SearcharxivSearch

arXiv subjects

S. Mosby

Publications and source records attributed to S. Mosby.

At least 19 recordsLinked to original sources

Meaurement of spin vs. TKE of $^{144}$Ba produced in spontaneous fission of $^{252}$Cf

We measure the average spin of $^{144}$Ba, a common fragment produced in $^{252}$Cf(sf), as a function of the total kinetic energy (TKE). We combined for the first time a twin Frisch-gridded ionization chamber with a world-class $\gamma$-ray spectrometer that was designed to measure high-multiplicity $\gamma$-ray events, Gammasphere. The chamber, loaded with a $^{252}$Cf(sf) source, provides a fission trigger, the TKE of the fragments, the approximate fragment masses, and the polar angle of the fission axis. Gammasphere provides the total $\gamma$-ray yield, fragment identification through the tagging of decay $\gamma$ rays, and the feeding of rotational bands in the fragments. We determine the dependence of the average spin of $^{144}$Ba on the fragments' TKE by correlating the fragment properties with the distribution of discrete levels that are fed. We find that the average spin only changes by about $0.5$ $\hbar$ across the TKE range of 158-203 MeV. The virtual independence of the spin on TKE suggests that spin is not solely generated through the statistical excitation of rotational modes, and more complex mechanisms are required.

nucl-ex

Enhanced production of 60Fe in massive stars

Massive stars are a major source of chemical elements in the cosmos, ejecting freshly produced nuclei through winds and core-collapse supernova explosions into the interstellar medium. Among the material ejected, long lived radioisotopes, such as 60Fe (iron) and 26Al (aluminum), offer unique signs of active nucleosynthesis in our galaxy. There is a long-standing discrepancy between the observed 60Fe/26Al ratio by {\gamma}-ray telescopes and predictions from supernova models. This discrepancy has been attributed to uncertainties in the nuclear reaction networks producing 60Fe, and one reaction in particular, the neutron-capture on 59Fe. Here we present experimental results that provide a strong constraint on this reaction. We use these results to show that the production of 60Fe in massive stars is higher than previously thought, further increasing the discrepancy between observed and predicted 60Fe/26Al ratios. The persisting discrepancy can therefore not be attributed to nuclear uncertainties, and points to issues in massive-star models.

nucl-ex

Properties of correlated fission fragments from neutron induced fission of Np-237 at incident neutron energies between 200 keV and 100 MeV

Neutron-induced fission of $^{237}$Np has been measured over a wide range of incident neutron energies using a twin Frisch-gridded ionization chamber (TFGIC) and a thin-backed $^{237}$Np target. These measurements were performed at the Los Alamos Neutron Science Center - Weapons Neutron Research (LANSCE - WNR) facility, which provides a collimated beam of neutrons with energies ranging from 100s of keV to 100s of MeV. The data were analyzed using the double-energy ($2E$) method, with mass-dependent corrections for prompt-fission neutrons and pulse height defect. Pre- and post-neutron evaporation average total kinetic energy ($\langle TKE\rangle$) values are reported for 54 incident neutron energies in the energy range $0.20 \le E_n \le 100.0$ MeV and compared to existing data and evaluations. Pre- and post-neutron evaporation mass yields were extracted with a full width at half maximum (FWHM) resolution of 4u and compared to existing data and evaluations. The present $\langle TKE\rangle$ and mass yield data agree with previous results and also with statistical models of $^{237}$Np$(n,f)$ at incident neutron energies between $E_n = 0.2 - 20.0$ MeV. A flattening of the $\langle TKE\rangle$ data is observed (relative to the prediction of the GEF model) above $E_n = 20.0$ MeV. However, the interpretation of this discrepancy is unclear as the analysis method's neglect of incomplete momentum transfer at high energies, as well as pre-equilibrium pre-fission phenomena likely have a significant impact on the measurement at such high incident neutron energies.

nucl-ex

Measurement of the $^{239}$Pu(n,f)/$^{235}$U(n,f) Cross-Section Ratio with the NIFFTE fission Time Projection Chamber

