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S. Kailas

Publications and source records attributed to S. Kailas.

At least 19 recordsLinked to original sources

Fusion systematics for weakly bound nuclei using neutron flow and collective degrees of freedom

A systematic analysis of the fusion cross sections around the Coulomb barrier energies with stable weakly bound ($^{6}$Li,$^{7}$Li,$^{9}$Be) and strongly bound $^{12}$C projectiles on various targets was performed by using neutron flow model and coupled channels approach. The analysis show that both the models are successful in explaining the near barrier fusion data. Further, it is also observed that the collective degrees of freedom as well as the neutron flow influence the near barrier fusion process involving weakly bound projectiles.

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Inclusive $α$ Production for $^{6}$Li+$^{51}$V System

Measurement of angular distributions and energy spectra of $α$ and deuterons through breakup, transfer and incomplete fusion processes to dis-entangle their relative contributions and to investigate relative importance of breakup-fusion compared to transfer. Inclusive $α$ production cross-sections have been measured for $^6$Li + $^{51}$V system near Coulomb barrier energies. Theoretical calculations for estimation of various reaction channels contributing to $α$ production have been performed with finite range coupled reaction method using \textsc{FRESCO} code. The cross-sections from non-capture breakup (NCBU) ($α$ + \textit{d}) and 1\textit{n}, 1\textit{p}, and 1\textit{d} transfer channels, compound nuclear decay channel and incomplete fusion (ICF) leading to $α$ production were estimated to get the cumulative production cross-sections. Contributions from breakup, transfer and incomplete fusion channels could reproduce the integral direct $α$ production cross-sections and their angular distributions quite well. The direct $α$ production cross-sections are in agreement with other targets. The $α$ production cross-sections are higher compared to the deuteron production. Kinematic analysis of the energy spectra of $α$ particles and deuterons suggest that $α$ particle spectra is dominated by breakp-fusion and deuteron spectra have contribution of breakup and transfer reactions. A systematic study of direct $α$ production with various targets follow a universal behavior on average but noticeable differences are observed for different targets. A ratio of $α$ and deuteron yields for a wide mass range of targets shows a saturation above barrier and an increasing production of $α$ particles relative to deuteron around Coulomb barrier.

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Unraveling the reaction mechanism for large alpha production and incomplete fusion in reactions involving weakly bound stable nuclei

The origin of the large $α$ particle production and incomplete fusion in reactions involving weakly-bound $α$+$x$ cluster nuclei still remains unresolved. While the (two-step) process of breakup followed by capture of the ``free" complementary fragment ($x$) is widely believed to be responsible, a few recent studies suggest the dominant role of (direct) cluster stripping. To achieve an unambiguous experimental discrimination between these two processes, a coincidence measurement between the outgoing $α$ particles and $γ$ rays from the heavy residues has been performed for the $^7$Li($α$+triton)+$^{93}$Nb system. Proper choice of kinematical conditions allowed for the first time a significant population of the region accessible only to the direct triton stripping process and not to breakup followed by the capture of the ``free'' triton (from the three-body continuum). This result, also supported by a cluster-transfer calculation, clearly establishes the dominance of the direct cluster-stripping mechanism in the large alpha production.

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Investigation of neutron transfer in $^{7}$Li+$^{124}$Sn reaction

The relative importance of neutron transfer and breakup process in reaction around Coulomb barrier energies have been studied for the $^{7}$Li+$^{124}$Sn system. Coupled channel calculations have been performed to understand the one neutron stripping and pickup cross sections along with the breakup in the $^{7}$Li+$^{124}$Sn system. The systematics of one and two neutron striping and pickup cross sections with $^7$Li projectile on several targets show an approximate universal behaviour that have been explained by a simple model. Complete reaction mechanism have been studied by comparing the reaction cross sections with cumulative cross sections of total fusion and one neutron transfer.

