arXiv subjects

S. Imajo

Publications and source records attributed to S. Imajo.

13 recordsLinked to original sources

arXiv2026

High-field fate of the Kitaev quantum spin liquid in $α$-RuCl$_3$

Kitaev quantum spin liquids (KQSLs) host fractionalized excitations described by itinerant Majorana quasiparticles and gapped $Z_2$ fluxes (visons), providing a platform for emergent topological matter. Whether such a state survives under strong magnetic fields, however, remains an open question. The layered honeycomb magnet $α$-RuCl$_3$ is a leading candidate material: an in-plane field of $\sim$ 7 T suppresses antiferromagnetic order and induces a quantum-disordered phase exhibiting signatures consistent with Majorana excitations, including an anomalous thermal Hall effect and field-angle-dependent specific heat. At higher fields, the magnetization approaches saturation, suggesting a transition to a spin-polarized state, yet the microscopic evolution between these limits remains unresolved. Here we report high-field specific heat measurements up to 24 T that reveal a distinct crossover at $μ_0H^*\approx$15 T, beyond which the perturbative Kitaev description breaks down. Above $H^*$, the characteristic six-fold angular modulation of the specific heat collapses and the excitation gap deviates from the predicted $H^3$ scaling. Meanwhile, the gap decreases with increasing field and the in-plane magnetization anisotropy persists up to $\sim$ 24 T, both in sharp contrast to a trivial spin-polarized state, indicating that KQSL signatures are preserved even at $\sim$ 90 % of magnetization saturation. These results reveal that the KQSL in $α$-RuCl$_3$ extends well beyond the perturbative window, persisting as a nonperturbative regime in which the Majorana and vison energy scales merge, before eventually giving way to spin polarization. This thermodynamic roadmap provides a basis for understanding how fractionalized phases evolve under strong magnetic fields.

cond-mat.str-el↗

arXiv2026

Neutron EDM Experiment with an Advanced Ultracold Neutron Source at TRIUMF

The TRIUMF Ultracold Advanced Neutron (TUCAN) collaboration has been developing a high-intensity ultracold neutron (UCN) source aimed at searching for the neutron electric dipole moment (EDM) with a sensitivity goal of $10^{-27}\ e{\rm cm}$. This article reports on recent progress in commissioning of the UCN source and in the development of the neutron EDM spectrometer. In its final configuration, the accelerator-driven super-thermal UCN source will enable a neutron EDM experiment with two orders of magnitude improved statistics compared to the current best experiment. Substantial progress in 2024 allowed the collaboration to operate the complete source system, with the exception of the liquid deuterium cold moderator, resulting in the first production of UCNs. The status of the EDM spectrometer is also presented, with emphasis on UCN handling components and magnetic subsystems relevant to field control, shielding, and magnetometry.

physics.ins-det↗

arXiv2026

Initial results of the TRIUMF ultracold advanced neutron source

We report the first results on ultracold neutron production from a new spallation-driven superfluid $^4$He (He-II) source at TRIUMF, which is being prepared for a new, precise measurement of the neutron electric dipole moment. A total of $(9.3 \pm 0.8)\times 10^{5}$ ultracold neutrons were observed at a proton beam current of \SI{37}{\uA}, when the target was irradiated for a period of \SI{60}{\s}. The results are in fair agreement with expectations based on a detailed simulation of neutron transport and ultracold neutron source cryogenics. There is some indication that the new source might not be as limited by the conduction of heat through the He-II as originally expected. The results indicate that the source is likely to make its ultimate production goals, once the liquid deuterium cold moderator system is completed, with the expectation that $5.7\times 10^7$~UCNs would be detected in the same experiment with full liquid levels. This would, for example, correspond to delivery of $1.4\times 10^6$~UCNs delivered to each of two nEDM measurement cells, and a statistical uncertainty of $1\times 10^{-27}~e$cm on the neutron EDM in 280 days of running.

