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S. M. Clayton

Publications and source records attributed to S. M. Clayton.

At least 37 records · Page 2Linked to original sources

The neutron electric dipole moment experiment at the Spallation Neutron Source

Novel experimental techniques are required to make the next big leap in neutron electric dipole moment experimental sensitivity, both in terms of statistics and systematic error control. The nEDM experiment at the Spallation Neutron Source (nEDM@SNS) will implement the scheme of Golub & Lamoreaux [Phys. Rep., 237, 1 (1994)]. The unique properties of combining polarized ultracold neutrons, polarized $^3$He, and superfluid $^4$He will be exploited to provide a sensitivity to $\sim 10^{-28}\,e{\rm \,\cdot\, cm}$. Our cryogenic apparatus will deploy two small ($3\,{\rm L}$) measurement cells with a high density of ultracold neutrons produced and spin analyzed in situ. The electric field strength, precession time, magnetic shielding, and detected UCN number will all be enhanced compared to previous room temperature Ramsey measurements. Our $^3$He co-magnetometer offers unique control of systematic effects, in particular the Bloch-Siegert induced false EDM. Furthermore, there will be two distinct measurement modes: free precession and dressed spin. This will provide an important self-check of our results. Following five years of "critical component demonstration," our collaboration transitioned to a "large scale integration" phase in 2018. An overview of our measurement techniques, experimental design, and brief updates are described in these proceedings.

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A boron-coated CCD camera for direct detection of Ultracold Neutrons (UCN)

A new boron-coated CCD camera is described for direct detection of ultracold neutrons (UCN) through the capture reactions $^{10}$B (n,$α$0$γ$)$^7$Li (6%) and $^{10}$B(n,$α$1$γ$)$^7$Li (94%). The experiments, which extend earlier works using a boron-coated ZnS:Ag scintillator, are based on direct detections of the neutron-capture byproducts in silicon. The high position resolution, energy resolution and particle ID performance of a scientific CCD allows for observation and identification of all the byproducts $α$, $^7$Li and $γ$ (electron recoils). A signal-to-noise improvement on the order of 10$^4$ over the indirect method has been achieved. Sub-pixel position resolution of a few microns is demonstrated. The technology can also be used to build UCN detectors with an area on the order of 1 m$^2$. The combination of micrometer scale spatial resolution, few electrons ionization thresholds and large area paves the way to new research avenues including quantum physics of UCN and high-resolution neutron imaging and spectroscopy.

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Monte Carlo Simulations of Trapped Ultracold Neutrons in the UCNτ Experiment

In the UCNτ experiment, ultracold neutrons (UCN) are confined by magnetic fields and the Earth's gravitational field. Field-trapping mitigates the problem of UCN loss on material surfaces, which caused the largest correction in prior neutron experiments using material bottles. However, the neutron dynamics in field traps differ qualitatively from those in material bottles. In the latter case, neutrons bounce off material surfaces with significant diffusivity and the population quickly reaches a static spatial distribution with a density gradient induced by the gravitational potential. In contrast, the field-confined UCN -- whose dynamics can be described by Hamiltonian mechanics -- do not exhibit the stochastic behaviors typical of an ideal gas model as observed in material bottles. In this report, we will describe our efforts to simulate UCN trapping in the UCNτ magneto-gravitational trap. We compare the simulation output to the experimental results to determine the parameters of the neutron detector and the input neutron distribution. The tuned model is then used to understand the phase space evolution of neutrons observed in the UCNτ experiment. We will discuss the implications of chaotic dynamics on controlling the systematic effects, such as spectral cleaning and microphonic heating, for a successful UCN lifetime experiment to reach a 0.01% level of precision.

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Solid deuterium surface degradation at ultracold neutron sources

Solid deuterium (sD_2) is used as an efficient converter to produce ultracold neutrons (UCN). It is known that the sD_2 must be sufficiently cold, of high purity and mostly in its ortho-state in order to guarantee long lifetimes of UCN in the solid from which they are extracted into vacuum. Also the UCN transparency of the bulk sD_2 material must be high because crystal inhomogeneities limit the mean free path for elastic scattering and reduce the extraction efficiency. Observations at the UCN sources at Paul Scherrer Institute and at Los Alamos National Laboratory consistently show a decrease of the UCN yield with time of operation after initial preparation or later treatment (`conditioning') of the sD_2. We show that, in addition to the quality of the bulk sD_2, the quality of its surface is essential. Our observations and simulations support the view that the surface is deteriorating due to a build-up of D_2 frost-layers under pulsed operation which leads to strong albedo reflections of UCN and subsequent loss. We report results of UCN yield measurements, temperature and pressure behavior of deuterium during source operation and conditioning, and UCN transport simulations. This, together with optical observations of sD_2 frost formation on initially transparent sD_2 in offline studies with pulsed heat input at the North Carolina State University UCN source results in a consistent description of the UCN yield decrease.

