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S. M. Hayden

Publications and source records attributed to S. M. Hayden.

71 records · Page 4Linked to original sources

Multiband superconductivity in NbSe_2 from heat transport

The thermal conductivity of the layered s-wave superconductor NbSe_2 was measured down to T_c/100 throughout the vortex state. With increasing field, we identify two regimes: one with localized states at fields very near H_c1 and one with highly delocalized quasiparticle excitations at higher fields. The two associated length scales are most naturally explained as multi-band superconductivity, with distinct small and large superconducting gaps on different sheets of the Fermi surface.

cond-mat.supr-con↗

Heat Conduction in the Vortex State of NbSe_2: Evidence for Multi-Band Superconductivity

The thermal conductivity kappa of the layered s-wave superconductor NbSe_2 was measured down to T_c/100 throughout the vortex state. With increasing field, we identify two regimes: one with localized states at fields very near H_c1 and one with highly delocalized quasiparticle excitations at higher fields. The two associated length scales are naturally explained as multi-band superconductivity, with distinct small and large superconducting gaps on different sheets of the Fermi surface. This behavior is compared to that of the multi-band superconductor MgB_2 and the conventional superconductor V_3Si.

cond-mat.supr-con↗

Heavy quasiparticles in the ferromagnetic superconductor ZrZn2

We report a study of the de Haas-van Alphen effect in the normal state of the ferromagnetic superconductor ZrZn2. Our results are generally consistent with an LMTO band structure calculation which predicts four exchange-split Fermi surface sheets. Quasiparticle effective masses are enhanced by a factor of about 4.9 implying a strong coupling to magnetic excitations or phonons. Our measurements provide insight in to the mechanism for superconductivity and unusual thermodynamic properties of ZrZn2.

cond-mat.supr-con↗

Magnetic Order in YBa$_2$Cu$_3$O$_{6+x}$ Superconductors

Polarized and unpolarized neutron diffraction has been used to search for magnetic order in YBa$_2$Cu$_3$O$_{6+x}$ superconductors. Most of the measurements were made on a high quality crystal of YBa$_2$Cu$_3$O$_{6.6}$. It is shown that this crystal has highly ordered ortho-II chain order, and a sharp superconducting transition. Inelastic scattering measurements display a very clean spin-gap and pseudogap with any intensity at 10 meV being 50 times smaller than the resonance intensity. The crystal shows a complicated magnetic order that appears to have three components. A magnetic phase is found at high temperatures that seems to stem from an impurity with a moment that is in the $a$-$b$ plane, but disordered on the crystal lattice. A second ordering occurs near the pseudogap temperature that has a shorter correlation length than the high temperature phase and a moment direction that is at least partly along the c-axis of the crystal. Its moment direction, temperature dependence, and Bragg intensities suggest that it may stem from orbital ordering of the $d$-density wave (DDW) type. An additional intensity increase occurs below the superconducting transition. The magnetic intensity in these phases does not change noticeably in a 7 Tesla magnetic field aligned approximately along the c-axis. Searches for magnetic order in YBa$_2$Cu$_3$O$_{7}$ show no signal while a small magnetic intensity is found in YBa$_2$Cu$_3$O$_{6.45}$ that is consistent with c-axis directed magnetic order. The results are contrasted with other recent neutron measurements.

cond-mat.supr-con↗

Observation of Two-dimensional Spin Fluctuations in the Bilayer Ruthenate Sr3Ru2O7 by Inelastic Neutron Scattering

We report the first observation of two-dimensional incommensurate magnetic fluctuations in the layered metallic perovskite Sr3Ru2O7. The wavevectors where the magnetic fluctuations are strongest are different from those observed in the superconducting single layer ruthenate Sr2RuO4 and appear to be determined by Fermi surface nesting. No antiferromagnetic ordering is observed for temperatures down to 1.5K. For temperatures T<20K, the fluctuations become predominately ferromagnetic. Our inelastic neutron scattering measurements provide concrete evidence of the coexistence of competing interactions in Sr3Ru2O7 and of the low energy scale of the fluctuations.

cond-mat.str-el↗

Superconducting Fluctuations and the Reduced Dimensionality of the Organic Superconductor $κ$- (BEDT-TTF)$_{2}$Cu(NCS)$_{2}$ as Observed through Measurements of the de Haas-van Alphen Effect

