of a prototype gas cell for in-gas-jet laser-ionization and spectroscopy studies using the low energy branch of the SPIRAL2-S$^3$ radioactive-ion-beam facility. The prototype aims to demonstrate the possibility to reduce the extraction time of radioactive ions from the gas cell, while implementing a controlled neutralization mechanism, necessary for laser-spectroscopy studies. Different simulation methods of ion processes in gas are comparatively discussed. Design considerations and detailed simulations of the ion extraction time and efficiency are presented. A study of the dynamics of electrons obtained in the gas cell by ionization is also performed to assess the achievable electron densities.

physics.ins-det

Direct transfer to $^{46,48}$K as a survey of the $\pi(s_{1/2})$$-\nu(sdpf)$ interaction

The collapse of the canonical $N=28$ magic number in nuclei with $Z<20$ has drawn significant interest as it relates to the emergence of an island of inversion centered on $^{42}$Si and $^{44}$S. In particular, interactions between the $\pi s_{1/2}$ orbital -- empty in $^{42}$Si and full in $^{44}$S -- and the neutron orbitals just above and below the $N=28$ gap are expected to be critical in this region, but remain relatively unexplored. In this paper, we expand upon the results of our previous study of the direct transfer reaction $^{47}$K(d,p$\gamma$)$^{48}$K [C.\,J.~Paxman \textit{et al.}, Phys. Rev. Lett. 134, 162504 (2025)] with the results of the complementary $^{47}$K(d,t$\gamma$)$^{46}$K reaction. Through this study, we present a comprehensive scan of the interaction between the critical $\pi s_{1/2}$ orbital and a broad range of neutron orbitals spanning nearly two full shells. We identify several discrepancies between the experimental results and state-of-the-art shell model calculations, which suggest a deficiency of the shell model to fully capture the complex proton configuration mixing in this region, highlighting a significant challenge for single-particle descriptions of the island of inversion.

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An experimental setup for the study of gas-cell processes for the S$^3$-Low Energy Branch

We present an experimental setup dedicated to the study of in-gas ion processes and characterization of gas stopping cells for the Low Energy Branch of the Super Separator Spectrometer (S$^3$) at SPIRAL2-GANIL. The first application is the development of a new gas stopper with a neutralization mechanism designed for faster extraction of the radioactive ions. This development should enable in-gas-jet laser spectroscopy and other low-energy experiments with shorter lived radioactive isotopes. We discuss in detail the motivation and objectives of these developments and we present the results of simulations performed in the design phase, as well as the first experimental results.

physics.ins-det

Laser spectroscopy and CP-violation sensitivity of actinium monofluoride

The apparent invariance of the strong nuclear force under combined charge conjugation and parity (CP) remains an open question in modern physics. Precision experiments with heavy atoms and molecules can provide stringent constraints on CP violation via searches for effects due to permanent electric dipole moments and other CP-odd properties in leptons, hadrons, and nuclei. Radioactive molecules have been proposed as highly sensitive probes for such searches, but experiments with most such molecules have so far been beyond technical reach. Here we report the first production and spectroscopic study of a gas-phase actinium molecule, $^{227}$AcF. We observe the predicted strongest electronic transition from the ground state, which is necessary for efficient readout in searches of symmetry-violating interactions. Furthermore, we perform electronic- and nuclear-structure calculations for $^{227}$AcF to determine its sensitivity to various CP-violating parameters, and find that a realistic, near-term experiment with a precision of 1 mHz would improve current constraints on the CP-violating parameter hyperspace by three orders of magnitude. Our results thus highlight the potential of $^{227}$AcF for exceptionally sensitive searches of CP violation.

physics.atom-ph

Science for Peace and the need for Civil Clauses at universities and civilian research institutions

