arXiv subjects

S. Li

Publications and source records attributed to S. Li.

At least 145 records · Page 8Linked to original sources

arXiv2021

Correlation Driven Transient Hole Dynamics Resolved in Space and Time in the Isopropanol Molecule

The possibility of suddenly ionized molecules undergoing extremely fast electron hole dynamics prior to significant structural change was first recognized more than 20 years ago and termed charge migration. The accurate probing of ultrafast electron hole dynamics requires measurements that have both sufficient temporal resolution and can detect the localization of a specific hole within the molecule. We report an investigation of the dynamics of inner valence hole states in isopropanol where we use an x-ray pump/x-ray probe experiment, with site and state-specific probing of a transient hole state localized near the oxygen atom in the molecule, together with an ab initio theoretical treatment. We record the signature of transient hole dynamics and make the first observation of dynamics driven by frustrated Auger-Meitner transitions. We verify that the hole lifetime is consistent with our theoretical prediction. This state-specific measurement paves the way to widespread application for observations of transient hole dynamics localized in space and time in molecules and thus to charge transfer phenomena that are fundamental in chemical and material physics.

physics.chem-ph↗

arXiv2021

Inherited Weak Topological Insulator Signatures in Topological Hourglass Semimetal Nb3XTe6 (X = Si, Ge)

Using spin-resolved and angle-resolved photoemission spectroscopy and first-principles calculations, we have identified bulk band inversion and spin polarized surface state evolved from a weak topological insulator (TI) phase in van der Waals materials Nb3XTe6 (X = Si, Ge). The fingerprints of weak TI homologically emerge with hourglass fermions, as multi nodal chains composed by the same pair of valence and conduction bands gapped by spin orbit coupling. The novel topological state, with a pair of valence and conduction bands encoding both weak TI and hourglass semimetal nature, is essential and guaranteed by nonsymmorphic symmetry. It is distinct from TIs studied previously based on band inversions without symmetry protections.

cond-mat.mtrl-sci↗

arXiv2021

A Constraint on Primordial $B$-Modes from the First Flight of the SPIDER Balloon-Borne Telescope

We present the first linear polarization measurements from the 2015 long-duration balloon flight of SPIDER, an experiment designed to map the polarization of the cosmic microwave background (CMB) on degree angular scales. Results from these measurements include maps and angular power spectra from observations of 4.8% of the sky at 95 and 150 GHz, along with the results of internal consistency tests on these data. While the polarized CMB anisotropy from primordial density perturbations is the dominant signal in this region of sky, Galactic dust emission is also detected with high significance; Galactic synchrotron emission is found to be negligible in the SPIDER bands. We employ two independent foreground-removal techniques in order to explore the sensitivity of the cosmological result to the assumptions made by each. The primary method uses a dust template derived from Planck data to subtract the Galactic dust signal. A second approach, employing a joint analysis of SPIDER and Planck data in the harmonic domain, assumes a modified-blackbody model for the spectral energy distribution of the dust with no constraint on its spatial morphology. Using a likelihood that jointly samples the template amplitude and $r$ parameter space, we derive 95% upper limits on the primordial tensor-to-scalar ratio from Feldman-Cousins and Bayesian constructions, finding $r<0.11$ and $r<0.19$, respectively. Roughly half the uncertainty in $r$ derives from noise associated with the template subtraction. New data at 280 GHz from SPIDER's second flight will complement the Planck polarization maps, providing powerful measurements of the polarized Galactic dust emission.

