arXiv subjects

S. Kolkowitz

Publications and source records attributed to S. Kolkowitz.

14 recordsLinked to original sources

arXiv2025

Laser cooling and qubit measurements on a forbidden transition in neutral Cs atoms

We experimentally demonstrate background-free, hyperfine-level-selective measurements of individual Cs atoms by simultaneous cooling to $5.3~\mu\rm K$ and imaging on the $6s_{1/2}\rightarrow 5d_{5/2}$ electric-quadrupole transition. We achieve hyperfine resolved detection with fidelity 0.9993(4) and atom retention of 0.9954(5), limited primarily by vacuum lifetime. Performing state measurements in a 3D cooling configuration enables repeated low loss measurements. A theoretical analysis of an extension of the demonstrated approach based on quenching of the excited state with an auxiliary field, identifies parameters for hyperfine-resolved measurements with a projected fidelity of $\sim 0.9995 $ in $\sim 60~\mu\rm s$.

quant-ph↗

arXiv2023

A physically motivated analytical expression for the temperature dependence of the zero-field splitting of the nitrogen-vacancy center in diamond

The temperature dependence of the zero-field splitting (ZFS) between the $|m_{s}=0\rangle$ and $|m_{s}=\pm 1\rangle$ levels of the nitrogen-vacancy (NV) center's electronic ground-state spin triplet can be used as a robust nanoscale thermometer in a broad range of environments. However, despite numerous measurements of this dependence in different temperature ranges, to our knowledge no analytical expression has been put forward that captures the scaling of the ZFS of the NV center across all relevant temperatures. Here we present a simple, analytical, and physically motivated expression for the temperature dependence of the NV center's ZFS that matches all experimental observations, in which the ZFS shifts in proportion to the occupation numbers of two representative phonon modes. In contrast to prior models our expression does not diverge outside the regions of fitting. We show that our model quantitatively matches experimental measurements of the ZFS from 15 to 500 K in single NV centers in ultra-pure bulk diamond, and we compare our model and measurements to prior models and experimental data.

cond-mat.mes-hall↗

arXiv2022

Temperature-dependent spin-lattice relaxation of the nitrogen-vacancy spin triplet in diamond

Spin-lattice relaxation within the nitrogen-vacancy (NV) center's electronic ground-state spin triplet limits its coherence times, and thereby impacts its performance in quantum applications. We report measurements of the relaxation rates on the NV center's $|m_{s}=0\rangle \leftrightarrow |m_{s}=\pm 1\rangle$ and $|m_{s}=-1\rangle \leftrightarrow |m_{s}=+1\rangle$ transitions as a function of temperature from 9 to 474 K in high-purity samples. We show that the temperature dependencies of the rates are reproduced by an ab initio theory of Raman scattering due to second-order spin-phonon interactions, and we discuss the applicability of the theory to other spin systems. Using a novel analytical model based on these results, we suggest that the high-temperature behavior of NV spin-lattice relaxation is dominated by interactions with two groups of quasilocalized phonons centered at 68.2(17) and 167(12) meV.

quant-ph↗

arXiv2022

New Horizons: Scalar and Vector Ultralight Dark Matter

The last decade has seen unprecedented effort in dark matter model building at all mass scales coupled with the design of numerous new detection strategies. Transformative advances in quantum technologies have led to a plethora of new high-precision quantum sensors and dark matter detection strategies for ultralight ($<10\,$eV) bosonic dark matter that can be described by an oscillating classical, largely coherent field. This white paper focuses on searches for wavelike scalar and vector dark matter candidates.

hep-ex↗

arXiv2022

Super-resolution Airy disk microscopy of individual color centers in diamond

Super-resolution imaging techniques enable nanoscale microscopy in fields such as physics, biology, and chemistry. However, many super-resolution techniques require specialized optical components, such as a helical-phase mask. We present a novel technique, Super-resolution Airy disk Microscopy (SAM) that can be used in a standard confocal microscope without any specialized optics. We demonstrate this technique, in combination with ground state depletion, to image and control nitrogen-vacancy (NV) centers in bulk diamond below the diffraction limit. A greater than 14-fold improvement in resolution compared to the diffraction limit is achieved, corresponding to a spatial resolution of 16.9(8) nm for a 1.3 NA microscope with 589 nm light. We make use of our enhanced spatial resolution to control the spins states of individual NV centers separated from each other by less than the diffraction limit, including pairs sharing the same orientation that are indistinguishable with a conventional electron spin resonance measurement.

