arXiv subjects

S. Fratini

Publications and source records attributed to S. Fratini.

51 records · Page 3Linked to original sources

arXiv2003

Incipient quantum melting of the one-dimensional Wigner lattice

A one--dimensional tight--binding model of electrons with long--range Coulomb interactions is studied in the limit where double site occupancy is forbidden and the Coulomb coupling strength $V$ is large with respect to the hopping amplitude $t$. The quantum problem of a kink--antikink pair generated in the Wigner lattice (the classical ground state for $t=0$) is solved for fillings $n=1/s$, where $s$ is an integer larger than 1. The pair energy becomes negative for a relatively high value of $V$, $V_c/t\approx s^3$. This signals the initial stage of the quantum melting of the Wigner lattice.

cond-mat.str-el↗

arXiv2003

Dynamical mean field theory of small polaron transport

We present a unified view of the transport properties of small-polarons in the Holstein model at low carrier densities, based on the Dynamical Mean Field Theory. The nonperturbative nature of the approach allows us to study the crossover from classical activated motion at high temperatures to coherent motion at low temperatures. Large quantitative discrepancies from the standard polaronic formulae are found. The scaling properties of the resistivity are analysed, and a simple interpolation formula is proposed in the nonadiabatic regime.

cond-mat.str-el↗

arXiv2003

Charge and spin order in one-dimensional electron systems with long-range Coulomb interactions

We study a system of electrons interacting through long--range Coulomb forces on a one--dimensional lattice, by means of a variational ansatz which is the strong--coupling counterpart of the Gutzwiller wave function. Our aim is to describe the quantum analogue of Hubbard's classical ``generalized Wigner crystal''. We first analyse charge ordering in a system of spinless fermions, with particular attention to the effects of lattice commensurability. We argue that for a general (rational) number of electrons per site $n$ there are three regimes, depending on the relative strength $V$ of the long--range Coulomb interaction (as compared to the hopping amplitude $t$). For very large $V$ the quantum ground state differs little from Hubbard's classical solution, for intermediate to large values of $V$ we recover essentially the Wigner crystal of the continuum model, and for small $V$ the charge modulation amounts to a small--amplitude charge--density wave. We then include the spin degrees of freedom and show that in the Wigner crystal regimes (i.e. for large $V$) they are coupled by an antiferromagnetic kinetic exchange $J$, which turns out to be smaller than the energy scale governing the charge degrees of freedom. Our results shed new light on the insulating phases of organic quasi--1D compounds where the long--range part of the interaction is unscreened, and magnetic and charge orderings coexist at low temperatures.

cond-mat.str-el↗

arXiv2002

Variational Wave Function for Generalized Wigner Lattices in One Dimension

We study a system of electrons on a one-dimensional lattice, interacting through the long range Coulomb forces, by means of a variational technique which is the strong coupling analog of the Gutzwiller approach. The problem is thus the quantum version of Hubbard's classical model of the generalized Wigner crystal [J. Hubbard, Phys. Rev. B 17, 494 (1978)]. The magnetic exchange energy arising from quantum fluctuations is calculated, and turns out to be smaller than the energy scale governing charge degrees of freedom. This approach could be relevant in insulating quasi-one-dimensional compounds where the long range Coulomb interactions are not screened. In these compounds charge order often appears at high temperatures and coexists with magnetic order at low temperatures.

cond-mat.str-el↗

arXiv2002

Polarization catastrophe in doped cuprates and metal-ammonia solutions: an analogy

On doping polar dielectrics, such as the cuprates or liquid ammonia, the long range polarization leads to the formation of bound states (polarons or solvated electrons). However, the exact role of such entities in the metal-insulator transition (MIT) still remains unclear. We suggest that the driving mechanism of the MIT is a polarization catastrophe that occurs due to their unscreened Coulomb interaction. This phenomenon is associated to a negative static dielectric constant, which could be the origin of both the superconducting transition in the cuprates -- where the doping ions are frozen in the lattice structure -- and the phase separation observed in liquid metal-ammonia solutions -- where the counter-ions are mobile.

