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S. Goriely

Publications and source records attributed to S. Goriely.

At least 19 recordsLinked to original sources

The impact of nuclear uncertainties on the p-process nucleosynthesis in Supernovae

The p-process is responsible for the production of the stable neutron-deficient nuclei heavier than iron observed in the solar system. However, important nuclear uncertainties still limit our understanding of this nucleosynthesis process. Among the most significant are the nuclear level densities (NLDs) and photon strength functions (PSFs) entering the calculation of photodisintegration rates under supernova conditions. We investigate both model (systematic) and parameter (statistical) uncertainties affecting NLDs and PSFs and quantify their impact on p-process nucleosynthesis in type-Ia and type-II supernovae. Correlated model uncertainties are estimated using several NLD and PSF models that reproduce available experimental observables. Uncorrelated parameter uncertainties are evaluated with a backward-forward Monte Carlo approach, in which parameter variations are constrained by measured reaction rates before being propagated to unknown cross sections of neutron-deficient nuclei. The resulting uncertainties are propagated through p-process calculations while preserving model correlations. To identify the reactions driving abundance uncertainties, we combine regularized linear-response modeling, stability analysis, and contribution and interaction decompositions. We find that photoneutron-emission uncertainties dominate the overall uncertainty budget. The leading source of uncertainty arises from local parameter variations still compatible with current experimental constraints, highlighting the lack of constraining nuclear data in the neutron-deficient region. For many p-nuclei, the dominant contribution originates either from the photoneutron emission of the p-nucleus itself or from a nearby $(\gamma,n)$ reaction along the same isotopic chain. While improved nuclear models remain important, many key reactions involve stable or near-stable nuclei and should be experimentally accessible.

nucl-th

Detection of actinides in CEMP-rs stars

The carbon-enhanced metal-poor stars with hybrid enrichments of slow- and rapid neutron-capture elements, the so-called CEMP-rs stars, still raise many questions due to their elusive abundance signatures. In our recent analysis, we found that heavy r process elements are enhanced in these objects and can be explained by the intermediate neutron-capture process (i-process) occurring in low-mass, very low-metallicity asymptotic giant branch (AGB) stars. However, the origin of actinides such as thorium and uranium is typically associated with explosive nucleosynthesis in highly neutron-rich environments, and their detection in stellar spectra remains challenging due to severe line blending from other elements and carbon-bearing molecules. In this work, we investigate the presence of thorium and uranium abundances in a sample of CEMP-rs stars using their high-resolution spectra obtained with the UVES spectrograph mounted on the UT2 (Kueyen) ESO VLT. Thorium is robustly detected in three stars, while uranium remains marginally detected, allowing only upper limits to be derived. Comparison with theoretical i-process nucleosynthesis models demonstrates that the observed abundances can be reproduced within uncertainties, supporting an i-process origin for these elements. This study reports the first detection of actinides in stars confirmed as CEMP-rs stars, providing new constraints on their nucleosynthetic history. Furthermore, these detections provide a potential way to estimate in the future the time elapsed since the proton-ingestion episode in AGB stars using cosmochronometry techniques, and more generally to place lower limits on the ages of the resulting white dwarf remnants.

astro-ph.SR

Stellar nucleosynthesis in the era of large surveys: S-process polluted binaries in GALAH DR4

Binary interactions during the AGB phase can lead to the formation of chemically peculiar stars with overabundances of s-process elements. Only a few hundreds of these stars have been subject to detailed chemical or dynamical studies. This work aims at compiling a systematic sample of s-process-polluted candidates using GALAH DR4. We also want to compare their properties with those of confirmed s-polluted stars to have stronger evidence of their nature. GALAH DR4 uses neural networks and automatic spectral analysis methods as well as data of a lower spectral resolution than normally used to characterise these objects. Because of this, we built a validation sample, for which we obtained UVES@VLT and HERMES@Mercator high-resolution spectra. We compare our stellar parameters and abundances with those of the survey and use this validation to define the thresholds that a star in GALAH DR4 must pass to be flagged as a good s-process-rich candidate. Based on our comparisons, we define thresholds on [s/Fe], [Y/Fe], [Zr/Fe], [Ba/Fe], and [La/Fe]. We identified 1059 stars in GALAH DR4 that are good candidates to be s-process polluted stars, covering a broad parameter space. They share many similarities with the samples of confirmed s-rich stars, especially their ratios of heavy over light s-elements ([hs/ls]), which strengthen our confidence in the purity of the sample. We find that only 7% of the candidates have measured orbital periods and eccentricities, limiting for now a full comparison with confirmed Ba and related stars. However, their binary fraction is, as expected, higher than the one we found for the full GALAH DR4 catalogue. Our sample of candidates is almost five times larger than the number of currently confirmed polluted stars. This and the fact that it has been homogeneously treated by GALAH open very interesting avenues to confront nucleosynthesis and binary evolution models.

