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S. Johnston

Publications and source records attributed to S. Johnston.

At least 19 recordsLinked to original sources

Observation of multipartite spin entanglement in a cuprate chain

Quantum materials are believed to host highly entangled states of matter, but probing and quantifying such entanglement has long remained experimentally elusive. Here, we use resonant inelastic X-ray scattering (RIXS) as a probe of multipartite spin entanglement. By projecting the RIXS cross section onto the appropriate spin excitation channel, we show that the Quantum Fisher Information can be extracted directly from the measured spin fluctuation spectrum. We detect at least 7-partite spin entanglement in the model one-dimensional cuprate Sr$_2$CuO$_3$, revealing one of the largest entanglement depths yet reported in a solid. The observed entanglement depth agrees with Hubbard-model expectations and persists to elevated temperatures. Our results establish RIXS as an experimental probe of many-body spin entanglement and provide a platform for extensions to charge and orbital sectors and nonequilibrium settings.

cond-mat.str-el

Precision Neutron Skins of $^{208}$Pb and $^{48}$Ca from Parity-Violating Electron Scattering

We have measured the parity-violating elastic electron scattering asymmetry in the PREX and CREX experiments on ${}^{208}$Pb and ${}^{48}$Ca respectively; these are both doubly-magic nuclei whose excited states can be discriminated from the ground state by the high resolution spectrometers in Hall A at Jefferson Lab. This asymmetry provides a precise determination of the weak charge form factor at one $Q^2$ and pins down the neutron radius in these two nuclei in a relatively clean and model-independent way. This is because the $Z^0$ boson of the weak interaction couples primarily to neutrons. The heavier lead nucleus, with a neutron excess, provides an interpretation of the neutron skin thickness in terms of properties of bulk neutron matter. For the lighter ${}^{48}$Ca nucleus, which is also rich in neutrons, comparisons to microscopic nuclear theory calculations are sensitive to poorly constrained 3-neutron forces. The weak neutral form factors $F_W(Q^2)$ were extracted to be $0.368 \pm 0.013$ at $Q = 0.3977 {\rm\ fm}^{-1}$ for $^{208}$Pb from PREX-2 and $0.1304 \pm 0.0055$ at $Q = 0.8733 {\rm\ fm}^{-1}$ for $^{48}$Ca. The form factor differences $(F_{ch}-F_W)(Q^2)$ were calculated to be $0.041 \pm 0.013$ at $Q = 0.3977 {\rm fm}^{-1}$ for $^{208}$Pb from PREX-2 and $0.0277 \pm 0.0055$ at $Q = 0.8733 {\rm fm}^{-1}$ for $^{48}$Ca. Correcting for Coulomb distortions and using nuclear model information, we find the neutron skin thicknesses to be $R^{208}_{\rm skin} = 0.283 \pm 0.071$ fm combining PREX-1 and PREX-2 and $R^{48}_{\rm skin} = 0.121 \pm 0.035$ fm. This paper provides a full description of the special experimental and data analysis techniques employed for precisely measuring these small asymmetries.

nucl-ex

Layer Architecture Shapes Electronic, Magnetic, and Lattice Interactions in Ruddlesden-Popper Nickelates

The discovery of superconductivity in Ruddlesden-Popper nickelates has raised a central question: how does layer architecture shape the electronic, magnetic, and lattice interactions relevant to pairing? Here, we report a detailed comparative study of the two polymorphs of La3Ni2O7--the alternating monolayer-trilayer (LNO-1313) and bilayer (LNO-2222) structures--and the related trilayer compound La4Ni3O10, using both Ni L3- and O K-edge RIXS. We find that LNO-1313 and La4Ni3O10 share strikingly similar electronic, magnetic, and lattice excitations, whereas bilayer LNO-2222 exhibits distinct features. Compared to LNO-2222, LNO-1313 and La4Ni3O10 have weaker orbital polarization, enhanced 3d8L character, a reduced out-of-plane magnetic-exchange scale, and stronger EPC. Within an effective local-moment framework, an entangled-dimer scenario provides a natural description of the spin excitations generated by strong antiferromagnetic interlayer coupling. Its advantage over conventional spin-wave theory is clearest in bilayer LNO-2222, where the interlayer coupling dominates the intralayer interactions. These findings provide critical experimental constraints for future theoretical models for the low-energy physics relevant to superconductivity in these layered nickelates.

cond-mat.str-el

A DQMC study of the spectral and conductive properties of the two-dimensional Holstein model