After the end of World War II, the commitment to confine scientific activities in universities and research institutions to peaceful and civilian purposes has entered, in the form of {\it Civil Clauses}, the charters of many research institutions and universities. In the wake of recent world events, the relevance and scope of such Civil Clauses has been questioned in reports issued by some governments and by the EU Commission, a development that opens the door to a possible blurring of the distinction between peaceful and military research. This paper documents the reflections stimulated by a panel discussion on this issue recently organized by the Science4Peace Forum. We review the adoptions of Civil Clauses in research organizations and institutions in various countries, present evidence of the challenges that are emerging to such Civil Clauses, and collect arguments in favour of maintaining the purely civilian and peaceful focus of public (non-military) research.

physics.soc-ph

Unbound neutron $\nu0d_{3/2}$ strength in $^{17}$C and the N=16 shell gap

Significant continuum strength has been observed to be populated in $^{17}$C produced in the d($^{16}$C,p) reaction at a beam energy of 17.2~MeV/nucleon. The strength appears at greater than $\sim$2~MeV above the single-neutron decay threshold and has been identified as arising from transfer into the neutron $0d_{3/2}$ orbital. Guided by shell model predictions the greater majority of the strength is associated with a 3/2$^+$ state at an excitation energy of 4.40$_{-0.14}^{+0.33}$ MeV and a much weaker 3/2$^+$ level at 5.60$_{-0.45}^{+1.35}$ MeV. The corresponding total widths were determined to be 3.45$_{-0.78}^{+1.82}$ and 1.6$_{-1.4}^{+4.6}$ MeV, respectively. From the backward angle proton differential cross sections and the branching ratios for neutron decay to the $^{16}$C(2$_{1}^{+}$) level, the corresponding spectroscopic factors to the ground state were deduced to be 0.47$\pm{10}$ and $<$0.09. Shell-model calculations employing the phenomenological SFO-tls interaction as well as Gamow Shell-Model calculations including continuum effects are in reasonable agreement with experiment, although the predicted strength lies at somewhat lower energy. The size of the N=16 shell gap ($\varepsilon_{ \nu0d_{3/2}}-\varepsilon _{\nu 1s_{1/2}}$) was estimated to be 5.08$_{-0.33}^{+0.43}$~MeV - some 1.3~MeV larger than found in the SFO-tls shell model calculation.

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Charge Radii Measurements of Exotic Tin Isotopes in the Proximity of $N=50$ and $N=82$

We report nuclear charge radii for the isotopes $^{104-134}$Sn, measured using two different collinear laser spectroscopy techniques at ISOLDE-CERN. These measurements clarify the arch-like trend in charge radii along the isotopic chain and reveal an odd-even staggering that is more pronounced near the $N=50$ and $N=82$ shell closures. The observed local trends are well described by both nuclear density functional theory and valence space in-medium similarity renormalization group calculations. Both theories predict appreciable contributions from beyond-mean-field correlations to the charge radii of the neutron-deficient tin isotopes. The models, however, fall short of reproducing the magnitude of the known $B(E2)$ transition probabilities, highlighting the remaining challenges in achieving a unified description of both ground-state properties and collective phenomena.

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Science4Peace: A Plea for Continued Peaceful International Scientific Cooperation (Input to the European Strategy for Particle Physics -- 2026 update)

The European Strategy for Particle Physics (ESPP) - 2026 update is taking place in a turbulent international climate. Many of the norms that have governed relations between states for decades are being broken or challenged. The future progress of science in general, and particle physics in particular, will depend on our ability to maintain peaceful international scientific collaboration in the face of political pressures. We plead that the ESPP 2026 update acknowledge explicitly the importance of peaceful international scientific collaboration, not only for the progress of science, but also as a precious bridge between geopolitical blocs. "Scientific thought is the common heritage of mankind" - Abdus Salam

