arXiv subjects

S. Imada

Publications and source records attributed to S. Imada.

At least 19 recordsLinked to original sources

arXiv2025

Hybridized and Localized 4f Electronic States of Nd-based Intermetallic Compounds in Cubic Symmetry Probed by High-Energy Photoemission

We have performed soft and hard X-ray photoemission spectroscopies on NdTi2Al20 and NdBe13 which show antiferromagnetic ordering at low temperatures. The Nd 3d core-level photoemission and Nd 3d-4f valence-band resonant photoemission spectra show finite 4f4 initial-state components in addition to the 4f3 configurations attributed to the c-f hybridization effects in NdTi2Al20, while the 4f3 initial-state components with localized character are dominant in NdBe13. These results imply the emergence of overscreening channel due to the two-channel Kondo effect in NdTi2Al20 through the the strong c-f hybridization effect.

cond-mat.str-el↗

arXiv2024

Observations of Non-thermal Velocity and Comparison with Alfv\'en Wave Turbulence Model in Solar Active Regions

We present a study of spectral line width measurements from the Extreme Ultraviolet Imaging Spectrometer (EIS) on {\it Hinode}. We used spectral line profiles of Fe {\sc xvi} 262.984 {\AA}, Fe {\sc xiv} 264.787 {\AA}, Fe {\sc xiv} 270.519 {\AA}, Fe {\sc xiv} 274.203 {\AA}, and Fe {\sc xv} 284.160 {\AA}, and studied 11 active regions. Previous studies of spectral line widths have shown that in hot loops in the cores of active regions, the observed non-thermal velocities are smaller than predicted from models of reconnection jets in the corona or shock heating associated with Alfv\'{e}n waves. The observed line widths are also inconsistent with models of chromospheric evaporation due to coronal nanoflares. We show that recent advances in higher resolution Alfv\'{e}n wave turbulence modeling enables us to obtain non-thermal velocities similar to those measured in active regions. The observed non-thermal velocities for the 11 active regions in our study are in the range of 17$-$30 $\rm km ~ s^{-1}$, consistent with the spectral line non-thermal widths predicted from our model of 16 interacting flux tubes, which are in the range of ~15$-$37 $\rm km ~ s^{-1}$.

astro-ph.SR↗

arXiv2024

Fingerprints of Mott and Slater gaps in the core-level photoemission spectra of antiferromagnetic iridates

We present Ir $4f$ core-level hard-x-ray photoemission spectroscopy (HAXPES) experiments conducted across antiferromagnetic (AFM) ordering transition in Ruddlesden-Popper iridates Sr$_2$IrO$_4$ and Sr$_3$Ir$_2$O$_7$. The Ir $4f$ spectra exhibit distinct changes between the AFM and paramagnetic (PM) phases, with the spectral difference $I_\text{PM}-I_\text{AFM}$ showing a contrasting behavior in the two compounds. By employing computational simulations using the local-density approximation combined with the dynamical mean-field theory method, we elucidate that $I_\text{PM}-I_\text{AFM}$ primary reflects the Slater or Mott-Hubbard character of the AFM insulating state rather than material specific details. This sensitivity to fine low-energy electronic structure arises from the dependence of charge-transfer responses to the sudden creation of a localized core hole on both metal-insulator transitions and long-range AFM ordering. Our result broadens the applications of core-level HAXPES as a tool for characterization of electronic structure.

cond-mat.str-el↗

arXiv2023

Impact of the ground-state $4f$ symmetry for anisotropic $cf$-hybridization in the heavy fermion superconductor CeNi$_{2}$Ge$_{2}$

We report the ground-state symmetry of the Ce $4f$ states in the heavy fermion superconductor CeNi$_{2}$Ge$_{2}$, yielding anisotropic $cf$-hybridization between the Ce $4f$ states and conducting electrons. By analyzing linear dichroism in soft x-ray absorption and core-level hard x-ray photoemission spectra, the $4f$ symmetry is determined as $\Sigma$-type $\Gamma_{7}$, promoting predominant hybridization with the conducting electrons originating from the Ge site. The band structures probed by the soft x-ray angle-resolved photoemission indicates that the Ge $4p$ components contribute to the band renormalization through the anisotropic hybridization effects, suggesting that the control of the electronic structures of Ge orbital gives an impact to achieve the exotic phenomena in CeNi$_{2}$Ge$_{2}$.