We study the dynamical properties of the two-dimensional square lattice Holstein Hamiltonian using numerically exact determinant quantum Monte Carlo simulations. In particular, we report systematic calculations of the model's single-particle spectral function and optical conductivity over a range of phonon energies, electron-phonon coupling strengths, carrier concentrations, and temperatures. In doing so, we map the evolution of the system from a dressed metallic phase to a (bi)polaron liquid/insulator to a charge-density-wave insulator as the carrier concentration is tuned from dilute values to half-filling. We corroborate these results using several equal-time correlation measurements and related proxy quantities reconstructed from time-displaced correlation measurements. This paper is also accompanied by an extensive open data set, covering over 16,640 unique parameter values.

cond-mat.str-el

Disentangling multi-spin dynamic correlations in the Heisenberg spin-$\frac{1}{2}$ chain

Higher-order correlations are essential for understanding exotic phases and uncovering universal aspects of quantum dynamics. While inelastic neutron scattering provides well-established access to two-particle correlations, measuring correlations in solids involving more than two particles remains a major challenge. Focusing on magnetic excitations in the Heisenberg spin-$\frac{1}{2}$ chain, we demonstrate that resonant inelastic X-ray scattering (RIXS) can selectively probe multi-spin dynamical correlations by exciting distinct intermediate states through energy detuning. Through theoretical modeling, we isolate the two- and multi- spin responses, and establish that: (i) The resonant energies of the two- and multi- spin dynamical correlations are separated by $\approx \frac{3}{4}J$; implying that the multi-spin part of the cross-section comes from intermediate states that contain spin flips; (ii) The spectral weight of the two-spin channel exhibits a Lorentzian resonant energy profile consistent with a single dominant electronic configuration, whereas the multi-spin channel response shows a Gaussian-like profile, implying contributions from multiple intermediate spin configurations. These characteristics are reproduced by exact diagonalization of the $t-J$ Hamiltonian, which further reveals that the widths of Lorentzian and Gaussian resonant energy profiles depend primarily on core-hole lifetime ($\Gamma/2$) and $\frac{2J}{\Gamma}$, respectively. Controlled access to multi-spin dynamics, using RIXS energy detuning as a knob, can open new pathways to explore many-body dynamics in quantum materials.

cond-mat.str-el

Murriyang cryogenic phased array feed: spectral-line results and noise-reduction methods

Spectral-line results from a new cryogenic phased array feed (cryoPAF) on the Murriyang telescope at Parkes are presented. This array offers a significant improvement in field of view, aperture efficiency, bandwidth, chromaticity and survey speed compared with conventional horn-fed receivers. We demonstrate this with measurements of sky calibrators and observations of 21-cm neutral hydrogen (HI) in the LMC and the nearby galaxy NGC 6744. Within 0.3 deg of the optical axis, the ratio of system temperature to dish aperture efficiency is 25 K and the ratio with beam efficiency is 21 K (at 1.4 GHz). For the previously measured $T_{sys} = 17$ K, respective efficiency values 0.7 and 0.8 are derived. Our HI observational results are in good agreement with previous results, although detailed comparison with multibeam observations of the LMC suggests that the earlier observations may have missed an extended component of low-column-density gas ($8\times 10^{18}$ cm$^{-2}$). We use the cryoPAF zoom-band and wideband data to make a preliminary investigation of whether the large number of simultaneous beams (72) permits the use of novel data reduction methods to reduce the effects of foreground/background continuum contamination and RFI. We also investigate if these methods can better protect against signal loss for the detection of faint, extended cosmological signals such as HI intensity maps. Using robust higher-order singular value decomposition (SVD) techniques, we find encouraging results for the detection of both compact and extended sources, including challenging conditions with high RFI occupancy and significant sky continuum structure. Examples are shown that demonstrate that 3D SVD techniques offer a significant improvement in noise reduction and signal capture compared with more traditional layered 2D techniques.

astro-ph.IM

Observation of correlated plasmons in low-valence nickelates

The discovery of nickelate superconductors has opened a new arena for studying the behavior of correlated electron liquids that give rise to unconventional superconductivity. While critical information about a material's charge dynamics is encoded in its plasmons, collective modes of the electron gas, these excitations have not yet been observed in nickelate materials. Here, we use resonant inelastic x-ray scattering (RIXS) to detect plasmons in the metallic, low-valence nickelate Pr4Ni3O8. Although qualitatively similar to those in cuprates, the nickelate plasmons are more heavily damped and have a lower velocity than those in a cuprate at comparable doping, which we attribute to reduced electronic hopping and enhanced screening of the long-range Coulomb interactions. Furthermore, the plasmons in Pr4Ni3O8 soften with increasing temperature, in contrast to the cuprate, where plasmons remain at nearly fixed energy but become more strongly damped. Taken together, these results reveal a distinct charge-screening landscape in nickelates and place quantitative constraints on analogies to cuprates.

