arXiv subjects

S. J. Rose

Publications and source records attributed to S. J. Rose.

At least 19 recordsLinked to original sources

arXiv2025

A comparison of time-dependent Cloudy astrophysical code simulations with experimental X-ray spectra from keV laser-generated argon plasmas

We have generated strongly photoionized Ar plasmas in experiments designed to use primarily X-ray L-shell line emission generated from Ag foils irradiated by the VULCAN high-power laser at the UK Central Laser Facility. The principle of the experiment is that use of line emission rather than the usual sub-keV quasi-blackbody source allows keV radiation to play a more dominant role compared to softer X-rays and thus mimic the effect of a blackbody with a higher effective spectral temperature. Our aim is to reproduce in the laboratory the extreme photoionization conditions found in accretion-powered astrophysical sources. In this paper, we compare the experimental results on K-$β$ X-ray Ar spectra with modelling using the time-dependent version of the Cloudy astrophysical code. The results indicate that photoionized laboratory plasmas can be successfully modelled with codes such as Cloudy that have been developed for application to astrophysical sources. Our comparison of simulation and experiment shows that the flux of sub-keV photons that photoionize the outer-shell electrons can have a significant effect, and that detailed measurements of the X-ray drive spectrum across all photon energy ranges are crucial for accurate modelling of experiments.

astro-ph.HE↗

arXiv2025

Bounding elastic photon-photon scattering at $\sqrt s \approx 1\,$MeV using a laser-plasma platform

We report on a direct search for elastic photon-photon scattering using x-ray and $γ$ photons from a laser-plasma based experiment. A gamma photon beam produced by a laser wakefield accelerator provided a broadband gamma spectrum extending to above $E_γ= 200$ MeV. These were collided with a dense x-ray field produced by the emission from a laser heated germanium foil at $E_x \approx 1.4$ keV, corresponding to an invariant mass of $\sqrt{s} = 1.22 \pm 0.22$ MeV. In these asymmetric collisions elastic scattering removes one x-ray and one high-energy $γ$ photon and outputs two lower energy $γ$ photons. No changes in the $γ$ photon spectrum were observed as a result of the collisions allowing us to place a 95% upper bound on the cross section of $1.5 \times 10^{15}\,μ$b. Although far from the QED prediction, this represents the lowest upper limit obtained so far for $\sqrt{s} \lesssim 1$ MeV.

hep-ex↗

arXiv2024

Extended X-ray absorption spectroscopy using an ultrashort pulse laboratory-scale laser-plasma accelerator

Laser-driven compact particle accelerators can provide ultrashort pulses of broadband X-rays, well suited for undertaking X-ray absorption spectroscopy measurements on a femtosecond timescale. Here the Extended X-ray Absorption Fine Structure (EXAFS) features of the K-edge of a copper sample have been observed over a 250 eV window in a single shot using a laser wakefield accelerator, providing information on both the electronic and ionic structure simultaneously. This unique capability will allow the investigation of ultrafast processes, and in particular, probing high-energy-density matter and physics far-from-equilibrium where the sample refresh rate is slow and shot number is limited. For example, states that replicate the tremendous pressures and temperatures of planetary bodies or the conditions inside nuclear fusion reactions. Using high-power lasers to pump these samples also has the advantage of being inherently synchronised to the laser-driven X-ray probe. A perspective on the additional strengths of a laboratory-based ultrafast X-ray absorption source is presented.

physics.plasm-ph↗

arXiv2024

Generation of photoionized plasmas in the laboratory of relevance to accretion-powered x-ray sources using keV line radiation

We describe laboratory experiments to generate X-ray photoionized plasmas of relevance to accretion-powered X-ray sources such as neutron star binaries and quasars, with significant improvements over previous work. A key quantity is referenced, namely the photoionization parameter. This is normally meaningful in an astrophysical steady-state context, but is also commonly used in the literature as a figure of merit for laboratory experiments that are, of necessity, time-dependent. We demonstrate emission-weighted values of ξ > 50 ergcm/s using laser-plasma X-ray sources, with higher results at the centre of the plasma which are in the regime of interest for several astrophysical scenarios. Comparisons of laboratory experiments with astrophysical codes are always limited, principally by the many orders of magnitude differences in time and spatial scales, but also other plasma parameters. However useful checks on performance can often be made for a limited range of parameters. For example, we show that our use of a keV line source, rather than the quasi-blackbody radiation fields normally employed in such experiments, has allowed the generation of the ratio of inner-shell to outer-shell photoionization expected from a blackbody source with ~keV spectral temperature. We compare calculations from our in-house plasma modelling code with those from Cloudy and find moderately good agreement for the time evolution of both electron temperature and average ionisation. However, a comparison of code predictions for a K-beta argon X-ray spectrum with experimental data reveals that our Cloudy simulation overestimates the intensities of more highly ionised argon species. This is not totally surprising as the Cloudy model was generated for a single set of plasma conditions, while the experimental data are spatially integrated.