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Measurement of the neutron lifetime using an asymmetric magneto- gravitational trap and in situ detection

The precise value of the mean neutron lifetime, $τ_n$, plays an important role in nuclear and particle physics and cosmology. It is a key input for predicting the ratio of protons to helium atoms in the primordial universe and is used to search for new physics beyond the Standard Model of particle physics. There is a 3.9 standard deviation discrepancy between $τ_n$ measured by counting the decay rate of free neutrons in a beam (887.7 $\pm$ 2.2 s) and by counting surviving ultracold neutrons stored for different storage times in a material trap (878.5$\pm$0.8 s). The experiment described here eliminates loss mechanisms present in previous trap experiments by levitating polarized ultracold neutrons above the surface of an asymmetric storage trap using a repulsive magnetic field gradient so that the stored neutrons do not interact with material trap walls and neutrons in quasi-stable orbits rapidly exit the trap. As a result of this approach and the use of a new in situ neutron detector, the lifetime reported here (877.7 $\pm$ 0.7 (stat) +0.4/-0.2 (sys) s) is the first modern measurement of $τ_n$ that does not require corrections larger than the quoted uncertainties.

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Search for the Neutron Decay n$\rightarrow$ X+$γ$ where X is a dark matter particle

In a recent paper submitted to Physical Review Letters, Fornal and Grinstein have suggested that the discrepancy between two different methods of neutron lifetime measurements, the beam and bottle methods can be explained by a previously unobserved dark matter decay mode, n$\rightarrow$ X+$γ$ where X is a dark matter particle. We have performed a search for this decay mode over the allowed range of energies of the monoenergetic gamma ray for X to be a dark matter particle. We exclude the possibility of a sufficiently strong branch to explain the lifetime discrepancy with greater than 4 sigma confidence.

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Performance of the upgraded ultracold neutron source at Los Alamos National Laboratory and its implication for a possible neutron electric dipole moment experiment

The ultracold neutron (UCN) source at Los Alamos National Laboratory (LANL), which uses solid deuterium as the UCN converter and is driven by accelerator spallation neutrons, has been successfully operated for over 10 years, providing UCN to various experiments, as the first production UCN source based on the superthermal process. It has recently undergone a major upgrade. This paper describes the design and performance of the upgraded LANL UCN source. Measurements of the cold neutron spectrum and UCN density are presented and compared to Monte Carlo predictions. The source is shown to perform as modeled. The UCN density measured at the exit of the biological shield was $184(32)$ UCN/cm$^3$, a four-fold increase from the highest previously reported. The polarized UCN density stored in an external chamber was measured to be $39(7)$ UCN/cm$^3$, which is sufficient to perform an experiment to search for the nonzero neutron electric dipole moment with a one-standard-deviation sensitivity of $σ(d_n) = 3\times 10^{-27}$ $e\cdot$cm.

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Evaluation of commercial nickel-phosphorus coating for ultracold neutron guides using a pinhole bottling method

We report on the evaluation of commercial electroless nickel phosphorus (NiP) coatings for ultracold neutron (UCN) transport and storage. The material potential of 50~$μ$m thick NiP coatings on stainless steel and aluminum substrates was measured to be $V_F = 213(5.2)$~neV using the time-of-flight spectrometer ASTERIX at the Lujan Center. The loss per bounce probability was measured in pinhole bottling experiments carried out at ultracold neutron sources at Los Alamos Neutron Science Center and the Institut Laue-Langevin. For these tests a new guide coupling design was used to minimize gaps between the guide sections. The observed UCN loss in the bottle was interpreted in terms of an energy independent effective loss per bounce, which is the appropriate model when gaps in the system and upscattering are the dominate loss mechanisms, yielding a loss per bounce of $1.3(1) \times 10^{-4}$. We also present a detailed discussion of the pinhole bottling methodology and an energy dependent analysis of the experimental results.