physics.optics↗

arXiv2022

Analysis of a Cesium lattice optical clock

We propose and analyze a Cesium lattice optical clock (CLOC) which has the potential for high performance and simple operation in a compact form factor using a forbidden optical transition in Cs atoms at 685 nm. Cs atoms are trapped in a 3D optical lattice using a magic trap wavelength of $\lambda_{\textrm m}=803~\textrm nm$. To reduce sensitivity to magnetic fields the atoms are probed on two cycling transitions with equal magnitude, but opposite magnetic shifts. Operation of the clock requires only three diode lasers at 685, 803, 852 nm and is simplified compared to other higher-performance optical clocks that rely on alkaline earth atoms or single trapped ions. Analysis shows a quantum noise limited stability of $8.4\times 10^{-16}/\sqrt\tau$ and the potential for reaching 1 ns timing uncertainty at 1 month with realistic system parameters.

quant-ph↗

arXiv2021

Probing charge dynamics in diamond with an individual color center

Control over the charge states of color centers in solids is necessary in order to fully utilize them in quantum technologies. However, the microscopic charge dynamics of deep defects in wide-bandgap semiconductors are complex, and much remains unknown. Here, we utilize single shot charge state readout of an individual nitrogen-vacancy (NV) center to probe charge dynamics of the surrounding defects in diamond. We show that the NV center charge state can be converted through the capture of holes produced by optical illumination of defects many microns away. With this method, we study the optical charge conversion of silicon-vacancy (SiV) centers and provide evidence that the dark state of the SiV center under optical illumination is SiV2-. These measurements illustrate that charge carrier generation, transport, and capture are important considerations in the design and implementation of quantum devices with color centers, and provide a novel way to probe and control charge dynamics in diamond.

cond-mat.mes-hall↗

arXiv2020

State-dependent phonon-limited spin relaxation of nitrogen-vacancy centers

Understanding the limits to the spin-coherence of the nitrogen-vacancy (NV) center in diamond is vital to realizing the full potential of this quantum system. We show that relaxation on the $|m_{s}=-1\rangle \leftrightarrow |m_{s}=+1\rangle$ transition occurs approximately twice as fast as relaxation on the $|m_{s}=0\rangle \leftrightarrow |m_{s}=\pm 1\rangle$ transitions under ambient conditions in native NVs in high-purity bulk diamond. The rates we observe are independent of NV concentration over four orders of magnitude, indicating they are limited by spin-phonon interactions. We find that the maximum theoretically achievable coherence time for an NV at 295 K is limited to 6.8(2) ms. Finally, we present a theoretical analysis of our results that suggests Orbach-like relaxation from quasilocalized phonons or contributions due to higher-order terms in the spin-phonon Hamiltonian are the dominant mechanism behind $|m_{s}=-1\rangle \leftrightarrow |m_{s}=+1\rangle$ relaxation, motivating future measurements of the temperature dependence of this relaxation rate.

cond-mat.mes-hall↗

arXiv2019

New Technologies for Discovery

For the field of high energy physics to continue to have a bright future, priority within the field must be given to investments in the development of both evolutionary and transformational detector development that is coordinated across the national laboratories and with the university community, international partners and other disciplines. While the fundamental science questions addressed by high energy physics have never been more compelling, there is acute awareness of the challenging budgetary and technical constraints when scaling current technologies. Furthermore, many technologies are reaching their sensitivity limit and new approaches need to be developed to overcome the currently irreducible technological challenges. This situation is unfolding against a backdrop of declining funding for instrumentation, both at the national laboratories and in particular at the universities. This trend has to be reversed for the country to continue to play a leadership role in particle physics, especially in this most promising era of imminent new discoveries that could finally break the hugely successful, but limited, Standard Model of fundamental particle interactions. In this challenging environment it is essential that the community invest anew in instrumentation and optimize the use of the available resources to develop new innovative, cost-effective instrumentation, as this is our best hope to successfully accomplish the mission of high energy physics. This report summarizes the current status of instrumentation for high energy physics, the challenges and needs of future experiments and indicates high priority research areas.

physics.ins-det↗

arXiv2017

Dynamics of interacting fermions under spin-orbit coupling in an optical lattice clock

