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S. Kawasaki

Publications and source records attributed to S. Kawasaki.

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Evidence for ferromagnetic spin-pairing superconductivity in UGe$_2$: A $^{73}$Ge-NQR study under pressure

We report that a novel type of superconducting order parameter has been realized in the ferromagnetic states in UGe$_2$ via $^{73}$Ge nuclear-quadrupole-resonance (NQR) experiments performed under pressure ($P$). Measurements of the nuclear spin-lattice relaxation rate $(1/T_1)$ have revealed an unconventional nature of superconductivity such that the up-spin band is gapped with line nodes, but the down-spin band remains gapless at the Fermi level. This result is consistent with that of a ferromagnetic spin-pairing model in which Cooper pairs are formed among ferromagnetically polarized electrons. The present experiment has shed new light on a possible origin of ferromagnetic superconductivity, which is mediated by ferromagnetic spin-density fluctuations relevant to the first-order transition inside the ferromagnetic states.

cond-mat.supr-con↗

Evidence for unconventional superconducting fluctuations in heavy-fermion compound CeNi2Ge2

We present evidence for unconventional superconducting fluctuations in a heavy-fermion compound CeNi$_2$Ge$_2$. The temperature dependence of the $^{73}$Ge nuclear-spin-lattice-relaxation rate $1/T_1$ indicates the development of magnetic correlations and the formation of a Fermi-liquid state at temperatures lower than $T_{\rm FL}=0.4$ K, where $1/T_1T$ is constant. The resistance and $1/T_1T$ measured on an as-grown sample decrease below $T_{\rm c}^{\rm onset} = 0.2$ K and $T_{\rm c}^{\rm NQR} = 0.1$ K, respectively; these are indicative of the onset of superconductivity. However, after annealing the sample to improve its quality, these superconducting signatures disappear. These results are consistent with the emergence of unconventional superconducting fluctuations in close proximity to a quantum critical point from the superconducting to the normal phase in CeNi$_2$Ge$_2$.

cond-mat.str-el↗

Evidence for Uniform Coexistence of Ferromagnetism and Unconventional Superconductivity in UGe_2: A ^73Ge-NQR Study under Pressure

We report on the itinerant ferromagnetic superconductor UGe_2 through ^73Ge-NQR measurements under pressure (P). The P dependence of the NQR spectrum signals a first-order transition from the low-temperature (T) and low-P ferromagnetic phase (FM2) to high-T and high-P one (FM1) around a critical pressure of P_x ~ 1.2 GPa. The superconductivity exhibiting a maximum value of T_sc=0.7 K at P_x ~ 1.2 GPa, was found to take place in connection with the P-induced first-order transition. The nuclear spin-lattice relaxation rate 1/T_1 has probed the ferromagnetic transition, exhibiting a peak at the Curie temperature as well as a decrease without the coherence peak below T_sc. These results reveal the uniformly coexistent phase of ferromagnetism and unconventional superconductivity with a line-node gap. We remark on an intimate interplay between the onset of superconductivity and the underlying electronic state for the ferromagnetic phases.

cond-mat.supr-con↗

Unconventional Superconductivity in Heavy Fermion Systems

We review the studies on the emergent phases of superconductvity and magnetism in the $f$-electron derived heavy-fermion (HF) systems by means of the nuclear-quadrupole-resonance (NQR) under pressure. These studies have unraveled a rich variety of the phenomena in the ground state of HF systems. In this article, we highlight the novel phase diagrams of magnetism and unconventional superconductivity (SC) in CeCu$_2$Si$_2$, HF antiferromagnets CeRhIn$_5$, and CeIn$_3$. A new light is shed on the difference and common features on the interplay between magnetism and SC on the magnetic criticality.

cond-mat.str-el↗

Ion acceleration during internal magnetic reconnection events in TST-2

Characteristics of ion acceleration in the internal magnetic reconnection events (IRE) have been studied by means of a neutral particle energy analyzer (NPA) in Tokyo Spherical Tokamak (TST-2). The major and minor radii are 0.38 m and 0.25m, respectively. The magnetic field strength is 0.3T and the maximum plasma current is up to 140 kA. The electron and ion temperatures are 0.4-0.5 keV and 0.1 keV, respectively and the electron density is ~1x1019 m-3. The NPA can be scanned toroidally from q = 74&deg; (cw) to q = 114&deg; (ccw), where q = 90&deg; corresponds to the perpendicular sightline. The direction of the plasma current is cw. The NPA signals are digitized at every 50 ms. The NPA is calibrated in the energy range of 0.1 keV < E < 8.4 keV. When the IRE occurs, it is observed that the plasma current increases by ~ 20% and the loop voltage drops from 0.6 V to-5 V for ~ 0.1 ms. The enhanced charge exchange flux is observed by more than one order of magnitude at ~ 1 keV for this reconnection phase. The ion temperature increases by 80 eV at IREs. The angle q dependence of increment of Ti shows that DTi (q = 74&deg;) is higher than that for q = 114&deg;. This observation suggests that an ion is accelerated initially in the direction of magnetic field lines. The time evolution of the ion distribution function is simulated with a Fokker-Planck code taking into account the electric field effects.