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Detection System for Neutron $β$ Decay Correlations in the UCNB and Nab experiments

We describe a detection system designed for precise measurements of angular correlations in neutron $β$ decay. The system is based on thick, large area, highly segmented silicon detectors developed in collaboration with Micron Semiconductor, Ltd. The prototype system meets specifications for $β$ electron detection with energy thresholds below 10 keV, energy resolution of $\sim$3 keV FWHM, and rise time of $\sim$50 ns with 19 of the 127 detector pixels instrumented. Using ultracold neutrons at the Los Alamos Neutron Science Center, we have demonstrated the coincident detection of $β$ particles and recoil protons from neutron $β$ decay. The fully instrumented detection system will be implemented in the UCNB and Nab experiments, to determine the neutron $β$ decay parameters $B$, $a$, and $b$.

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A new method for measuring the neutron lifetime using an in situ neutron detector

The neutron lifetime is important in understanding the production of light nuclei in the first minutes after the big bang and it provides basic information on the charged weak current of the standard model of particle physics. Two different methods have been used to measure the neutron lifetime: disappearance measurements using bottled ultracold neutrons and decay rate measurements using neutron beams. The best measurements using these two techniques give results that differ by nearly 4 standard deviations. In this paper we describe a new method for measuring surviving neutrons in neutron lifetime measurements using bottled ultracold neutrons that provides better characterization of systematic uncertainties and enables higher precision than previous measurement techniques. We present results obtained using our method.

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Position-sensitive detection of ultracold neutrons with an imaging camera and its implications to spectroscopy

Position-sensitive detection of ultracold neutrons (UCNs) is demonstrated using an imaging charge-coupled device (CCD) camera. A spatial resolution less than 15 $μ$m has been achieved, which is equivalent to an UCN energy resolution below 2 pico-electron-volts through the relation $δE = m_0g δx$. Here, the symbols $δE$, $δx$, $m_0$ and $g$ are the energy resolution, the spatial resolution, the neutron rest mass and the gravitational acceleration, respectively. A multilayer surface convertor described previously is used to capture UCNs and then emits visible light for CCD imaging. Particle identification and noise rejection are discussed through the use of light intensity profile analysis. This method allows different types of UCN spectroscopy and other applications.

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Measurement of spin-flip probabilities for ultracold neutrons interacting with nickel phosphorus coated surfaces

We report a measurement of the spin-flip probabilities for ultracold neutrons interacting with surfaces coated with nickel phosphorus. For 50~$μ$m thick nickel phosphorus coated on stainless steel, the spin-flip probability per bounce was found to be $β_{\rm NiP\;on\;SS} = (3.3^{+1.8}_{-5.6}) \times 10^{-6}$. For 50~$μ$m thick nickel phosphorus coated on aluminum, the spin-flip probability per bounce was found to be $β_{\rm NiP\;on\;Al} = (3.6^{+2.1}_{-5.9}) \times 10^{-6}$. For the copper guide used as reference, the spin flip probability per bounce was found to be $β_{\rm Cu} = (6.7^{+5.0}_{-2.5}) \times 10^{-6}$. The results on the nickel phosphorus-coated surfaces may be interpreted as upper limits, yielding $β_{\rm NiP\;on\;SS} < 6.2 \times 10^{-6}$ (90\% C.L.) and $β_{\rm NiP\;on\;Al} < 7.0 \times 10^{-6}$ (90\% C.L.) for 50~$μ$m thick nickel phosphorus coated on stainless steel and 50~$μ$m thick nickel phosphorus coated on aluminum, respectively. Nickel phosphorus coated stainless steel or aluminum provides a solution when low-cost, mechanically robust, and non-depolarizing UCN guides with a high-Fermi-potential are needed.

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An apparatus for studying electrical breakdown in liquid helium at 0.4 K and testing electrode materials for the SNS nEDM experiment

We have constructed an apparatus to study DC electrical breakdown in liquid helium at temperatures as low as 0.4 K and at pressures between the saturated vapor pressure and $\sim$600 torr. The apparatus can house a set of electrodes that are 12 cm in diameter with a gap of $1-2$ cm between them, and a potential up to $\pm 50$ kV can be applied to each electrode. Initial results demonstrated that it is possible to apply fields exceeding 100 kV/cm in a 1 cm gap between two electropolished stainless steel electrodes 12 cm in diameter for a wide range of pressures at 0.4 K. We also measured the current between two electrodes. Our initial results, $I<1$ pA at 45 kV, correspond to a lower bound on the effective volume resistivity of LHe of $ρ_V > 5\times10^{18}$ $Ω\cdot$cm. This lower bound is 5 times larger than the bound previously measured. We report the design, construction, and operational experience of the apparatus, as well as initial results.