The $^{239}$Pu(n,f)/$^{235}$U(n,f) cross-section ratio has been measured with the fission Time Projection Chamber (fissionTPC) from 100 keV to 100 MeV. The fissionTPC provides three-dimensional reconstruction of fission-fragment ionization profiles, allowing for a precise quantification of measurement uncertainties. The measurement was performed at the Los Alamos Neutron Science Center which provides a pulsed white source of neutrons. The data are recommended to be used as a cross-section ratio shape. A discussion of the status of the absolute normalization and comparisons to ENDF evaluations and previous measurements is included.

nucl-ex

Measurement of material isotopics and atom number ratio with alpha-particle spectroscopy for the NIFFTE fission Time Projection Chamber actinide target

We present the results of a measurement of isotopic concentrations and atomic number ratio of a double-sided actinide target with alpha-spectroscopy and mass spectrometry. The double-sided actinide target, with primarily Pu-239 on one side and U-235 on the other, was used in the fission Time Projection Chamber (fissionTPC) for a measurement of the neutron-induced fission cross-section ratio between the two isotopes. The measured atomic number ratio is intended to provide an absolute normalization of the measured fission cross-section ratio. The Pu-239/U-235 atom number ratio was measured with a combination of mass spectrometry and alpha-spectroscopy with a planar silicon detector with uncertainties of less than 1%.

nucl-ex

Isotopically resolved neutron total cross sections at intermediate energies

The neutron total cross sections $\sigma_{tot}$ of $^{16,18}$O, $^{58,64}$Ni, $^{103}$Rh, and $^{112,124}$Sn have been measured at the Los Alamos Neutron Science Center (LANSCE) from low to intermediate energies (3 $\leq E_{lab} \leq$ 450 MeV) by leveraging waveform-digitizer technology. The $\sigma_{tot}$ relative differences between isotopes are presented, revealing additional information about the isovector components needed for an accurate optical-model description away from stability. Digitizer-enabled $\sigma_{tot}$-measurement techniques are discussed and a series of uncertainty-quantified dispersive optical model (DOM) analyses using these new data is presented, validating the use of the DOM for modeling light systems ($^{16,18}$O) and systems with open neutron shells ($^{58,64}$Ni and $^{112,124}$Sn). The valence-nucleon spectroscopic factors extracted for each isotope reaffirm the usefulness of high-energy proton reaction cross sections for characterizing depletion from the mean-field expectation.

nucl-ex

Neutron Induced Fission Fragment Angular Distributions, Anisotropy, and Linear Momentum Transfer Measured with the NIFFTE Fission Time Projection Chamber

The Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) collaboration has performed measurements with a fission time projection chamber (fissionTPC) to study the fission process by reconstructing full three-dimensional tracks of fission fragments and other ionizing radiation. The amount of linear momentum imparted to the fissioning nucleus by the incident neutron can be inferred by measuring the opening angle between the fission fragments. Using this measured linear momentum, fission fragment angular distributions can be converted to the center-of-mass frame for anisotropy measurements. Angular anisotropy is an important experimental observable for understanding the quantum mechanical state of the fissioning nucleus and vital to determining detection efficiency for cross section measurements. Neutron linear momentum transfer to fissioning $^{235}$U, $^{238}$U, and $^{239}$Pu and fission fragment angular anisotropy of $^{235}$U and $^{238}$U as a function of neutron energies in the range 130 keV--250 MeV are presented.

nucl-ex

1H(n,el) as a Cross Section Reference in a White Source Neutron Beam With the fissionTPC

We provide a quantitative description of a method to measure neutron-induced fission cross sections in ratio to elastic hydrogen scattering in a white-source neutron beam with the fission Time Projection Chamber. This detector has measured precision fission cross section ratios using actinide references such as $^{235}$U(n,f) and $^{238}$U(n,f). However, by employing a more precise reference such as the H(n,el) cross section there is the potential to further reduce the evaluation uncertainties of the measured cross sections. In principle the fissionTPC could provide a unique measurement by simultaneously measuring both fission fragments and proton recoils over a large solid angle. We investigate one method with a hydrogenous gas target and with the neutron energy determined by the proton recoil kinematics. This method enables the measurement to be performed in a white-source neutron beam and with the current configuration of the fissionTPC. We show that while such a measurement is feasible in the energy range of 0.5 MeV to $\sim$10 MeV, uncertainties on the proton detection efficiency and the neutron energy resolution do not allow us to preform a fission ratio measurement to the desired precision. Utilizing either a direct measurement of the neutron time-of-flight for the recoil proton or a mono-energetic neutron source or some combination of both would provide a path to a sub-percent precision measurement.