nucl-ex↗

arXiv2026

Ultracold Neutron Guide-Coating Facility at U.Winnipeg

We report the construction and commissioning of a new ultracold neutron (UCN) guide-coating facility at the University of Winnipeg. The facility employs pulsed laser deposition (PLD) to produce diamond-like carbon (DLC) coatings on cylindrical UCN guides up to 1 m in length with a 200 mm outer diameter. DLC is a promising material for UCN transport and storage due to its high real component of the optical potential, low neutron absorption cross section, and low depolarization probabilities. First coating attempts on a full length aluminum UCN guide and matching blank flange were successfully coated with a carbon film with density of 2.3 g/cm$^3$, corresponding to optical potentials of 200 neV, as measured by X-ray reflectometry (XRR). Coating thicknesses were measured to be 90 nm for the UCN guide and 180 nm for the flange with no evidence of delamination. The implementation of a plasma plume collimator and plasma feed back control via a time of flight in vacuum ion probe produced a film with an XRR measured density of 2.8 g/cm$^3$, corresponding to an optical potential of 240 neV. This 80 nm thick film had poor adhesion to the aluminum tube substrate. These results establish a baseline for the coating facility. Ongoing and future work focuses on improving the diamond content of films and adhesion through plasma plume collimation, TOF ion probe feed back, and pre/post treatment methods with the goal of providing high quality DLC UCN guides for the TUCAN experiment at TRIUMF.

physics.ins-det↗

arXiv2025

Cryogenic systems for the TUCAN EDM experiment

The TUCAN (TRIUMF UltraCold Advanced Neutron) Collaboration is completing a new ultracold neutron (UCN) source. The UCN source will deliver UCNs to a neutron electric dipole moment (EDM) experiment. The EDM experiment is projected to be capable of an uncertainty of $1\times 10^{-27}~e$cm, competitive with other planned projects, and a factor of ten more precise than the present world's best. The TUCAN source is based on a UCN production volume of superfluid helium (He-II), held at 1~K, and coupled to a proton-driven spallation target. The production rate in the source is expected to be in excess of $10^7$~UCN/s; since UCN losses can be small in superfluid helium, this should allow us to build up a large number of UCNs. The spallation-driven superfluid helium technology is the principal aspect making the TUCAN project unique. The superfluid production volume was recently cooled, for the first time, and successfully filled with superfluid helium. The design principles of the UCN source are described, along with some of the challenging cryogenic milestones that were recently passed.

physics.ins-det↗

arXiv2023

A diffuse scattering model of ultracold neutrons on wavy surfaces

Metal tubes plated with nickel-phosphorus are used in many fundamental physics experiments using ultracold neutrons (UCN) because of their ease of fabrication. These tubes are usually polished to a average roughness of 25-150 nm. However, there is no scattering model that accurately describes UCN scattering on such a rough guide surface with a mean-square roughness larger than 5 nm. We therefore developed a scattering model for UCN in which scattering from random surface waviness with a size larger than the UCN wavelength is described by a microfacet Bidirectional Reflectance Distribution Function model (mf-BRDF model), and scattering from smaller structures by the Lambert's cosine law (Lambert model). For the surface waviness, we used the statistical distribution of surface slope measured by an atomic force microscope on a sample piece of guide tube as input of the model. This model was used to describe UCN transmission experiments conducted at the pulsed UCN source at J-PARC. In these experiments, a UCN beam collimated to a divergence angle smaller than $\pm 6^{\circ}$ was directed into a guide tube with a mean-square roughness of 6.4 nm to 17 nm at an oblique angle, and the UCN transport performance and its time-of-flight distribution were measured while changing the angle of incidence. The mf-BRDF model combined with the Lambert model with scattering probability $p_{L} = 0.039\pm0.003$ reproduced the experimental results well. We have thus established a procedure to evaluate the characteristics of UCN guide tubes with a surface roughness of approximately 10 nm.

physics.ins-det↗

arXiv2023

Quantum oscillations in a centrosymmetric skyrmion-hosting magnet GdRu2Si2

We have performed magnetic torque and resistivity measurements on a centrosymmetric skyrmion-host GdRu2Si2, in which the dominant magnetic interaction leading to skyrmion formation is under debate. We observe both the de Haas-van Alphen and Shubnikov-de Haas oscillations in the forced ferromagnetic phase. The angular dependence of the quantum oscillation frequencies can be reproduced by the ab-initio calculation. The de Haas-van Alphen oscillation is also observed in the double-Q phase with a different frequency to that in the forced ferromagnetic phase, indicating a Fermi surface reconstruction due to the coupling between localized spins and conduction electrons. Based on these experimental findings, the magnetic interactions in this system are discussed.