astro-ph.SR

Skyrme-Hartree-Fock-Bogoliubov mass models on a 3D mesh: V. The N2LO extension of the Skyrme EDF

We present BSkG5, the latest entry in the Brussels-Skyrme-on-a-Grid (BSkG) series and the first large-scale nuclear structure model based on next-to-next-to-leading order (N2LO) Skyrme energy density functional (EDF). By extending the traditional Skyrme EDF ansatz with central terms containing up to four gradients, we are able to combine an excellent global description of nuclear ground state properties with a stiff equation of state for pure neutron matter that is consistent with all astronomical observations of neutron stars. More precisely, the new model matches the accuracy of earlier BSkG models but with two parameters less: we achieve root-mean-square deviations of 0.649 MeV for 2457 atomic masses, 0.0267 fm for 810 charge radii, and 0.43 MeV for 45 primary fission barriers of actinide nuclei. We demonstrate that the complexities of N2LO EDFs are not insurmountable, even for demanding many-body calculations.

nucl-th

Improved microscopic nuclear level densities within the triaxial Hartree-Fock-Bogoliubov plus combinatorial method

New developments have been brought to our energy-, spin- and parity-dependent nuclear level densities based on the microscopic combinatorial method. Our new calculation is based on the BSkG3 mean-field model which relies on a three-dimensional coordinate-space representation of the nucleus, allowing for the spontaneous breaking of ground state rotational, axial and reflection symmetry. In particular, we now account for the impact of possible triaxial deformation of nuclear ground states on the level density. This has two effects on our calculations: the additional freedom of the single-particle levels affects the intrinsic level density while the absence of a rotational symmetry axis results in a larger collective correction. The present model reproduces the experimental s- and p-wave neutron resonance spacings with a degree of accuracy comparable to that of the best global models available. It is also shown that the model gives a reliable extrapolation at low energies where experimental data on the cumulative number of levels can be extracted. The predictions are also in good agreement with the experimental data extracted from the Oslo method. Total level densities for more than 8500 nuclei are made available in a table format for practical applications. For the nuclei for which experimental s-wave spacings and enough low-lying states exist, renormalization factors are provided to reproduce simultaneously both observables. The same combinatorial method is used to estimate the nuclear level densities at the fission saddle points of actinides and at the shape isomer deformation. Finally, the new nuclear level densities are applied to the calculation of radiative neutron capture cross sections and compared with those obtained with our previous combinatorial model.

nucl-th

The intermediate neutron capture process. VI. Proton ingestion and i-process in rotating magnetic asymptotic giant branch stars

The intermediate neutron-capture process (i-process) can occur during proton ingestion events (PIEs), which may take place in the early evolutionary phases of asymptotic giant branch (AGB) stars. We investigate the impact of rotational and magnetic mixing on i-process nucleosynthesis in low-metallicity, low-mass AGB stars. We computed AGB models with [Fe/H] = $-2.5$ and $-1.7$ and initial masses of 1 and 1.5 $M_{\odot}$ using the STAREVOL code, including a network of 1160 nuclei coupled to transport equations. Rotating models incorporate a calibrated Tayler-Spruit (TS) dynamo to account for core rotation rates inferred from asteroseismic observations of solar-metallicity sub-giants and giants. Initial rotation velocities of 0, 30, and 90 km s$^{-1}$ were considered, along with varying assumptions for magnetic mixing. We find that rotation without magnetic fields strongly suppresses the i-process due to the production of primary $^{14}$N, which is subsequently converted into $^{22}$Ne $-$ a potent neutron poison during the PIE. Including magnetic fields via the TS dynamo restores the models close to their non-rotating counterparts: strong core-envelope coupling suppresses shear mixing and prevents primary $^{14}$N synthesis, yielding i-process nucleosynthesis similar to non-rotating models. We also find that rotational mixing during the AGB phase is insufficient to affect the occurrence of PIEs. Proton ingestion event-driven nucleosynthesis proceeds similarly in asteroseismic-calibrated magnetic rotating AGB stars and non-rotating stars, producing identical abundance patterns.

