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S. M. Frolov

Publications and source records attributed to S. M. Frolov.

At least 19 recordsLinked to original sources

Realistic quantum device data synthesized by consumer AI and how to identify it

With the advance of generative artificial intelligence (AI) synthetic texts and images have become commonplace. These capabilities offer clear benefits, but have also raised a number of ethical concerns that often have to do with misrepresenting AI outputs as genuine material. A lesser known capability of generative AI is to perform the basic analysis, processing and even synthesis of numerical data. This raises the question of whether AI can be used to imitate experimental data that an expert would consider scientifically meaningful and on par with data in the figures of peer-reviewed manuscripts? In this paper, we focus on synthesizing data inspired by well-known experiments done frequently on quantum electronic devices. This field is related to information technologies such as spintronics and quantum computing, and is considered data-rich and data-driven. We demonstrate that it is possible to generate dramatic signals associated with iconic effects such as quantum bit control, Majorana fermions, Josephson effects, quantum dots and wires using widely available ChatGPT. We find that because some of the clearest data from quantum devices can be expressed in terms of relatively basic mathematical models, AI does not need to learn on the specialized body of data. Instead, knowledge of the physics equations and of the basic features of experimental signals can go a long way towards building a realistic dataset. We also demonstrate that real data can be augmented by AI, and that AI can mimic the noise of common scientific instruments. To help assure that published data come from experiments and are not synthesized by AI, we recommend sharing large volumes of the primary data. While it is straightforward for AI to mimic a few sets of data, consistently generating long measured sequences poses sufficient barriers to the proliferation of undisclosed synthetic data.

cond-mat.mes-hall

Comparison of Origins of Re-Entrant Supercurrents at High In-Plane Magnetic Fields in Planar InAs-Al Josephson Junctions

Hybrid superconductor-semiconductor systems with large spin-orbit coupling are important platforms for realizing topological or triplet superconductivity. Planar Josephson junctions made using these materials are predicted to enter the topological state by tuning the phase difference between the two superconductors from 0 to $π$. The 0-$π$ transition can be driven by magnetic field through Zeeman splitting of subbands in the semiconductor. It is expected to manifest as a node, or a re-entrance, in the critical current. Here we present re-entrant switching currents from several InAs/Al planar Josephson junctions in high in-plane magnetic fields. We find that re-entrances in some devices conform with expected signatures for topological or 0-$π$ transitions. However, we show that the data can also be explained in terms of mode interference in the junction in the presence of disorder. We also present simulations of supercurrent interference under in-plane fields that can reproduce re-entrances due to corrugated weak link without invoking the Zeeman effect or topology.

cond-mat.mes-hall

Report on reproducibility in condensed matter physics

We present recommendations to improve reproducibility and replicability in condensed matter physics. This area of physics has consistently produced both fundamental insights into the workings of matter and transformative inventions. Our recommendations result from a collaboration that includes researchers from academia and government laboratories, scientific journalists, legal professionals, representatives of publishers, professional societies, and other experts. The group met in person in May 2024 at a conference at the University of Pittsburgh to discuss the growing challenges related to research reproducibility and replicability in condensed matter physics. In this report, we discuss best practices and policies at all stages of the scientific process to safeguard the value of condensed matter. We hope this report will lay the groundwork for a broader conversation to develop subfield-specific recommendations.

cond-mat.other

Model for missing Shapiro steps due to bias-dependent resistance

Majorana zero modes are predicted in several solid state systems such as hybrid superconductor-semiconductor structures and topological insulators coupled to superconductors. One of the expected signatures of Majorana modes is the fractional 4$π$ Josephson effect. Evidence in favor of this effect often comes from a.c. Josephson effect measurements and focuses on the observation of missing first or higher odd-numbered Shapiro steps. However, the disappearance of the odd Shapiro steps has also been reported in conventional Josephson junctions where no Majorana modes are expected. In this paper, we present a phenomenological model that displays suppression of the odd Shapiro steps. We perform resistively-shunted junction model calculations and introduce peaks in differential resistance as function of the bias current. In the presence of only the standard 2$π$ Josephson current, for chosen values of peak positions and amplitudes, we can suppress the odd Shapiro steps, or any steps, thus providing a possible explanation for the observation of missing Shapiro steps.

cond-mat.mes-hall

Missing odd-order Shapiro steps do not uniquely indicate fractional Josephson effect

