arXiv subjects

S. Majumdar

Publications and source records attributed to S. Majumdar.

At least 19 recordsLinked to original sources

arXiv2026

Resonant photoionization dynamics during optical trapping of lithium atoms

Photoionization induced by trapping and auxiliary laser fields is an inherent feature of many laser-cooling and optical trapping experiments, yet its microscopic dynamics are rarely investigated directly. In this work, we employ a reaction microscope implementing an event-by-event photoionization time retrieval technique to extend momentum-resolved photoelectron spectroscopy to continuous-wave laser--atom interactions. We investigate low-intensity multicolor photoionization of laser-cooled lithium atoms confined in an all-optical trap. Complete three-dimensional electron momentum distributions and kinetic-energy spectra recorded for different laser wavelengths and polarization configurations identify resonant excitation of the $5p$ and $5f$ states and reveal an additional ionization channel following spontaneous decay from the $5f$ to the $4d$ state. A pronounced polarization dependence of the photoionization yield is explained by magnetic-sublevel selection rules and the coherent interference of different virtual excitation pathways. These results demonstrate that reaction microscopy combined with event-by-event time reconstruction provides a powerful approach for investigating microscopic electronic dynamics in laser-cooled atomic systems and offers new insight into photoionization processes occurring during optical trapping.

physics.atom-ph↗

arXiv2025

Relevance of Murchison Widefield Array Interplanetary Scintillation Observations to Heliospheric Transient Catalogues

We have conducted a comprehensive comparison of interplanetary scintillation (IPS) observations taken by the Murchison Widefield Array (MWA) with several heliospheric transient event catalogues, over a time period of 7 months during solar minimum. From this analysis we have found that of the 84% of catalogued events that have MWA IPS data available, 68% of them appear in MWA observations. Of the enhancements first identified in IPS observations, only 58% have a potential match with a catalogued event. The majority of enhancements that were identified in the IPS observations were situated greater than 10$^\circ$ from the ecliptic plane. Two such features were selected for detailed analysis, connecting their solar origins to their propagation through the heliosphere. The first of these features was created by a coronal mass ejection (CME), captured over two successive MWA observations and recorded in several catalogues. The second feature has the potential of being a stream interaction region (SIR) travelling out of the ecliptic plane. This particular SIR was not recorded in any catalogue. Thus the MWA shows promise in detecting heliospheric transients that other commonly-used techniques may overlook. These results show the strength of the MWA in having unbridled access to the heliosphere, able to make remote observations of events far out of the ecliptic as it is not restrained to the orbits of spacecraft. We demonstrate how the inclusion of MWA IPS data can potentially boost the number of CME and SIR events that are characterised.

astro-ph.SR↗

arXiv2024

Successive ferroelectric orders and magnetoelectric coupling without long-range magnetic order in highly frustrated pyrochlore compounds: Sm$_2$Ti$_{2-x}$V$_x$O$_7$

Sm$_2$Ti$_2$O$_7$, a member of rare-earth titanate pyrochlores, exhibits dipolar-octupolar antiferromagnetism below $T_N$ = 0.35 K. We observed two ferroelectric transitions at 182 ($T_{FE1}$) and 52 K ($T_{FE2}$), significantly higher than $T_N$ for Sm$_2$Ti$_{2-x}$V$_x$O$_7$ ($x$ = 0, 0.1). Although the ferroelectric transition temperatures remain unchanged, the polarization value decreases considerably with V doping. A structural transition to a polar $R3m$ rhombohedral phase from the cubic $Fd\bar{3}m$ structure occurs at $T_{FE1}$, involving a distortion in the pyochlore lattice. Remarkably, significant linear magnetoelectric coupling is observed in both compounds, with further enhancement of magnetoelectric coupling due to magnetic V doping. The existence of magnetoelectric coupling without long-range magnetic order in a frustrated pyrochlore system could enable the tailoring of magnetoelectric coupling properties, which can be further fine-tuned through V doping. The emergence of ferroelectricity in a frustrated magnetic system introduces an intriguing aspect to these compounds and paves the way for developing ferroelectric order driven by the alleviation of magnetic frustration in pyrochlore systems.

