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S. Lalkovski

Publications and source records attributed to S. Lalkovski.

14 recordsLinked to original sources

Probing the quantum phase transition around $N\approx60$ via mass measurements of technetium isotopes

The masses of neutron-rich $^{104-106}$Tc isotopes were measured using the JYFLTRAP double Penning trap and found to deviate from the Atomic Mass Evaluation 2020 by $-79(25)$, $40(12)$ and $94(41)$ keV, respectively. In the case of $^{105,106}$Tc, the updated $Q_\beta$ values are in agreement with a previous JYFLTRAP measurement, disagreeing with the values from the mass evaluation. The new mass values result in a more linear trend in two-neutron separation energies indicating that technetium ($Z=43$) isotopes around $N \approx 60$ are not a part of the island of shape coexistence around $^{100}$Zr$_{60}$.

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Shape evolution in even-mass $^{98-104}$Zr isotopes via lifetime measurements using the $γγ$-coincidence technique

The Zirconium (Z = 40) isotopic chain has attracted interest for more than four decades. The abrupt lowering of the energy of the first $2^+$ state and the increase in the transition strength B(E2; $2_1^\rightarrow 0_1^+$ going from $^{98}$Zr to $^{100}$Zr has been the first example of "quantum phase transition" in nuclear shapes, which has few equivalents in the nuclear chart. Although a multitude of experiments have been performed to measure nuclear properties related to nuclear shapes and collectivity in the region, none of the measured lifetimes were obtained using the Recoil Distance Doppler Shift method in the $γγ$-coincidence mode where a gate on the direct feeding transition of the state of interest allows a strict control of systematical errors. This work reports the results of lifetime measurements for the first yrast excited states in $^{98-104}$Zr carried out to extract reduced transition probabilities. The new lifetime values in $γγ$-coincidence and $γ$-single mode are compared with the results of former experiments. Recent predictions of the Interacting Boson Model with Configuration Mixing, the Symmetry Conserving Configuration Mixing model based on the Hartree-Fock-Bogoliubov approach and the Monte Carlo Shell Model are presented and compared with the experimental data.

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Is Seniority a Partial Dynamic Symmetry in the First $νg_{9/2}$ Shell?

The low-lying structures of the midshell $νg_{9/2}$ Ni isotopes $^{72}$Ni and $^{74}$Ni have been investigated at the RIBF facility in RIKEN within the EURICA collaboration. Previously unobserved low-lying states were accessed for the first time following $β$ decay of the mother nuclei $^{72}$Co and $^{74}$Co. As a result, we provide a complete picture in terms of the seniority scheme up to the first $(8^+)$ levels for both nuclei. The experimental results are compared to shell-model calculations in order to define to what extent the seniority quantum number is preserved in the first neutron $g_{9/2}$ shell. We find that the disappearance of the seniority isomerism in the $(8^+_1)$ states can be explained by a lowering of the seniority-four $(6^+)$ levels as predicted years ago. For $^{74}$Ni, the internal de-excitation pattern of the newly observed $(6^+_2)$ state supports a restoration of the normal seniority ordering up to spin $J=4$. This property, unexplained by the shell-model calculations, is in agreement with a dominance of the single-particle spherical regime near $^{78}$Ni.

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Structure of the neutron mid-shell nuclei $^{111,113}_{\quad \ 47}$Ag$_{64,66}$

$^{111}$Ag and $^{113}$Ag were produced in induced fission reaction, where yrast and near-yrast states were populated. To interpret the new data the Interacting Boson-Fermion model was used. A good agreement with the experimental data is achieved, suggesting that the two Ag nuclei have a well developed collectivity, superimposed on $πg_{9/2}^{-3}$ excitations previously observed throughout the entire isotopic chain.

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The mutable nature of particle-core excitations with spin in the one-valence-proton nucleus 133Sb

The gamma-ray decay of excited states of the one-valence-proton nucleus 133Sb has been studied using cold-neutron induced fission of 235U and 241Pu targets, during the EXILL campaign at the ILL reactor in Grenoble. By using a highly efficient HPGe array, coincidences between gamma-rays prompt with the fission event and those delayed up to several tens of microseconds were investigated, allowing to observe, for the first time, high-spin excited states above the 16.6 micros isomer. Lifetimes analysis, performed by fast-timing techniques with LaBr3(Ce) scintillators, reveals a difference of almost two orders of magnitude in B(M1) strength for transitions between positive-parity medium-spin yrast states. The data are interpreted by a newly developed microscopic model which takes into account couplings between core excitations (both collective and non-collective) of the doubly magic nucleus 132Sn and the valence proton, using the Skyrme effective interaction in a consistent way. The results point to a fast change in the nature of particle-core excitations with increasing spin.