astro-ph.SR

Modeling Ultra-High-Energy Cosmic Rays propagation using the input from Configuration Interaction Shell Model

The dipole response of a nuclear system, characterized by its photon strength function (PSF), is a key ingredient of many applications of nuclear structure, ranging from nuclear reactor design and nuclear waste transmutation to astrophysical models of nucleosynthesis and stellar evolution. While the majority of those applications require the knowledge of PSF of mid-mass and heavy nuclei, there is now renewed interest in $E1$ strength distributions of light nuclei in the framework of the PANDORA project, which aims at an understanding of the mass distribution of ultrahigh-energy cosmic radiation (UHECR).UHECR is of extragalactic origin and its interaction along the travel path is dominated by photoabsorption of cosmic background radiation boosted to the Giant Dipole Resonance (GDR) energy region in the center-of-mass system. Thus, systematic knowledge of the photoabsorption cross sections in light nuclei and of their subsequent particle decay is required. The purpose of this work is to enhance the database of available theoretical evaluations of PSF of light nuclei that are necessary in the studies of UHECR propagation. We employ the Configuration Interaction Shell Model (CI-SM) approach to provide predictions of $E1$ dipole response for $p$ and $sd$-shell nuclei, with mass number $A$ between 7 and 40. Theoretical predictions are compared to available data and to existing predictions from phenomenological and microscopic models. Finally, the impact of using of CI-SM PSF on the predicted propagation of a $^{40}$Ca UHECR source is studied.

nucl-th

Exploring the statistical properties of the neutron-deficient $^{109}$In isotope with the Oslo method

The nuclear level density (NLD) and the $\gamma$-ray strength function (GSF) of the neutron-deficient $^{109}$In isotope were extracted for the first time with data from the $^{106}$Cd$(\alpha,p\gamma)^{109}$In reaction using a combination of the Oslo and the shape methods. Both quantities are consistent with those of neighboring Cd and Sn nuclei, but show substantial discrepancies with currently available model predictions. In contrast to earlier observations in the neighboring isotopic chains, $^{109}$In does not exhibit any significant enhancement of the dipole strength near the neutron separation energy. To interpret this feature, random-phase time-blocking approximation calculations have been performed for $^{109}$In and the neighboring $^{110,112}$Sn nuclei. The experimental data were also employed to estimate cross sections and rates of the radiative neutron- and proton-capture reactions, $^{108}$In($n,\gamma)$$^{109}$In and $^{108}$Cd($p,\gamma)$$^{109}$In, respectively, with the reaction code TALYS. Our ($p,\gamma)$ cross section is in excellent agreement with direct measurements over a wide range of proton energies, while the ($n,\gamma)$ cross section demonstrates notable deviations from predictions in the JINA REACLIB library. The new results on the statistical properties of $^{109}$In provide valuable constraints that may help address the problem of large model uncertainties compromising the accuracy of astrophysical $p$-process simulations.

nucl-ex

High-Resolution Laser Spectroscopy on the Hyperfine Structure of $^{255}$Fm (Z=100)

We report on high-resolution laser spectroscopy of $^{255}$Fm ($T_{1/2} = 20$h), one of the heaviest nuclides available from reactor breeding. The hyperfine structures in two different atomic ground-state transitions at 398.4~nm and 398.2~nm were probed by in-source laser spectroscopy at the RISIKO mass separator in Mainz, using the PI-LIST high-resolution ion source. Experimental results were combined with hyperfine fields from various atomic ab-initio calculations, in particular using MultiConfigurational Dirac-Hartree-Fock theory, as implemented in GRASP18. In this manner, the nuclear magnetic dipole and electric quadrupole moments were derived to be $\mu = -0.75(5)~ \mu_\textrm{N}$ and $Q_\textrm{S} = +5.84(13)$~eb, respectively. The magnetic moment indicates occupation of the $\nu$~7/2[613] Nilsson orbital, while the large quadrupole moment confirms strong, stable prolate deformation consistent with systematics in the heavy actinides. Comparisons with available expectation values from nuclear theory show good agreement, providing a stringent benchmark for the used theoretical models. These results revise earlier data and establish $^{255}$Fm as a reference isotope for future high-resolution studies.