astro-ph.CO↗

arXiv2021

Event Reconstruction in a Liquid Xenon Time Projection Chamber with an Optically-Open Field Cage

nEXO is a proposed tonne-scale neutrinoless double beta decay ($0νββ$) experiment using liquid ${}^{136}Xe$ (LXe) in a Time Projection Chamber (TPC) to read out ionization and scintillation signals. Between the field cage and the LXe vessel, a layer of LXe ("skin" LXe) is present, where no ionization signal is collected. Only scintillation photons are detected, owing to the lack of optical barrier around the field cage. In this work, we show that the light originating in the skin LXe region can be used to improve background discrimination by 5% over previous published estimates. This improvement comes from two elements. First, a fraction of the $γ$-ray background is removed by identifying light from interactions with an energy deposition in the skin LXe. Second, background from ${}^{222}Rn$ dissolved in the skin LXe can be efficiently rejected by tagging the $α$ decay in the ${}^{214}Bi-{}^{214}Po$ chain in the skin LXe.

physics.ins-det↗

arXiv2021

Interplay of anionic quasi-atom and interstitial point defects in electrides: abnormal interstice occupation and colossal charge state of point defects in dense FCC-lithium

Electrides are an emerging class of materials with highly-localized electrons in the interstices of a crystal that behave as anions. The presence of these unusual interstitial quasi-atom (ISQ) electrons leads to interesting physical and chemical properties, and wide potential applications for this new class of materials. Crystal defects often have a crucial influence on the properties of materials. Introducing impurities has been proved to be an effective approach to improve the properties of a material and to expand its applications. However, the interactions between the anionic ISQs and the crystal defects in electrides are as yet unknown. Here, dense FCC-Li was employed as an archetype to explore the interplay between anionic ISQs and interstitial impurity atoms in this electride. This work reveals a strong coupling among the interstitial impurity atoms, the ISQs, and the matrix Li atoms near to the defects. This complex interplay and interaction mainly manifest as the unexpected tetrahedral interstitial occupation of impurity atoms and the enhancement of electron localization in the interstices. Moreover, the Be impurity occupying the octahedral interstice shows the highest negative charge state (Be8-) discovered thus far. These results demonstrate the rich chemistry and physics of this emerging material, and provide a new basis for enriching their variants for a wide range of applications.

cond-mat.mtrl-sci↗

arXiv2021

Measurement of the Ar(e,e$^\prime$ p) and Ti(e,e$^\prime$ p) cross sections in Jefferson Lab Hall A

The E12-14-012 experiment, performed in Jefferson Lab Hall A, has collected exclusive electron-scattering data (e,e$^\prime$p) in parallel kinematics using natural argon and natural titanium targets. Here, we report the first results of the analysis of the data set corresponding to beam energy of 2,222 MeV, electron scattering angle 21.5 deg, and proton emission angle -50 deg. The differential cross sections, measured with $\sim$4% uncertainty, have been studied as a function of missing energy and missing momentum, and compared to the results of Monte Carlo simulations, obtained from a model based on the Distorted Wave Impulse Approximation.

nucl-ex↗

arXiv2021

Ruling out color transparency in quasi-elastic $^{12}$C(e,e'p) up to $Q^2$ of 14.2 (GeV/c)$^2$

Quasielastic $^{12}$C$(e,e'p)$ scattering was measured at space-like 4-momentum transfer squared $Q^2$~=~8, 9.4, 11.4, and 14.2 (GeV/c)$^2$, the highest ever achieved to date. Nuclear transparency for this reaction was extracted by comparing the measured yield to that expected from a plane-wave impulse approximation calculation without any final state interactions. The measured transparency was consistent with no $Q^2$ dependence, up to proton momenta of 8.5~GeV/c, ruling out the quantum chromodynamics effect of color transparency at the measured $Q^2$ scales in exclusive $(e,e'p)$ reactions. These results impose strict constraints on models of color transparency for protons.

nucl-ex↗

arXiv2020

Design and pre-flight performance of SPIDER 280 GHz receivers

In this work we describe upgrades to the Spider balloon-borne telescope in preparation for its second flight, currently planned for December 2021. The Spider instrument is optimized to search for a primordial B-mode polarization signature in the cosmic microwave background at degree angular scales. During its first flight in 2015, Spider mapped ~10% of the sky at 95 and 150 GHz. The payload for the second Antarctic flight will incorporate three new 280 GHz receivers alongside three refurbished 95- and 150 GHz receivers from Spider's first flight. In this work we discuss the design and characterization of these new receivers, which employ over 1500 feedhorn-coupled transition-edge sensors. We describe pre-flight laboratory measurements of detector properties, and the optical performance of completed receivers. These receivers will map a wide area of the sky at 280 GHz, providing new information on polarized Galactic dust emission that will help to separate it from the cosmological signal.

