arXiv subjects

S. Michimasa

Publications and source records attributed to S. Michimasa.

At least 19 recordsLinked to original sources

arXiv2026

Single-particle strength toward N = 32: Spectroscopy of 51 Ca via the 50 Ca(d, p) reaction

States in the neutron-rich isotope 51 Ca were populated via the 50 Ca(d, p) transfer reaction in inverse kinematics at a beam energy of about 14 AMeV. The experiment was performed using a decelerated radioactive 50 Ca beam from the OEDO facility and the TiNA2 silicon array in combination with the SHARAQ magnetic spectrometer at RIBF/RIKEN. The energies of excited states in 51 Ca were reconstructed via missing mass spectroscopy, and angular distributions of protons were measured to extract differential cross sections. From a comparison with adiabatic distorted wave approximation (ADWA) calculations, spectroscopic factors were deduced for several states, including the ground state and excited states up to 4.2 MeV. These results are compared with shell-model calculations, as well as ab initio valence-space in-medium similarity renormalization group (VS-IMSRG) predictions. The data support the assignment of the 1/2- and 5/2- single-particle states and provide evidence for a candidate 9/2+ state with a structure consistent with neutron excitation into the 0g9/2 orbital. These findings contribute new constraints on the single-particle structure and shell evolution in neutron-rich calcium isotopes.

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arXiv2026

High-Precision Mass Measurements of Proton-Rich Rh, Pd, Cd isotopes in the vicinity of 100Sn and Impact on X-Ray Burst and Supernova Nucleosynthesis

Using the ZeroDegree multi-reflection time-of-flight mass spectrograph of the CRISMASS project at RIKEN Radioactive Isotope Beam Factory, we performed high-precision mass measurements of proton-rich nuclei near the doubly magic nucleus 100Sn, achieving uncertainties on the order of 10 keV. The masses of 91Rh, 92Pd, and 96Cd were determined for the first time with high precision, and the accuracy of several additional masses was substantially improved. Incorporating the new data into X-ray burst simulations significantly reduces the abundance uncertainties in the $A$ = 90-100 region, shifting the reaction flow toward $A$ = 90 production and suppressing the synthesis of heavier nuclei. Further investigation of the $\nu p$-process indicates that 99Rh plays a significant role in the reaction flow within the mass region studied. These high-precision mass measurements refine the mass surface near 100Sn and provide critical constraints on models of proton-rich nucleosynthesis.

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arXiv2026

First Extraction of the Matter Radius of $^{132}$Sn via Proton Elastic Scattering at 200 MeV/Nucleon

The angular distribution of the differential cross sections for proton elastic scattering from $^{132}$Sn at 196-210 MeV/nucleon was successfully measured over a momentum transfer range of 0.80 to 2.1 fm$^{-1}$. Using a relativistic impulse approximation, the root-mean-square matter radius of $^{132}$Sn was extracted to be $4.758^{+0.023}_{-0.024}$ fm, which was compared with the state-of-the-art ab initio calculations. Combined with the charge radius measured at ISOLDE, there are no theoretical calculations consistent with both matter and charge radii within the experimental errors.

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arXiv2025

Precision mass measurements around ${}^{84}$Mo rule out ZrNb cycle formation in the rapid proton-capture process at type I X-ray bursts

The rapid proton-capture ($rp$-) process is one of the primary, explosive thermonuclear burning processes that drive type I X-ray bursts. A possible termination of the $rp$-process at around ${}^{84}$Mo was previously suggested by the formation of a ZrNb cycle. We report here precision mass measurements at around ${}^{84}$Mo, which have concluded the possibility of the cycle. The experiment was conducted using the multi-reflection time-of-flight spectrograph at RIKEN RI Beam Factory, and the masses of ${}^{79}$Y, ${}^{83}$Nb, ${}^{84}$Mo, ${}^{88}$Ru, and an isomer in ${}^{78}$Y were measured. For ${}^{84}$Mo, and ${}^{88}$Ru, and the isomeric state of ${}^{78}$Y, their masses are experimentally determined for the first time with uncertainties of $\delta m \approx 20~{\rm keV/c^2}$. The mass precision of ${}^{79}$Y and ${}^{83}$Nb is improved to $13~{\rm keV/c^2}$ and $9.6~{\rm keV/c^2}$, respectively. The new $\alpha$-separation energy of ${}^{84}$Mo, 1.434(83) MeV, unambiguously rules out the possibility of forming the ZrNb cycle. The X-ray burst simulation with the new masses shows that our measurements effectively remove the large final abundance uncertainties in the $A=80-90$ mass region. The new mass values improve the prediction power for the composition of the nuclear ashes in X-ray bursts.