cond-mat.str-el

Non-reciprocal circular dichroism of axial phonons coupled to ferro-rotational order

Circular dichroism (CD) in X-ray absorption, defined as the difference in absorption between opposite circular polarizations, is fundamentally enabled by the breaking of time-reversal symmetry or inversion symmetry. It is therefore sensitive to magnetism, chirality, and their interplay. In contrast, the sample symmetry alone is insufficient to determine whether CD in resonant inelastic X-ray scattering (RIXS) is allowed. Rather, RIXS-CD is governed by both the sample symmetry and the scattering geometry. Here, using RIXS, we identify circularly polarized phonons coupled to ferro-rotational order in MnTiO$_3$, which we refer to as ferro-axial phonons. Their excitations provide a direct demonstration of non-reciprocal RIXS-CD, in which the dichroic response changes upon reversing the propagation direction of the incident X-rays, although the system globally preserves both inversion and time-reversal symmetries. We propose that a condensate of these phonons, manifested as standing waves, underlies the ferro-rotational order in MnTiO$_3$. The observed non-reciprocal CD reflects the interplay among photon helicity, phonon polarization, and ferro-rotational order.

cond-mat.str-el

Evolutionary Map of the Universe: A pilot survey to detect high Galactic latitude pulsars in variance images with ASKAP

It has been proposed that radio pulsars can be distinguished from other point-like radio sources in continuum images by their unique interstellar scintillation signatures. Using data from the Australian Square Kilometre Array Pathfinder (ASKAP) Evolutionary Map of the Universe (EMU) survey, we conducted a pilot survey of radio pulsars at high Galactic latitude regions via the variance imaging method. Out of approximately 59,800 compact radio sources detected in a ~480 square degree survey area, we identified 20 highly variable sources. Among them, 9 are known pulsars, 1 is a known radio star, 1 is an ultra-long period source, 3 are radio star candidates, and the remaining 6 are pulsar candidates. Notably, we discovered two strongly scintillating pulsars: one with a period of 85.707 ms and a dispersion measure (DM) of 19.4 pc/cm^3, and another with a period of 5.492 ms and a DM of 29.5 pc/cm^3. In addition, a third pulsar was discovered in the variance images, with a period of 14.82 ms and a DM of 39.0 pc/cm^3. This source shows a steep radio spectrum and a high degree of circular polarisation. These results underscore the strong potential of variance imaging for pulsar detection in full EMU and future radio continuum surveys planned with Square Kilometre Array (SKA).

astro-ph.IM

Frequency evolution of pulsar emission: Further evidence for fan beam model

Aims. We explore frequency-dependent changes in pulsar radio emission by analyzing their profile widths and emission heights, assessing whether the simple radius-to-frequency mapping (RFM) or the fan beam model can describe the data. Methods. Using wideband (704-4032 MHz) Murriyang (Parkes) observations of over 100 pulsars, we measured profile widths at multiple intensity levels, fit Gaussian components, and used aberration-retardation effects to estimate emission altitudes. We compared trends in width evolution and emission height with a fan beam model. Results. Similar to other recent studies, we find that while many pulsars show profiles narrowing with increasing frequency, a substantial fraction show the reverse. The Gaussian decomposition of the profiles reveals that the peak locations of the components vary little with frequency. However, the component widths do, in general, narrow with increasing frequency. This argues that propagation effects are responsible for the width evolution of the profiles rather than emission height. Overall, the evolution of the emission height with frequency is unclear, and clouded by the assumptions in the model. Spin-down luminosity correlates weakly with profile narrowing but not with emission height. Conclusions. The classic picture where pulsars emit at a single emission height which decreases with increasing observing frequency cannot explain the diversity in behavior observed here. Instead, pulsar beams likely originate from extended regions at multiple altitudes, with fan-beam or patchy structures dominating their frequency evolution. Future models must incorporate realistic plasma physics and multi-altitude emission to capture the range of pulsar behaviors.

