arXiv subjects

S. Goriely

Publications and source records attributed to S. Goriely.

At least 73 records · Page 4Linked to original sources

arXiv2019

Reference Database for Photon Strength Functions

Photon strength functions describing the average response of the nucleus to an electromagnetic probe are key input information in the theoretical modelling of nuclear reactions. Consequently they are important for a wide range of fields such as nuclear structure, nuclear astrophysics, medical isotope production, fission and fusion reactor technologies. They are also sources of information for widely used reaction libraries such as the IAEA Reference Input Parameter Library and evaluated data files such as EGAF. In the past two decades, the amount of reaction gamma-ray data measured to determine photon strength functions has grown rapidly. Different experimental techniques have led to discrepant results and users are faced with the dilemma which (if any) of the divergent data to adopt. We report on a coordinated effort to compile and assess the existing experimental data on photon strength functions from the giant dipole resonance region to energies below the neutron separation energy. The assessment of the discrepant data at energies around or below the neutron separation energy has been possible only in a few cases where adequate information on the model-dependent analysis and estimation of uncertainties was available. In the giant dipole resonance region, we adopt the recommendations of the new IAEA photonuclear data library. We also present global empirical and semi-microscopic models that describe the photon strength functions in the entire energy region and reproduce reasonably well most of the experimental data. The compiled experimental photon strengths and recommended model calculations are available from the PSF database hosted at the IAEA (URL:www-nds.iaea.org/PSFdatabase).

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arXiv2019

$γ$-ray Strength Function for Barium Isotopes

Photoneutron cross sections were measured for $^{137}$Ba and $^{138}$Ba at energies below two-neutron threshold using quasi-monochromatic $γ$-ray beams produced in laser Compton-scattering at the NewSUBARU synchrotron radiation facility. The photoneutron data are used to constrain the $γ$-ray strength function on the basis of the Hartree-Fock-Bogolyubov plus quasi-particle random phase approximation using the Gogny D1M interaction. Supplementing the experimentally constrained $γ$-ray strength function with the zero-limit E1 and M1 contributions which are unique to the deexcitation mode, we discuss radiative neutron capture cross sections relevant to the s-process nucleosynthesis of barium isotopes in the vicinity of the neutron magic number 82.

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arXiv2019

IAEA Photonuclear Data Library 2019

Photo-induced reaction cross section data are of importance for a variety of current or emerging applications, such as radiation shielding design and radiation transport analyses, calculations of absorbed dose in the human body during radiotherapy, physics and technology of fission reactors (influence of photo-reactions on neutron balance) and fusion reactors (plasma diagnostics and shielding), activation analyses, safeguards and inspection technologies, nuclear waste transmutation, medical isotope production and astrophysical applications. Since the release of the IAEA Photonuclear Data Library in 1999 however, new experimental data as well as new methods to assess the reliability of experimental cross sections have become available. Theoretical models and input parameters used to evaluate photo-induced reactions have improved significantly over the years. In addition, new measurements of partial photoneutron cross sections using mono-energetic photon beams and advanced neutron detection systems have been performed allowing for the validation of the evaluations and assessments of the experimental data. Furthermore, technological advances have led to the construction of new and more powerful gamma-beam facilities, therefore new data needs are emerging. We report our coordinated efforts to address these data needs and present the results of the new evaluations of more than 200 nuclides included in the new updated IAEA Photonuclear Data Library, where the photon energy goes up to 200 MeV. We discuss the new assessment method and make recommendations to the user community in cases where the experimental data are discrepant and the assessments disagree. In addition, in the absence of experimental data, we present model predictions for photo-induced reaction cross section on nuclides of potential interest to medical radioisotope production.

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arXiv2019

Unified equations of state for cold non-accreting neutron stars with Brussels-Montreal functionals. I. Role of symmetry energy

The theory of the nuclear energy-density functional is used to provide a unified and thermodynamically consistent treatment of all regions of cold non-accreting neutron stars. In order to assess the impact of our lack of complete knowledge of the density dependence of the symmetry energy on the constitution and the global structure of neutron stars, we employ four different functionals. All of them were precision fitted to essentially all the nuclear-mass data with the Hartree-Fock-Bogoliubov method and two different neutron-matter equations of state based on realistic nuclear forces. For each functional, we calculate the composition, the pressure-density relation, and the chemical potentials throughout the star. We show that uncertainties in the symmetry energy can significantly affect the theoretical results for the composition and global structure of neutron stars. To facilitate astrophysical applications, we construct analytic fits to our numerical results.