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A multilayer surface detector for ultracold neutrons

A multilayer surface detector for ultracold neutrons (UCNs) is described. The top $^{10}$B layer is exposed to the vacuum chamber and directly captures UCNs. The ZnS:Ag layer beneath the $^{10}$B layer is a few microns thick, which is sufficient to detect the charged particles from the $^{10}$B(n,$α$)$^7$Li neutron-capture reaction, while thin enough so that ample light due to $α$ and $^7$Li escapes for detection by photomultiplier tubes. One-hundred-nm thick $^{10}$B layer gives high UCN detection efficiency, as determined by the mean UCN kinetic energy, detector materials and others. Low background, including negligible sensitivity to ambient neutrons, has also been verified through pulse-shape analysis and comparisons with other existing $^3$He and $^{10}$B detectors. This type of detector has been configured in different ways for UCN flux monitoring, development of UCN guides and neutron lifetime research.

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Measurement of the Formation Rate of Muonic Hydrogen Molecules

Background: The rate λ_ppμ characterizes the formation of ppμ molecules in collisions of muonic pμ atoms with hydrogen. In measurements of the basic weak muon capture reaction on the proton to determine the pseudoscalar coupling g_P, capture occurs from both atomic and molecular states. Thus knowledge of λ_ppμ is required for a correct interpretation of these experiments. Purpose: Recently the MuCap experiment has measured the capture rate Λ_S from the singlet pμ atom, employing a low density active target to suppress ppμ formation (PRL 110, 12504 (2013)). Nevertheless, given the unprecedented precision of this experiment, the existing experimental knowledge in λ_ppμ had to be improved. Method: The MuCap experiment derived the weak capture rate from the muon disappearance rate in ultra-pure hydrogen. By doping the hydrogen with 20 ppm of argon, a competing process to ppμ formation was introduced, which allowed the extraction of λ_ppμ from the observed time distribution of decay electrons. Results: The ppμ formation rate was measured as λ_ppμ= (2.01 +- 0.06(stat) +- 0.03(sys)) 10^6 s^-1. This result updates the λ_ppμ value used in the above mentioned MuCap publication. Conclusions: The 2.5x higher precision compared to earlier experiments and the fact that the measurement was performed at nearly identical conditions to the main data taking, reduces the uncertainty induced by λ_ppμ to a minor contribution to the overall uncertainty of Λ_S and g_P, as determined in MuCap. Our final value for λ_ppμ shifts Λ_S and g_P by less than one tenth of their respective uncertainties compared to our results published earlier.

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Determination of the Free Neutron Lifetime

We present the status of current US experimental efforts to measure the lifetime of the free neutron by the "beam" and "bottle" methods. BBN nucleosynthesis models require accurate measurements with 1 second uncertainties, which are currently feasible. For tests of physics beyond the standard model, future efforts will need to achieve uncertainties well below 1 second. We outline paths achieve both.

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A high-pressure hydrogen time projection chamber for the MuCap experiment

The MuCap experiment at the Paul Scherrer Institute performed a high-precision measurement of the rate of the basic electroweak process of nuclear muon capture by the proton, $μ^- + p \rightarrow n + ν_μ$. The experimental approach was based on the use of a time projection chamber (TPC) that operated in pure hydrogen gas at a pressure of 10 bar and functioned as an active muon stopping target. The TPC detected the tracks of individual muon arrivals in three dimensions, while the trajectories of outgoing decay (Michel) electrons were measured by two surrounding wire chambers and a plastic scintillation hodoscope. The muon and electron detectors together enabled a precise measurement of the $μp$ atom's lifetime, from which the nuclear muon capture rate was deduced. The TPC was also used to monitor the purity of the hydrogen gas by detecting the nuclear recoils that follow muon capture by elemental impurities. This paper describes the TPC design and performance in detail.

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High electric field development for the SNS nEDM Experiment

A new experiment to search for the permanent electric dipole moment of the neutron is being developed for installation at the Spallation Neutron Source at Oak Ridge National Laboratory. This experiment will be performed in liquid helium at ? 0:4 K and requires a large electric field (E ~ 75 kV/cm) to be applied in liquid helium. We have constructed a new HV test apparatus to study electric breakdown in liquid helium. Initial results demonstrated that it is possible to apply fields exceeding 100 kV/cm in a 1 cm gap between two electropolished stainless steel electrodes12 cm in diameter for a wide range of pressures.

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