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Competing quasifission and asymmetric fusion-fission in neutron-deficient sub-lead nuclei

To disentangle the role of shell effects and dynamics, fission fragment mass distributions of $^{191}$Au, a nucleus in the newly identified island of mass asymmetric fission in the sub-lead region, have been measured down to excitation energy of $\approx$20 MeV above the fission barrier via two different entrance channels, viz. $^{16}$O+$^{175}$Lu and $^{37}$Cl+$^{154}$Sm reactions. Apart from having signature of the shell effects in both the cases, clear experimental evidence of quasifission has been observed in the mass distributions of the Cl induced reaction, that has also been substantiated by the theoretical calculations. This crucial evidence along with a systematic analysis of available experimental data has revealed that the dynamics in the entrance channel has significant influence on most of the reactions used earlier to explore the persistence of recently discovered mass asymmetry in $β$-delayed fission at low energy in this mass region, ignoring which might lead to ambiguity in interpreting the heavy-ion data.

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Systematics of direct-$α$ production with weakly and strongly bound projectiles

The production of $α$-particles in reactions using both the strongly and weakly bound projectiles at energies around the Coulomb barrier show several interesting features. To understand these, the role of various reaction mechanisms responsible for $α$-production, such as non-capture breakup, capture of only one of the fragments subsequent to projectile breakup and their contribution to reaction cross sections have been investigated. A systematic study of the $α$-particle production based on available data for various projectile target systems have been performed and a classification based on projectile type is obtained.

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Deep-inelastic multinucleon transfer processes in the $^{16}$O+$^{27}$Al reaction

The reaction mechanism of deep-inelastic multinucleon transfer processes in the $^{16}$O+$^{27}$Al reaction at an incident $^{16}$O energy ($E_{\rm lab}=134$ MeV) substantially above the Coulomb barrier has been studied both experimentally and theoretically. Elastic-scattering angular distribution, total kinetic energy loss spectra and angular distributions for various transfer channels have been measured. The $Q$-value- and angle-integrated isotope production cross sections have been deduced. To obtain deeper insight into the underlying reaction mechanism, we have carried out a detailed analysis based on the time-dependent Hartree-Fock (TDHF) theory. A recently developed method, TDHF+GEMINI, has been applied to evaluate production cross sections for secondary products. From a comparison between the experimental and theoretical cross sections, we find that the theory qualitatively reproduces the experimental data. Significant effects of secondary light-particle emissions are demonstrated. Possible interplay between fusion-fission, deep-inelastic, multinucleon transfer and particle evaporation processes are discussed.

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Exploring contributions from incomplete fusion in $^{6,7}$Li+$^{209}$Bi and $^{6,7}$Li+$^{198}$Pt reactions

We use the breakup absorption model to simultaneously describe the measured cross-sections of the Complete fusion (CF), Incomplete fusion (ICF), and Total fusion (TF) in nuclear reactions induced by weakly bound nuclei $^{6,7}$Li on $^{209}$Bi and $^{198}$Pt targets. The absorption cross-sections are calculated using the Continuum Discretized Coupled Channels (CDCC) method with different choices of short range imaginary potentials to get the ICF, CF and TF cross-sections. It is observed that the cross-sections for deuteron-ICF/deuteron-capture are of similar magnitude as the $α$-ICF/$α$-capture, in case of $^{6}$Li projectile, while the cross-sections for triton-ICF/triton-capture is more dominant than $α$-ICF/$α$-capture in case of $^{7}$Li projectile. Both these observations are also corroborated by the experimental data. The ratio of ICF to TF cross-sections, which defines the value of fusion suppression factor is found to be in agreement with the data available from the literature. The cross-section ratio of CF/TF and ICF/TF show opposite behavior, the former decreases while the latter increases as the energy is lowered, which shows the dominance of ICF at below barrier energies. We have also studied the correlation of the ICF cross-sections with the non-capture breakup (NCBU) cross-sections as a function of energy, which shows that the NCBU is more significant than ICF at below barrier energies.

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Probing transfer to unbound states of the ejectile with weakly bound 7Li on 93Nb

The two-step process of transfer followed by breakup is explored by measuring a rather complete set of exclusive data for reaction channels populating states in the ejectile continua of the $^7$Li+$^{93}$Nb system at energies close to the Coulomb barrier. The cross sections for $α+α$ events from one proton pickup were found to be smaller than those for $α+d$ events from one neutron stripping and $α+t$ events from direct breakup of $^7$Li. Coupled channels Born approximation and continuum discretized coupled channels calculations describe the data well and support the conclusion that the $α+d$ and $α+α$ events are produced by direct transfer to unbound states of the ejectile.