cond-mat.str-el↗

arXiv2023

A Comprehensive Simulation of Solar Wind Formation from the Solar Interior: Significant Cross-field Energy Transport by Interchange Reconnection near the Sun

The physical connection between thermal convection in the solar interior and the solar wind remains unclear due to their significant scale separation. Using an extended version of the three-dimensional radiative magnetohydrodynamic code RAMENS, we perform the first comprehensive simulation of the solar wind formation, starting from the wave excitation and the small-scale dynamo below the photosphere. The simulation satisfies various observational constraints as a slow solar wind emanating from the coronal hole boundary. The magnetic energy is persistently released in the simulated corona, showing a hot upward flow at the interface between open and closed fields. To evaluate the energetic contributions from Alfv\'en wave and interchange reconnection, we develop a new method to quantify the cross-field energy transport in the simulated atmosphere. The measured energy transport from closed coronal loops to open field accounts for approximately half of the total. These findings suggest a significant role of the supergranular-scale interchange reconnection in solar wind formation.

astro-ph.SR↗

arXiv2023

Bulk superconductivity in Pb-substituted BiS$_{\bf 2}$-based compounds studied by hard-x-ray spectroscopy

In this study, we investigate the bulk electronic structure of Pb-substituted LaO$_{0.5}$F$_{0.5}$BiS$_2$ single crystals, using two types of hard-x-ray spectroscopy. High-energy-resolution fluorescence-detected x-ray absorption spectroscopy revealed a spectral change at low temperatures. Using density functional theory (DFT) simulations, we find that the temperature-induced change originates from a structural phase transition, similar to the pressure-induced transition in LaO$_{0.5}$F$_{0.5}$BiS$_2$. This finding suggests that the mechanism of bulk superconductivity induced by Pb substitution is the same as that under high pressure. Furthermore, a novel low-valence state with a mixture of divalent and trivalent Bi ions is discovered using hard x-ray photoemission spectroscopy with the aid of DFT calculations.

cond-mat.supr-con↗

arXiv2021

Non-Equilibrium Ionization Plasma During Large Solar Limb Flare Observed by Hinode/EIS

This study on plasma heating considers the time-dependent ionization process during a large solar flare on September 10, 2017, observed by Hinode/EIS. The observed FeXXIV / FeXXIII ratios increase downstream of the reconnection outflow, and they are consistent with the time-dependent ionization effect at a constant electron temperature Te = 25 MK. Moreover, this study also shows that the non-thermal velocity, which can be related to the turbulent velocity, reduces significantly along the downstream of the reconnection outflow, even when considering the time-dependent ionization process.

astro-ph.SR↗

arXiv2020

The Prominent Charge-Transfer Effects of Trinuclear Complexes with Nominally High Nickel Valences

Recently synthesized Rh-Ni trinuclear complexes hexacoordinated with sulfur ions, 3-aminopropanethiolate (apt) metalloligand [Ni{Rh(apt)$_{3}$}$_{2}$](NO$_{3}$)$_{n}$ ($n$ = 2, 3, 4), are found to be chemically interconvertible between the nominal Ni$^{2+}$ and Ni$^{4+}$ states. In order to clarify the origins of their interconvertible nature and the stability of such a high oxidation state as the tetravalency from the physical point of view, we have systematically investigated the local 3$d$ electronic structures of [Ni{Rh(apt)$_{3}$}$_{2}$](NO$_{3}$)$_{n}$ by means of soft X-ray core-level absorption spectroscopy (XAS). The experimental data have been reproduced by the single-site configuration-interaction cluster-model simulations, which indicate that the charge-transferred configurations are more stable than the nominal $d$-electron-number configuration for $n=3,4$ leading to the prominent charge-transfer effects. These are also supported by S $K$-edge XAS of [Ni{Rh(apt)$_{3}$}$_{2}$](NO$_{3}$)$_{n}$. Our results imply that the found charge-transfer effects have a key role to realize the interconvertible nature as well as the stability of the high oxidization state of the Ni ions.

cond-mat.str-el↗

arXiv2019

Effect of morphological asymmetry between leading and following sunspots on the prediction of solar cycle activity