astro-ph.HE

Hamiltonian parameter inference from resonant inelastic x-ray scattering with active learning

Identifying model Hamiltonians is a vital step toward creating predictive models of materials. Here, we combine Bayesian optimization with the EDRIXS numerical package to infer Hamiltonian parameters from resonant inelastic X-ray scattering (RIXS) spectra within the single atom approximation. To evaluate the efficacy of our method, we test it on experimental RIXS spectra of NiPS3, NiCl2, Ca3LiOsO6, and Fe2O3, and demonstrate that it can reproduce results obtained from hand-fitted parameters to a precision similar to expert human analysis while providing a more systematic mapping of parameter space. Our work provides a key first step toward solving the inverse scattering problem to extract effective multi-orbital models from information-dense RIXS measurements, which can be applied to a host of quantum materials. We also propose atomic model parameter sets for two materials, Ca3LiOsO6 and Fe2O3, that were previously missing from the literature.

cond-mat.str-el

High Voltage Delivery and Distribution for the NEXT-100 Time Projection Chamber

A critical element in the realization of large liquid and gas time projection chambers (TPCs) is the delivery and distribution of high voltages into and around the detector. Such experiments require of order tens of kilovolts to enable electron drift over meter-scale distances. This paper describes the design and operation of the cathode feedthrough and high voltage distribution through the field cage of the NEXT-100 experiment, an underground TPC that will search for neutrinoless double beta decay $0\nu\beta\beta$. The feedthrough has been demonstrated to hold pressures up to 20~bar and sustain voltages as high as -65~kV, and the TPC is operating stably at its design high voltages. The system has been realized within the constraints of a stringent radiopurity budget and is now being used to execute a suite of sensitive double beta decay analyses.

physics.ins-det

The Thousand-Pulsar-Array programme on MeerKAT -- XVI. Mapping the Galactic magnetic field with pulsar observations

Measuring the magnetic field of the Milky Way reveals the structure and evolution of the galaxy. Pulsar rotation measures (RMs) provide a means to probe this Galactic magnetic field (GMF) in three dimensions. We use the largest single-origin data set of pulsar measurements, from the MeerKAT Thousand-Pulsar-Array, to map out GMF components parallel to pulsar lines of sight. We also present these measurements for easy integration into the consolidated RM catalogue, RMTable. Focusing on the Galactic disk, we investigate competing theories of how the GMF relates to the spiral arms, comparing our observational map with five analytic models of magnetic field structure. We also analyse RMs to extragalactic radio sources, to help build up a three-dimensional picture of the magnetic structure of the galaxy. In particular, our large number of measurements allows us to investigate differing magnetic field behaviour in the upper and lower halves of the Galactic plane. We find that the GMF is best explained as following the spiral arms in a roughly bisymmetric structure, with antisymmetric parity with respect to the Galactic plane. This picture is complicated by variations in parity on different spiral arms, and the parity change location appears to be shifted by a distance of 0.15 kpc perpendicular to the Galactic plane. This indicates a complex relationship between the large-scale distributions of matter and magnetic fields in our galaxy. Future pulsar discoveries will help reveal the origins of this relationship with greater precision, as well as probing the locations of local magnetic field inhomogenities.

astro-ph.GA

Flat tails in FRB and pulsar energy distributions: implications for optimizing nearby FRB surveys

Fast radio bursts (FRBs) are energetic, short-duration radio pulses of unclear origin. To explore effective survey strategies for detecting FRBs from nearby globular clusters (GCs), we investigate the burst energy distribution, which has a strong influence on the detection rate. We re-analyze FRBs and pulsars exhibiting broad energy distributions by fitting their high-energy tails with power-law models. Two cosmological repeating FRBs (FRB 20201124A and FRB 20220912A), one nearby FRB (FRB 20200120E), and two pulsars (RRATs J1846$-$0257 and J1854+0306), exhibit power-law indices of $\alpha \gtrsim -1$, suggesting that their bright pulses contribute significantly to the total radio pulse energy. The brightest bursts from these sources can be fitted with a power-law model ($\alpha_{\rm Bri} = -0.26 \pm 0.05$), suggesting that an extremely flat index is required to naturally derive high-luminosity FRBs from low-luminosity sources. We present detailed survey strategies for FAST, MeerKAT and Parkes cryoPAF in the search for FRBs in nearby GCs using different power-law indices, recommending targets for observation. We suggest that combining observations with FAST ($\sim3$ hours) and Parkes cryoPAF (10$-$20 hours) is practicable for discovering new FRBs in nearby GCs.