Quantum statistics and symmetrization dictate that identical fermions do not interact via s-wave collisions. However, in the presence of spin-orbit coupling (SOC), fermions prepared in identical internal states with distinct momenta become distinguishable. The resulting strongly interacting system can exhibit exotic topological and pairing behaviors, many of which are yet to be observed in condensed matter systems. Ultracold atomic gases offer a promising pathway for simulating these rich phenomena. Two recent experiments reported the observation of single atom SOC in optical lattice clocks (OLCs) based on alkaline-earth atoms. In these works encoding the effective spin degree of freedom in the long-lived electronic clock states significantly reduced the detrimental effects of spontaneous emission and heating that have thus far hindered the study of interacting SOC with alkali atoms. Beyond first studies of interacting SOC with alkali atoms in a bulk gas and with two particles in a lattice, here we enter a new regime of many-body interacting SOC in an OLC. Using clock spectroscopy, we observe the precession of the collective magnetization and the emergence of spin locking effects arising from an interplay between p-wave and SOC-induced exchange interactions. The many-body dynamics are well captured by a collective XXZ spin model, which describes a broad class of condensed matter systems ranging from superconductors to quantum magnets. Furthermore, our work will aid in the design of next-generation OLCs by offering a route for avoiding the observed large density shifts caused by SOC-induced exchange interactions.

physics.atom-ph↗

arXiv2016

Spin-orbit coupled fermions in an optical lattice clock

Engineered spin-orbit coupling (SOC) in cold atom systems can aid in the study of novel synthetic materials and complex condensed matter phenomena. Despite great advances, alkali atom SOC systems are hindered by heating from spontaneous emission, which limits the observation of many-body effects, motivating research into potential alternatives. Here we demonstrate that SOC can be engineered to occur naturally in a one-dimensional fermionic 87Sr optical lattice clock (OLC). In contrast to previous SOC experiments, in this work the SOC is both generated and probed using a direct ultra-narrow optical clock transition between two electronic orbital states. We use clock spectroscopy to prepare lattice band populations, internal electronic states, and quasimomenta, as well as to produce SOC dynamics. The exceptionally long lifetime of the excited clock state (160 s) eliminates decoherence and atom loss from spontaneous emission at all relevant experimental timescales, allowing subsequent momentum- and spin-resolved in situ probing of the SOC band structure and eigenstates. We utilize these capabilities to study Bloch oscillations, spin-momentum locking, and Van Hove singularities in the transition density of states. Our results lay the groundwork for the use of OLCs to probe novel SOC phases of matter.

cond-mat.quant-gas↗

arXiv2012

Measuring mechanical motion with a single spin

We study theoretically the measurement of a mechanical oscillator using a single two level system as a detector. In a recent experiment, we used a single electronic spin associated with a nitrogen vacancy center in diamond to probe the thermal motion of a magnetized cantilever at room temperature {Kolkowitz et al., Science 335, 1603 (2012)}. Here, we present a detailed analysis of the sensitivity limits of this technique, as well as the possibility to measure the zero point motion of the oscillator. Further, we discuss the issue of measurement backaction in sequential measurements and find that although backaction heating can occur, it does not prohibit the detection of zero point motion. Throughout the paper we focus on the experimental implementation of a nitrogen vacancy center coupled to a magnetic cantilever; however, our results are applicable to a wide class of spin-oscillator systems. Implications for preparation of nonclassical states of a mechanical oscillator are also discussed.

cond-mat.mes-hall↗

arXiv2008

Systematic study of trace radioactive impurities in candidate construction materials for EXO-200

The Enriched Xenon Observatory (EXO) will search for double beta decays of 136Xe. We report the results of a systematic study of trace concentrations of radioactive impurities in a wide range of raw materials and finished parts considered for use in the construction of EXO-200, the first stage of the EXO experimental program. Analysis techniques employed, and described here, include direct gamma counting, alpha counting, neutron activation analysis, and high-sensitivity mass spectrometry.

physics.ins-det↗

arXiv2008

A microfabricated sensor for thin dielectric layers

We describe a sensor for the measurement of thin dielectric layers capable of operation in a variety of environments. The sensor is obtained by microfabricating a capacitor with interleaved aluminum fingers, exposed to the dielectric to be measured. In particular, the device can measure thin layers of solid frozen from a liquid or gaseous medium. Sensitivity to single atomic layers is achievable in many configurations and, by utilizing fast, high sensitivity capacitance read out in a feedback system onto environmental parameters, coatings of few layers can be dynamically maintained. We discuss the design, read out and calibration of several versions of the device optimized in different ways. We specifically dwell on the case in which atomically thin solid xenon layers are grown and stabilized, in cryogenic conditions, from a liquid xenon bath.

physics.gen-ph↗