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arXiv2024

Isochronous mass spectrometry at the RIKEN Rare-RI Ring facility

A dedicated isochronous storage ring, named the Rare-RI Ring, was constructed at the RI Beam Factory of RIKEN, aiming at precision mass measurements of nuclei located in uncharted territories of the nuclear chart. The Rare-RI Ring employs the isochronous mass spectrometry technique with the goal to achieve a relative mass precision of $10^{-6}$ within a measurement time of less than 1 ms. The performance of the facility was demonstrated through mass measurements of neutron-rich nuclei with well-known masses. Velocity or magnetic rigidity is measured for every particle prior to its injection into the ring, wherein its revolution time is accurately determined. The latter quantity is used to determine the mass of the particle, while the former one is needed for non-isochronicity corrections. Mass precisions on the order of $10^{-5}$ were achieved in the first commissioning, which demonstrates that Rare-RI Ring is a powerful tool for mass spectrometry of short-lived nuclei.

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arXiv2023

Enlarged deformation region in neutron-rich Zr isotopes by the second intruder orbit

Nuclear deformations and density profiles of neutron-rich even-even Zr isotopes are investigated using the Skyrme-Hartree-Fock-Bogoliubov method. Large quadrupole and hexadecapole deformations are predicted along with large enhancement of the total reaction cross sections at the neutron number $N=60$-74. Strong nuclear deformation starting at $N=60$ is induced by the occupation of the intruder orbit with the asymptotic quantum number $[nn_zΛ]Ω$ = [550]1/2 originating from the spherical $0h_{11/2}$ orbit. The deformation region is further enlarged from $N=72$ to 74 owing to the occupation of the next intruder orbit with [530]1/2 originating from the spherical $1f_{7/2}$ orbit. This characteristic nuclear deformation is crucially reflected in the systematic behavior of the nuclear radii and the density profiles near the nuclear surface.

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arXiv2022

A new study of the $N=32$ and $N=34$ shell gap for Ti and V by the first high-precision MRTOF mass measurements at BigRIPS-SLOWRI

The atomic masses of $^{55}$Sc, $^{56,58}$Ti, and $^{56-59}$V have been determined using the high-precision multi-reflection time-of-flight technique. The radioisotopes have been produced at RIKEN's RIBF facility and delivered to the novel designed gas cell and multi-reflection system (ZD MRTOF), which has been recently commissioned downstream of the ZeroDegree spectrometer following the BigRIPS separator. For $^{56,58}$Ti and $^{56-59}$V the mass uncertainties have been reduced down to the order of $10\,\mathrm{keV}$, shedding new light on the $N=34$ shell effect in Ti and V isotopes by the first high-precision mass measurements of the critical species $^{58}$Ti and $^{59}$V. With the new precision achieved, we reveal the non-existence of the $N=34$ empirical two-neutron shell gaps for Ti and V, and the enhanced energy gap above the occupied $νp_{3/2}$ orbit is identified as a feature unique to Ca. We perform new Monte Carlo shell model calculations including the $νd_{5/2}$ and $νg_{9/2}$ orbits and compare the results with conventional shell model calculations, which exclude the $νg_{9/2}$ and the $νd_{5/2}$ orbits. The comparison indicates that the shell gap reduction in Ti is related to a partial occupation of the higher orbitals for the outer two valence neutrons at $N=34$.