physics.soc-ph

Beta delayed neutron emission of $N=84$ $^{132}$Cd

Using the time-of-flight technique, we measured the beta-delayed neutron emission of $^{132}$Cd. From our large-scale shell model (LSSM) calculation using the N$^3$LO interaction [Z.Y. Xu et al., Phys. Rev. Lett. 131, 022501 (2023)], we suggest the decay is dominated by the transformation of a neutron in the $g_{7/2}$ orbital, deep below the Fermi surface, into a proton in the $g_{9/2}$ orbital. We compare the beta-decay half-lives and neutron branching ratios of nuclei with $Z<50$ and $N\geq82$ obtained with our LSSM with those of leading "global" models such as Finite-Range Droplet Model (FRDM). Our calculations match known half-lives and neutron branching ratios well and suggest that current leading models overestimate the yet-to-be-measured half-lives. Our model, backed by the $^{132}$Cd decay data presented here, offers robust predictive power for nuclei of astrophysical interest such as $r$-process waiting points.

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Spectroscopy of $^{52}$K

The first spectroscopy of $^{52}$K was investigated via in-beam $\gamma$-ray spectroscopy at the RIKEN Radioactive Isotope Beam Factory after one-proton and one-neutron knockout from $^{53}$Ca and $^{53}$K beams impinging on a 15-cm liquid hydrogen target at $\approx$ 230~MeV/nucleon. The energy level scheme of $^{52}$K was built using single $\gamma$ and $\gamma$-$\gamma$ coincidence spectra. The spins and parities of the excited states were established based on momentum distributions of the fragment after the knockout reaction and based on exclusive cross sections. The results were compared to state-of-the-art shell model calculations with the SDPF-Umod interaction and ab initio IMSRG calculations with chiral effective field theory nucleon-nucleon and three-nucleon forces.

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Mirror nucleon-transfer reactions from $^{18}$Ne and $^{18}$O

The $^{18}$Ne(d,t)$^{17}$Ne and $^{18}$Ne(d,$^3$He)$^{17}$F single-nucleon pickup reactions were measured at 16.5 MeV/nucleon in inverse kinematics together with elastic and inelastic scattering channels. The full set of measured exclusive differential cross sections was compared with the mirror reaction channels on stable $^{18}$O after consistent reanalysis using coupled reaction channels calculations. Within this interpretation scheme, most of the spectroscopic factors extracted for the population of unbound states in $^{17}$F match within uncertainties with their mirror partners in $^{17}$O. However, for the deeply-bound neutron removal channel to $^{17}$Ne, a significant symmetry breaking with the mirror proton-removal channel leading to $^{17}$N is evidenced by an overall single-particle strength reduction.

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Probing exotic cross-shell interactions at N=28 with single-neutron transfer on 47K

We present the first measurement of the $^{47}$K($d,p\gamma$)$^{48}$K transfer reaction, performed in inverse kinematics using a reaccelerated beam of $^{47}$K. The level scheme of $^{48}$K has been greatly extended with nine new bound excited states identified and spectroscopic factors deduced. Detailed comparisons with SDPF-U and SDPF-MU shell-model calculations reveal a number of discrepancies with these results, and a preference for SDPF-MU is found. Intriguingly, an apparent systematic overestimation of spectroscopic factors and a poor reproduction of the energies for 1$^-$ states suggests that the mixing between the $\pi s^{\,\,\,1}_{1/2} d^{\,\,\,4}_{3/2}$ and $\pi s^{\,\,\,2}_{1/2} d^{\,\,\,3}_{3/2}$ proton configurations in $^{48}$K is not correctly described using current interactions, challenging our descriptions of light $N=28$ nuclei.

