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S. Jöhr

Publications and source records attributed to S. Jöhr.

4 recordsLinked to original sources

Strain-Induced Metal-to-Insulator Transition in Antiferromagnetic SrCrO$_3$ Thin Films

Antiferromagnetic (AF) metals are rare, yet they combine properties attractive for spintronic devices like robustness against stray fields and electrical readout. Among AF metal oxide candidates, SrCrO$_3$ remains largely unexplored due to its notoriously difficult synthesis. In this paper, we demonstrate the growth of high-quality SrCrO$_3$ thin films by magnetron sputtering on substrates that impose a wide range of tensile and compressive strains. Muon spin relaxation experiments, supported by x-ray magnetic dichroism, unveil the emergence of an AF phase with dilute magnetic disorder at low temperatures, while resistivity measurements confirm the simultaneous metallic ground state of SrCrO$_3$ under low strain. As both compressive and tensile strain increase, a metal-to-insulator transition is induced in the films, while the onset of the magnetic transition temperature remains unchanged. Moreover, an intriguing resistivity upturn, accompanied by a change in the dominant charge-carrier type, occurs at a temperature that correlates with strain. These observations suggest a complex strain-dependent band structure, with strain-induced Jahn-Teller distortions or tilting of the CrO$_6$ octahedra that emerge depending on the sign of the strain, as inferred from density functional theory calculations.

cond-mat.mtrl-sci

Electronic reconstruction forming a $C_2$-symmetric Dirac semimetal in Ca$_3$Ru$_2$O$_7$

Electronic band structures in solids stem from a periodic potential reflecting the structure of either the crystal lattice or an electronic order. In the stoichiometric ruthenate Ca$_3$Ru$_2$O$_7$, numerous Fermi surface sensitive probes indicate a low-temperature electronic reconstruction. Yet, the causality and the reconstructed band structure remain unsolved. Here, we show by angle-resolved photoemission spectroscopy, how in Ca$_3$Ru$_2$O$_7$ a $C_2$-symmetric massive Dirac semimetal is realized through a Brillouin-zone preserving electronic reconstruction. This Dirac semimetal emerges in a two-stage transition upon cooling. The Dirac point and band velocities are consistent with constraints set by quantum oscillation, thermodynamic, and transport experiments, suggesting that the complete Fermi surface is resolved. The reconstructed structure -- incompatible with translational-symmetry-breaking density waves -- serves as an important test for band structure calculations of correlated electron systems.

cond-mat.str-el

Disentangling Intertwined Quantum States in a Prototypical Cuprate Superconductor

Spontaneous symmetry breaking constitutes a paradigmatic classification scheme of matter. However, broken symmetry also entails domain degeneracy that often impedes identification of novel low symmetry states. In quantum matter, this is additionally complicated by competing intertwined symmetry breaking orders. A prime example is that of unconventional superconductivity and density-wave orders in doped cuprates in which their respective symmetry relation remains a key question. Using uniaxial pressure as a domain-selective stimulus in combination with x-ray diffraction, we unambiguously reveal that the fundamental symmetry of the charge order in the prototypical cuprate La$_{1.88}$Sr$_{0.12}$CuO$_4$ is characterized by uniaxial stripes. We further demonstrate the direct competition of this stripe order with unconventional superconductivity via magnetic field tuning. The stripy nature of the charge-density-wave state established by our study is a prerequisite for the existence of a superconducting pair-density-wave -- a theoretical proposal that clarifies the interrelation of intertwined quantum phases in unconventional superconductors -- and paves the way for its high-temperature realization.

cond-mat.str-el

Multiple- to single-gap superconductivity crossover in Nb$_5$Ir$_{3-x}$Pt$_x$O alloys

By using mostly the muon-spin rotation/relaxation ($μ$SR) technique, we investigate the superconductivity (SC) of Nb$_5$Ir$_{3-x}$Pt$_x$O ($x = 0$ and 1.6) alloys, with $T_c = 10.5$ K and 9.1 K, respectively. At a macroscopic level, their superconductivity was studied by electrical resistivity, magnetization, and specific-heat measurements. In both compounds, the electronic specific heat and the low-temperature superfluid density data suggest a nodeless SC. The superconducting gap value and the specific heat discontinuity at $T_c$ are larger than that expected from the Bardeen-Cooper-Schrieffer theory in the weak-coupling regime, indicating strong-coupling superconductivity in the Nb$_5$Ir$_{3-x}$Pt$_x$O family. In Nb$_5$Ir$_3$O, multigap SC is evidenced by the field dependence of the electronic specific heat coefficient and the superconducting Gaussian relaxation rate, as well as by the temperature dependence of the upper critical field. Pt substitution suppresses one of the gaps, and Nb$_5$Ir$_{1.4}$Pt$_{1.6}$O becomes a single-gap superconductor. By combining our extensive experimental results, we provide evidence for a multiple- to single-gap SC crossover in the Nb$_5$Ir$_{3-x}$Pt$_x$O family.

cond-mat.supr-con