arXiv subjects

S. Kubono

Publications and source records attributed to S. Kubono.

At least 19 recordsLinked to original sources

arXiv2026

High-Precision Mass Measurements of Proton-Rich Rh, Pd, Cd isotopes in the vicinity of 100Sn and Impact on X-Ray Burst and Supernova Nucleosynthesis

Using the ZeroDegree multi-reflection time-of-flight mass spectrograph of the CRISMASS project at RIKEN Radioactive Isotope Beam Factory, we performed high-precision mass measurements of proton-rich nuclei near the doubly magic nucleus 100Sn, achieving uncertainties on the order of 10 keV. The masses of 91Rh, 92Pd, and 96Cd were determined for the first time with high precision, and the accuracy of several additional masses was substantially improved. Incorporating the new data into X-ray burst simulations significantly reduces the abundance uncertainties in the $A$ = 90-100 region, shifting the reaction flow toward $A$ = 90 production and suppressing the synthesis of heavier nuclei. Further investigation of the $\nu p$-process indicates that 99Rh plays a significant role in the reaction flow within the mass region studied. These high-precision mass measurements refine the mass surface near 100Sn and provide critical constraints on models of proton-rich nucleosynthesis.

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arXiv2025

Precise measurement of the $\gamma$-decay probability of the Hoyle state with a new triple coincidence-detection method

We measured the $\gamma$-decay probability of the Hoyle state with a new method of triple coincidence detection of a scattered $\alpha$ particle, a recoil $\rm ^{12}C$ nucleus, and a $\gamma$ ray in inelastic alpha scattering on $\rm ^{12}C$. This method successfully enabled a low-background measurement and a precise determination of the $\gamma$-decay probability of the Hoyle state as $\Gamma_\mathrm{\gamma}/\Gamma=[4.00 \pm 0.22 \mathrm{(sta.)} \pm 0.18 \mathrm{(sys.)}]\times10^{-4}$, which is consistent with the previous literature value. Therefore, we concluded that the literature value can be reliably used in the study of nucleosynthesis in the universe.

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arXiv2025

The beta decay of Tz=-2 64Se and its descendants: the T=2 isobaric multiplet

In this paper we present our results on the decay of 64Se. It is the heaviest Tz=-2 nucleus that both beta decays and has a stable mirror partner Tz=+2, thus allowing comparison with charge exchange reaction studies. The beta decays of 64Se and its descendants were studied at the RIKEN Nishina Center (Tokyo, Japan) following their production in the fragmentation of 78Kr on a beryllium target. Beta-delayed gamma-ray and particle radiation was identified for each of the nuclei in the decay chain allowing us to obtain decay schemes for 64Se, 64As, and 63Ge. Thus new excited states could be found for the descendant nuclei, including the interesting case of the N=Z nucleus 64Ge. Furthermore we observed for the first time the beta-delayed proton emission of 64Se and 64As. Based on these results we obtained proton branching ratios of 48.0(9)% in 64Se decay and 4.4(1)% in 64As decay. We obtained a half-life value of 22.5(6) ms for 64Se decay and half-lives slightly more precise than those in the literature for each nucleus involved in the decay chain. Using our results on the excited levels of 64As and the mass excess in the literature for 63Ge we obtained -39588(50) keV for the mass excess of 64As. Then based on the IMME we obtained the mass excess of -27429(88) keV for 64Se by extrapolation. The mirror process of 64Se beta decay, the charge exchange reaction 64Zn(3He,t)64Ga, has already been measured allowing us to study the mirror symmetry through the comparison of the weak force (beta decay) and strong force (charge exchange reaction). An interpretation of the decay schemes based on the idea of the Anti Analogue State is proposed.

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arXiv2025

Precision mass measurements around ${}^{84}$Mo rule out ZrNb cycle formation in the rapid proton-capture process at type I X-ray bursts