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arXiv2019

Nuclear level densities and gamma-ray strength functions of $^{180,181,182}$Ta

Particle-$γ$ coincidence experiments were performed at the Oslo Cyclotron Laboratory with the $^{181}$Ta(d,X) and $^{181}$Ta($^{3}$He,X) reactions, to measure the nuclear level densities (NLDs) and $γ$-ray strength functions ($γ$SFs) of $^{180, 181, 182}$Ta using the Oslo method. The Back-shifted Fermi-Gas, Constant Temperature plus Fermi Gas, and Hartree-Fock-Bogoliubov plus Combinatorial models where used for the absolute normalisations of the experimental NLDs at the neutron separation energies. The NLDs and $γ$SFs are used to calculate the corresponding $^{181}$Ta(n,$γ$) cross sections and these are compared to results from other techniques. The energy region of the scissors resonance strength is investigated and from the data and comparison to prior work it is concluded that the scissors strength splits into two distinct parts. This splitting may allow for the determination of triaxiality and a $γ$ deformation of $14.9^{\circ} \pm 1.8^{\circ}$ was determined for $^{181}$Ta.

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arXiv2018

Photoneutron reaction cross section measurements on 94Mo and 90Zr relevant to the p-process nucleosynthesis

The photodisintegration cross sections for the 94Mo(γ,n) and 90Zr(γ,n) reactions have been experimentally investigated with quasi-monochromatic photon beams at the High Intensity γ-ray Source (HIγS) facility of the Triangle Universities Nuclear Laboratory (TUNL). The energy dependence of the photoneutron reaction cross sections was measured with high precision from the respective neutron emission thresholds up to 13.5 MeV. These measurements contribute to a broader investigation of nuclear reactions relevant to the understanding of the p-process nucleosynthesis. The results are compared with the predictions of Hauser-Feshbach statistical model calculations using two different models for the dipole γ-ray strength function. The resulting 94Mo(γ,n) and 90Zr(γ,n) photoneutron stellar reaction rates as a function of temperature in the typical range of interest for the p-process nucleosynthesis show how sensitive the photoneutron stellar reaction rate can be to the experimental data in the vicinity of the neutron threshold.

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arXiv2018

The $γ$-ray strength function for Thallium isotopes relevant to the $^{205}$Pb - $^{205}$Tl chronometry

Photoneutron cross sections were measured for $^{203}$Tl and $^{205}$Tl at energies between the one- and two-neutron thresholds using quasi-monochromatic $γ$-ray beams produced in laser Compton-scattering at the NewSUBARU synchrotron radiation facility. Our new measurement results in cross sections significantly different from the previously reported bremsstrahlung experiment, leading to rather different GDR parameters, in particular to lower GDR peak energies and higher peak cross sections. The photoneutron data are used to constrain the $γ$-ray strength function on the basis of the Hartree-Fock-Bogolyubov plus quasi-particle random phase approximation using the Gogny D1M interaction. Supplementing the experimentally constrained $γ$-ray strength function with the zero-limit E1 and M1 contributions for the de-excitation mode, we estimate the Maxwellian-averaged cross section for the s-process branching-point nucleus $^{204}$Tl in the context of the $^{205}$Pb - $^{205}$Tl chronometry.