physics.atom-ph

Abundance of heavy r-process elements in CEMP-rs stars: The role of the i-process

Carbon-enhanced metal-poor (CEMP) stars are ancient stars enriched in carbon and heavy elements. Some of these stars exhibit enhanced s-process and/or r-process elements, hence are classified as CEMP-s, CEMP-rs, or CEMP-r. This classification is challenging due to the limited availability of heavy element abundances, particularly among r-process elements. Heavy r-process elements such as terbium, holmium, thulium, ytterbium, lutetium, tantalum, and iridium have rarely been measured because their sensitive lines are located in the ultraviolet. However, they provide sensitive diagnostics of the s-, r-, and i- nucleosynthetic processes. In this work, we aim to obtain a secure classification of CEMP-s and -rs stars and investigate whether the i-process can account for the measured abundance patterns in CEMP-rs stars. We derive the abundance profiles, notably for twelve heavy r-elements, including, in some cases, tantalum, using high-resolution UVES spectra of seventeen CEMP-s and -rs stars. Based on indicators such as the [s/r] abundance ratio or the model-independent 'abundance distance', nine stars are confirmed as CEMP-rs and six as CEMP-s. The classification of two objects remains uncertain. The i-process satisfactorily reproduces the abundance patterns of CEMP-rs stars. However, larger samples are needed to confirm trends with metallicity and clarify how CEMP-rs stars differ from CEMP-s stars.

astro-ph.SR

TENDL-astro: a new nuclear data set for astrophysics interest

In this work, we are presenting a new database of astrophysical interest, based on calculations performed with the nuclear reaction code TALYS. Four quantities are systematically calculated for over 8000 nuclides: cross sections, reaction rates, Maxwellian Averaged Cross Sections (or MACS) at 30 keV and partition functions. For cross sections and reaction rates, nine reactions are considered, induced by neutron, proton or alpha. The main complement of this database compared to existing ones is that the impact of reaction models ({\it e.g.} level density, gamma strength function, and optical model) is estimated by varying 9 different models, and by proposing calculated values for each of them, together with averages, standard deviations and other statistical quantities. This new database, called TENDL-astro, version 2023, is available online (https://tendl.web.psi.ch/tendl\_2023/astro/astro.html) and linked to the well-known TENDL database, used in a variety of applications.

nucl-th

What to expect from microscopic nuclear modelling for k$_{\rm eff}$ calculations ?

Comparisons between predicted and benchmark k$_{\rm eff}$ values from criticality-safety systems are often used as metrics to estimate the quality of evaluated nuclear data libraries. Relevant nuclear data for these critical systems generally come from a mixture of expert knowledge and phenomenological predictions. In the present work, we use solely microscopic nuclear modelling from TALYS to estimate actinides cross sections and angular distributions, and we compare the calculated MCNP k$_{\rm eff}$ values for fast systems between the JEFF-3.3 evaluated library, phenomenological and microscopic modelling. The conclusion is that even if the evaluated library leads to the most adequate results, the microscopic nuclear modelling can reach very similar results for these integral quantities. It demonstrates the remarkable advances in the recent decades of microscopic nuclear reaction ingredients for applied integral observables.

nucl-th

Photoneutron reactions on gold in the giant dipole resonance region: reaction cross sections and average kinetic energies of $(\gamma,\,xn)$ photoneutrons