The rapid proton-capture ($rp$-) process is one of the primary, explosive thermonuclear burning processes that drive type I X-ray bursts. A possible termination of the $rp$-process at around ${}^{84}$Mo was previously suggested by the formation of a ZrNb cycle. We report here precision mass measurements at around ${}^{84}$Mo, which have concluded the possibility of the cycle. The experiment was conducted using the multi-reflection time-of-flight spectrograph at RIKEN RI Beam Factory, and the masses of ${}^{79}$Y, ${}^{83}$Nb, ${}^{84}$Mo, ${}^{88}$Ru, and an isomer in ${}^{78}$Y were measured. For ${}^{84}$Mo, and ${}^{88}$Ru, and the isomeric state of ${}^{78}$Y, their masses are experimentally determined for the first time with uncertainties of $\delta m \approx 20~{\rm keV/c^2}$. The mass precision of ${}^{79}$Y and ${}^{83}$Nb is improved to $13~{\rm keV/c^2}$ and $9.6~{\rm keV/c^2}$, respectively. The new $\alpha$-separation energy of ${}^{84}$Mo, 1.434(83) MeV, unambiguously rules out the possibility of forming the ZrNb cycle. The X-ray burst simulation with the new masses shows that our measurements effectively remove the large final abundance uncertainties in the $A=80-90$ mass region. The new mass values improve the prediction power for the composition of the nuclear ashes in X-ray bursts.

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arXiv2025

Impact of newly measured $\beta$\nobreakdash-delayed neutron emitters around \myisoSimp{78}{Ni} on light element nucleosynthesis in the neutrino-wind following a neutron star merger

Neutron emission probabilities and half-lives of 37 beta-delayed neutron emitters from 75Ni to 92Br were measured at the RIKEN Nishina Center in Japan, including 11 one-neutron and 13 two-neutron emission probabilities and 6 half-lives measured for the first time, which supersede theoretical estimates. These nuclei lie in the path of the weak r-process occurring in neutrino-driven winds from the accretion disk formed after the merger of two neutron stars, synthesizing elements in the A~80 abundance peak. The presence of such elements dominates the accompanying kilonova emission over the first few days and has been identified in the AT2017gfo event, associated with the gravitational wave detection GW170817. Abundance calculations based on over 17000 simulated trajectories describing the evolution of matter properties in the merger outflows show that the new data lead to an increase of 50-70 percent in the abundance of Y, Zr, Nb, and Mo. This enhancement is large compared to the scatter of relative abundances observed in old very metal-poor stars and is therefore significant in the comparison with other possible astrophysical processes contributing to light-element production. These results underline the importance of including experimental decay data for very neutron-rich beta-delayed neutron emitters into r-process models.

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arXiv2024

Isospin breaking in the $^{71}$Kr and $^{71}$Br mirror system

Isospin symmetry is a fundamental concept in nuclear physics. Even though isospin symmetry is partially broken, it holds approximately for most nuclear systems, which makes exceptions very interesting from the nuclear structure perspective. In this framework, it is expected that the spins and parities of the ground states of mirror nuclei should be the same, in particular for the simplest systems where a proton is exchanged with a neutron or vice versa. In this work, we present evidence that this assumption is broken in the mirror pair $^{71}$Br and $^{71}$Kr system. Our conclusions are based on a high-statistics $\beta$ decay study of $^{71}$Kr and on state-of-the-art shell model calculations. In our work, we also found evidence of a new state in $^{70}$Se, populated in the $\beta$-delayed proton emission process which can be interpreted as the long sought coexisting 0$^+$ state.

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arXiv2022

Deep underground laboratory measurement of $^{13}$C($α$,$n$)$^{16}$O in the Gamow windows of the $s$- and $i$-processes

The $^{13}$C($α$,$n$)$^{16}$O reaction is the main neutron source for the slow-neutron-capture (s-) process in Asymptotic Giant Branch stars and for the intermediate (i-) process. Direct measurements at astrophysical energies in above-ground laboratories are hindered by the extremely small cross sections and vast cosmic-ray induced background. We performed the first consistent direct measurement in the range of $E_{\rm c.m.}=$0.24 MeV to 1.9 MeV using the accelerators at the China Jinping Underground Laboratory (CJPL) and Sichuan University. Our measurement covers almost the entire i-process Gamow window in which the large uncertainty of the previous experiments has been reduced from 60\% down to 15\%, eliminates the large systematic uncertainty in the extrapolation arising from the inconsistency of existing data sets, and provides a more reliable reaction rate for the studies of the s- and i-processes along with the first direct determination of the alpha strength for the near-threshold state.