We report measurements of the de Haas-van Alphen (DHVA) effect and AC susceptibility in the layered organic superconductor $κ$-(BEDT-TTF)$_{2}$Cu(NCS)$_{2}$. The amplitude of the DHVA oscillations is attenuated over a wide field range above the irreversibility line, B_irr(B), below which a rigid flux lattice is formed. Thus the DHVA effect provides a unique probe of the superconducting fluctuations at high fields in this material. We compare our measurements with other determinations of the superconducting phase diagram of $κ$-(BEDT-TTF)$_{2}$Cu(NCS)$_{2}$.

cond-mat.supr-con↗

Spin waves and electronic interactions in La2CuO4

The magnetic excitations of the square-lattice spin-1/2 antiferromagnet and high-Tc parent La2CuO4 are determined using high-resolution inelastic neutron scattering. Sharp spin waves with absolute intensities in agreement with theory including quantum corrections are found throughout the Brillouin zone. The observed dispersion relation shows evidence for substantial interactions beyond the nearest-neighbor Heisenberg term, which can be understood in terms of a cyclic or ring exchange due to the strong hybridization path around the Cu4O4 square plaquettes.

cond-mat.str-el↗

A polarized neutron-scattering study of the Cooper-pair moment in Sr2RuO4

We report a study of the magnetization density in the mixed state of the unconventional superconductor S2RuO4. On entering the superconducting state we find no change in the magnitude or distribution of the induced moment for a magnetic field of 1 Tesla applied within the RuO2 planes. Our results are consistent with a spin-triplet Cooper pairing with spins lying in the basal plane. This is in contrast with similar experiments performed on conventional and high-Tc superconductors.

cond-mat.supr-con↗

The connection between superconducting phase correlations and spin excitations in YBa$_2$Cu$_3$O$_{6.6}$: A magnetic field study

One of the most striking universal properties of the high-transition-temperature (high-$T_c$) superconductors is that they are all derived from the hole-doping of their insulating antiferromagnetic (AF) parent compounds. From the outset, the intimate relationship between magnetism and superconductivity in these copper-oxides has intrigued researchers. Evidence for this link comes from neutron scattering experiments that show the unambiguous presence of short-range AF correlations (excitations) in cuprate superconductors. Even so, the role of such excitations in the pairing mechanism and superconductivity is still a subject of controversy. For YBa$_2$Cu$_3$O$_{6+x}$, where $x$ controls the hole-doping level, the most prominent feature in the magnetic excitations spectra is the ``resonance''. Here we show that for underdoped YBa$_2$Cu$_3$O$_{6.6}$, where $x$ and $T_c$ are below the optimal values, modest magnetic fields suppress the resonance significantly, much more so for fields approximately perpendicular rather than parallel to the CuO$_2$ planes. Our results indicate that the resonance measures pairing and phase coherence, suggesting that magnetism plays an important role in the superconductivity of cuprates. The persistence of a field effect above $T_c$ favors mechanisms with preformed pairs in the normal state of underdoped cuprates.

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The Magnetic Excitation Spectrum and Thermodynamics of High-$T_c$ Superconductors

Inelastic neutron scattering was used to study the wavevector- and frequency-dependent magnetic fluctuations in single crystals of superconducting YBa$_2$Cu$_3$O$_{6+x}$. The spectra contain several important features, including a gap in the superconducting state, a pseudogap in the normal state and the much-discussed resonance peak. The appearance of the pseudogap determined from transport and nuclear resonance coincides with formation of the resonance in the magnetic excitations. The exchange energy associated with the resonance has the temperature and doping dependences as well as the magnitude to describe approximately the electronic specific heat near the superconducting transition temperature ($T_c$).

cond-mat.supr-con↗

The strongly enhanced magnetic excitations near the quantum critical point of Cr$_{1-x}$V$_x$ and why strong exchange enhancement need not imply heavy fermion behavior