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arXiv2018

Determination of the photodisintegration reaction rates involving charged particles: systematical calculations and proposed measurements based on Extreme Light Infrastructure - Nuclear Physics (ELI-NP)

Photodisintegration reaction rates involving charged particles are of relevance to the p-process nucleosynthesis that aims at explaining the production of the stable neutron-deficient nuclides heavier than iron. In this study, the cross sections and astrophysical rates of (g,p) and (g,a) reactions for about 3000 target nuclei with 10<Z<100 ranging from stable to proton dripline nuclei are computed. To study the sensitivity of the calculations to the optical model potentials (OMPs), both the phenomenological Woods-Saxon and the microscopic folding OMPs are taken into account. The systematic comparisons show that the reaction rates, especially for the (g,a) reaction, are dramatically influenced by the OMPs. Thus the better determination of the OMP is crucial to reduce the uncertainties of the photodisintegration reaction rates involving charged particles. Meanwhile, a gamma-beam facility at ELI-NP is being developed, which will open new opportunities to experimentally study the photodisintegration reactions of astrophysics interest. Considering both the important reactions identified by the nucleosynthesis studies and the purpose of complementing the experimental results for the reactions involving p-nuclei, the measurements of six (g,p) and eight (g,a) reactions based on the gamma-beam facility at ELI-NP and the ELISSA detector for the charged particles detection are proposed, and the GEANT4 simulations are correspondingly performed. The minimum required energies of the gamma-beam to measure these reactions are estimated. It is shown that the direct measurements of these photonuclear reactions within the Gamow windows at T_9=2.5 for p-process are fairly feasible and promising at ELI-NP. The expected experimental results will be used to constrain the OMPs of the charged particles, which can eventually reduce the uncertainties of the reaction rates for the p-process nucleosynthesis.

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arXiv2018

Photoneutron cross sections for Ni isotopes: Toward understanding $(n,γ)$ cross sections relevant to the weak s-process nucleosynthesis

Photoneutron cross sections were measured for $^{58}$Ni, $^{60}$Ni, $^{61}$Ni, and $^{64}$Ni at energies between the one-neutron and two-neutron thresholds using quasi-monochromatic $γ$-ray beams produced in laser Compton-scattering at the NewSUBARU synchrotron radiation facility. The new photoneutron data are used to extract the $γ$-ray strength function above the neutron threshold complementing the information obtained by the Oslo method below the threshold. We discuss radiative neutron capture cross sections and the Maxwellian-averaged cross sections for Ni isotopes including $^{63}$Ni, a branching point nucleus along the weak s-process path. The cross sections are calculated with the experimentally constrained $γ$-ray strength functions from the Hartree-Fock-Bogolyubov plus quasi-particle-random phase approximation based on the Gogny D1M interaction for both $E1$ and $M1$ components and supplemented with the $M1$ upbend.

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arXiv2018

When binaries keep track of recent nucleosynthesis: The Zr - Nb pair in extrinsic stars as an s-process diagnostic

Barium stars are s-process enriched giants. They owe their chemical peculiarities to a past mass transfer phase. During which they were polluted by their binary companion, which at the time was an AGB star, but is now an extinct white dwarf. Barium stars are thus ideal targets for understanding and constraining the s-process in low and intermediate-mass AGB stars. We derive the abundances of a large number of heavy elements in order to shed light on the conditions of operation of the neutron source responsible for the production of s-elements in the former companions of the barium stars. Adopting a recently used methodology(Neyskens et al. 2015), we analyse a sample of 18 highly enriched barium stars observed with the high-resolution HERMES spectrograph mounted on the MERCATOR telescope (La Palma). We determine the stellar parameters and abundances using MARCS model atmospheres. In particular, we derive the Nb/Zr ratio which was previously shown to be a sensitive thermometer for the s-process nucleosynthesis. Indeed, in barium stars, $^{93}Zr$ has fully decayed into mono-isotopic $^{93}Nb$ , so Nb/Zr is a measure of the temperature-sensitive $^{93}Zr/Zr$ isotopic ratio. HD 28159, previously classified as K5III and initially selected to serve as a reference cool K star for our abundance analysis, turns out to be enriched in s-process elements, and as such is a new barium star. Four stars, characterised by high nitrogen abundances, also tend to have high [Nb/Zr] and [hs/ls] ratios. The derived Zr and Nb abundances provide more accurate constraints on the s-process neutron source, identified to be $^{13}C(alpha,n)^{16}O$ for barium stars. The comparison with stellar evolution and nucleosynthesis models shows that the investigated barium stars were polluted by a low-mass (2-3 Solar mass) AGB star. HD 100503 is potentially identified as the highest metallicity CEMP-rs star yet discovered.