cond-mat.mtrl-sci↗

arXiv2024

Coupled linear Schrödinger equations: Control and stabilization results

This article presents some controllability and stabilization results for a system of two coupled linear Schrödinger equations in the one-dimensional case where the state components are interacting through the Kirchhoff boundary conditions. Considering the system in a bounded domain, the null boundary controllability result is shown. The result is achieved thanks to a new Carleman estimate, which ensures a boundary observation. Additionally, this boundary observation together with some trace estimates, helps us to use the Gramian approach, with a suitable choice of feedback law, to prove that the system under consideration decays exponentially to zero at least as fast as the function $e^{-2ωt}$ for some $ω>0$.

math.AP↗

arXiv2023

Magnetization, dielectric and thermal studies in the double perovskite polycrystalline compound Tm2CoMnO6

We report here a comprehensive study on structural, magnetic, caloric and electronic properties of the monoclinic phase of double perovskite compound Tm2CoMnO6 (TCMO) in its polycrysttaline format. Magnetic measurements confirm the presence of thermal hysteresis in magnetization indicates towards a first order magnetic transition at its critical point (Tc). Our study finds the metamagnetic jump in isothermal M(H) at 2 K that signifies the rare earth spin allignement in loop cycling above a certain critical field. This jump is only present at very low T that dies out as the T raises. M(H) measurements at different temperature stipulate that Co2+ and Mn4+ do not order completely inspite of strong ferromagnetic correlation that is against the previous study on TCMO. The concurrence of structral, magnetic and dielectric anomaly at Tc suggest its possible magnetostructural copuling. We found a high dielectric constant (2700) in TCMO and the Maxwell-Wagner electrial loss spectrum analysis hints towards a long range hopping mechanism. Sizeable magnetocaloric effect in terms of entropy change across the transition temperatures has been obtained from heat capacity data that clearly corroborates its intrinsic behaviour.

cond-mat.mtrl-sci↗

arXiv2022

Unconventional topological phase transition from semimetal to insulator in SnBi2Te4: Role of anomalous thermal expansion

We propose SnBi2Te4 to be a novel candidate material exhibiting temperature (T) mediated transitions between rich topological phases. From a combined theoretical and experimental studies, we find that SnBi2Te4 goes from a low-T topological semimetallic phase to a high-T (room temperature) topological insulating phase via an intermediate topological metallic phase. Single crystals of SnBi2Te4 are characterized by various experimental probes including Synchrotron based X-ray diffraction, magnetoresistance, Hall effect, Seebeck coefficient, magnetization and angle-resolved photoemission spectroscopy (ARPES). X-ray diffraction data confirms an anomalous thermal expansion of the unit cell volume below 100 K, which significantly affects the bulk band structure and hence the transport properties, as confirmed by our density functional theory calculations. Simulated surface states at 15 K agree fairly well with our ARPES data and are found to be robust with varying T. This indirectly supports the experimentally observed paramagnetic singularity in the entire T-range. The proposed coexistence of rich topological phases is a rare occurrence, yet paves a fertile ground to tune various topological phases in a material driven by structural distortion.

cond-mat.str-el↗

arXiv2021

Bulk Rashba spin splitting and Dirac surface state in $p$-type (Bi$_{0.9}$Sb$_{0.1})_2$Se$_3$ single crystal

We report bulk Rashba spin splitting (RSS) and associated Dirac surface state in (Bi$_{0.9}$Sb$_{0.1})_2$Se$_3$, exhibiting dominant $p$-type conductivity. We argue from the synchrotron diffraction studies that origin of the bulk RSS is due to a structural transition to a non-centrosymmetric $R3m$ phase below $\sim$ 30 K. The Shubnikov-de Haas Van (SdH) oscillations observed in the magnetoresistance curves at low temperature and the Landau level fan diagram, as obtained from these oscillations, confirm the presence of nontrivial Dirac surface state. The magnetization data at low temperature exhibit substantial orbital magnetization consistent with the bulk RSS. The existance of both the bulk RSS and Dirac surface states are confirmed by first principles density functional theory calculations. Coexistence of orbital magnetism, bulk RSS, and Dirac surface state is unique for $p$-type (Bi$_{0.9}$Sb$_{0.1})_2$Se$_3$, making it an ideal candidate for spintronic applications.

cond-mat.str-el↗

arXiv2019

Natural ferroelectric order near ambient temperature in HoFeO3: A member of RFeO3 orthoferrites