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arXiv2022

Beta decay of the very neutron-deficient $^{60}$Ge and $^{62}$Ge nuclei

We report here the results of a study of the $β$ decay of the proton-rich Ge isotopes, $^{60}$Ge and $^{62}$Ge, produced in an experiment at the RIKEN Nishina Center. We have improved our knowledge of the half-lives of $^{62}$Ge (73.5(1) ms), $^{60}$Ge (25.0(3) ms) and its daughter nucleus, $^{60}$Ga (69.4(2) ms). We measured individual $β$-delayed proton and $γ$ emissions and their related branching ratios. Decay schemes and absolute Fermi and Gamow-Teller transition strengths have been determined. The mass excesses of the nuclei under study have been deduced. A total $β$-delayed proton-emission branching ratio of 67(3)% has been obtained for $^{60}$Ge. New information has been obtained on the energy levels populated in $^{60}$Ga and on the 1/2$^-$ excited state in the $βp$ daughter $^{59}$Zn. We extracted a ground state to ground state feeding of 85.3(3)% for the decay of $^{62}$Ge. Eight new $γ$ lines have been added to the de-excitation of levels populated in the $^{62}$Ga daughter.

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arXiv2021

Advancement of Photospheric Radius Expansion and Clocked Type-I X-Ray Burst Models with the New $^{22}$Mg$(α,p)^{25}$Al Reaction Rate Determined at Gamow Energy

We report the first (in)elastic scattering measurement of $^{25}\mathrm{Al}+p$ with the capability to select and measure in a broad energy range the proton resonances in $^{26}$Si contributing to the $^{22}$Mg$(α,p)$ reaction at type I x-ray burst energies. We measured spin-parities of four resonances above the $α$ threshold of $^{26}$Si that are found to strongly impact the $^{22}$Mg$(α,p)$ rate. The new rate advances a state-of-the-art model to remarkably reproduce light curves of the GS 1826$-$24 clocked burster with mean deviation $<9$ % and permits us to discover a strong correlation between the He abundance in the accreting envelope of photospheric radius expansion burster and the dominance of $^{22}$Mg$(α,p)$ branch.

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arXiv2021

Persistence of the ${Z=28}$ shell gap in ${A=75}$ isobars: Identification of a possible ${(1/2^-)}$ $μ$s isomer in ${^{75}}$Co and $β$ decay to ${^{75}}$Ni

Background: The evolution of shell structure around doubly magic exotic nuclei is of great interest in nuclear physics and astrophysics. In the `southwest' region of $^{78}$Ni, the development of deformation might trigger a major shift in our understanding of explosive nucleosynthesis. To this end, new spectroscopic information on key close-lying nuclei is very valuable. Purpose: We intend to measure the isomeric and $β$ decay of $^{75}$Co, with one-proton and two-neutron holes relative to $^{78}$Ni, to access new nuclear structure information in $^{75}$Co and its $β$-decay daughters $^{75}$Ni and $^{74}$Ni. Methods: The nucleus $^{75}$Co is produced in relativistic in-flight fission reactions of $^{238}$U at the Radioactive Ion Beam Factory in the RIKEN Nishina Center. Its isomeric and $β$ decay are studied exploiting the BigRIPS and EURICA setups. Results: We obtain partial $β$-decay spectra for $^{75}$Ni and $^{74}$Ni, and report a new isomeric transition in $^{75}$Co. The energy [$E_γ=1914(2)$ keV] and half-life [$t_{1/2}=13(6)$ $μ$s] of the delayed $γ$ ray lend support for the existence of a $J^π=(1/2^-)$ isomeric state at 1914(2) keV. A comparison with PFSDG-U shell-model calculations provides a good account for the observed states in $^{75}$Ni, but the first calculated $1/2^-$ level in $^{75}$Co, a prolate $K=1/2$ state, is predicted about 1 MeV below the observed $(1/2^-)$ level. Conclusions: The spherical-like structure of the lowest-lying excited states in $^{75}$Ni is proved. In the case of $^{75}$Co, the results suggest that the dominance of the spherical configurations over the deformed ones might be stronger than expected below $^{78}$Ni. Further experimental efforts to discern the nature of the $J^π=(1/2^-)$ isomer are necessary.