The morphological asymmetry of leading and following sunspots is a well-known characteristic of the solar surface. In the context of large-scale evolution of the surface magnetic field, the asymmetry has been assumed to have only a negligible effect. Using the surface flux transport model, we show that the morphological asymmetry of leading and following sunspots has a significant impact on the evolution of the large-scale magnetic field on the solar surface. By evaluating the effect of the morphological asymmetry of each bipolar magnetic region (BMR), we observe that the introduction of the asymmetry in the BMR model significantly reduces its contribution to the polar magnetic field, especially for large and high-latitude BMRs. Strongly asymmetric BMRs can even reverse the regular polar field formation. The surface flux transport simulations based on the observed sunspot record shows that the introduction of the morphological asymmetry reduces the root-mean-square difference from the observed axial dipole strength by 30--40 percent. These results indicate that the morphological asymmetry of leading and following sunspots has a significant effect on the solar cycle prediction.

astro-ph.SR↗

arXiv2018

Semi-conservative reduced speed of sound technique for low Mach number flows with large density variations

The reduced speed of sound technique (RSST) has been used for efficient simulation of low Mach number flows in solar and stellar convection zones. The basic RSST equations are hyperbolic, and are suitable for parallel computation by domain decomposition. The application of RSST is limited to cases where density perturbations are much smaller than the background density. In addition, non-conservative variables are required to be evolved using this method, which is not suitable in cases where discontinuities like shock waves co-exist in a single numerical domain. In this study, we suggest a new semi-conservative formulation of the RSST that can be applied to low Mach number flows with large density variations. We derive the wave speed of the original and newly suggested methods to clarify that these methods can reduce the speed of sound without affecting the entropy wave. The equations are implemented using the finite volume method. Several numerical tests are carried out to verify the suggested methods. The analysis and numerical results show that the original RSST is not applicable when mass density variations are large. In contrast, the newly suggested methods are found to be efficient in such cases. We also suggest variants of the RSST that conserve momentum in the machine precision. The newly suggested variants are formulated as semi-conservative equations, which reduce to the conservative form of the Euler equations when the speed of sound is not reduced. This property is advantageous when both high and low Mach number regions are included in the numerical domain. The newly suggested forms of RSST can be applied to a wider range of low Mach number flows.

physics.comp-ph↗

arXiv2018

Electron Power-Law Spectra in Solar and Space Plasmas

Particles are accelerated to very high, non-thermal energies in solar and space plasma environments. While energy spectra of accelerated electrons often exhibit a power law, it remains unclear how electrons are accelerated to high energies and what processes determine the power-law index $\delta$. Here, we review previous observations of the power-law index $\delta$ in a variety of different plasma environments with a particular focus on sub-relativistic electrons. It appears that in regions more closely related to magnetic reconnection (such as the `above-the-looptop' solar hard X-ray source and the plasma sheet in Earth's magnetotail), the spectra are typically soft ($\delta \gtrsim$ 4). This is in contrast to the typically hard spectra ($\delta \lesssim$ 4) that are observed in coincidence with shocks. The difference implies that shocks are more efficient in producing a larger non-thermal fraction of electron energies when compared to magnetic reconnection. A caveat is that during active times in Earth's magnetotail, $\delta$ values seem spatially uniform in the plasma sheet, while power-law distributions still exist even in quiet times. The role of magnetotail reconnection in the electron power-law formation could therefore be confounded with these background conditions. Because different regions have been studied with different instrumentations and methodologies, we point out a need for more systematic and coordinated studies of power-law distributions for a better understanding of possible scaling laws in particle acceleration as well as their universality.