astro-ph.HE↗

arXiv2024

Dielectronic satellite emission from a solid-density Mg plasma: relationship to models of ionisation potential depression

We report on experiments where solid-density Mg plasmas are created by heating with the focused output of the Linac Coherent Light Source x-ray free-electron-laser. We study the K-shell emission from the Helium and Lithium-like ions using Bragg crystal spectroscopy. Observation of the dielectronic satellites in Lithium-like ions confirms that the M-shell electrons appear bound for these high charge states. An analysis of the intensity of these satellites indicates that when modelled with an atomic-kinetics code, the ionisation potential depression model employed needs to produce depressions for these ions which lie between those predicted by the well known Stewart-Pyatt and Ecker-Kroll models. These results are largely consistent with recent Density Functional Theory calculations.

hep-ex↗

arXiv2023

Monte Carlo modelling of the linear Breit-Wheeler process within the GEANT4 framework

A linear Breit-Wheeler module for the code Geant4 has been developed. This allows signal-to-noise ratio calculations of linear Breit-Wheeler detection experiments to be performed within a single framework. The interaction between two photon sources is modelled by treating one as a static field, then photons from the second source are sampled and tracked through the field. To increase the efficiency of the module, we have used a Gaussian process regression, which can lead to an increase in the calculation rate by a factor of up to 1000. To demonstrate the capabilities of this module, we use it to perform a parameter scan, modelling an experiment based on that recently reported by Kettle et al. [1]. We show that colliding $50\,$fs duration $γ$-rays, produced through bremsstrahlung emission of a $100\,$pC, $2\,$GeV laser wakefield accelerator beam, with a $50\,$ps X-ray field, generated by a germanium burn-through foil heated to temperatures $>\,150\,$eV, this experiment is capable of producing $>1\,$ Breit-Wheeler pair per shot.

physics.plasm-ph↗

arXiv2022

SpK: A fast atomic and microphysics code for the high-energy-density regime

SpK is part of the numerical codebase at Imperial College London used to model high energy density physics (HEDP) experiments. SpK is an efficient atomic and microphysics code used to perform detailed configuration accounting calculations of electronic and ionic stage populations, opacities and emissivities for use in post-processing and radiation hydrodynamics simulations. This is done using screened hydrogenic atomic data supplemented by the NIST energy level database. An extended Saha model solves for chemical equilibrium with extensions for non-ideal physics, such as ionisation potential depression, and non thermal equilibrium corrections. A tree-heap (treap) data structure is used to store spectral data, such as opacity, which is dynamic thus allowing easy insertion of points around spectral lines without a-priori knowledge of the ion stage populations. Results from SpK are compared to other codes and descriptions of radiation transport solutions which use SpK data are given. The treap data structure and SpK's computational efficiency allows inline post-processing of 3D hydrodynamics simulations with a dynamically evolving spectrum stored in a treap.

physics.plasm-ph↗

arXiv2022

L-shell X-ray conversion yields for laser-irradiated tin and silver foils

We have employed the VULCAN laser facility to generate a laser plasma X-ray source for use in photoionisation experiments. A nanosecond laser pulse with an intensity of order ${10}^{15}$ W{cm}$^{-2}$ was used to irradiate thin Ag or Sn foil targets coated onto a parylene substrate, and the L-shell emission in the $3.3-4.4$ keV range was recorded for both the laser-irradiated and non-irradiated sides. Both the experimental and simulation results show higher laser to X-ray conversion yields for Ag compared with Sn, with our simulations indicating yields approximately a factor of two higher than found in the experiments. Although detailed angular data were not available experimentally, the simulations indicate that the emission is quite isotropic on the laser-irradiated side, but shows close to a cosine variation on the non-irradiated side of the target as seen experimentally in previous work.

physics.plasm-ph↗

arXiv2021

Temperature Equilibration Due to Charge State Fluctuations in Dense Plasmas

The charge states of ions in dense plasmas fluctuate due to collisional ionization and recombination. Here we show how, by modifying the ion interaction potential, these fluctuations can mediate energy exchange between the plasma electrons and ions. Moreover, we develop a theory for this novel electron-ion energy transfer mechanism. Calculations using a random walk approach for the fluctuations suggest that the energy exchange rate from charge state fluctuations could be comparable to direct electron-ion collisions. This mechanism is, however, predicted to exhibit a complex dependence on the temperature and ionization state of the plasma, which could contribute to our understanding of significant variation in experimental measurements of equilibration times.