Topological superconductivity is expected to spur Majorana zero modes -- exotic states that are also considered a quantum technology asset. Fractional Josephson effect is their manifestation in electronic transport measurements, often under microwave irradiation. A fraction of induced resonances, known as Shapiro steps, should vanish, in a pattern that signifies the presence of Majorana modes. Here we report patterns of Shapiro steps expected in topological Josephson junctions, such as the missing first Shapiro step, or several missing odd-order steps. But our junctions, which are InAs quantum wells with Al contacts, are studied near zero magnetic field, meaning that they are not in the topological regime. We also observe other patterns such as missing even steps and several missing steps in a row, not relevant to topological superconductivity. Potentially responsible for our observations is rounding of not fully developed steps superimposed on non-monotonic resistance versus voltage curves, but several origins may be at play. Our results demonstrate that any single pattern, even striking, cannot uniquely identify topological superconductivity, and a multifactor approach is necessary to unambiguously establish this important phenomenon.

cond-mat.mes-hall

Zero-bias conductance peaks at zero applied magnetic field due to stray fields from integrated micromagnets in hybrid nanowire quantum dots

Many recipes for realizing topological superconductivity rely on broken time-reversal symmetry, which is often attained by applying a substantial external magnetic field. Alternatively, using magnetic materials can offer advantages through low-field operation and design flexibility on the nanoscale. Mechanisms for lifting spin degeneracy include exchange coupling, spin-dependent scattering, spin injection-all requiring direct contact between the bulk or induced superconductor and a magnetic material. Here, we implement locally broken time-reversal symmetry through dipolar coupling from nearby micromagnets to superconductor-semiconductor hybrid nanowire devices. Josephson supercurrent is hysteretic due to micromangets switching. At or around zero external magnetic field, we observe an extended presence of Andreev bound states near zero voltage bias. We also show a zero-bias peak plateau of a non-quantized value. Our findings largely reproduce earlier results where similar effects were presented in the context of topological superconductivity in a homogeneous wire, and attributed to more exotic time-reversal breaking mechanisms [1]. In contrast, our stray field profiles are not designed to create Majorana modes, and our data are compatible with a straightforward interpretation in terms of trivial states in quantum dots. At the same time, the use of micromagnets in hybrid superconductor-semiconductor devices shows promise for future experiments on topological superconductivity.

cond-mat.mes-hall

Supercurrent through a single transverse mode in nanowire Josephson junctions

Hybrid superconductor-semiconductor materials are fueling research in mesoscopic physics and quantum technology. Recently demonstrated smooth $β$-Sn superconductor shells, due to the increased induced gap, are expanding the available parameter space to new regimes. Fabricated on quasiballistic InSb nanowires, with careful control over the hybrid interface, Sn shells yield measurable switching currents even when nanowire resistance is of order 10kohm. In this regime Cooper pairs travel through a purely 1D quantum wire for at least part of their trajectory. Here, we focus on the evolution of proximity-induced supercurrent in magnetic field parallel to the nanowire. Long decay up to fields of 1T is observed. At the same time, the decay for higher occupied subbands is notably faster in some devices but not in others. We analyze this using a tight-binding numerical model that includes the Zeeman, orbital and spin-orbit effects. When the first subband is spin polarized, we observe a dramatic suppression of supercurrent, which is also confirmed by the model and suggests an absence of significant triplet supercurrent generation.

cond-mat.supr-con

Matters Arising from S. Vaitiekenas et al., "Zero-bias peaks at zero magnetic field in ferromagnetic hybrid nanowires" Nature Physics 2021

In 2021 Nature Physics published a paper by Vaitiekenas, Liu, Krogstrup and Marcus titled "Zero-bias peaks at zero magnetic field in ferromagnetic hybrid nanowires". The paper reports low temperature transport measurements on semiconductor InAs nanowires with two partly overlapping shells -- a shell of EuS, a magnetic insulator, and a shell of Al, a metal that becomes superconducting at temperatures below 1.2K. The paper claims that (1) the data are consistent with induced topological superconductivity and Majorana zero modes (MZMs), and (2) that this is facilitated by the breaking of the time reversal symmetry through a direct magnetic interaction with the EuS shell. In this Matters Arising, we present an alternative explanation which is based on trivial effects that are likely to appear in the reported geometry. Specifically, first, we find that data the authors present in support of the topological superconductivity claim can originate from unintended quantum dots in their devices, a widely known likely explanation that is not being discussed in the paper. Second, our analysis of the setup, supported by our numerical micromagnetic simulations, shows similar effects could be obtained due to stray magnetic fields from the region of the EuS shell damaged during Al etching. This basic picture should come before the exotic interpretation in terms of magnetic exchange interaction with a ferromagnetic insulator.

cond-mat.mes-hall

Evidence of $ϕ$0-Josephson junction from skewed diffraction patterns in Sn-InSb nanowires

We study Josephson junctions based on InSb nanowires with Sn shells. We observe skewed critical current diffraction patterns: the maxima in forward and reverse current bias are at different magnetic flux, with a displacement of 20-40 mT. The skew is greatest when the external field is nearly perpendicular to the nanowire, in the substrate plane. This orientation suggests that spin-orbit interaction plays a role. We develop a phenomenological model and perform tight-binding calculations, both methods reproducing the essential features of the experiment. The effect modeled is the $ϕ$0-Josephson junction with higher-order Josephson harmonics. The system is of interest for Majorana studies: the effects are either precursor to or concomitant with topological superconductivity. Current-phase relations that lack inversion symmetry can also be used to design quantum circuits with engineered nonlinearity.