In this work, we present new data on the $^{197}$Au photoneutron reactions in and above the giant dipole resonance region, obtained by using 8 to 39~MeV quasi-monochromatic $\gamma$-ray beams produced at the NewSUBARU facility in Japan and a high-and-flat efficiency neutron detection system. We report absolute cross sections and mean photoneutron energies for the $^{197}$Au$(\gamma,\,inX)$ reactions with $i$~=~1 to 4. The photoabsorption cross section was obtained as the sum of the $(\gamma,\,inX)$ reaction cross sections. The giant dipole resonance parameter values were obtained by fitting the experimental photoabsorption cross sections. The present photoabsorption cross sections are in good agreement with the Saclay results of Veyssiere~\emph{et al.}. Thus, our study does not support the recommendation of Berman~\emph{et al.} of lowering the Saclay photoabsorption cross sections by 8$\%$. We observed a non-statistical high-energy neutron emission in the $(\gamma,\,n)$ reaction in the low-energy region between $S_n$ and 10~MeV. The present results are compared with data from the literature and statistical model calculations performed with the TALYS and EMPIRE codes.

nucl-ex

The impact of mass uncertainties on the r-process nucleosynthesis in neutron star mergers

Theoretical predictions of element yields from the rapid neutron capture (r-) process are subject to large uncertainties due to incomplete knowledge of nuclear properties and approximative hydrodynamical modeling of matter ejection. A major source of uncertainty in determining ejecta composition and radioactive decay heat is the lack of nuclear mass data for exotic neutron-rich nuclei produced during neutron irradiation. We examine both model (systematic) and parameter (statistical) uncertainties affecting nuclear mass predictions and their impact on r-process nucleosynthesis, and consequently, the composition of neutron star merger ejecta. To estimate the effect of model uncertainties, we consider five nuclear mass models that accurately describe known masses. We also use a backward-forward Monte Carlo method to estimate uncorrelated uncertainties from local variations in model parameters, constraining them to experimentally known masses before propagating them to unknown masses of neutron-rich nuclei. These mass uncertainties are then applied to a 1.38-1.38 M$_{\odot}$ neutron star merger model, considering a wide range of ejecta trajectories. We find that uncorrelated parameter uncertainties lead to ejected abundance uncertainties of 20% up to A $\simeq$ 130, 40% between A=150 and 200, with peaks around A $\simeq$ 140 and A $\simeq$ 203, leading to deviations of 100-300%. While correlated model uncertainties generally exceed parameter uncertainties for most nuclei, both have a significant impact on heavy element production. Overall, improvements in nuclear models are essential to reducing uncertainties in r-process predictions. Both correlated model uncertainties and coherent determination of parameter uncertainties are crucial for sensitivity analysis in r-process nucleosynthesis.

astro-ph.HE

Production of Lithium and Heavy Elements in AGB Stars Experiencing PIEs

Asymptotic giant branch (AGB) stars can experience proton ingestion events (PIEs), leading to a rich nucleosynthesis. During a PIE, the intermediate neutron capture process (i-process) develops, leading to the production of trans-iron elements. It is also suggested that lithium is produced during these events. We investigate the production of lithium and trans-iron elements in AGB stars experiencing a PIE with $1<M_{\rm ini}/M_{\odot}< 3$ and $-3< \mathrm{[Fe/H]} <0$. We find that lithium is produced in all PIE models with surface abundances $3<$ A(Li) $<5$. The surface enrichment and overall AGB lithium yield increases with decreasing stellar mass. The lithium enrichment is accompanied by a production of $^{13}$C with $3<^{12}$C/$^{13}$C$<9$ at the surface just after the PIE. AGB stars experiencing PIE may be related to J-type carbon stars whose main features are excesses of lithium and $^{13}$C. In addition to Li and $^{13}$C, heavy elements (e.g., Sr, Ba, Eu, Pb) are significantly produced in low-metallicity stars up to [Fe/H]$\simeq-1$. The yields of our models are publicly available. Additionally, of interest to the Li nucleosynthesis, we provide an updated fitting formula for the $^{7}$Be($e^-,\nu_e$)$^{7}$Li electron capture rate.

astro-ph.SR

Proton ingestion in asymptotic giant branch stars as a possible explanation for J-type stars and AB2 grains