cond-mat↗

arXiv2002

Polarization catastrophe in the polaronic Wigner crystal

We consider a three dimensional Wigner crystal of electrons lying in a host ionic dielectric. Owing to their interaction with the lattice polarization, each localized electron forms a polaron. We study the collective excitations of such a polaronic Wigner crystal at zero temperature, taking into account the quantum fluctuations of the polarization within the Feynman harmonic approximation. We show that, contrary to the ordinary electron crystal, the system undergoes a polarization catastrophe when the density is increased. An optical signature of this instability is derived, whose trend agrees with the experiments carried out in Nd-based cuprates.

cond-mat.str-el↗

arXiv2002

Electronic susceptibilities in systems with anisotropic Fermi surfaces

The low temperature dependence of the spin and charge susceptibilities of an anisotropic electron system in two dimensions is analyzed. It is shown that the presence of inflection points at the Fermi surface leads, generically, to a $ T \log T $ dependence, and a more singular behavior, $χ\sim T ^{3/4} \log T$, is also possible. Applications to quasi two-dimensional materials are discussed.

cond-mat.str-el↗

arXiv2001

Energy radiation of moving cracks

The energy radiated by moving cracks in a discrete background is analyzed. The energy flow through a given surface is expressed in terms of a generalized Poynting vector. The velocity of the crack is determined by the radiation by the crack tip. The radiation becomes more isotropic as the crack velocity approaches the instability threshold.

cond-mat.mtrl-sci↗

arXiv2001

Anomalous optical absorption in overdoped cuprates near the charge-ordering instability

We propose an interpretation for the hump observed in the optical conductivity at or below a few hundreds of cm$^{-1}$, in overdoped cuprates like the electron-doped Nd_{2-x}Ce_xCuO_{4-y} at x\gtrsim 0.15 and the hole-doped Bi_2Sr_2CuO_6 and La_{2-x}Sr_xCuO_4. This interpretation is based on the direct excitation of charge collective modes, which become nearly critical in the proximity to a charge-ordering instability. The nearly critical character of these excitations entails a peculiar temperature dependence and a pseudo-scaling form of the lineshapes, which are in agreement with the experimental data.

cond-mat.supr-con↗

arXiv2000

Jahn-Teller, Charge and Magnetic Ordering in half-doped Manganese Oxides

The phase diagram of half-doped manganite systems of formula A_{0.5}A'_{0.5}MnO_3 is investigated within a single-orbital model incorporating magnetic double-exchange and superexchange, together with intersite Coulomb and electron-lattice interactions. Strong Jahn-Teller and breathing mode deformations compete together and result in shear lattice deformations. The latters stabilize the charge-ordered CE-type phase, which undergo first-order transitions with temperature or magnetic field to either Ferromagnetic metallic or Paramagnetic insulating phases. An essential feature is the self-consistent screening of Coulomb and electron-phonon interactions in the ferromagnetic phase.

cond-mat.str-el↗

arXiv2000

Is the Quantum Melting of a Polaron Wigner Crystal an Insulator-to-Superconductor transition ?

On examining the stability of a Wigner Crystal (WC) in an ionic dielectric, two competitive effects due to Polaron formation are found to be important: (i) the screening of the Coulomb forces which destabilizes the crystal, compensated by (ii) the increase of the carrier mass (polaron mass). The quantum melting of the Polaron Wigner Crystal (PWC) is examined. By calculating the quantum fluctuations of both the electrons and the polarization, we show that there is a competition between the dissociation of the Polarons at the insulator-to-metal transition (IMT), and a melting towards a polaron liquid. We find that at strong coupling ($α> α^*$), a liquid state of polarons cannot exist, and the IMT is driven by polaron dissociation. Next, we show that the dipolar interactions between localized polarons are responsible for a phonon instability of the PWC as the density increases. This provides a new mechanism for the IMT in doped dielectrics. Examining the sign of the dielectric constant of the PWC, we conjecture that such an instability could yield an Insulator-to-Superconductor transition.