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arXiv2018

Crustal heating in accreting neutron stars from the nuclear energy-density functional theory. I. Proton shell effects and neutron-matter constraint

Observations of soft X-ray transients in quiescence suggest the existence of heat sources in the crust of accreting neutron stars. Heat is thought to be released by electroweak and nuclear processes triggered by the burying of ashes of X-ray bursts. The heating is studied using a fully quantum approach taking consistently into account nuclear shell effects. We have followed the evolution of ashes made of $^{56}$Fe employing the nuclear energy-density functional theory. Both the outer and inner crusts are described using the same functional, thus ensuring a unified and thermodynamically consistent treatment. To assess the role of the neutron-matter constraint, we have employed the set of accurately calibrated Brussels-Montreal functionals BSk19, BSk20, and BSk21 and for comparison the SLy4 functional. Due to nuclear shell effects, the fully accreted crust is found to be much less stratified than in previous studies. In particular, large regions of the inner crust contain clusters with the magic number $Z=14$. The heat deposited in the outer crust is tightly constrained by experimental atomic mass data. The shallow heating we obtain does not exceed $0.2$~MeV and is therefore not enough to explain the cooling of some soft X-ray transients. The total heat released in the crust is very sensitive to details of the nuclear structure and is predicted to lie in the range from $1.5$~MeV to $1.7$~MeV. The evolution of an accreted matter element and therefore the location of heat sources are governed to a large extent by the existence of nuclear shell closures. Ignoring these effects in the inner crust, the total heat falls to $\sim 0.6$~MeV. The neutron-matter constraint is also found to play a key role. The large amount of heat obtained by Steiner et al. (2012) could thus be traced back to unrealistic neutron-matter equations of state.

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arXiv2018

The gamma-ray strength function of $^{89}$Y and $^{90}$Y

In this work, we present new data on the $^{89}$Y($γ$,n) cross section studied with a quasi-monochromatic photon beam produced at the NewSUBARU synchrotron radiation facility in Japan contributing torwards resolving a long standing discrepancy between existing measurements of this cross section. Results for $γ$-ray strength function below threshold obtained by applying the Oslo method to $^{89}$Y($p,p'γ$)$^{89}$Y coincidences combined with the $^{89}$Y($γ$,n) data this providing experimental data for the $γ$-ray strength function of $^{89}$Y for $γ$ energies in the range of $\approx 1.6$ Mev to $\approx$ 20 MeV. A low-energy enhancement is seen for $γ$-rays below $\approx 2.5$ MeV. Shell-model calculations indicate that this feature is caused by strong, low-energy $M1$ transitions at high excitation energies. The nuclear level density and $γ$-ray strength function have been extracted from $^{89}$Y($d,p γ$)$^{90}$Y coincidences using the Oslo method. Using the ($γ,n$) and ($d,pγ$) data as experimental constraints, we have calculated the $^{89}$Y($n,γ$)$^{90}$Y cross section with the TALYS reaction code. Our results have been compared with directly measured (n,$γ$) cross sections and evaluations. The $N=50$ isotope $^{89}$Y is an important bottleneck in the s-process and the magnitude of the $^{89}$Y(n,$γ)$ cross section is key to understanding how s-process stars produce heavy isotopes.

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arXiv2018

Verification of detailed balance for $γ$ absorption and emission in Dy isotopes

The photo-neutron cross sections of $^{162,163}\rm{Dy}$ have been measured for the first time in an energy region from the neutron threshold ($S_n$) up to $\approx$ $13$~MeV. The ($γ$,n) reaction was induced with quasi-monochromatic laser Compton-scattered $γ$ rays, produced at the NewSUBARU laboratory. The corresponding $γ$-ray strength functions ($γ$SF) have been calculated from the photo-neutron cross sections. The data are compared to reanalyzed $γ$SFs of $^{160-164}\rm{Dy}$, which are measured below $S_n$. The excellent agreement with the photo-neutron data at $S_n$ confirms the principle of detailed balance. Thus, a complete $γ$SF is established covering in total the energy region of 1 MeV $\leq$ E$_γ$ $\leq$ 13 MeV. These mid-shell well-deformed dysprosium isotopes all show scissors resonances with very similar structures. We find that our data predict the same integrated scissors strength as ($γ,γ^\prime$) data when integrated over the same energy range, which shows that the scissors mode very likely is consistent with the generalized Brink hypothesis. Finally, using the $γ$SFs as input in the reaction code TALYS, we have deduced radiative neutron-capture cross sections and compared them to direct measurements. We find a very good agreement within the uncertainties, which gives further support to the experimentally determined $γ$SFs.