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arXiv2022

The new MRTOF mass spectrograph following the ZeroDegree spectrometer at RIKEN's RIBF facility

A newly assembled multi-reflection time-of-flight mass spectrograph (MRTOF-MS) at RIKEN's RIBF facility became operational for the first time in spring 2020; further modifications and performance tests using stable ions were completed in early 2021. By using a pulsed-drift-tube technique to modify the ions' kinetic energy in a wide range, we directly characterize the dispersion function of the system for use in a new procedure for optimizing the voltages applied to the electrostatic mirrors. Thus far, a mass resolving power of $R_m > 1\,000\,000$ is reached within a total time-of-flight of only $12.5\,\mathrm{ms}$, making the spectrometer capable of studying short-lived nuclei possessing low-lying isomers. Detailed information about the setup and measurement procedure is reported, and an alternative in-MRTOF ion selection scheme to remove molecular contaminants in the absence of a dedicated deflection device is introduced. The setup underwent an initial on-line commissioning at the BigRIPS facility at the end of 2020, where more than 70 nuclear masses have been measured. A summary of the commissioning experiments and results from a test of mass accuracy will be presented.

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arXiv2022

First application of mass measurement with the Rare-RI Ring reveals the solar r-process abundance trend at A=122 and A=123

The Rare-RI Ring (R3) is a recently commissioned cyclotron-like storage ring mass spectrometer dedicated to mass measurements of exotic nuclei far from stability at Radioactive Isotope Beam Factory (RIBF) in RIKEN. The first application of mass measurement using the R3 mass spectrometer at RIBF is reported. Rare isotopes produced at RIBF, $^{127}$Sn, $^{126}$In, $^{125}$Cd, $^{124}$Ag, $^{123}$Pd, were injected in R3. Masses of $^{126}$In, $^{125}$Cd, and $^{123}$Pd were measured whereby the mass uncertainty of $^{123}$Pd was improved. This is the first reported measurement with a new storage ring mass spectrometery technique realized at a heavy-ion cyclotron and employing individual injection of the pre-identified rare nuclei. The latter is essential for the future mass measurements of the rarest isotopes produced at RIBF. The impact of the new $^{123}$Pd result on the solar $r$-process abundances in a neutron star merger event is investigated by performing reaction network calculations of 20 trajectories with varying electron fraction $Y_e$. It is found that the neutron capture cross section on $^{123}$Pd increases by a factor of 2.2 and $β$-delayed neutron emission probability, $P_\mathrm{1n}$, of $^{123}$Rh increases by 14\%. The neutron capture cross section on $^{122}$Pd decreases by a factor of 2.6 leading to pileup of material at $A=122$, thus reproducing the trend of the solar $r$-process abundances. The trend of the two-neutron separation energies (S$_\mathrm{2n}$) was investigated for the Pd isotopic chain. The new mass measurement with improved uncertainty excludes large changes of the S$_\mathrm{2n}$ value at $N=77$. Such large increase of the S$_\mathrm{2n}$ values before $N=82$ was proposed as an alternative to the quenching of the $N=82$ shell gap to reproduce $r$-process abundances in the mass region of $A=112-124$.

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arXiv2022

Large enhancement of total reaction cross sections at the edge of the island of inversion in Ti, Cr, and Fe isotopes

A systematic analysis of nuclear deformation is made for neutron-rich Ti, Cr, and Fe isotopes to explore the nuclear structure in the island of inversion near N = 40, where strong nuclear deformation is predicted. The nuclear ground states are obtained by the Skyrme Hartree-Fock method in three-dimensional coordinate space, which properly describes any nuclear shape. Three types of Skyrme interactions are employed to generate various deformed states in its isotopic chain. We find that in the island of inversion the occupation of highly elongated intruder orbits induces not only large quadrupole deformation but also large hexadecapole deformation. This appears as a sizable enhancement of the nuclear matter radius, showing the characteristic shell effect of the density profile near the nuclear surface. We show that the edge of the island of inversion, where the intruder orbit starts being occupied, can be determined by measuring the enhancement of the total reaction cross section at high incident energy. The possibility of constraining the hexadecapole deformation by a measurement of the total reaction cross sections is discussed.