physics.plasm-ph↗

Estimation of Power Balance in Steady State LHCD Discharges on TRIAM-1M

On TRIAM-1M, a long duration discharge for more than 5 h was achieved successfully by fully non-inductive lower hybrid current drive. Heat load distribution to the plasma facing components (PFCs) in the 5 h discharge was investigated by using calorimetric measurements. The injected RF power was coincident with the total amount of heat load to PFCs estimated by calorimetric measurement. The power balance including the portion of direct loss power of fast electron, heat flux due to the charge exchange process was able to be estimated in this long duration discharge.

physics.plasm-ph↗

Transport barrier formation by LHCD on TRIAM-1M

Internal transport barrier (ITB) has been obtained in full lower hybrid current driven (LHCD) plasmas on a superconducting tokamak, TRIMA-1M (R=0.84m, a x b=0.12mx0.18m, BT<8T). The formation of ITB depends on the current density profile, j(r), varied by the power deposition of the lower hybrid (LH). The plasma with ITB can be maintained by the LH power deposited around the foot point of ITB up to 25 sec, which corresponds to more than 100 times of current diffusion time, $τ$L/R. ITB is terminated by the reduction of current drive efficiency caused by metal impurities accumulation. In some condition, self-organized slow sawtooth oscillations (SSSO) of plasma current, density, temperature, and so on with the period comparable to the current diffusion time have been also observed during ITB discharge. The oscillation has the capability of particle exhaust, as the result, it may play an role in the avoidance of the impurity accumulation and the dilution in the future steady state fusion plasma with ITB, as the edge-localized mode in H-mode.

physics.plasm-ph↗

Novel superconductivity on the magnetic criticality in heavy-fermion systems : a systematic study of NQR under pressure

We report the discovery of exotic superconductivity (SC) and novel magnetism in heavy-fermion (HF) compounds, CeCu$_2$Si$_2$, CeRhIn$_5$ and CeIn$_3$ through nuclear-quadrupole-resonance (NQR) measurements under pressure ($P$). The exotic SC in a homogeneous CeCu$_2$Si$_2$ revealed antiferromagnetic critical fluctuations at the border to antiferromagnetism (AFM) or marginal AFM. The uniform mixed phase of SC and AFM in CeCu$_2$(Si$_{1-x}$Ge$_x$)$_2$ emerges on a microscopic level, once a tiny amount of 1%Ge($x=0.01$) is substituted for Si to expand its lattice. The application of minute pressure ($P\sim 0.19$ GPa) suppresses the sudden emergence of the AFM caused by doping Ge. The persistence of the low-lying magnetic excitations at temperatures lower than $T_c$ and $T_N$ is ascribed due to the uniform mixed phase of SC and AFM. Likewise, the $P$-induced HF superconductor CeRhIn$_5$ coexists with AFM on a microscopic level in $P = 1.5$ - 1.9 GPa. The unconventional gapless nature of SC in the low-lying excitation spectrum emerges due to the uniform mixed phase of AFM and SC. By contrast, in CeIn$_3$, we propose that the magnetic excitations such as spin-density fluctuations induced by the first-order phase transition from the AFM to the paramagnetism (PM) might mediate attractive interaction to form the Cooper pairs in the novel phase of AFM.

cond-mat.str-el↗

Exotic superconductivity in the coexistent phase of antiferromagnetism and superconductivity in CeCu2(Si0.98Ge0.02)2: A Cu-NQR study under hydrostatic pressure

We report a pressure ($P$) effect on CeCu$_2$(Si$_{0.98}$Ge$_{0.02}$)$_2$ where an antiferromagnetic (AFM) order at $T_N \sim$ 0.75 K coexists with superconductivity below $T_c \sim$ 0.4 K\@. At pressures exceeding $P = 0.19$ GPa, the AFM order is suppressed, which demonstrates that the sudden emergence of AFM order due to the Ge doping is ascribed to the intrinsic lattice expansion. The exotic superconductivity at $P = 0$ GPa is found to evolve into a typical heavy-fermion one with a line-node gap above $P = 0.91$ GPa\@. We highlight that the anomalous enhancement in nuclear spin-lattice relaxation rate $1/T_1$ that follows a $T_1T$ = const. behavior well below $T_c$ at $P$ = 0 GPa is characterized by the persistence of low-lying magnetic excitations, which may be inherent to the coexistent state of antiferromagnetism and superconductivity.