astro-ph.SR↗

arXiv2017

Improvement of solar cycle prediction: Plateau of solar axial dipole moment

Aims. We report the small temporal variation of the axial dipole moment near the solar minimum and its application to the solar cycle prediction by the surface flux transport (SFT) model. Methods. We measure the axial dipole moment using the photospheric synoptic magnetogram observed by the Wilcox Solar Observatory (WSO), the ESA/NASA Solar and Heliospheric Observatory Michelson Doppler Imager (MDI), and the NASA Solar Dynamics Observatory Helioseismic and Magnetic Imager (HMI). We also use the surface flux transport model for the interpretation and prediction of the observed axial dipole moment. Results. We find that the observed axial dipole moment becomes approximately constant during the period of several years before each cycle minimum, which we call the axial dipole moment plateau. The cross-equatorial magnetic flux transport is found to be small during the period, although the significant number of sunspots are still emerging. The results indicates that the newly emerged magnetic flux does not contributes to the build up of the axial dipole moment near the end of each cycle. This is confirmed by showing that the time variation of the observed axial dipole moment agrees well with that predicted by the SFT model without introducing new emergence of magnetic flux. These results allows us to predict the axial dipole moment in Cycle 24/25 minimum using the SFT model without introducing new flux emergence. The predicted axial dipole moment of Cycle 24/25 minimum is 60--80 percent of Cycle 23/24 minimum, which suggests the amplitude of Cycle 25 even weaker than the current Cycle 24. Conclusions. The plateau of the solar axial dipole moment is an important feature for the longer prediction of the solar cycle based on the SFT model.

astro-ph.SR↗

arXiv2017

Study on Precursor Activity of the X1.6 Flare in the Great AR 12192 with SDO, IRIS, and Hinode

The physical properties and its contribution to the onset of solar flare are still unclear although chromospheric brightening is considered a precursor phenomenon of flare. Many studies suggested that photospheric magnetic field changes cause destabilization of large-scale coronal structure. We aim to understand how a small photospheric change contributes to a flare and to reveal how the intermediary chromosphere behaves in the precursor phase. We analyzed the precursor brightening of the X1.6 flare on 2014 October 22 in the AR 12192 using the Interface Region Imaging Spectrograph (IRIS) and Hinode/EUV Imaging Spectrometer (EIS) data. We investigated a localized jet with the strong precursor brightening, and compared the intensity, Doppler velocity, and line width in C II, Mg II k, Si IV lines by IRIS and He II, Fe XII, Fe XV lines by Hinode/EIS. We also analyzed photospheric magnetic field and chromospheric/coronal structures using Solar Dynamics Observatory (SDO)/Helioseismic and Magnetic Imager (HMI) and Atmospheric Imaging Assembly (AIA). We found a significant blueshift (~ 100 km/s), which is related to the strong precursor brightening over a characteristic magnetic field structure, and the blueshift was observed at all the temperature. This might indicate that the flow is accelerated by Lorentz force. Moreover, the large-scale coronal loop that connects the foot-points of the flare ribbons was destabilized just after the precursor brightening with the blueshift. It suggests that magnetic reconnection locally occurred in the lower chromosphere and it triggered magnetic reconnection of the X1.6 flare in the corona.

astro-ph.SR↗

arXiv2017

UV/EUV High-Throughput Spectroscopic Telescope: A Next Generation Solar Physics Mission white paper

The origin of the activity in the solar corona is a long-standing problem in solar physics. Recent satellite observations, such as Hinode, Solar Dynamics Observatory (SDO), Interface Region Imaging Spectrograph (IRIS), show the detail characteristics of the solar atmosphere and try to reveal the energy transfer from the photosphere to the corona through the magnetic fields and its energy conversion by various processes. However, quantitative estimation of energy transfer along the magnetic field is not enough. There are mainly two reason why it is difficult to observe the energy transfer from photosphere to corona; 1) spatial resolution gap between photosphere (a few 0.1 arcsec) and corona (a few arcsec), 2) lack in temperature coverage. Furthermore, there is not enough observational knowledge of the physical parameters in the energy dissipation region. There are mainly three reason why it is difficult to observe in the vicinity of the energy dissipation region; 1) small spatial scale, 2) short time scale, 3) low emission. It is generally believed that the energy dissipation occurs in the very small scale and its duration is very short (10 second). Further, the density in the dissipation region might be very low. Therefore, the high spatial and temporal resolution UV/EUV spectroscopic observation with wide temperature coverage is crucial to estimate the energy transport from photosphere to corona quantitatively and diagnose the plasma dynamics in the vicinity of the energy dissipation region. Main Science Target for the telescope is quantitative estimation for the energy transfer from the photosphere to the corona, and clarification of the plasma dynamics in the vicinity of the energy dissipation region, where is the key region for coronal heating, solar wind acceleration, and/or solar flare, by the high spatial and temporal resolution UV/EUV spectroscopy.