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Ionization potential of radium monofluoride

The ionization potential (IP) of radium monofluoride (RaF) was measured to be 4.969(2)[10] eV, revealing a relativistic enhancement in the series of alkaline earth monofluorides. The results are in agreement with a relativistic coupled-cluster prediction of 4.969[7] eV, incorporating up to quantum electrodynamics corrections. Using the same computational methodology, an improved calculation for the dissociation energy ($D_{0}$) of 5.54[5] eV is presented. This confirms that radium monofluoride joins the small group of diatomic molecules for which $D_{0}>\mathrm{IP}$, paving the way for precision control and interrogation of its Rydberg states.

physics.atom-ph

Spectroscopy of deeply bound orbitals in neutron-rich Ca isotopes

The calcium isotopes are an ideal system to investigate the evolution of shell structure and magic numbers. Although the properties of surface nucleons in calcium have been well studied, probing the structure of deeply bound nucleons remains a challenge. Here, we report on the first measurement of unbound states in $^{53}$Ca and $^{55}$Ca, populated from \ts{54,56}Ca($p,pn$) reactions at a beam energy of around 216 MeV/nucleon at the RIKEN Radioactive Isotopes Beam Factory. The resonance properties, partial cross sections, and momentum distributions of these unbound states were analyzed. Orbital angular momentum $l$ assignments were extracted from momentum distributions based on calculations using the distorted wave impulse approximation (DWIA) reaction model. The resonances at excitation energies of 5516(41)\,keV in $^{53}$Ca and 6000(250)\,keV in $^{55}$Ca indicate a significant $l$\, =\,3 component, providing the first experimental evidence for the $\nu 0f_{7/2}$ single-particle strength of unbound hole states in the neutron-rich Ca isotopes. The observed excitation energies and cross-sections point towards extremely localized and well separated strength distributions, with some fragmentation for the $\nu 0f_{7/2}$ orbital in $^{55}$Ca. These results are in good agreement with predictions from shell-model calculations using the effective GXPF1Bs interaction and \textit{ab initio} calculations and diverge markedly from the experimental distributions in the nickel isotones at $Z=28$.

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Radiative lifetime of the A 2{\Pi}1/2 state in RaF with relevance to laser cooling

The radiative lifetime of the $A$ $^2 \Pi_{1/2}$ (v=0) state in radium monofluoride (RaF) is measured to be 35(1) ns. The lifetime of this state and the related decay rate $\Gamma = 2.86(8) \times 10^7$ $s^{-1}$ are of relevance to the laser cooling of RaF via the optically closed $A$ $^2 \Pi_{1/2} \leftarrow X$ $^2\Sigma_{1/2}$ transition, which makes the molecule a promising probe to search for new physics. RaF is found to have a comparable photon-scattering rate to homoelectronic laser-coolable molecules. Thanks to its highly diagonal Franck-Condon matrix, it is expected to scatter an order of magnitude more photons than other molecules when using just 3 cooling lasers, before it decays to a dark state. The lifetime measurement in RaF is benchmarked by measuring the lifetime of the $8P_{3/2}$ state in Fr to be 83(3) ns, in agreement with literature.

physics.atom-ph

Validation of the $^{10}\mathrm{Be}$ Ground-State Molecular Structure Using $^{10}\mathrm{Be}(p,p\alpha)^{6}\mathrm{He}$ Triple Differential Reaction Cross-Section Measurements

The cluster structure of the neutron-rich isotope $^{10}$Be has been probed via the $(p,p\alpha)$ reaction at 150 MeV/nucleon in inverse kinematics and in quasifree conditions. The populated states of $^{6}$He residues were investigated through missing mass spectroscopy. The triple differential cross-section for the ground-state transition was extracted for quasifree angle pairs ($\theta_{p}$, $\theta_{\alpha}$) and compared to distorted-wave impulse approximation reaction calculations performed in a microscopic framework using successively the Tohsaki-Horiuchi-Schuck-R\"opke product wave-function and the wave-function deduced from Antisymmetrized Molecular Dynamics calculations. The remarkable agreement between calculated and measured cross-sections in both shape and magnitude validates the molecular structure description of the $^{10}$Be ground-state, configured as an $\alpha$-$\alpha$ core with two valence neutrons occupying $\pi$-type molecular orbitals.

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