Inelastic neutron scattering reveals strong spin fluctuations with energies as high as 0.4eV in the nearly antiferromagnetic metal Cr$_{0.95}$V$_{0.05}$. The magnetic response is well described by a modified Millis-Monien-Pines function. From the low-energy response, we deduce a large exchange enhancement, more than an order of magnitude larger than the corresponding enhancement of the low-temperature electronic heat capacity $γT$. A scaling relationship between $γ$ and the inverse of the wavevector- averaged spin relaxation rate $Γ_{\text{ave}}$ is demonstrated for a number of magnetically correlated metals

cond-mat.str-el↗

Spin gap and magnetic coherence in a clean high-T_c superconductor

A notable aspect of high-temperature superconductivity in the copper oxides is the unconventional nature of the underlying paired-electron state. A direct manifestation of the unconventional state is a pairing energy - that is, the energy required to remove one electron from the superconductor - that varies (between zero and a maximum value) as a function of momentum or wavevector: the pairing energy for conventional superconductors is wavevector-independent. The wavefunction describing the superconducting state will include not only the pairing of charges, but also of the spins of the paired charges. Each pair is usually in the form of a spin singlet, so there will also be a pairing energy associated with transforming the spin singlet into the higher energy spin triplet form without necessarily unbinding the charges. Here we use inelastic neutron scattering to determine the wavevector-dependence of spin pairing in La_{2-x}Sr_xCuO_4, the simplest high-temperature superconductor. We find that the spin pairing energy (or 'spin gap') is wavevector independent, even though superconductivity significantly alters the wavevector dependence of the spin fluctuations at higher energies.

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Absolute measurements of the high-frequency magnetic dynamics in high-Tc superconductors

We review recent measurements of the high-frequency dynamic magnetic susceptibility in the high-$T_c$ superconducting systems La$_{2-x}$Sr$_{x}$CuO$_4$ and YBa$_2$Cu$_3$O$_{6+x}$. Experiments were performed using the chopper spectrometers HET and MARI at the ISIS spallation source. We have placed our measurements on an absolute intensity scale, this allows systematic trends to be seen and comparisons with theory to be made. We find that the insulating S=1/2 antiferromagnetic parent compounds show a dramatic renormalization of the spin wave intensity. The effect of doping on the response is to cause broadenings in wave vector and large redistributions of spectral weight in the frequency spectrum.

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Nearly Singular Magnetic Fluctuations in the Normal State of a High-T_c Cuprate Superconductor

Polarized and unpolarized neutron scattering was used to measure the wave vector- and frequency-dependent magnetic fluctuations in the normal state (from the superconducting transition temperature, T_c=35, up to 350 K) of single crystals of La_{1.86}Sr_{0.14}CuO_4. The peaks which dominate the fluctuations have amplitudes that decrease as T^{-2} and widths that increase in proportion to the thermal energy, k_B T (where k_B is Boltzmann's constant), and energy transfer added in quadrature. The nearly singular fluctuations are consistent with a nearby quantum critical point.

cond-mat.str-el↗

A Comparison of the High-Frequency Magnetic Fluctuations in Insulating and Superconducting La2-xSrxCuO4

Inelastic neutron scattering performed at a spallation source is used to make absolute measurements of the dynamic susceptibility of insulating La2CuO4 and superconducting La2-xSrxCuO4 over the energy range 15<EN<350 meV. The effect of Sr doping on the magnetic excitations is to cause a large broadening in wavevector and a substantial change in the spectrum of the local spin fluctuations. Comparison of the two compositions reveals a new energy scale of 22 meV in La1.86Sr0.14CuO4.

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New magnetic coherence effect in superconducting La_{2-x}Sr_{x}CuO_{4}

We have used inelastic neutron scattering to examine the magnetic fluctuations at intermediate frequencies in the simplest high temperature superconductor, La_{2-x}Sr_{x}Cu_{4}. The suppression of the low energy magnetic response in the superconducting state is accompanied by an increase in the response at higher energies. Just above a threshold energy of ~7 meV there is additional scattering present below T_{c} which is characterised by an extraordinarily long coherence length, in excess of 50 Å.

cond-mat↗

High-Frequency Spin Waves in YBa2Cu3O6.15

Pulsed neutron spectroscopy is used to make absolute measurements of the dynamic magnetic susceptibility of insulating YBa2Cu3O6.15. Acoustic and optical modes, derived from in- and out-of-phase oscillation of spins in adjacent CuO2 planes, dominate the spectra and are observed up to 250 meV. The optical modes appear first at 74 meV. Linear-spin-wave theory gives an excellent description of the data and yields intra- and inter-layer exchange constants of J_parallel =125 meV and J_perp = 11 meV respectively and a spin-wave intensity renormalization Z_chi = 0.4.

cond-mat↗