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Evolution of fusion hindrance for asymmetric systems at deep sub barrier energies

Measurements of fusion cross-sections of 7Li and 12C with 198Pt at deep sub-barrier energies are reported to unravel the role of the entrance channel in the occurrence of fusion hindrance. The onset of fusion hindrance has been clearly observed in 12C + 198Pt system but not in 7Li + 198Pt system, within the measured energy range. Emergence of the hindrance, moving from lighter (6,7Li) to heavier (12C,16O) projectiles is explained employing a model that considers a gradual transition from a sudden to adiabatic regime at low energies. The model calculation reveals a weak effect of the damping of coupling to collective motion for the present systems as compared to that obtained for systems with heavier projectiles.

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Fission barrier, damping of shell correction and neutron emission in the fission of A$\sim$200

Decay of $^{210}$Po compound nucleus formed in light and heavy-ion induced fusion reactions has been analyzed simultaneously using a consistent prescription for fission barrier and nuclear level density incorporating shell correction and its damping with excitation energy. Good description of all the excitation functions have been achieved with a fission barrier of 21.9 $\pm$ 0.2 MeV. For this barrier height, the predicted statistical pre-fission neutrons in heavy-ion fusion-fission are much smaller than the experimental values, implying the presence of dynamical neutrons due to dissipation even at these low excitation energies ($\sim$ 50~MeV) in the mass region A $\sim$ 200. When only heavy-ion induced fission excitation functions and the pre-fission neutron multiplicities are included in the fits, the deduced best fit fission barrier depends on the assumed fission delay time during which dynamical neutrons can be emitted. A fission delay of (0.8 $\pm$ 0.1 )$\times 10^{-19}$ s has been estimated corresponding to the above fission barrier height assuming that the entire excess neutrons over and above the statistical model predictions are due to the dynamics. The present observation has implication on the study of fission time scale/ nuclear viscosity using neutron emission as a probe.

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Understanding fusion and its suppression for the $^{9}$Be projectile with different targets

The role of the breakup process and one neutron stripping on the near barrier fusion are investigated for the weakly bound projectile $^{9}$Be on $^{28}$Si, $^{89}$Y, $^{124}$Sn, $^{144}$Sm and $^{208}$Pb targets. Continuum-discretized coupled channels (CDCC) calculations for the breakup with a $^{8}$Be + n model of the $^{9}$Be nucleus and coupled reactions channels (CRC) calculations for the one neutron stripping to several single particle states in the target are performed for these systems. A good description of the experimental fusion cross sections above the Coulomb barrier is obtained from the CDCC-CRC calculations for all the systems. The calculated incomplete fusion probabilities for different target systems are found to be consistent with the systematic behaviour of the complete fusion suppression factors as a function of target atomic mass, obtained from the experimental data.

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Nuclear temperatures from the evaporation fragment spectra and observed anomalies

The extreme back-angle evaporation spectra of alpha, lithium, beryllium, boron and carbon from different compound nuclei near A=100 (EX=76-210 MeV) have been compared with the predictions of standard statistical model codes such as 'CASCADE' and 'GEMINI'. It was found that the shapes of the alpha spectra agree well with the predictions of the statistical models. However the spectra of lithium, beryllium, boron and carbon show significantly gentler slopes implying higher temperature of the residual nuclei, even though the spectra satisfy all other empirical criteria of statistical emissions. The observed slope anomaly was found to be largest for lithium and decreases at higher excitation energy. These results could not be understood by adjusting the parameters of the statistical models or from reaction dynamics and might require examining the statistical model from a quantum mechanical perspective.