physics.plasm-ph↗

arXiv2021

A laser-plasma platform for photon-photon physics

We describe a laser-plasma platform for photon-photon collision experiments to measure fundamental quantum electrodynamic processes such as the linear Breit-Wheeler process with real photons. The platform has been developed using the Gemini laser facility at the Rutherford Appleton Laboratory. A laser wakefield accelerator and a bremsstrahlung convertor are used to generate a collimated beam of photons with energies of hundreds of MeV, that collide with keV x-ray photons generated by a laser heated plasma target. To detect the pairs generated by the photon-photon collisions, a magnetic transport system has been developed which directs the pairs onto scintillation-based and hybrid silicon pixel single particle detectors. We present commissioning results from an experimental campaign using this laser-plasma platform for photon-photon physics, demonstrating successful generation of both photon sources, characterisation of the magnetic transport system and calibration of the single particle detectors, and discuss the feasibility of this platform for the observation of the Breit-Wheeler process. The design of the platform will also serve as the basis for the investigation of strong-field quantum electrodynamic processes such as the nonlinear Breit-Wheeler and the Trident process, or eventually, photon-photon scattering.

physics.plasm-ph↗

arXiv2020

Calculating Opacity in Hot, Dense Matter using Second-Order Electron-Photon and Two-Photon Transitions to Approximate Line Broadening

Calculations of the opacity of hot, dense matter require models for plasma line broadening. However, the most general theories are too complex to calculate directly and some approximation is inevitably required. The most widely-used approaches focus on the line centre, where a Lorentzian shape is obtained. Here, we demonstrate that in the opposite limit, far from the line centre, the opacity can be expressed in terms of second-order transitions, such as electron-photon and two-photon processes. We suggest that this insight could form the basis for a new approach to improve calculations of opacity in hot, dense matter. Preliminary calculations suggest that this approach could yield increased opacity away from absorption lines.

physics.plasm-ph↗

arXiv2019

Single-shot multi-keV X-ray absorption spectroscopy using an ultrashort laser wakefield accelerator source

Single-shot absorption measurements have been performed using the multi-keV X-rays generated by a laser wakefield accelerator. A 200 TW laser was used to drive a laser wakefield accelerator in a mode which produced broadband electron beams with a maximum energy above 1 GeV and a broad divergence of $\approx15$ miliradians FWHM. Betatron oscillations of these electrons generated $1.2\pm0.2\times10^6$ photons/eV in the 5 keV region, with a signal-to-noise ratio of approximately 300:1. This was sufficient to allow high-resolution XANES measurements at the K-edge of a titanium sample in a single shot. We demonstrate that this source is capable of single-shot, simultaneous measurements of both the electron and ion distributions in matter heated to eV temperatures by comparison with DFT simulations. The unique combination of a high-flux, large bandwidth, few femtosecond duration X-ray pulse synchronised to a high-power laser will enable key advances in the study of ultra-fast energetic processes such as electron-ion equilibration.

physics.plasm-ph↗

arXiv2019

The Blind Implosion-Maker - Automated Inertial Confinement Fusion experiment design

The design of inertial confinement fusion experiments, alongside improving the development of energy density physics theory and experimental methods, is one of the key challenges in the quest for nuclear fusion as a viable energy source. Recent challenges in achieving a high-yield implosion at the National Ignition Facility (NIF) have led to new interest in considering a much wider design parameter space than normally studied. Here we report an algorithmic approach that can produce reasonable ICF designs with minimal assumptions. In particular we use the genetic algorithm metaheuristic, in which `populations' of implosions are simulated, the design of capsule is described by a `genome', natural selection removes poor designs, high quality designs are `mated' with each other based on their yield, and designs undergo `mutations' to introduce new ideas. We show that it takes ~5x10^4 simulations for the algorithm to find an original NIF design. We also link this method to other parts of the design process and look towards a completely automated ICF experiment design process - changing ICF from an experiment design problem to an algorithm design problem.

physics.plasm-ph↗

arXiv2019

Nuclear level densities and gamma-ray strength functions of $^{180,181,182}$Ta

Particle-$γ$ coincidence experiments were performed at the Oslo Cyclotron Laboratory with the $^{181}$Ta(d,X) and $^{181}$Ta($^{3}$He,X) reactions, to measure the nuclear level densities (NLDs) and $γ$-ray strength functions ($γ$SFs) of $^{180, 181, 182}$Ta using the Oslo method. The Back-shifted Fermi-Gas, Constant Temperature plus Fermi Gas, and Hartree-Fock-Bogoliubov plus Combinatorial models where used for the absolute normalisations of the experimental NLDs at the neutron separation energies. The NLDs and $γ$SFs are used to calculate the corresponding $^{181}$Ta(n,$γ$) cross sections and these are compared to results from other techniques. The energy region of the scissors resonance strength is investigated and from the data and comparison to prior work it is concluded that the scissors strength splits into two distinct parts. This splitting may allow for the determination of triaxiality and a $γ$ deformation of $14.9^{\circ} \pm 1.8^{\circ}$ was determined for $^{181}$Ta.