cond-mat.str-el↗

Gapless Magnetic and Quasiparticle Excitations due to the Coexistence of Antiferromagnetism and Superconductivity in CeRhIn$_5$ : A study of $^{115}$In-NQR under Pressure

We report systematic measurements of ac-susceptibility, nuclear-quadrupole-resonance spectrum, and nuclear-spin-lattice-relaxation time ($T_1$) on the pressure ($P$)- induced heavy-fermion (HF) superconductor CeRhIn$_5$. The temperature ($T$) dependence of $1/T_1$ at $P$ = 1.6 GPa has revealed that antiferromagnetism (AFM) and superconductivity (SC) coexist microscopically, exhibiting the respective transition at $T_N = 2.8$ K and $T^{MF}_c$ = 0.9 K. It is demonstrated that SC does not yield any trace of gap opening in low-lying excitations below $T_c^{onset} = 2$ K, but $T_c^{MF} = 0.9$ K, followed by a $T_1T$ = const law. These results point to the unconventional characteristics of SC coexisting with AFM. We highlight that both of the results deserve theoretical work on the gapless nature in low-lying excitation spectrum due to the coexistence of AFM and SC and the lack of the mean-field regime below $T_c^{onset} = 2$ K.

cond-mat.str-el↗

Anisotropic spin fluctuations in heavy-fermion superconductor CeCoIn5: In-NQR and Co-NMR studies

We report In-NQR and Co-NMR experiments of CeCoIn$_5$ that undergoes a superconducting transition with a record high $T_{\rm c}$ = 2.3 K to date among heavy-fermion superconductors. At zero magnetic field, an anomalous temperature ($T$) dependence of nuclear spin-lattice relaxation rate $1/T_1$ of $^{115}$In is explained by the relation $1/T_1\propto T\cdotχ_Q(T)^{3/4}$ based on the anisotropic spin-fluctuations model in case of the proximity to an antiferromagnetic (AFM) quantum critical point (QCP). The novel behavior of $1/T_1\sim T^{1/4}$ over a wide $T$ range of $T_{\rm c} < T < 40$ K arises because the staggered susceptibility almost follows the Curie law $χ_Q(T)\propto 1/(T+θ)$ with $θ= 0.6$ K and hence $1/T_1\propto T/(T+0.6)^{3/4}\sim T^{1/4}$ for $θ< T$. We highlight that the behavior $1/T_1\sim T^{1/4}$ is due to the proximity to the anisotropic AFM QCP relevant with its layered structure, and is not associated with the AFM QCP for isotropic 3D systems. We have also found that the AFM spin fluctuations in CeCoIn$_5$ are suppressed by small magnetic field so that $θ=0.6$ K at $H$=0 increases to $θ= 2.5$ K at $H$ = 1.1 T, reinforcing that CeCoIn$_5$ is closely located at the QCP.

cond-mat.str-el↗

Coexistence of Antiferromagnetism and Superconductivity near the Quantum Criticality in Heavy Fermion Compound CeRhIn$_5$

We report a study on the interplay between antiferromagnetism (AFM) and superconductivity (SC) in a heavy-fermion compound CeRhIn$_5$ under pressure $P=1.75$ GPa. The onset of the magnetic order is evidenced from a clear split of $^{115}$In-NQR spectrum due to the spontaneous internal field below the Néel temperature $T_N=2.5$ K. Simultaneously, bulk SC below $T_c=2.0$ K is demonstrated by the observation of the Meissner diamagnetism signal whose size is the same as in the exclusively superconducting phase. These results indicate that the AFM coexists homogeneously with the SC at a microscopic level.

cond-mat.str-el↗

^{115}In-NQR evidence for unconventional superconductivity in CeIn_3 under pressure

We report evidence for unconventional superconductivity in CeIn_3 at a pressure P = 2.65 GPa above critical pressure (P_c ~ 2.5 GPa) revealed by the measurements of nuclear-spin-lattice-relaxation time (T_1) and ac-susceptibility (ac-chi). Both the measurements of T_1 and ac-chi have pointed to a superconducting transition at T_c = 95 mK, which is much lower than an onset temperature T_{onset} = 0.15 K at zero resistance. The temperature dependence of 1/T_1 shows no coherence peak just below T_c, indicative of an unconventional nature for the superconductivity induced in CeIn_3.

cond-mat.str-el↗

Different routes to charge disproportionation in perovskites-type Fe oxides

Iron perovskites CaFeO_3 and La_{0.33}Sr_{0.67}FeO_3 show charge disproportionation, resulting in charge-ordered states with Fe^{3+}:Fe^{5+} =1:1 and =2:1, respectively. We have made photoemission and unrestricted Hartree-Fock band-structure calculation of CaFeO_3 and compared it with La_{0.33}Sr_{0.67}FeO_3. With decreasing temperature, a gradual decrease of the spectral weight near the Fermi level occurred in CaFeO_3 as in La_{0.33}Sr_{0.67}FeO_3 although lattice distortion occurs only in CaFeO_3. Hartree-Fock calculations have indicated that both the breathing and tilting distortions are necessary to induce the charge disproportionation in CaFeO_3, while no lattice distortion is necessary for the charge disproportionation in La_{0.33}Sr_{0.67}FeO_3.