Current scenario in multiferroics demands a breakthrough discovery of promising materials after BiFeO3. Recently, the controversial discovery of room temperature ferroelectricity (FE) in SmFeO3 [PRL 107, 117201 (2011); 113, 217203 (2014)] inspires the investigation of HoFeO3. Here, we report a natural ferroelectric order below 210 K (TFE) along c-axis with reasonably large polarization and low-field strong magnetoelectric coupling. Synchrotron and neutron diffraction results confirm that a shift of O atoms along c-axis of polar Pbn21 structure causes FE in HoFeO3. The exchange striction mechanism is suggested to elucidate the ferroelectric order. The results create a renewed attention for searching promising candidates with a natural ferroelectric order and higher TFE in the rest of the RFeO3 series.

cond-mat.mtrl-sci↗

arXiv2019

Magnetic and electric behaviors of DyMn$_2$O$_5$: effect of hole doping

DyMn$_2$O$_5$ is an intriguing multiferroic material showing multiple magnetic, electric and structural transitions. We present here the systematic study on the effect of Sr doping at the Dy site of DyMn$_2$O$_5$ through magnetic and dielectric measurements. Doping of divalent Sr at the Dy site is expected to enhance the Mn$^{4+}$:Mn$^{3+}$ ratio and it will also dilute the Dy site. Our study indicates large enhancement in the magnetic anomaly observed close to 43 K, which we believe to be related to the increased ferromagnetic correlations on Sr doping. Gradual increase in coercive field at 3 K with the Sr doping and decrease in bond length of adjacent Mn$^{4+}$ ions further support the enhancement of ferromagnetic corelations in the system. The parent sample shows a large magnetocaloric effect around 12 K, the magnitude of which found to decrease with increasing Sr concentration. The doping also enhances the anomaly at around 28 K observed in the dielectric permittivity versus temperature data, and this anomaly was earlier claimed to be associated with the spin reorientation as well as a simultaneous transition from one ferroelectric state to other. The electric orderings observed below 25 K are found to be susceptible to the applied magnetic field, and supports the view of Ratcliff II {\it et al.}(Phys. Rev. B {\bf 72}, 060407(R)(2005)) of concomitant changes in the magnetic structure associated with the multiple electric transitions.

cond-mat.str-el↗

arXiv2019

High-temperature ferroelectric order and magnetic field-cooled effect driven magnetoelectric coupling in R2BaCuO5 (R= Er, Dy, Sm)

The high-temperature ferroelectric order and a remarkable magnetoelectric effect driven by the magnetic field cooling are reported in R2BaCuO5 (R = Er, Dy, Sm) series. The ferroelectric (FE) orders are observed at much higher temperatures than their magnetic orders for all three members. The value of FE Curie temperature (TFE) is considerably high as ~ 235 K with the polarization value (P) of ~ 1410 μC/m2 for a 4 kV/cm poling field in case of Er2BaCuO5, whereas the values of TFE and P are also promising as ~ 232 K and ~ 992 μC/m2 for Dy2BaCuO5, and ~ 184 K and ~ 980 μC/m2 for Sm2BaCuO5. The synchrotron diffraction studies of Dy2BaCuO5 confirm a structural transition at TFE to a polar Pna21 structure, which correlates the FE order. An unusual magnetoelectric coupling is observed below the R order for Er and Dy compounds and below the Cu order for Sm compound, when the pyroelectric current is recorded only with the magnetic field both in heating and cooling cycles i.e. typical magnetic field cooled effect. The magnetic field cooled effect driven emergence of polarization is ferroelectric in nature, as it reverses due to the opposite poling field. The unexplored R2BaCuO5 series attracts the community for large TFE, high P value, and strange magnetoelectric consequences.

cond-mat.mtrl-sci↗

arXiv2019

Ferroelectric order associated with an ordered occupancy at the octahedral site of the inverse spinel structure of multiferroic NiFe2O4

We report a ferroelectric order at ~ 98 K for NiFe2O4, which carries an inverse spinel structure with a centrosymmetric Fd3m structure at room temperature. The value of spontaneous electric polarization is considerably high as ~ 0.29 μC/cm2 for 5 kV/cm poling field. The electric polarization decreases considerably (~ 17 %) around liquid nitrogen temperature upon application of 50 kOe field, proposing a significant magnetoelectric coupling. The synchrotron diffraction studies confirm a structural transition at ~ 98 K to a noncentrosymmetric structure of P4122 space group. The occurrence of polar order is associated with an ordered occupancy of Ni and Fe atoms at the octahedral sites of the P4122 structure, instead of random occupancies at the octahedral site of the inverse spinel structure. The results propose that NiFe2O4 is a new type-II multiferroic material.