nucl-ex↗

arXiv2017

X-ray line coincidence photopumping in a solar flare

Line coincidence photopumping is a process where the electrons of an atomic or molecular species are radiatively excited through the absorption of line emission from another species at a coincident wavelength. There are many instances of line coincidence photopumping in astrophysical sources at optical and ultraviolet wavelengths, with the most famous example being Bowen fluorescence (pumping of O III 303.80 A by He II), but none to our knowledge in X-rays. However, here we report on a scheme where a He-like line of Ne IX at 11.000 A is photopumped by He-like Na X at 11.003 A, which predicts significant intensity enhancement in the Ne IX 82.76 A transition under physical conditions found in solar flare plasmas. A comparison of our theoretical models with published X-ray observations of a solar flare obtained during a rocket flight provides evidence for line enhancement, with the measured degree of enhancement being consistent with that expected from theory, a truly surprising result. Observations of this enhancement during flares on stars other than the Sun would provide a powerful new diagnostic tool for determining the sizes of flare loops in these distant, spatially-unresolved, astronomical sources.

astro-ph.SR↗

arXiv2017

Energy dependence of the prompt $γ$-ray emission from the $(d,p)$-induced fission of $^{234}\mathrm{U}^{}$ and $^{240}\mathrm{Pu}^{}$

Prompt fission $γ$-rays are responsible for approximately 5\% of the total energy released in fission, and therefore important to understand when modelling nuclear reactors. In this work we present prompt $γ$-ray emission characteristics in fission, for the first time as a function of the nuclear excitation energy of the fissioning system. Emitted $γ$-ray spectra were measured, and $γ$-ray multiplicities and average and total $γ$ energies per fission were determined for the $^{233}$U(d,pf) reaction for excitation energies between 4.8 and 10 MeV, and for the $^{239}$Pu(d,pf) reaction between 4.5 and 9 MeV. The spectral characteristics show no significant change as a function of excitation energy above the fission barrier, despite the fact that an extra $\sim$5 MeV of energy is potentially available in the excited fragments for $γ$-decay. The measured results are compared to model calculations made for prompt $γ$-ray emission with the fission model code GEF. Further comparison with previously obtained results from thermal neutron induced fission is made to characterize possible differences arising from using the surrogate (d,p) reaction.

nucl-ex↗

arXiv2017

Low-energy enhancement and fluctuations of $γ$-ray strength functions in $^{56,57}$Fe: test of the Brink-Axel hypothesis

Nuclear level densities and $γ$-ray strength functions of $^{56,57}$Fe have been extracted from proton-$γ$ coincidences. A low-energy enhancement in the $γ$-ray strength functions up to a factor of 30 over common theoretical E1 models is confirmed. Angular distributions of the low-energy enhancement in $^{57}$Fe indicate its dipole nature, in agreement with findings for $^{56}$Fe. The high statistics and the excellent energy resolution of the large-volume LaBr$_{3}$(Ce) detectors allowed for a thorough analysis of $γ$ strength as function of excitation energy. Taking into account the presence of strong Porter-Thomas fluctuations, there is no indication of any significant excitation-energy dependence in the $γ$-ray strength function, in support of the generalized Brink-Axel hypothesis.

nucl-ex↗

arXiv2016

Study of the 238U(d,p) surrogate reaction via the simultaneous measurement of gamma-decay and fission probabilities

We investigated the 238U(d,p) reaction as a surrogate for the n + 238U reaction. For this purpose we measured for the first time the gamma-decay and fission probabilities of 239U* simultaneously and compared them to the corresponding neutron-induced data. We present the details of the procedure to infer the decay probabilities, as well as a thorough uncertainty analysis, including parameter correlations. Calculations based on the continuum-discretized coupled-channels and distorted-wave Born approximations were used to correct our data from detected protons originating from elastic and inelastic deuteron breakup. In the region where the fission and gamma-decay probabilities compete, the corrected fission probability is in agreement with neutron-induced data, whereas the gamma-decay probability is much higher than the neutron-induced data. The performed statistical-model calculations are not able to explain these results.

nucl-ex↗