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arXiv2020

Development and operation of an electrostatic time-of-flight detector for the Rare RI storage Ring

An electrostatic time-of-flight detector named E-MCP has been developed for quick diagnostics of circulating beam and timing measurement in mass spectrometry at the Rare-RI Ring in RIKEN. The E-MCP detector consists of a conversion foil, potential grids, and a microchannel plate. Secondary electrons are released from the surface of the foil when a heavy ion hits it. The electrons are accelerated and deflected by 90$^\circ$ toward the microchannel plate by electrostatic potentials. A thin carbon foil and a thin aluminum-coated mylar foil were used as conversion foils. We obtained time resolutions of 69(1) ps and 43(1) ps (standard deviation) for a $^{84}$Kr beam at an energy of 170 MeV/u when using the carbon and the aluminum-coated mylar foils, respectively. A detection efficiency of approximately 90% was obtained for both foils. The E-MCP detector equipped with the carbon foil was installed inside the Rare-RI Ring to confirm particle circulation within a demonstration experiment on mass measurements of nuclei around $^{78}$Ge produced by in-flight fission of uranium beam at the RI Beam Factory in RIKEN. Periodic time signals from circulating ions were clearly observed. Revolution times for $^{78}$Ge, $^{77}$Ga, and $^{76}$Zn were obtained. The results confirmed successful circulation of the short-lived nuclei inside the Rare-RI Ring.

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arXiv2020

Parity-transfer $({}^{16}{\rm O},{}^{16}{\rm F}(0^-,{\rm g.s.}))$ reaction as a selective probe of isovector $0^-$ states in nuclei

We demonstrate that the parity-transfer $({}^{16}{\rm O},{}^{16}{\rm F}(0^-,{\rm g.s.}))$ reaction provides a selective probe of isovector $0^-$ excitations in nuclei. This reaction selectively populates unnatural-parity states through a $0^+ \to 0^-$ transition in the projectile. The excitation-energy spectrum of $^{12}\mathrm{B}$ was reconstructed via the ${}^{12}{\rm C}({}^{16}{\rm O},{}^{16}{\rm F}(0^-,{\rm g.s.}))$ reaction at 247~MeV/u from the coincident detection of the ${}^{15}\mathrm{O}+p$ decay products of ${}^{16}\mathrm{F}$. The known $0^{-}$ state at $E_x = 9.3~{\rm MeV}$ was clearly observed with an enhanced forward cross section, confirming the selectivity of the reaction. Structures observed at $E_x = 6.6 \pm 0.4$ and $14.8 \pm 0.3~{\rm MeV}$ exhibit forward-peaked angular distributions and are suggested to contain significant $0^-$ strength. These results demonstrate that the parity-transfer reaction provides a powerful probe of $0^-$ excitations and highlight its potential for systematic studies of spin-isospin modes, including pion-related dynamics, in nuclei.

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arXiv2018

How different is the core of $^{25}$F from $^{24}$O$_{g.s.}$?

The neutron-shell structure of $^{25}$F was studied using quasi-free (p,2p) knockout reaction at 270A MeV in inverse kinematics. The sum of spectroscopic factors of $π$0d$_{5/2}$ orbital is found to be $1.0 \pm 0.3$. However, the spectroscopic factor for the ground-state to ground-state transition ($^{25}$F, $^{24}$O$_{g.s.}$) is only $0.36\pm 0.13$, and $^{24}$O excited states are produced from the 0d$_{5/2}$ proton knockout. The result shows that the $^{24}$O core of $^{25}$F nucleus significantly differs from a free $^{24}$O nucleus, and the core consists of 35% $^{24}$O$_{g.s}$. and 65% excited $^{24}$O.

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arXiv2018

Spectroscopy of pionic atoms in $\mathbf{{}^{122}{\textbf Sn}({\textit d},{}^3{\textbf He})}$ reaction and angular dependence of the formation cross sections

We observed the atomic $1s$ and $2p$ states of $π^-$ bound to ${}^{121}{\rm Sn}$ nuclei as distinct peak structures in the missing mass spectra of the ${}^{122}{\rm Sn}(d,{}^3{\rm He})$ nuclear reaction. A very intense deuteron beam and a spectrometer with a large angular acceptance let us achieve potential of discovery, which includes capability of determining the angle-dependent cross sections with high statistics. The $2p$ state in a Sn nucleus was observed for the first time. The binding energies and widths of the pionic states are determined and found to be consistent with previous experimental results of other Sn isotopes. The spectrum is measured at finite reaction angles for the first time. The formation cross sections at the reaction angles between 0 and $2^\circ$ are determined. The observed reaction-angle dependence of each state is reproduced by theoretical calculations. However, the quantitative comparison with our high-precision data reveals a significant discrepancy between the measured and calculated formation cross sections of the pionic $1s$ state.