cond-mat.mtrl-sci↗

arXiv2019

Magnetic states of Ni-Mn-Sn based shape memory alloy: a combined muon spin relaxation and neutron diffraction study

The fascinating multiple magnetic states observed in the Ni-Mn-Sn based metamagnetic shape memory alloy are addressed through a combined muon spin relaxation (muSR) and neutron powder diffraction studies. The material used in the present investigation is an off-stoichiometric alloy of nominal composition, Ni[2.04]Mn[1.4]Sn[0.56]. This prototypical alloy, similar to other members in the Ni-Mn-Sn series, orders ferromagnetically below T[CA] (= 320 K), and undergoes martensitic type structural transition at T[MS] (= 290 K), which is associated with the sudden loss of magnetization. The sample regains its magnetization below another magnetic transition at T[CM] = 260 K. Eventually, the composition shows a step-like anomaly at T[B] = 120 K, which is found to coincide with the blocking temperature of exchange bias effect observed in the alloy. In our study, the initial asymmetry A_[10] ) of the $μ$SR data falls rapidly below T[CA], indicating the onset of bulk magnetic order. A[10] regains its full asymmetry value below T[MS] suggesting the collapse of the ferromagnetic order into a fully disordered paramagnetic state. Below the second magnetic transition at T[CM], asymmetry drops again, confirming the re-entrance of a long range ordered state. Interestingly, A[10] increases sluggishly below T[B], indicating that the system attains a disordered/glassy magnetic phase below T[B], which is responsible for the exchange bias and frequency dispersion in the ac susceptibility data as previously reported. The neutron powder diffraction data do not show any magnetic superlattice reflections, ruling out the possibility of a long range antiferromagnetic state at low temperatures. The ground state is likely to be comprised of a concentrated metallic spin-glass in the backdrop of an ordered ferromagnetic state.

cond-mat.str-el↗

arXiv2018

Magnetic Order and Lattice Instabilities in Ni$_{2}$Mn$_{1+x}$Sn$_{1-x}$ Heusler based Magnetic Shape-Memory Alloys

The magnetic correlations in the austenite phase and the consequent martensitic transition in inverse magnetocaloric alloys, Ni$_{2}$Mn$_{1+x}$Sn$_{1-x}$, have been a matter of debate for decades. We conclusively establish using {\it ab initio} phonon calculations that the spin alignment of excess Mn at the Sn site (Mn$_{Sn}$) with the existing Mn in the unit cell in the high temperature cubic phase of Ni-Mn-Sn alloy is ferromagnetic (FM), and not ferrimagnetic (FI), resolving a long lasting controversy. Using first principles density functional perturbation theory (DFPT), we observe an instability of the TA$_{2}$ mode along the $Γ$-M direction in the FM phase, very similar to that observed in the prototypical ferromagnetic shape memory alloy (FSMA) Ni$_{2}$MnGa. This specific instability is not observed in the FI phase. Further finite temperature first principles lattice dynamics calculations reveal that at 300 K the FM phase becomes mechanically stable, while the FI phase continue to remain unstable providing credence to the fact that the high-temperature phase has FM order. These results will be primordial to understand the magneto-structural properties of this class of compounds.

cond-mat.str-el↗

arXiv2018

Unconventional transport behavior in the Quaternary Heusler compounds CoFeTiSn and CoFeVGa

We report here the electrical transport and magnetic properties of the newly synthesized quaternary Heusler compound CoFeTiSn and CoFeVGa. We observe a striking change in the electronic transport properties of CoFeTiSn as the system undergoes the paramagnetic to ferromagnetic transition. While the sample shows an activated semiconducting behaviour in the paramagnetic phase, it turns abruptly to a metallic phase with the onset of ferromagnetic transition. We have compared the system with other Hesuler compounds showing similar anomaly in transport, and it appears that CoFeTiSn has much similarities with the Fe$_2$VAl compound having pseudogap in the paramagnetic phase. In sharp contrast, CoFeVGa shows a predominantly semiconducting behaviour down to 90 K, below which it shows a window of metallic region. Both the compositions show negative Seebeck coefficient varying linearly with temperature. The value of the Seebeck coefficient of CoFeTiSn is comparable to that of many Heusler alloys identified as potential thermoelectric materials.

cond-mat.mtrl-sci↗

arXiv2018

Magnetoelastic coupling and ferromagnetic-type in-gap spin excitations in multiferroic $α$-Cu$_2$V$_2$O$_7$