cond-mat.str-el↗

arXiv2023

Characterization of electroless nickel-phosphorus plating for ultracold-neutron storage

Electroless nickel plating is an established industrial process that provides a robust and relatively low-cost coating suitable for transporting and storing ultracold neutrons (UCN). Using roughness measurements and UCN-storage experiments we characterized UCN guides made from polished aluminum or stainless-steel tubes plated by several vendors. All electroless nickel platings were similarly suited for UCN storage with an average loss probability per wall bounce of $2.8\cdot10^{-4}$ to $4.1\cdot10^{-4}$ for energies between 90 neV and 190 neV, or a ratio of imaginary to real Fermi potential $η$ of $1.7\cdot10^{-4}$ to $3.3\cdot10^{-4}$. Measurements at different elevations indicate that the energy dependence of UCN losses is well described by the imaginary Fermi potential. Some special considerations are required to avoid an increase in surface roughness during the plating process and hence a reduction in UCN transmission. Increased roughness had only a minor impact on storage properties. Based on these findings we chose a vendor to plate the UCN-production vessel that will contain the superfluid-helium converter for the new TRIUMF UltraCold Advanced Neutron (TUCAN) source, achieving acceptable UCN-storage properties with ${η=3.5(5)\cdot10^{-4}}$.

nucl-ex↗

arXiv2022

Enhanced superconducting pairing strength near a nonmagnetic nematic quantum critical point

The quest for high-temperature superconductivity at ambient pressure is a central issue in physics. In this regard, the relationship between unconventional superconductivity and the quantum critical point (QCP) associated with the suppression of some form of symmetry-breaking order to zero temperature has received particular attention. The key question is how the strength of the electron pairs changes near the QCP, and this can be verified by high-field experiments. However, such studies are limited mainly to superconductors with magnetic QCPs, and the possibility of unconventional mechanisms by which nonmagnetic QCP promotes strong pairing remains a nontrivial issue. Here, we report systematic measurements of the upper critical field $H_{\rm c2}$ in nonmagnetic FeSe$_{1-x}$Te$_{x}$ superconductors, which exhibit a QCP of electronic nematicity characterized by spontaneous rotational-symmetry breaking. As the magnetic field increases, the superconducting phase of FeSe$_{1-x}$Te$_{x}$ shrinks to a narrower dome surrounding the nematic QCP. The analysis of $H_{\rm c2}$ reveals that the Pauli-limiting field is enhanced toward the QCP, implying that the pairing interaction is significantly strengthened via nematic fluctuations emanated from the QCP. Remarkably, this nonmagnetic nematic QCP is not accompanied by a divergent effective mass, distinct from the magnetically mediated pairing. Our observation opens up a nonmagnetic route to high-temperature superconductivity.

cond-mat.supr-con↗

arXiv2021

Normal state specific heat in the cuprates La$_{2-x}$Sr$_x$CuO$_4$ and Bi$_{2+y}$Sr$_{2-x-y}$La$_x$CuO$_{6+δ}$ near the critical point of the pseudogap phase

The specific heat $C$ of the cuprate superconductors La$_{2-x}$Sr$_x$CuO$_4$ and Bi$_{2+y}$Sr$_{2-x-y}$La$_x$CuO$_{6+δ}$ was measured at low temperature (down to $0.5~{\rm K}$), for dopings $p$ close to $p^\star$, the critical doping for the onset of the pseudogap phase. A magnetic field up to $35~{\rm T}$ was applied to suppress superconductivity, giving direct access to the normal state at low temperature, and enabling a determination of $C_e$, the electronic contribution to the normal-state specific heat, at $T \to 0$. In La$_{2-x}$Sr$_x$CuO$_4$ at $x=p = 0.22$, $0.24$ and $0.25$, $C_e / T = 15-16~{\rm mJmol}^{-1}{\rm K}^{-2}$ at $T = 2~{\rm K}$, values that are twice as large as those measured at higher doping ($p > 0.3$) and lower doping ($p < 0.15$). This confirms the presence of a broad peak in the doping dependence of $C_e$ at $p^\star\simeq 0.19$, as previously reported for samples in which superconductivity was destroyed by Zn impurities. Moreover, at those three dopings, we find a logarithmic growth as $T \to 0$, such that $C_e / T \sim {\rm B}\ln(T_0/T)$. The peak vs $p$ and the logarithmic dependence vs $T$ are the two typical thermodynamic signatures of quantum criticality. In the very different cuprate Bi$_{2+y}$Sr$_{2-x-y}$La$_x$CuO$_{6+δ}$, we again find that $C_e / T \sim {\rm B}\ln(T_0/T$) at $p \simeq p^\star$, strong evidence that this $\ln(1/T)$ dependence - first discovered in the cuprates La$_{1.8-x}$Eu$_{0.2}$Sr$_x$CuO$_4$ and La$_{1.6-x}$Nd$_{0.4}$Sr$_x$CuO$_4$ - is a universal property of the pseudogap critical point. All four materials display similar values of the $\rm B$ coefficient, indicating that they all belong to the same universality class.