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Enhanced time response of 1-in. LaBr3(Ce) crystals by leading edge and constant fraction techniques

We have characterized in depth the time response of three detectors equipped with cylindrical LaBr$_{3}$ (Ce) crystals with dimensions of 1-in. in height and 1-in. in diameter, and having nominal Ce doping concentration of 5%, 8% and 10%. Measurements were performed at $^{60}$Co and $^{22}$Na γ-ray energies against a fast BaF$_{2}$ reference detector. The time resolution was optimized by the choice of the photomultiplier bias voltage and the fine tuning of the parameters of the constant fraction discriminator, namely the zero-crossing and the external delay. We report here on the optimal time resolution of the three crystals. It is observed that timing properties are influenced by the amount of Ce doping and the crystal homogeneity. For the crystal with 8% of Ce doping the use of the ORTEC 935 CFD at very shorts delays in addition to the Hamamatsu R9779 PMT has made it possible to improve the LaBr$_{3}$(Ce) time resolution from the best literature value at 60Co photon energies to below 100 ps.

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Co-existing structures in 105Ru

New positive-parity states, having a band-like structure, were observed in 105Ru. The nucleus was produced in induced fission reaction and the prompt gamma-rays, emitted from the fragments, were detected by the EUROBALL III multi-detector array. The partial scheme of excited 105Ru levels is analyzed within the Triaxial-Rotor-plus-Particle approach.

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Core-coupled states and split proton-neutron quasi-particle multiplets in 122-126Ag

Neutron-rich silver isotopes were populated in the fragmentation of a 136Xe beam and the relativistic fission of 238U. The fragments were mass analyzed with the GSI Fragment separator and subsequently implanted into a passive stopper. Isomeric transitions were detected by 105 HPGe detectors. Eight isomeric states were observed in 122-126Ag nuclei. The level schemes of 122,123,125Ag were revised and extended with isomeric transitions being observed for the first time. The excited states in the odd-mass silver isotopes are interpreted as core-coupled states. The isomeric states in the even-mass silver isotopes are discussed in the framework of the proton-neutron split multiplets. The results of shell-model calculations, performed for the most neutron-rich silver nuclei are compared to the experimental data.

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Observation of Positive-Parity Bands in $^{109}$Pd and $^{111}$Pd: Enhanced $γ$-Softness

The neutron-rich nuclei $^{109}$Pd and $^{111}$Pd were produced as fission fragments following the $^{30}$Si + $^{168}$Er reaction at 142 MeV. Using the identification based on the coincidences with the complementary fission fragments, the only positive-parity bands observed so far in $^{109}$Pd and $^{111}$Pd emerged from this work. A band, built on top of the 5/2$^+$ ground state exhibiting $ΔI$ = 1 energy-level staggering, was observed in each of these nuclei. Both nuclei of interest, $^{109}$Pd and $^{111}$Pd, are suggested to lie in the transitional region of Pd isotopes of maximum $γ$-softness. The ground states of both nuclei are predicted by TRS calculations to be extremely $γ$-soft with shallow triaxial minima. The first crossing in the new bands is proposed to be due to an alignment of $h^2_{11/2}$ neutrons.

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Fast-timing measurements in 95,96Mo

Half-lives of the 19/2+ and 21/2+ states in 95Mo and of the 8+ and 10+ states in 96Mo were measured. Matrix elements for yrast transitions in 95Mo and 96Mo are discussed.

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Single-particle isomeric states in 121Pd and 117Ru

Neutron-rich nuclei were populated in a relativistic fission of 238U. Gamma-rays with energies of 135 keV and 184 keV were associated with two isomeric states in 121Pd and 117Ru. Half-lives of 0.63(5) microseconds and 2.0(3) micrisecondss were deduced and the isomeric states were interpreted in terms of deformed single-particle states.

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In-beam fast-timing measurements in 103,105,107Cd

Fast-timing measurements were performed recently in the region of the medium-mass 103,105,107Cd isotopes, produced in fusion evaporation reactions. Emitted gamma-rays were detected by eight HPGe and five LaBr3:Ce detectors working in coincidence. Results on new and re-evaluated half-lives are discussed within a systematic of transition rates. The $7/2_1^+$ states in 103,105,107Cd are interpreted as arising from a single-particle excitation. The half-life analysis of the $11/2_1^-$ states in 103,105,107Cd shows no change in the single-particle transition strength as a function of the neutron number.

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IBM-1 calculations towards the neutron-rich nucleus $^{106}$Zr

The neutron-rich N=66 isotonic and A=106 isobaric chains, covering regions with varying types of collectivity, are interpreted in the framework of the interacting boson model. Level energies and electric quadrupole transition probabilities are compared with available experimental information. The calculations for the known nuclei in the two chains are extrapolated towards the neutron-rich nucleus $^{106}$Zr.

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Ground-gamma band mixing and evolution of collectivity in even-even neutron-rich nuclei with 40<Z<50

We propose an extended band mixing formalism capable of describing the ground-gamma band interaction in a wide range of collective spectra beyond the regions of well deformed nuclei. On this basis we explain the staggering effects observed in the gamma bands of Mo, Ru and Pd nuclei providing a consistent interpretation of new experimental data in the neutron rich region. As a result the systematic behavior of the odd-even staggering effect and some general characteristics of the spectrum such as the mutual disposition of the bands, the interaction strength and the band structures is explained as the manifestation of respective changes in collective dynamics of the system.

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