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Exploring the breakup and transfer coupling effects in 9Be elastic scattering

Two cluster structures of 9Be namely, 5He+4He and 8Be+n have been considered for its breakup to describe the available data on elastic scattering for 9Be projectile with 28Si, 64Zn and 144Sm targets. The results of these calculations suggest that the breakup coupling effects are significant for 5He+4He cluster model at above the barrier energies, while they are dominant at relatively lower energies for 8Be+n model. The addition of one neutron stripping channel in the 8Be+n model gives an overall good description of the elastic data for all the systems considered. The couplings generated by breakup in 8Be+n model have different behaviour than the coupling effects obtained within the 5He+4He model, the former being more prominent at lower energies and for the heavier target systems. The behaviour of extracted dynamic polarisation potentials (DPP) generated due to breakup and one neutron transfer couplings have been investigated.

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Role of the cluster structure of $^7$Li in the dynamics of fragment capture

Exclusive measurements of prompt $γ$-rays from the heavy-residues with various light charged particles in the $^7$Li + $^{198}$Pt system, at an energy near the Coulomb barrier (E/$V_b$ $\sim$ 1.6) are reported. Recent dynamic classical trajectory calculations, constrained by the measured fusion, $α$ and $t$ capture cross-sections have been used to explain the excitation energy dependence of the residue cross-sections. These calculations distinctly illustrate a two step process, breakup followed by fusion in case of the capture of $t$ and $α$ clusters; whereas for $^{6}$He + $p$ and $^{5}$He + $d$ configurations, massive transfer is inferred to be the dominant mechanism. The present work clearly demonstrates the role played by the cluster structures of $^7$Li in understanding the reaction dynamics at energies around the Coulomb barrier.

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Total cross sections for neutron-nucleus scattering

Systematics of neutron scattering cross sections on various materials for neutron energies up to several hundred MeV are important for ADSS applications. Ramsauer model is well known and widely applied to understand systematics of neutron nucleus total cross sections. In this work, we examined the role of nuclear effective radius parameter (r$_0$) on Ramsauer model fits of neutron total cross sections. We performed Ramsauer model global analysis of the experimental neutron total cross sections reported by W. P. Abfalterer, F. B. Bateman, {\it et. al.,}, from 20MeV to 550MeV for nuclei ranging from Be to U . The global fit functions which can fit total cross section data over periodic table are provided along with the required global set of parameters. The global fits predict within $\pm 8%$ deviation to data, showing the scope for improvement. It has been observed that a finer adjustment of r$_0$ parameter alone can give very good Ramsauer model description of neutron total scattering data within $\pm 4%$ deviation. The required r$_0$ values for Ramsauer model fits are shown as a function of nuclear mass number and an empirical formula is suggested for r$_0$ values as a function of mass number. In optical model approach for neutron scattering, we have modified the real part of Koning-Deleroche potentails to fit the neutron total cross sections using SCAT2 code. The modified potentails have a different energy dependence beyond 200MeV of neutron energy and fit the total cross sections from Al to Pb.

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Sub- and above barrier fusion of loosely bound $^6$Li with $^{28}$Si

Fusion excitation functions are measured for the system $^6$Li+$^{28}$Si using the characteristic $γ$-ray method, encompassing both the sub-barrier and above barrier regions, viz., $E_{lab}$= 7-24 MeV. Two separate experiments were performed, one for the above barrier region ($E_{lab}$= 11-24 MeV) and another for the below barrier region ($E_{lab}$= 7-10 MeV). The results were compared with our previously measured fusion cross section for the $^7$Li+$^{28}$Si system. We observed enhancement of fusion cross section at sub-barrier regions for both $^6$Li and $^7$Li, but yield was substantially larger for $^6$Li. However, for well above barrier regions, similar type of suppression was identified for both the systems.

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Sub-barrier fusion excitation for the system $^7$Li+$^{28}$Si

The sub-barrier fusion excitation functions are measured for the first time for the system $^7$Li +$^{28}$Si by the characteristic $γ$-ray method in the energy range $E_{lab}$= 7-11.5 MeV. The results show an enhancement, below the barrier, by about a factor of two when compared with the one-dimensional barrier penetration (1D BPM) model. Introduction of coupling with the rotational 2$^{+}$ state (1.779MeV) of the target improves the fit somewhat, but still an enhancement of about 25-40% remains.

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