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arXiv2020

Mass measurements for $T_{z}=-2$ $fp$-shell nuclei $^{40}$Ti, $^{44}$Cr, $^{46}$Mn, $^{48}$Fe, $^{50}$Co and $^{52}$Ni

By using isochronous mass spectrometry (IMS) at the experimental cooler storage ring CSRe, masses of short-lived $^{44}$Cr, $^{46}$Mn, $^{48}$Fe, $^{50}$Co and $^{52}$Ni were measured for the first time and the precision of the mass of $^{40}$Ti was improved by a factor of about 2. Relative precisions of $δm/m=(1-2)\times$10$^{-6}$ have been achieved. Details of the measurements and data analysis are described. The obtained masses are compared with the Atomic-Mass Evaluation 2016 (AME$^{\prime}$16) and with theoretical model predictions. The new mass data enable us to extract the higher order coefficients, $d$ and $e$, of the quartic form of the isobaric multiplet mass equation (IMME) for the $fp$-shell isospin quintets. Unexpectedly large $d$- and $e$-values for $A=44$ quintet are found. By re-visiting the previous experimental data on $β$-delayed protons from $^{44}$Cr decay, it is suggested that the observed anomaly could be due to the misidentification of the $T=2$, $J^π=0^{+}$ isobaric analog state (IAS) in $^{44}$V.

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arXiv2019

Constraining the $^{12}$C+$^{12}$C astrophysical S-factors with the $^{12}$C+$^{13}$C measurements at very low energies

We use an underground counting lab with an extremely low background to perform an activity measurement for the $^{12}$C+$^{13}$C system with energies down to $E\rm_{c.m.}$=2.323 MeV, at which the $^{12}$C($^{13}$C,$p$)$^{24}$Na cross section is found to be 0.22(7) nb. The $^{12}$C+$^{13}$C fusion cross section is derived with a statistical model calibrated using experimental data. Our new result of the $^{12}$C+$^{13}$C fusion cross section is the first decisive evidence in the carbon isotope systems which rules out the existence of the astrophysical S-factor maximum predicted by the phenomenological hindrance model, while confirming the rising trend of the S-factor towards lower energies predicted by other models, such as CC-M3Y+Rep, DC-TDHF, KNS, SPP and ESW. After normalizing the model predictions with our data, a more reliable upper limit is established for the $^{12}$C+$^{12}$C fusion cross sections at stellar energies.

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arXiv2019

Masses of ground and isomeric states of $^{101}$In and configuration-dependent shell evolution in odd-$A$ indium isotopes

We report first precision mass measurements of the $1/2^-$ isomeric and $9/2^+$ ground states of $^{101}$In. The determined isomeric excitation energy continues a smooth trend of odd-$A$ indium isotopes up to the immediate vicinity of $N=50$ magic number. This trend can be confirmed by dedicated shell model calculations only if the neutron configuration mixing is considered. We find that the single particle energies are different for different states of the same isotope. The presented configuration-dependent shell evolution, type II shell evolution, in odd-$A$ nuclei is discussed for the first time. Our results will facilitate future studies of single-particle neutron states.

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arXiv2018

Isochronous mass measurements of $T_z=-1$ $fp$-shell nuclei from projectile fragmentation of $^{58}$Ni

Atomic masses of seven $T_z=-1$, $fp$-shell nuclei from $^{44}$V to $^{56}$Cu and two low-lying isomers, $^{44m}$V ($J^π=6^+$) and $^{52m}$Co ($J^π=2^+$), have been measured with relative precisions of $1-4\times 10^{-7}$ with Isochronous Mass Spectrometry (IMS) at CSRe. The masses of $^{56}$Cu, $^{52g,52m}$Co, and $^{44m}$V were measured for the first time in this experiment. The Mass Excesses ($ME^{\prime}$s) of $^{44}$V, $^{48}$Mn, $^{50}$Fe, and $^{54}$Ni are determined with an order of magnitude improved precision compared to the literature values. $^{52g,52m}$Co and $^{56}$Cu are found to be $370$~keV and $400$~keV more bound, respectively, while $^{44g,44m}$V are $\sim 300$~keV less bound than the extrapolations in the Atomic-Mass Evaluation 2012 (AME$^{\prime}$12). The masses of the four $T_z=-1/2$ nuclei $^{45}$V, $^{47}$Cr, $^{49}$Mn, and $^{51}$Fe are re-determined to be in agreement, within the experimental errors, with the recent JYFLTRAP measurements or with the previous IMS measurements in CSRe. Details of the measurements and data analysis are described, and the impact of the new $ME$ values on different aspects in nuclear structure are investigated and discussed.