We investigate magnetoelectric coupling and low-energy magnetic excitations in multiferroic $α$-Cu$_2$V$_2$O$_7$ by detailed thermal expansion, magnetostriction, specific heat and magnetization measurements in magnetic fields up to 15~T and by high-field/high-frequency electron spin resonance studies. Our data show negative thermal expansion in the temperature range $\leq 200$~K under study. Well-developed anomalies associated with the onset of multiferroic order (canted antiferromagnetism with a significant magnetic moment and ferroelectricity) imply pronounced coupling to the structure. We detect anomalous entropy changes in the temperature regime up to $\sim 80$~K which significantly exceed the spin entropy. Failure of Grüneisen scaling further confirms that several dominant ordering phenomena are concomitantly driving the multiferroic order. By applying external magnetic fields, anomalies in the thermal expansion and in the magnetization are separated. Noteworthy, the data clearly imply the development of a canted magnetic moment at temperatures above the structural anomaly. Low-field magnetostriction supports the scenario of exchange-striction driven multiferroicity. We observe low-energy magnetic excitations well below the antiferromagnetic gap, i.e., a ferromagnetic-type resonance branch associated with the canted magnetic moment arising from Dzyaloshinsii-Moriya interactions. The anisotropy parameter $\tilde{D}=1.6(1)$~meV indicates a sizeable ratio of DM- and isotropic magnetic exchange.

cond-mat.str-el↗

arXiv2017

Observation of non-Fermi liquid behavior in hole doped Eu2Ir2O7

The Weyl semimetallic compound Eu2Ir2O7 along with its hole doped derivatives (which is achieved by substituting trivalent Eu by divalent Sr) are investigated through transport, magnetic and calorimetric studies. The metal-insulator transition (MIT) temperature is found to get substantially reduced with hole doping and for 10% Sr doping the composition is metallic down to temperature as low as 5 K. These doped compounds are found to violate the Mott-Ioffe-Regel condition for minimum electrical conductivity and show distinct signature of non-Fermi liquid behavior at low temperature. The MIT in the doped compounds does not correlate with the magnetic transition point and Anderson-Mott type disorder induced localization may be attributed to the ground state insulating phase. The observed non-Fermi liquid behavior can be understood on the basis of disorder induced distribution of spin orbit coupling parameter which is markedly different in case of Ir4+ and Ir5+ ions.

cond-mat.str-el↗

arXiv2017

Upper limits on the 21-cm Epoch of Reionization power spectrum from one night with LOFAR

We present the first limits on the Epoch of Reionization (EoR) 21-cm HI power spectra, in the redshift range $z=7.9-10.6$, using the Low-Frequency Array (LOFAR) High-Band Antenna (HBA). In total 13\,h of data were used from observations centred on the North Celestial Pole (NCP). After subtraction of the sky model and the noise bias, we detect a non-zero $Δ^2_{\rm I} = (56 \pm 13 {\rm mK})^2$ (1-$σ$) excess variance and a best 2-$σ$ upper limit of $Δ^2_{\rm 21} < (79.6 {\rm mK})^2$ at $k=0.053$$h$cMpc$^{-1}$ in the range $z=$9.6-10.6. The excess variance decreases when optimizing the smoothness of the direction- and frequency-dependent gain calibration, and with increasing the completeness of the sky model. It is likely caused by (i) residual side-lobe noise on calibration baselines, (ii) leverage due to non-linear effects, (iii) noise and ionosphere-induced gain errors, or a combination thereof. Further analyses of the excess variance will be discussed in forthcoming publications.

astro-ph.CO↗

arXiv2016

Giant Positive Magnetoresistance and field-induced metal insulator transition in Cr2NiGa

We report here the magneto-transport properties of the newly synthesized Heusler compound Cr2NiGa which crystallizes in a disordered cubic B2 structure belonging to Pm-3m space group. The sample is found to be paramagnetic down to 2 K with metallic character. On application of magnetic field, a significantly large increase in resistivity is observed which corresponds to magnetoresistance as high as 112% at 150 kOe of field at the lowest temperature. Most remarkably, the sample shows negative temperature coefficient of resistivity below about 50 K under the application of field gretare than or equal to 80 kOe, signifying a field-induced metal to `insulating' transition. The observed magnetoresistance follows Kohler's rule below 20 K indicating the validity of the semiclassical model of electronic transport in metal with a single relaxation time. A multi-band model for electronic transport, originally proposed for semimetals, is found to be appropriate to describe the magneto-transport behavior of the sample.

cond-mat.str-el↗