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arXiv2017

Pygmy and core polarization dipole modes in $^{206}$Pb: connecting nuclear structure to stellar nucleosynthesis

A high-resolution study of the electromagnetic response of $^{206}$Pb below the neutron separation energy is performed using a ($\vecγ$,$γ'$) experiment at the HI$\vecγ$S facility. Nuclear resonance fluorescence with 100% linearly polarized photon beams is used to measure spins, parities, branching ratios, and decay widths of excited states in $^{206}$Pb from $4.9$ to $8.1$MeV. The extracted $Σ$$B$(E1)$\uparrow$ and $Σ$$B$(M1)$\uparrow$ values for the total electric and magnetic dipole strength below the neutron separation energy are 0.9$\pm$0.2e$^2$fm$^2$ and 8.3$\pm$2.0$μ_{N}^2$, respectively. These measurements are found to be in very good agreement with the predictions from an energy-density functional (EDF) plus quasiparticle phonon model (QPM). Such a detailed theoretical analysis allows to separate the pygmy dipole resonance from both the tail of the giant dipole resonance and multi-phonon excitations. Combined with earlier photonuclear experiments above the neutron separation energy, one extracts a value for the electric dipole polarizability of $^{206}$Pb of $α_{D}\!=\!122\pm10$mb/MeV. When compared to predictions from both the EDF+QPM and accurately calibrated relativistic EDFs, one deduces a range for the neutron-skin thickness of $R_{\rm skin}^{206}\!=\!0.12$-$0.19$fm and a corresponding range for the slope of the symmetry energy of $L\!=\!48$-$60$MeV. This newly obtained information is also used to estimate the Maxwellian-averaged radiative cross section $^{205}$Pb(n,$γ$)$^{206}$Pb at 30keV to be $σ\!=\!130\!\pm\!25$mb. The astrophysical impact of this measurement--on both the s-process in stellar nucleosynthesis and on the equation of state of neutron-rich matter--is discussed.

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arXiv2017

Quasicontinuum $γ$-decay of $^{91,92}$Zr: benchmarking indirect ($n,γ$) cross section measurements for the $s$-process

Nuclear level densities (NLDs) and $γ$-ray strength functions ($γ$SFs) have been extracted from particle-$γ$ coincidences of the $^{92}$Zr($p,p' γ$)$^{92}$Zr and $^{92}$Zr($p,d γ$)$^{91}$Zr reactions using the Oslo method. The new $^{91,92}$Zr $γ$SF data, combined with photonuclear cross sections, cover the whole energy range from $E_γ \approx 1.5$~MeV up to the giant dipole resonance at $E_γ \approx 17$~MeV. The wide-range $γ$SF data display structures at $E_γ \approx 9.5$~MeV, compatible with a superposition of the spin-flip $M1$ resonance and a pygmy $E1$ resonance. Furthermore, the $γ$SF shows a minimum at $E_γ \approx 2-3$~MeV and an increase at lower $γ$-ray energies. The experimentally constrained NLDs and $γ$SFs are shown to reproduce known ($n, γ$) and Maxwellian-averaged cross sections for $^{91,92}$Zr using the {\sf TALYS} reaction code, thus serving as a benchmark for this indirect method of estimating ($n, γ$) cross sections for Zr isotopes.