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arXiv2018

Possible determination of high-lying single particle components with (p,d) reactions

A detailed feasibility study on deducing the high-lying single-particle components (HLSPCs), which are important but used to be ignored, in the ground and low-lying excited states of even-even light nuclei is performed by analyses of $(p,d)$ reactions with \nuc{12}{C}, \nuc{24}{Mg}, \nuc{28}{Si}, and \nuc{40}{Ca} targets at 51.93 MeV. Coupled reaction channels (CRC) analyses have been made for $(p,d)$ transitions to the $j$-forbidden excited states in \nuc{11}{C} (${\tfrac{5}{2}}^-$, 4.32 MeV), \nuc{23}{Mg} (${\tfrac{7}{2}}^+$, 2.05 MeV), \nuc{27}{Si} (${\tfrac{7}{2}}^+$, 2.16 MeV) and \nuc{39}{Ca} (${\tfrac{9}{2}}^-$, 3.64 MeV), including the major allowed transition components together with direct components of HLSPCs. Spectroscopic amplitudes of the HLSPCs are deduced by fitting the angular distributions of the ground and the $j$-forbidden excited states simultaneously. The present analysis demonstrates for the first time that information about HLSPCs in atomic nuclei can be obtained from analysis of $(p,d)$ reactions.

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arXiv2018

Commissioning of the BRIKEN detector for the measurement of very exotic beta-delayed neutron emitters

A new detection system has been installed at the RIKEN Nishina Center (Japan) to investigate decay properties of very neutron-rich nuclei. The setup consists of three main parts: a moderated neutron counter, a detection system sensitive to the implantation and decay of radioactive ions, and gamma-ray detectors. We describe here the setup, the commissioning experiment and some selected results demonstrating its performance for the measurement of half-lives and beta-delayed neutron emission probabilities. The methodology followed in the analysis of the data is described in detail. Particular emphasis is placed on the correction of the accidental neutron background.

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arXiv2018

The Masses of the $T_z=-3/2$ Nuclei $^{27}$P and $^{29}$S

Isochronous mass spectrometry has been applied in the storage ring CSRe to measure the masses of the $T_z=-3/2$ nuclei $^{27}$P and $^{29}$S. The new mass excess value $ME$($^{29}$S) $=-3094(13)$~keV is 66(52)~keV larger than the result of the previous $^{32}$S($^3$He,$^{6}$He)$^{29}$S reaction measurement in 1973 and a factor of 3.8 more precise. The new result for $^{29}$S, together with those of the $T=3/2$ isobaric analog states (IAS) in $^{29}$P, $^{29}$Si, and $^{29}$Al, fit well into the quadratic form of the Isobaric Multiplet Mass Equation IMME. The mass excess of $^{27}$P has been remeasured to be $ME(^{27}$P$)=-685(42)$ keV. By analyzing the linear and quadratic coefficients of the IMME in the $T_z=-3/2$ $sd$-shell nuclei, it was found that the ratio of the Coulomb radius parameters is $R\approx0.96$ and is nearly the same for all $T=3/2$ isospin multiplets. Such a nearly constant $R$-value, apparently valid for the entire light mass region with $A>9$, can be used to set stringent constraints on the isovector and isotensor components of the isospin non-conserving forces in theoretical calculations.

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arXiv2018

Mass Measurements of Neutron-Deficient Y, Zr, and Nb Isotopes and Their Impact on $rp$ and $νp$ Nucleosynthesis Processes

Using isochronous mass spectrometry at the experimental storage ring CSRe in Lanzhou, the masses of $^{82}$Zr and $^{84}$Nb were measured for the first time with an uncertainty of $\sim 10$ keV, and the masses of $^{79}$Y, $^{81}$Zr, and $^{83}$Nb were re-determined with a higher precision. %The latter differ significantly from their literature values. The latter are significantly less bound than their literature values. Our new and accurate masses remove the irregularities of the mass surface in this region of the nuclear chart. Our results do not support the predicted island of pronounced low $α$ separation energies for neutron-deficient Mo and Tc isotopes, making the formation of Zr-Nb cycle in the $rp$-process unlikely. The new proton separation energy of $^{83}$Nb was determined to be 490(400)~keV smaller than that in the Atomic Mass Evaluation 2012. This partly removes the overproduction of the $p$-nucleus $^{84}$Sr relative to the neutron-deficient molybdenum isotopes in the previous $νp$-process simulations.

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