astro-ph.IM↗

arXiv2020

Novel observation of isospin structure of short-range correlations in calcium isotopes

Short Range Correlations (SRCs) have been identified as being responsible for the high momentum tail of the nucleon momentum distribution, n(k). Hard, short-range interactions of nucleon pairs generate the high momentum tail and imprint a universal character on n(k) for all nuclei at large momentum. Triple coincidence experiments have shown a strong dominance of np pairs, but these measurements involve large final state interactions. This paper presents the results from Jefferson Lab experiment E08014 which measured inclusive electron scattering cross-section from Ca isotopes. By comparing the inclusive cross section from 48Ca to 40Ca in a kinematic region dominated by SRCs we provide a new way to study the isospin structure of SRCs.

nucl-ex↗

arXiv2020

Probabilistic teleportation of a quantum dot spin qubit

Electron spin s in semiconductor quantum dot s have been intensively studied for implementing quantum computation and high fidelity single and two qubit operation s have recently been achieved . Quantum teleportation is a three qubit protocol exploiting quantum entanglement and it serv es as a n essential primitive for more sophisticated quantum algorithm s Here, we demonstrate a scheme for quantum teleportation based on direct Bell measurement for a single electron spin qubit in a triple quantum dot utilizing the Pauli exclusion principle to create and detect maximally entangled state s . T he single spin polarization is teleported from the input qubit to the output qubit with a fidelity of 0.9 1 We find this fidelity is primarily limited by singlet triplet mixing which can be improved by optimizing the device parameters Our results may be extended to quantum algorithms with a larger number of se miconductor spin qubit s

cond-mat.mes-hall↗

arXiv2020

Search For Electron-Antineutrinos Associated With Gravitational-Wave Events GW150914, GW151012, GW151226, GW170104, GW170608, GW170814, and GW170817 at Daya Bay

Providing a possible connection between neutrino emission and gravitational-wave (GW) bursts is important to our understanding of the physical processes that occur when black holes or neutron stars merge. In the Daya Bay experiment, using data collected from December 2011 to August 2017, a search has been performed for electron-antineutrino signals coinciding with detected GW events, including GW150914, GW151012, GW151226, GW170104, GW170608, GW170814, and GW170817. We used three time windows of $\mathrm{\pm 10~s}$, $\mathrm{\pm 500~s}$, and $\mathrm{\pm 1000~s}$ relative to the occurrence of the GW events, and a neutrino energy range of 1.8 to 100 MeV to search for correlated neutrino candidates. The detected electron-antineutrino candidates are consistent with the expected background rates for all the three time windows. Assuming monochromatic spectra, we found upper limits (90% confidence level) on electron-antineutrino fluence of $(1.13~-~2.44) \times 10^{11}~\rm{cm^{-2}}$ at 5 MeV to $8.0 \times 10^{7}~\rm{cm^{-2}}$ at 100 MeV for the three time windows. Under the assumption of a Fermi-Dirac spectrum, the upper limits were found to be $(5.4~-~7.0)\times 10^{9}~\rm{cm^{-2}}$ for the three time windows.