astro-ph.HE

Discovery and Timing of Four $\gamma$-ray Millisecond Pulsars

We discovered four millisecond pulsars (MSPs) in searches of 80 $\gamma$-ray sources conducted from 2015 to 2017 with the Murriyang radio telescope of the Parkes Observatory. We provide an overview of the survey and focus on the results of a follow-up pulsar timing campaign. Using Fermi Large Area Telescope data, we have detected $\gamma$-ray pulsations from all four pulsars, and by combining radio and $\gamma$-ray data we obtain improved timing solutions. We also provide flux density distributions for the radio pulsars and flux-calibrated and phase-aligned radio and $\gamma$-ray pulse profiles. Some of the pulsars may be suitable for radio pulsar timing array experiments. PSR J0646-5455, PSR J1803-4719, and PSR J2045-6837 are in typical, nearly circular white dwarf binaries with residual eccentricities proportional to their binary periods. PSR J1833-3840 is a black widow pulsar with the longest known period, Pb = 0.9 d, and a very soft radio spectrum. PSR J0646-5455 has a strong, Vela-like $\gamma$-ray pulse profile and is suitable for inclusion in the $\gamma$-ray Pulsar Timing Array (GPTA). Despite this, it is possibly one of the lowest-efficiency $\gamma$-ray MSPs known. Indeed, all four new $\gamma$-ray MSPs have lower-than-average efficiency, a potential indication of bias in earlier searches. Finally, we retrospectively evaluate the efficiency of this survey: while only four new MSPs were directly discovered, subsequent campaigns have found pulsars in a further 19 of our targets, an excellent 30% efficiency.

astro-ph.HE

Cooper-Pair Localization in the Magnetic Dynamics of a Cuprate Ladder

We investigate the spin dynamics of the cuprate ladder Sr$_{2.5}$Ca$_{11.5}$Cu$_{24}$O$_{41}$ to elucidate the behavior of its intrinsically doped holes. Combining high-resolution neutron spectroscopy and density matrix renormalization group calculations enables a comprehensive analysis of the collective magnetic dynamics. We find a general absence of magnetic signatures from unpaired charges, indicating holes within the system form strongly bound localized Cooper pairs. A one-band Hubbard model fails to match the spectral features but a straightforward extension to a large attractive nearest-neighbor interaction quantitatively explains our results. Our finding shows the significance of additional interactions beyond the long-predicted quantum spin pairing in the ($d$-wave) charge pairing process. Considering the parallels between ladders and two-dimensional cuprates, these results are potentially relevant for square lattices as well.

cond-mat.str-el

Dispersive dark excitons in van der Waals ferromagnet CrI3

Spin-flip dark excitons are optical-dipole-forbidden quasiparticles with remarkable potential in optoelectronics, especially when they are realized within cleavable van der Waals materials. Despite this potential, dark excitons have not yet been definitively identified in ferromagnetic van der Waals materials. Here, we report two dark excitons in a model ferromagnetic material CrI3 using high-resolution resonant inelastic x-ray scattering (RIXS) and show that they feature narrower linewidths compared to the bright excitons previously reported in this material. These excitons are shown to have spin-flip character, to disperse as a function of momentum, and to change through the ferromagnetic transition temperature. Given the versatility of van der Waals materials, these excitons hold promise for new types of magneto-optical functionality.

cond-mat.str-el

Observation of anisotropic dispersive dark exciton dynamics in CrSBr

Many-body excitons in CrSBr are attracting intense interest in view of their highly anisotropic magneto-optical coupling and their potential for novel optical interfaces within spintronic and magnonic devices. Characterizing the orbital character and propagation of these electronic excitations is crucial for understanding and controlling their behavior; however, this information is challenging to access. Ultra-high resolution resonant inelastic x-ray scattering is a momentum-resolved technique that can address these crucial questions. We present measurements collected at the Cr $L_3$-edge which show a rich spectrum of excitations with a variety of spin-orbital characters. While most of these excitations appear to be localized, the dispersion of the lowest energy dark exciton indicates that it is able to propagate along both the $a$ and $b$ directions within the planes of the crystal. This two-dimensional character is surprising as it contrasts with electrical conductivity and the behavior of the bright exciton, both of which are strongly one-dimensional. The discovery of this propagating dark exciton highlights an unusual coexistence of one- and two-dimensional electronic behaviors in CrSBr.

cond-mat.str-el