cond-mat.str-el↗

Coexistence of antiferromagnetism and superconductivity in heavy-fermions systems

We report the novel pressure(P)-temperature(T) phase diagrams of antiferromagnetism (AF) and superconductivity (SC) in CeRhIn$_5$, CeIn$_3$ and CeCu$_2$Si$_2$ revealed by the NQR measurement. In the itinerant helical magnet CeRhIn$_5$, we found that the Néel temperature $T_N$ is reduced at $P \geq$ 1.23 GPa with an emergent pseudogap behavior. The coexistence of AF and SC is found in a narrow P range of 1.63 - 1.75 GPa, followed by the onset of SC with line-node gap over a wide P window 2.1 - 5 GPa. In CeIn$_3$, the localized magnetic character is robust against the application of pressure up to $P \sim$ 1.9 GPa, beyond which the system evolves into an itinerant regime in which the resistive superconducting phase emerges. We discuss the relationship between the phase diagram and the magnetic fluctuations. In CeCu$_2$Si$_2$, the SC and AF coexist on a microscopic level once its lattice parameter is expanded. We remark that the underlying marginal antiferromagnetic state is due to collective magnetic excitations in the superconducting state in CeCu$_2$Si$_2$. An interplay between AF and SC is discussed on the SO(5) scenario that unifies AF and SC. We suggest that the SC and AF in CeCu$_2$Si$_2$ have a common mechanism.

cond-mat.str-el↗

Pressure-Temperature Phase Diagram of Antiferromagnetism and Superconductivity in CeRhIn5 and CeIn3 : In-NQR Study under Pressure

We report the novel pressure($P$) - temperature($T$) phase diagram of antiferromagnetism and superconductivity in CeRhIn$_5$ and CeIn$_3$ revealed by the $^{115}$In nuclear-spin-lattice-relaxation ($T_1$) measurement. In the itinerant magnet CeRhIn$_5$, we found that the Néel temperature $T_N$ is reduced at $P \geq$ 1.23 GPa with an emergent pseudogap behavior. In CeIn$_3$, the localized magnetic character is robust against the application of pressure up to $P \sim$ 1.9 GPa, beyond which the system evolves into an itinerant regime in which the resistive superconducting phase emerges. We discuss the relationship between the phase diagram and the magnetic fluctuations.

cond-mat.str-el↗

Unique Spin Dynamics and Unconventional Superconductivity in the Layered Heavy Fermion Compound CeIrIn_5:NQR Evidence

We report measurements of the ^{115}In nuclear spin-lattice relaxation rate (1/T_1) between T=0.09 K and 100 K in the new heavy fermion (HF) compound CeIrIn_5. At 0.4 K < T < 100 K, 1/T_1 is strongly T-dependent, which indicates that CeIrIn_5 is much more itinerant than known Ce-based HFs. We find that 1/T_1T, subtracting that for LaIrIn_5, follows a 1/(T+θ)^{3/4} variation with θ=8 K. We argue that this novel feature points to anisotropic, due to a layered crystal structure, spin fluctuations near a magnetic ordering. The bulk superconductivity sets in at 0.40 K below which the coherence peak is absent and 1/T_1 follows a T^3 variation, which suggests unconventional superconductivity with line-node gap.

cond-mat.supr-con↗

Pressure-induced anomalous magnetism and unconventional superconductivity in CeRhIn5 : 115In-NQR Study under Pressure

We report $^{115}$In nuclear-quadrupole-resonance (NQR) measurements of the pressure($P$)-induced superconductor CeRhIn$_5$ in the antiferromagnetic (AF) and superconducting (SC) states. In the AF region, the internal field $H_{int}$ at the In site is substantially reduced from $H_{int}=1.75$ kOe at P=0 to 0.39 kOe at $P=1.23$ GPa, while the Néel temperature slightly changes with increasing $P$. This suggests that either the size in the ordered moment $M_{Q}(P)$ or the angle $θ(P)$ between the direction of $M_{Q}(P)$ and the tetragonal $c$ axis is extrapolated to zero at $P^*=1.6 \pm 0.1$ GPa at which a bulk SC transition is no longer emergent. In the SC state at $P=2.1$ GPa, the nuclear spin-lattice relaxation rate $^{115}(1/T_1)$ has revealed a $T^3$ dependence without the coherence peak just below $T_c$, giving evidence for the unconventional superconductivity. The dimensionality of the magnetic flutuations in the normal state are also discussed.

cond-mat.str-el↗