cond-mat.supr-con↗

arXiv2019

Effects of Electron Correlations and Chemical Pressures on Superconductivity of $β^{\prime\prime}$-type Organic Compounds

We investigate low-temperature electronic states of the series of organic conductors $β^{\prime\prime}$-(BEDT-TTF)$_4$[(H$_3$O)M(C$_2$O$_4$)$_3$]G, where BEDT-TTF is bis(ethylenedithio)tetrathiafulvalene, and M and G represent trivalent metal ions and guest organic molecules, respectively. Our structural analyses reveal that the replacement of M and G give rise to systematic change in the cell parameters, especially in the $b$-axis length, which has positive correlation with the superconducting transition temperature $T_{\rm c}$. Analyses of temperature and magnetic field dependences of the electrical resistance including the Shubnikov-de Haas oscillations elucidates that the variation of charge disproportionation, effective mass and the number of itinerant carriers, can be systematically explained by the change of the $b$-axis length. The changes of the transfer integrals induced by stretching/compressing the $b$-axis are confirmed by the band calculation. We discuss that electron correlations in quarter-filled electronic bands lead to charge disproportionation and the possibility of a novel pairing mechanism of superconductivity mediated by charge degrees of freedom.

cond-mat.str-el↗

arXiv2015

Pulsed UCN production using a Doppler shifter at J-PARC

We have constructed a Doppler-shifter-type pulsed ultra-cold neutron (UCN) source at the Materials and Life Science Experiment Facility (MLF) of the Japan Proton Accelerator Research Complex (J-PARC). Very-cold neutrons (VCNs) with 136-$\mathrm{m/s}$ velocity in a neutron beam supplied by a pulsed neutron source are decelerated by reflection on a m=10 wide-band multilayer mirror, yielding pulsed UCN. The mirror is fixed to the tip of a 2,000-rpm rotating arm moving with 68-$\mathrm{m/s}$ velocity in the same direction as the VCN. The repetition frequency of the pulsed UCN is $8.33~\mathrm{Hz}$ and the time width of the pulse at production is $4.4~\mathrm{ms}$. In order to increase the UCN flux, a supermirror guide, wide-band monochromatic mirrors, focus guides, and a UCN extraction guide have been newly installed or improved. The $1~\mathrm{MW}$-equivalent count rate of the output neutrons with longitudinal wavelengths longer than $58~\mathrm{nm}$ is $1.6 \times 10^{2}~\mathrm{cps}$, while that of the true UCNs is $80~\mathrm{cps}$. The spatial density at production is $1.4~\mathrm{UCN/cm^{3}}$. This new UCN source enables us to research and develop apparatuses necessary for the investigation of the neutron electric dipole moment (nEDM).

physics.ins-det↗

arXiv2014

Beam energy dependence of charged pion ratio in $^{28}$Si + In reactions

The double differential cross sections for $^{nat}$In($^{28}$Si, $π^{\pm}$) reactions are measured at 400, 600, and 800 MeV/nucleon. Both $π^+$ and $π^-$ are found to be emitted isotropically from a single moving source. The $π^- / π^+$ yield ratio is determined as a function of the charged pion energy between 25 and 100 MeV. The experimental results significantly differ from the prediction of the standard transport model calculation using the code PHITS. This discrepancy suggests that more theoretical works are required to deduce firm information on the nuclear symmetry energy from the $π^- / π^+$ yield ratio.

nucl-ex↗