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arXiv2016

Large-scale deformed quasiparticle random-phase approximation calculations of the $γ$-ray strength function using the Gogny force

Valuable theoretical predictions of nuclear dipole excitations in the whole chart are of great interest for different nuclear applications, including in particular nuclear astrophysics. Here we present large-scale calculations of the $E1$ $γ$-ray strength function obtained in the framework of the axially-symmetric deformed QRPA based on the finite-range Gogny force. This approach is applied to even-even nuclei, the strength function for odd nuclei being derived by interpolation. The convergence with respect to the adopted number of harmonic oscillator shells and the cut-off energy introduced in the 2-quasiparticle (2-$qp$) excitation space is analyzed. The calculations performed with two different Gogny interactions, namely D1S and D1M, are compared. A systematic energy shift of the $E1$ strength is found for D1M relative to D1S, leading to a lower energy centroid and a smaller energy-weighted sum rule for D1M. When comparing with experimental photoabsorption data, the Gogny-QRPA predictions are found to overestimate the giant dipole energy by typically $\sim$2 MeV. Despite the microscopic nature of our self-consistent Hartree-Fock-Bogoliubov plus QRPA calculation, some phenomenological corrections need to be included to take into account the effects beyond the standard 2-$qp$ QRPA excitations and the coupling between the single-particle and low-lying collective phonon degrees of freedom. For this purpose, three prescriptions of folding procedure are considered and adjusted to reproduce experimental photoabsorption data at best. All of them are shown to lead to rather similar predictions of the $E1$ strength, both at low energies and for exotic neutron-rich nuclei. Predictions of $γ$-ray strength functions and Maxwellian-averaged neutron capture rates for the whole Sn isotopic chain are also discussed and compared with previous theoretical calculations.

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arXiv2016

Experimentally constrained ($p,γ$)$^{89}$Y and ($n,γ$)$^{89}$Y reaction rates relevant to the $p$-process nucleosynthesis

The nuclear level density and the $γ$-ray strength function have been extracted for $^{89}$Y, using the Oslo Method on $^{89}$Y($p,p' γ$)$^{89}$Y coincidence data. The $γ$-ray strength function displays a low-energy enhancement consistent with previous observations in this mass region ($^{93-98}$Mo). Shell-model calculations give support that the observed enhancement is due to strong, low-energy $M1$ transitions at high excitation energies. The data were further used as input for calculations of the $^{88}$Sr($p,γ$)$^{89}$Y and $^{88}$Y($n,γ$)$^{89}$Y cross sections with the TALYS reaction code. Comparison with cross-section data, where available, as well as with values from the BRUSLIB library, shows a satisfying agreement.

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arXiv2016

Solar r-process-constrained actinide production in neutrino-driven winds of supernovae

Long-lived radioactive nuclei play an important role as nucleo-cosmochronometers and as cosmic tracers of nucleosynthetic source activity. In particular nuclei in the actinide region like thorium, uranium, and plutonium can testify to the enrichment of an environment by the still enigmatic astrophysical sources that are responsible for the production of neutron-rich nuclei by the rapid neutron-capture process (r-process). Supernovae and merging neutron-star (NS) or NS-black hole binaries are considered as most likely sources of the r-nuclei. But arguments in favour of one or the other or both are indirect and make use of assumptions; they are based on theoretical models with remaining simplifications and shortcomings. An unambiguous observational determination of a production event is still missing. In order to facilitate searches in this direction, e.g.\ by looking for radioactive tracers in stellar envelopes, the interstellar medium or terrestrial reservoirs, we provide improved theoretical estimates and corresponding uncertainty ranges for the actinide production ($^{232}$Th, $^{235,236,238}$U, $^{237}$Np, $^{244}$Pu, and $^{247}$Cm) in neutrino-driven winds of core-collapse supernovae. Since state-of-the-art supernova models do not yield r-process viable conditions ---but still lack, for example, the effects of strong magnetic fields--- we base our investigation on a simple analytical, Newtonian, adiabatic and steady-state wind model and consider the superposition of a large number of contributing components, whose nucleosynthesis-relevant parameters (mass weight, entropy, expansion time scale, and neutron excess) are constrained by the assumption that the integrated wind nucleosynthesis closely reproduces the solar system distribution of r-process elements. We also test the influence of uncertain nuclear physics.

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