astro-ph.SR↗

arXiv2015

Photoemission System with Polarized Hard X-rays for Probing Ground State Symmetry of Strongly Correlated Materials

We have developed a polarized hard X-ray photoemission (HAXPES) system to study the ground-state symmetry of strongly correlated materials. The linear polarization of the incoming X-ray beam is switched by the transmission-type phase retarder composed of two diamond (100) crystals. The best degree of the linear polarization $P_L$ is $-0.96$, containing the vertical polarization component of 98%. A newly developed low temperature two-axis manipulator enables easy polar and azimuthal rotations to select the detection direction of photoelectrons. The lowest temperature achieved is 9 K, offering us a chance to access the ground state even for the strongly correlated electron systems in cubic symmetry. The co-axial sample monitoring system with the long-working-distance microscope enables us to keep measuring the same region on the sample surface before and after rotation procedures. Combining this sample monitoring system with a micro-focused X-ray beam by means of an ellipsoidal Kirkpatrick-Baez mirror (25 $μ$m $\times$ 25 $μ$m (FWHM)), we have demonstrated the polarized valence-band HAXPES on NiO for voltage application as resistive random access memories to reveal the origin of the metallic spectral weight near the Fermi level.

cond-mat.str-el↗

arXiv2014

Formation of a Flare-Productive Active Region: Observation and Numerical Simulation of NOAA AR 11158

We present a comparison of the Solar Dynamics Observatory (SDO) analysis of NOAA Active Region (AR) 11158 and numerical simulations of flux-tube emergence, aiming to investigate the formation process of this flare-productive AR. First, we use SDO/Helioseismic and Magnetic Imager (HMI) magnetograms to investigate the photospheric evolution and Atmospheric Imaging Assembly (AIA) data to analyze the relevant coronal structures. Key features of this quadrupolar region are a long sheared polarity inversion line (PIL) in the central delta-sunspots and a coronal arcade above the PIL. We find that these features are responsible for the production of intense flares, including an X2.2-class event. Based on the observations, we then propose two possible models for the creation of AR 11158 and conduct flux-emergence simulations of the two cases to reproduce this AR. Case 1 is the emergence of a single flux tube, which is split into two in the convection zone and emerges at two locations, while Case 2 is the emergence of two isolated but neighboring tubes. We find that, in Case 1, a sheared PIL and a coronal arcade are created in the middle of the region, which agrees with the AR 11158 observation. However, Case 2 never builds a clear PIL, which deviates from the observation. Therefore, we conclude that the flare-productive AR 11158 is, between the two cases, more likely to be created from a single split emerging flux than from two independent flux bundles.

astro-ph.SR↗

arXiv2013

Bulk Nature of Layered Perovskite Iridates beyond the Mott Scenario : An Approach from Bulk Sensitive Photoemission Study

We present genuine bulk Ir 5d jeff states of layered perovskite iridates obtained by hard-x-ray photoemission spectroscopy (HAXPES) with s- and p-polarized lights. HAXPES spectra of Sr2IrO4 and Ba2IrO4 are well reproduced by the quasi-particle densities of states calculated by the local density approximation with dynamical mean-field theory (LDA+DMFT). It is demonstrated that the insulating nature of the iridates is triggered by antiferromagnetic correlation (Slater type) combined with electron correlation (Mott type). The extremely-low-energy bulk-sensitive photoemission spectroscopy reveals "bad metallic" states in the paramagnetic phase of the iridates, suggesting strongly renormalized metallic states above the Neel temperature as predicted by the LDA+DMFT.

cond-mat.str-el↗

arXiv2013

Evidence for Hot Fast Flow above a Solar Flare Aracade

Solar flares are one of the main forces behind space weather events. However the mechanism that drives such energetic phenomena is not fully understood. The standard eruptive flare model predicts that magnetic reconnection occurs high in the corona where hot fast flows are created. Some imaging or spectroscopic observations have indicated the presence of these hot fast flows but there have been no spectroscopic scanning observation to date to measure the two-dimensional structure quantitatively. We analyzed a flare that occurred on the west solar limb on 27 January 2012 observed by the Hinode EUV Imaging Spectrometer (EIS) and found that the hot (~30MK) fast (>500 km/s) component was located above the flare loop. This is consistent with magnetic reconnection taking place above the flare loop.

astro-ph.SR↗