cond-mat.supr-con↗

arXiv1999

Melting of a Wigner Crystal in an Ionic Dielectric

The melting of a Wigner Crystal of electrons placed into a host polar material is examined as a function of the density and the temperature. When the coupling to the longitudinal optical modes of the host medium is turned on, the WC is progressively transformed into a polaronic Wigner Crystal. We estimate the critical density for crystal melting at zero temperature using the Lindeman criterion. We show that above a certain critical value of the Frohlich electron-phonon coupling, the melting towards a quantum liquid of polarons is not possible, and the insulator-to-metal transition is driven by the ionization of the polarons (polaron dissociation). The phase diagram at finite temperature is obtained by making use of the same Lindeman criterion. Results are also provided in the case of an anisotropic electron band mass, showing that the scenario of polaron dissociation can be relevant in anisotropic compounds such as the superconducting cuprates at rather moderate e-ph couplings.

cond-mat.str-el↗

arXiv1998

Polaron Crystallization and Melting: Effects of the Long-Range Coulomb Forces

On examining the stability of a Wigner crystal in an ionic dielectric, two competitive effects due to the polaron formation are found to be important: (i) the screening of the Coulomb force, which destabilizes the crystal, compensated by (ii) the increase of the carrier mass (polaron mass). The competition between the two effects is carefully studied, and the quantum melting of the polaronic Wigner crystal is examined by varying the density at zero temperature. By calculating the quantum fluctuations of both the electron and the polarization, we show that there is a competition between the dissociation of the polarons at the insulator-to-metal transition (IMT), and a melting towards a polaron liquid. We find that at strong coupling, a liquid state of dielectric polarons cannot exist, and the IMT is driven by the polaron dissociation. Next, taking into account the dipolar interactions between localized carriers, we show that these are responsible for an instability of the transverse vibrational modes of the polaronic Wigner crystal as the density increases. This provides a new mechanism for the IMT in doped dielectrics, which yields interesting dielectric properties below and beyond the transition. An optical signature of such a mechanism for the IMT is provided.

cond-mat.supr-con↗

arXiv1997

Polaron Dissociation at the Insulator-to-Metal Transition

Considering the long range Coulomb interactions between large polarons in dielectrics, we propose a model for their crystallization when no bipolarons are formed. As the density increases, the melting is examined at $T=OK$. One possibility is the delocalization towards a liquid state of polarons. However, we show that this cannot happen if the electron-phonon coupling is larger than some critical value. The other competing mechanism is the dissociation of the polarons themselves, favored owing to their large mass at strong coupling. Finally, we propose a phase diagram for the insulator-to metal transition as a function of the density and electron-phonon coupling.

cond-mat↗

arXiv1997

Dynamical mean-field theory of the small polaron

A dynamical mean-field theory of the small polaron problem is presented, which becomes exact in the limit of infinite dimensions. The ground state properties and the one-electron spectral function are obtained for a single electron interacting with Einstein phonons by a mapping of the lattice problem onto a polaronic impurity model. The one-electron propagator of the impurity model is calculated through a continued fraction expansion (CFE), both at zero and finite temperature, for any electron-phonon coupling and phonon energy. In contrast to the ground state properties such as the effective polaron mass, which have a smooth behaviour, spectral properties exhibit a sharp qualitative change at low enough phonon frequency: beyond a critical coupling, one energy gap and then more and more open in the density of states at low energy, while the high energy part of the spectrum is broad and can be explained by a strong coupling adiabatic approximation. As a consequence narrow and coherent low-energy subbands coexist with an incoherent featureless structure at high energy. The subbands denote the formation of quasiparticle polaron states. Also, divergencies of the self-energy may occur in the gaps. At finite temperature such effect triggers an important damping and broadening of the polaron subbands. On the other hand, in the large phonon frequency regime such a separation of energy scales does not exist and the spectrum has always a multipeaked structure.

cond-mat↗