astro-ph.HE↗

arXiv2020

Study of muonium emission from laser-ablated silica aerogel

The emission of muonium ($μ^+e^-$) atoms into vacuum from silica aerogel with laser ablation on its surface was studied with various ablation structures at room temperature using the subsurface muon beams at TRIUMF and Japan Proton Accelerator Research Complex (J-PARC). Laser ablation was applied to produce holes or grooves with typical dimensions of a few hundred $μ$m to a few mm, except for some extreme conditions. The measured emission rate tends to be higher for larger fractions of ablation opening and for shallower depths. More than a few ablation structures reach the emission rates similar to the highest achieved in the past measurements. The emission rate is found to be stable at least for a couple of days. Measurements of spin precession amplitudes for the produced muonium atoms and remaining muons in a magnetic field determine a muonium formation fraction of $(65.5 \pm 1.8)$%. The precession of the polarized muonium atoms is also observed clearly in vacuum. A projection of the emission rates measured at TRIUMF to the corresponding rates at J-PARC is demonstrated taking the different beam condition into account reasonably.

physics.ins-det↗

arXiv2020

Cloud-cloud collision as drivers of the chemical complexity in Galactic Centre molecular clouds

G+0.693-0.03 is a quiescent molecular cloud located within the Sagittarius B2 (Sgr B2) star-forming complex. Recent spectral surveys have shown that it represents one of the most prolific repositories of complex organic species in the Galaxy. The origin of such chemical complexity, along with the small-scale physical structure and properties of G+0.693-0.03, remains a mystery. In this paper, we report the study of multiple molecules with interferometric observations in combination with single-dish data in G+0.693-0.03. Despite the lack of detection of continuum source, we find small-scale (0.2 pc) structures within this cloud. The analysis of the molecular emission of typical shock tracers such as SiO, HNCO, and CH$_3$OH unveiled two molecular components, peaking at velocities of 57 and 75 km s$^{-1}$. They are found to be interconnected in both space and velocity. The position-velocity diagrams show features that match with the observational signatures of a cloud-cloud collision. Additionally, we detect three series of class \rom{1} methanol masers known to appear in shocked gas, supporting the cloud-cloud collision scenario. From the maser emission we provide constraints on the gas kinetic temperatures ($\sim$30-150 K) and H$_2$ densities (10$^4$-10$^5$ cm$^{-2}$). These properties are similar to those found for the starburst galaxy NGC253 also using class \rom{1} methanol masers, suggested to be associated with a cloud-cloud collision. We conclude that shocks driven by the possible cloud-cloud collision is likely the most important mechanism responsible for the high level of chemical complexity observed in G+0.693-0.03.

astro-ph.GA↗

arXiv2020

Pattern formation of the three-layer Saffman-Taylor problem in a radial Hele-Shaw cell

The three-layer Saffman-Taylor problem introduces two coupled moving interfaces separating the three fluids. A very recent weakly nonlinear analysis of this problem in a radial Hele-Shaw cell setup has shown that the morphologies of the emerging fingering patterns strongly depend on the initial thickness of the intermediate layer connecting the two interfaces. Here we go beyond the weakly nonlinear regime and explore full nonlinear interfacial dynamics using a spectrally accurate boundary integral method. We quantify the nonlinear instability of both interfaces as the relevant physical parameters (e.g., viscosities and surface tensions) are varied and show that our nonlinear computations are in good agreement with the experimental observations and the weakly nonlinear analysis. Nonlinear simulations reveal that due to the existence of a second interface, the classical highly branched morphologies are replaced by less unstable structures in which finger tip-splitting and finger competition phenomena are evidently restrained as the initial annulus' thickness is reduced. In addition, these novels patterns develop fingers with a series of low-amplitude bumps at their tips, associated with the enhanced growth of high-frequency modes promoted by the increasing coupling strength of interfaces.

physics.flu-dyn↗

arXiv2020

Probing few-body nuclear dynamics via 3H and 3He (e,e'p)pn cross-section measurements