J-type stars are a subclass of carbon stars that are generally Li-rich, not enriched in s-elements, and have low $^{12}$C/$^{13}$C ratios. They were suggested to be the manufacturers of the pre-solar grains of type AB2 (having low $^{12}$C/$^{13}$C and supersolar $^{14}$N/$^{15}$N). In this Letter, we investigate the possibility that J-type stars are early asymptotic giant branch (AGB) stars that experienced a proton ingestion event (PIE). We used the stellar evolution code STAREVOL to compute AGB stellar models with initial masses of 1, 2, and 3 $M_{\odot}$ and metallicities [Fe/H] $= -0.5$ and 0.0. We included overshooting above the thermal pulse and used a network of 1160 nuclei coupled to the transport equations. In solar-metallicity AGB stars, PIEs can be triggered if a sufficiently high overshoot is considered. These events lead to low $^{12}$C/$^{13}$C ratios, high Li abundances, and no enrichment in s-elements. We find that the $2-3$ $M_{\odot}$ AGB models experiencing a PIE can account for most of the observational features of J-type stars and AB2 grains. The remaining tensions between models and observations are (1) the low $^{14}$N/$^{15}$N ratio of some AB2 grains and of 2 out of 13 J-type stars, (2) the high $^{26}$Al/$^{27}$Al of some AB2 grains, and (3) the J-type stars with A(Li) $<2$. Extra mixing mechanisms can alleviate some of these tensions, such as thermohaline or rotation. This work highlights a possible match between AGB stellar models that undergo a PIE and J-type stars and AB2 grains. To account for other types of carbon stars, such as N-type stars, PIEs should only develop in a fraction of solar-metallicity AGB stars. Additional work is needed to assess how the occurrence of PIEs depends on mixing parameters and initial conditions, and therefore to further confirm or exclude the proposed scenario.

astro-ph.SR

Photoneutron cross section measurements on $^{208}$Pb in the Giant Dipole Resonance region

Photoneutron reactions on $^{208}$Pb in the Giant Dipole Resonance energy region have been investigated at the $\gamma$-ray beam line of the NewSUBARU facility in Japan. The measurements made use of quasi-monochromatic laser Compton backscattering $\gamma$-ray beams in a broad energy range, from the neutron threshold up to 38 MeV, and of a flat-efficiency moderated $^3$He neutron detection system along with associated neutron-multiplicity sorting methods. We report absolute cross sections and mean photoneutron energies for the $^{208}$Pb$(\gamma,\,inX)$ reactions with $i$~=~1 to 4. The fine structure present in the $^{208}$Pb$(\gamma,\,n)$ cross sections at incident energies lower than 13~MeV has been observed. The photoabsorption cross section has been obtained as the sum of the $(\gamma,\,inX)$ reaction cross sections. By reproducing the measured ring-ratio values at excitation energies below the two neutron separation energy, we were able to extract estimations on the $^{208}$Pb$(\gamma,\,n)$ photoneutron energy spectra and on the partial photoneutron cross sections for leaving the residual $^{207}$Pb in its ground and first two excited states. The present results are compared with data from the literature and statistical model calculations.

nucl-ex

Giant Dipole Resonance photofission and photoneutron reactions in $^{238}$U and $^{232}$Th

New measurements of photofission and photoneutron reactions on $^{238}$U and $^{232}$Th in the Giant Dipole Resonance (GDR) energy region have been performed at the laser Compton-scattering $\gamma$-ray source of the NewSUBARU synchrotron radiation facility using a high-and-flat efficiency moderated $^3$He detection array. The neutron-multiplicity sorting of high-multiplicity fission neutron coincidence events has been performed using a dedicated energy dependent, multiple firing statistical treatment. The photoneutron $(\gamma,\,in)$ with $i$~=~1~--~3 and photofission $(\gamma,\,F)$ reactions have been discriminated by considering a Gaussian distribution of prompt-fission-neutron (PFN) multiplicities predicted by the theory of evaporation in sequential neutron emission from excited fission fragments. We report experimental $(\gamma,\,n)$, $(\gamma,\,2n)$, $(\gamma,\,3n)$ and $(\gamma,\,F)$ cross sections, average energies of PFNs and of $(\gamma,\,in)$ photoneutrons, as well as the mean number of PFNs per fission act and the width of the PFNs multiplicity distribution. Based on these primary experimental results and combined with reasonable assumptions, we extract also the first- and second-chance fission contributions. The new experimental results are compared with statistical-model calculations performed with the EMPIRE-3.2 Malta and TALYS-1.964 codes on the present data and with prompt fission emission calculations obtained with the Los Alamos model in the frame of the most probable fragmentation approach with and without sequential emission.

nucl-ex