cond-mat.mes-hall

Comment on "Ballistic Majorana Nanowire Devices" by Gul et al. Nature Nanotechnology 2018

This work re-analyzes Gul et al. Nature Nanotechnology 2018 "Ballistic Majorana nanowire devices" using fuller data from the original experiments released in 2023 on Zenodo. The authors have prepared a correction to their article that appeared in Nature Nanotechnology in 2024. However, the correction does not address the concerns we identify here. We demonstrate that the fuller data contain extensive evidence for quantum dots and disorder that are completely inconsistent with the authors' conclusion that they have achieved ballistic devices containing zero bias peaks of likely Majorana origin. We show how data selection, data cropping and undisclosed data processing played a role in composing the figures of the final published paper.

cond-mat.mes-hall

Large Second-Order Josephson Effect in Planar Superconductor-Semiconductor Junctions

We investigate the current-phase relations of Al/InAs-quantum well planar Josephson junctions fabricated using nanowire shadowing technique. Based on several experiments, we conclude that the junctions exhibit an unusually large second-order Josephson harmonic, the $\sin(2φ)$ term. First, superconducting quantum interference devices (dc-SQUIDs) show half-periodic oscillations, tunable by gate voltages as well as magnetic flux. Second, Josephson junction devices exhibit kinks near half-flux quantum in supercurrent diffraction patterns. Third, half-integer Shapiro steps are present in the junctions. Similar phenomena are observed in Sn/InAs quantum well devices. We perform data fitting to a numerical model with a two-component current phase relation. Analysis including a loop inductance suggests that the sign of the second harmonic term is negative. The microscopic origins of the observed effect remain to be understood. We consider alternative explanations which can account for some but not all of the evidence.

cond-mat.mes-hall

Role of a capping layer on the crystalline structure of Sn thin films grown at cryogenic temperatures on InSb substrates

Metal deposition with cryogenic cooling is widely utilized in the condensed matter community for producing ultra-thin epitaxial superconducting layers on semiconductors. However, a drawback arises when these films return to room temperature, as they tend to undergo dewetting. This issue is mitigated by capping the films with an amorphous layer. In this study, we examined the impact of different in-situ fabricated caps on the structural characteristics of Sn thin films deposited at 80 K on InSb substrates. Regardless of the type of capping, we observed that the films remained smooth upon returning to room temperature and were epitaxial on InSb in the cubic Sn ($α$-Sn) phase. However, we noted a correlation between alumina capping with an electron beam evaporator and an increased presence of tetragonal Sn ($β$-Sn) grains. This suggests that heating from the alumina source may contribute to a partial phase transition in the Sn layer. The existence of the $β$-Sn phase induced superconducting behavior of the films by percolation effect. This study highlights the potential for modifying the structural properties of cryogenic Sn thin films through in-situ capping, paving the way for precise control in the production of superconducting Sn films for integration into quantum computing platforms.

cond-mat.mtrl-sci

"Smoking gun" signatures of topological milestones in trivial materials by measurement fine-tuning and data postselection

Exploring the topology of electronic bands is a way to realize new states of matter with possible implications for information technology. Because bands cannot always be observed directly, a central question is how to tell that a topological regime has been achieved. Experiments are often guided by a prediction of a unique signal or a pattern, called "the smoking gun". Examples include peaks in conductivity, microwave resonances, and shifts in interference fringes. However, many condensed matter experiments are performed on relatively small, micron or nanometer-scale, specimens. These structures are in the so-called mesoscopic regime, between atomic and macroscopic physics, where phenomenology is particularly rich. In this paper, we demonstrate that the trivial effects of quantum confinement, quantum interference and charge dynamics in nanostructures can reproduce accepted smoking gun signatures of triplet supercurrents, Majorana modes, topological Josephson junctions and fractionalized particles. The examples we use correspond to milestones of topological quantum computing: qubit spectroscopy, fusion and braiding. None of the samples we use are in the topological regime. The smoking gun patterns are achieved by fine-tuning during data acquisition and by subsequent data selection to pick non-representative examples out of a fluid multitude of similar patterns that do not generally fit the "smoking gun" designation. Building on this insight, we discuss ways that experimentalists can rigorously delineate between topological and non-topological effects, and the effects of fine-tuning by deeper analysis of larger volumes of data.

cond-mat.mes-hall

Delocalized states in three-terminal superconductor-semiconductor nanowire devices