We report the first measurement of the \eep three-body breakup reaction cross sections in helium-3 ($^3$He) and tritium ($^3$H) at large momentum transfer ($\langle Q^2 \rangle \approx 1.9$ (GeV/c)$^2$) and $x_B>1$ kinematics, where the cross section should be sensitive to quasielastic (QE) scattering from single nucleons. The data cover missing momenta $40 \le p_{miss} \le 500$ MeV/c that, in the QE limit with no rescattering, equals the initial momentum of the probed nucleon. The measured cross sections are compared with state-of-the-art ab-initio calculations. Overall good agreement, within $\pm20\%$, is observed between data and calculations for the full $p_{miss}$ range for $^3$H and for $100 \le p_{miss} \le 350$ MeV/c for $^3$He. Including the effects of rescattering of the outgoing nucleon improves agreement with the data at $p_{miss} > 250$ MeV/c and suggests contributions from charge-exchange (SCX) rescattering. The isoscalar sum of $^3$He plus $^3$H, which is largely insensitive to SCX, is described by calculations to within the accuracy of the data over the entire $p_{miss}$ range. This validates current models of the ground state of the three-nucleon system up to very high initial nucleon momenta of $500$ MeV/c.

nucl-ex↗

arXiv2020

Measurement of the scintillation and ionization response of liquid xenon at MeV energies in the EXO-200 experiment

Liquid xenon (LXe) is employed in a number of current and future detectors for rare event searches. We use the EXO-200 experimental data to measure the absolute scintillation and ionization yields generated by $γ$ interactions from $^{228}$Th (2615~keV), $^{226}$Ra (1764~keV) and $^{60}$Co (1332~keV and 1173~keV) calibration sources, over a range of electric fields. The $W$-value that defines the recombination-independent energy scale is measured to be $11.5~\pm~0.5$~(syst.)~$\pm~0.1$~(stat.) eV. These data are also used to measure the recombination fluctuations in the number of electrons and photons produced by the calibration sources at the MeV-scale, which deviate from extrapolations of lower-energy data. Additionally, a semi-empirical model for the energy resolution of the detector is developed, which is used to constrain the recombination efficiency, i.e., the fraction of recombined electrons that result in the emission of a detectable photon. Detailed measurements of the absolute charge and light yields for MeV-scale electron recoils are important for predicting the performance of future neutrinoless double beta decay detectors.

physics.ins-det↗

arXiv2020

Measurement of the Spectral Shape of the beta-decay of 137Xe to the Ground State of 137Cs in EXO-200 and Comparison with Theory

We report on a comparison between the theoretically predicted and experimentally measured spectra of the first-forbidden non-unique $β$-decay transition $^{137}\textrm{Xe}(7/2^-)\to\,^{137}\textrm{Cs}(7/2^+)$. The experimental data were acquired by the EXO-200 experiment during a deployment of an AmBe neutron source. The ultra-low background environment of EXO-200, together with dedicated source deployment and analysis procedures, allowed for collection of a pure sample of the decays, with an estimated signal-to-background ratio of more than 99-to-1 in the energy range from 1075 to 4175 keV. In addition to providing a rare and accurate measurement of the first-forbidden non-unique $β$-decay shape, this work constitutes a novel test of the calculated electron spectral shapes in the context of the reactor antineutrino anomaly and spectral bump.

nucl-ex↗

arXiv2020

Particle Identification Using Boosted Decision Trees in the Semi-Digital Hadronic Calorimeter Prototype

The CALICE Semi-Digital Hadronic CALorimeter (SDHCAL) prototype using Glass Resistive Plate Chambers as a sensitive medium is the first technological prototype of a family of high-granularity calorimeters developed by the CALICE collaboration to equip the experiments of future leptonic colliders. It was exposed to beams of hadrons, electrons and muons several times in the CERN PS and SPS beamlines between 2012 and 2018. We present here a new method of particle identification within the SDHCAL using the Boosted Decision Trees (BDT) method applied to the data collected in 2015. The performance of the method is tested first with Geant4-based simulated events and then on the data collected by the SDHCAL in the energy range between 10 and 80~GeV with 10~GeV energy steps. The BDT method is then used to reject the electrons and muons that contaminate the SPS hadron beams.

physics.ins-det↗