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arXiv2017

Structure of 55Sc and development of the N=34 subshell closure

The low-lying structure of $^{55}$Sc has been investigated using in-beam $γ$-ray spectroscopy with the $^{9}$Be($^{56}$Ti,$^{55}$Sc+$γ$)$X$ one-proton removal and $^{9}$Be($^{55}$Sc,$^{55}$Sc+$γ$)$X$ inelastic-scattering reactions at the RIKEN Radioactive Isotope Beam Factory. Transitions with energies of 572(4), 695(5), 1539(10), 1730(20), 1854(27), 2091(19), 2452(26), and 3241(39) keV are reported, and a level scheme has been constructed using $γγ$ coincidence relationships and $γ$-ray relative intensities. The results are compared to large-scale shell-model calculations in the $sd$-$pf$ model space, which account for positive-parity states from proton-hole cross-shell excitations, and to it ab initio shell-model calculations from the in-medium similarity renormalization group that includes three-nucleon forces explicitly. The results of proton-removal reaction theory with the eikonal model approach were adopted to aid identification of positive-parity states in the level scheme; experimental counterparts of theoretical $1/2^{+}_{1}$ and $3/2^{+}_{1}$ states are suggested from measured decay patterns. The energy of the first $3/2^{-}$ state, which is sensitive to the neutron shell gap at the Fermi surface, was determined. The result indicates a rapid weakening of the $N=34$ subshell closure in $pf$-shell nuclei at $Z>20$, even when only a single proton occupies the $πf_{7/2}$ orbital.

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arXiv2016

Separated flow operation of the SHARAQ spectrometer for in-flight proton decay experiments

New operation mode, "separated flow mode", has been developed for in-flight proton decay experiments with the SHARAQ spectrometer. In the separated flow mode, the protons and the heavy-ion products are separated and measured in coincidence at two different focal planes of SHARAQ. The ion-optical properties of the new mode were studied by using a proton beam at $246~{\rm MeV}$, and the momentum vector was properly reconstructed from the parameters measured in the focal plane of SHARAQ. In the experiment with the $({}^{16}{\rm O},{}^{16}{\rm F})$ reaction at a beam energy of $247~{\rm MeV/u}$, the outgoing ${}^{15}{\rm O}+p$ produced by the decay of ${}^{16}{\rm F}$ were measured in coincidence with SHARAQ. High energy resolutions of $100~{\rm keV}$ (FWHM) and $\sim 2~{\rm MeV}$ were achieved for the relative energy of $535~{\rm keV}$, and the ${}^{16}{\rm F}$ energy of $3940~{\rm MeV}$, respectively.

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arXiv2012

Well-developed deformation in 42Si

Excited states in 38,40,42Si nuclei have been studied via in-beam gamma-ray spectroscopy with multi-nucleon removal reactions. Intense radioactive beams of 40S and 44S provided at the new facility of the RIKEN Radioactive Isotope Beam Factory enabled gamma-gamma coincidence measurements. A prominent gamma line observed with an energy of 742(8) keV in 42Si confirms the 2+ state reported in an earlier study. Among the gamma lines observed in coincidence with the 2+ -> 0+ transition, the most probable candidate for the transition from the yrast 4+ state was identified, leading to a 4+_1 energy of 2173(14) keV. The energy ratio of 2.93(5) between the 2+_1 and 4+_1 states indicates well-developed deformation in 42Si at N=28 and Z=14. Also for 38,40Si energy ratios with values of 2.09(5) and 2.56(5) were obtained. Together with the ratio for 42Si, the results show a rapid deformation development of Si isotopes from N=24 to N=28.

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arXiv2009

Spectroscopy of 32Ne and the Island of Inversion

We report on the first spectroscopic study of the N=22 nucleus 32Ne at the newly completed RIKEN Radioactive Ion Beam Factory. A single gamma-ray line with an energy of 722(9) keV was observed in both inelastic scattering of a 226 MeV/u 32Ne beam on a Carbon target and proton removal from 33Na at 245 MeV/u. This transition is assigned to the de-excitation of the first J^pi = 2+ state in 32Ne to the 0+ ground state. Interpreted through comparison with state-of-the-art shell model calculations, the low excitation energy demonstrates that the Island of Inversion extends to at least N=22 for the Ne isotopes.

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