We fabricate three-terminal hybrid devices with a nanowire segment proximitized by a superconductor, and with two tunnel probe contacts on either side of that segment. We perform simultaneous tunneling measurements on both sides. We identify some states as delocalized above-gap states observed on both ends, and some states as localized near one of the tunnel barriers. Delocalized states can be traced from zero to finite magnetic fields beyond 0.5 T. In the parameter regime of delocalized states, we search for correlated subgap resonances required by the Majorana zero mode hypothesis. While both sides exhibit ubiquitous low-energy features at high fields, no correlation is inferred. Simulations using a one-dimensional effective model suggest that delocalized states may belong to lower one-dimensional subbands, while the localized states originate from higher subbands. To avoid localization in higher subbands, disorder may need to be further reduced to realize Majorana zero modes.

cond-mat.mes-hall

Planar Josephson Junctions Templated by Nanowire Shadowing

More and more materials, with a growing variety of properties, are built into electronic devices. This is motivated both by increased device performance and by the studies of materials themselves. An important type of device is a Josephson junction based on the proximity effect between a quantum material and a superconductor, useful for fundamental research as well as for quantum and other technologies. When both junction contacts are placed on the same surface, such as a two-dimensional material, the junction is called ``planar". One outstanding challenge is that not all materials are amenable to the standard planar junction fabrication. The device quality, rather than the intrinsic characteristics, may be defining the results. Here, we introduce a technique in which nanowires are placed on the surface and act as a shadow mask for the superconductor. The advantages are that the smallest dimension is determined by the nanowire diameter and does not require lithography, and that the junction is not exposed to chemicals such as etchants. We demonstrate this method with an InAs quantum well, using two superconductors - Al and Sn, and two semiconductor nanowires - InAs and InSb. The junctions exhibit critical current levels consistent with transparent interfaces and uniform width. We show that the template nanowire can be operated as a self-aligned electrostatic gate. Beyond single junctions, we create SQUIDs with two gate-tunable junctions. We suggest that our method can be used for a large variety of quantum materials including van der Waals layers, topological insulators, Weyl semimetals and future materials for which proximity effect devices is a promising research avenue.

cond-mat.mes-hall

Spin and Orbital Spectroscopy in the Absence of Coulomb Blockade in Lead Telluride Nanowire Quantum Dots

We investigate quantum dots in semiconductor PbTe nanowire devices. Due to the accessibility of ambipolar transport in PbTe, quantum dots can be occupied both with electrons and holes. Owing to a very large dielectric constant in PbTe of order 1000, we do not observe Coulomb blockade which typically obfuscates the orbital and spin spectra. We extract large and highly anisotropic effective Lande g-factors, in the range 20-44. The absence of Coulomb blockade allows direct readout, at zero source-drain bias, of spin-orbit hybridization energies of up to 600 microelectronvolt. These spin properties make PbTe nanowires, the recently synthesized members of group IV-VI materials family, attractive as a materials platform for quantum technology, such as spin and topological qubits.

cond-mat.mes-hall

Hysteretic magnetoresistance in nanowire devices due to stray fields induced by micromagnets

We study hysteretic magnetoresistance in InSb nanowires due to stray magnetic fields from CoFe micromagnets. Devices without any ferromagnetic components show that the magnetoresistance of InSb nanowires commonly exhibits either a local maximum or local minimum at zero magnetic field. Switching of microstrip magnetizations then results in positive or negative hysteretic dependence as conductance maxima or minima shift with respect to the global external field. Stray fields are found to be in the range of tens of millitesla, comparable to the scale over which the nanowire magnetoresistance develops. We observe that the stray field signal is similar to that obtained in devices with ferromagnetic contacts (spin valves). We perform micromagnetic simulations which are in reasonable agreement with the experiment. The use of locally varying magnetic fields may bring new ideas for Majorana circuits in which nanowire networks require control over field orientation at the nanoscale.

cond-mat.mes-hall

Non-Majorana states yield nearly quantized conductance in superconductor-semiconductor nanowire devices

Conductance at zero source-drain voltage bias in InSb nanowire/NbTiN superconductor devices exhibits peaks that are close to a quantized value of $2e^2/h$. The nearly quantized resonances evolve in the tunnel barrier strength, magnetic field and magnetic field orientation in a way consistent with Majorana zero modes. Our devices feature two tunnel probes on both ends of the nanowire separated by a 400 nm nanowire segment covered by the superconductor. We only find nearly quantized zero bias peaks localized to one end of the nanowire, while conductance dips are observed for the same parameters on the other end. This undermines the Majorana explanation as Majorana modes must come in pairs. We do identify states delocalized from end to end near zero magnetic field and at higher electron density, which is not in the basic Majorana regime. We lay out procedures for assessing the nonlocality of subgap wavefunctions and provide a classification of nanowire bound states based on their localization.

cond-mat.mes-hall