nucl-ex

Enhanced low-energy $\gamma$-decay strength of $^{70}$Ni and its robustness within the shell model

Neutron-capture reactions on very neutron-rich nuclei are essential for heavy-element nucleosynthesis through the rapid neutron-capture process, now shown to take place in neutron-star merger events. For these exotic nuclei, radiative neutron capture is extremely sensitive to their $\gamma$-emission probability at very low $\gamma$ energies. In this work, we present measurements of the $\gamma$-decay strength of $^{70}$Ni over the wide range $1.3 \leq E_{\gamma} \leq 8 $ MeV. A significant enhancement is found in the $\gamma$-decay strength for transitions with $E_\gamma < 3$ MeV. At present, this is the most neutron-rich nucleus displaying this feature, proving that this phenomenon is not restricted to stable nuclei. We have performed $E1$-strength calculations within the quasiparticle time-blocking approximation, which describe our data above $E_\gamma \simeq 5$ MeV very well. Moreover, large-scale shell-model calculations indicate an $M1$ nature of the low-energy $\gamma$ strength. This turns out to be remarkably robust with respect to the choice of interaction, truncation and model space, and we predict its presence in the whole isotopic chain, in particular the neutron-rich $^{72,74,76}\mathrm{Ni}$.

nucl-ex

Three-body correlations in the ground-state decay of 26O

Background: Theoretical calculations have shown that the energy and angular correlations in the three-body decay of the two-neutron unbound O26 can provide information on the ground-state wave function, which has been predicted to have a dineutron configuration and 2n halo structure. Purpose: To use the experimentally measured three-body correlations to gain insight into the properties of O26, including the decay mechanism and ground-state resonance energy. Method: O26 was produced in a one-proton knockout reaction from F27 and the O24+n+n decay products were measured using the MoNA-Sweeper setup. The three-body correlations from the O26 ground-state resonance decay were extracted. The experimental results were compared to Monte Carlo simulations in which the resonance energy and decay mechanism were varied. Results: The measured three-body correlations were well reproduced by the Monte Carlo simulations but were not sensitive to the decay mechanism due to the experimental resolutions. However, the three-body correlations were found to be sensitive to the resonance energy of O26. A 1σ upper limit of 53 keV was extracted for the ground-state resonance energy of O26. Conclusions: Future attempts to measure the three-body correlations from the ground-state decay of O26 will be very challenging due to the need for a precise measurement of the O24 momentum at the reaction point in the target.

nucl-ex

Search for unbound 15Be states in the 3n+12Be channel

15Be is expected to have low-lying 3/2+ and 5/2+ states. A first search did not observe the 3/2+ [A. Spyrou et al., Phys. Rev. C 84, 044309 (2011)], however, a resonance in 15Be was populated in a second attempt and determined to be unbound with respect to 14Be by 1.8(1) MeV with a tentative spin-parity assignment of 5/2+ [J. Snyder et al., Phys. Rev. C 88, 031303(R) (2013)]. Search for the predicted 15Be 3/2+ state in the three-neutron decay channel. A two-proton removal reaction from a 55 MeV/u 17C beam was used to populate neutron-unbound states in 15Be. The two-, three-, and four-body decay energies of the 12Be + neutron(s) detected in coincidence were reconstructed using invariant mass spectroscopy. Monte Carlo simulations were performed to extract the resonance and decay properties from the observed spectra. The low-energy regions of the decay energy spectra can be described with the first excited unbound state of 14Be (E_x=1.54 MeV, E_r=0.28 MeV). Including a state in 15Be that decays through the first excited 14Be state slightly improves the fit at higher energies though the cross section is small. A 15Be component is not needed to describe the data. If the 3/2+ state in 15Be is populated, the decay by three-neutron emission through 14Be is weak, less than or equal to 11% up to 4 MeV. In the best fit, 15Be is unbound with respect to 12Be by 1.4 MeV (unbound with respect to $14Be by 2.66 MeV) with a strength of 7%.

nucl-ex

Observation of a low-lying neutron-unbound state in 19C

Proton removal reactions from a secondary 22N beam were utilized to populate unbound states in neutron-rich carbon isotopes. Neutrons were measured with the Modular Neutron Array (MoNA) in coincidence with carbon fragments. A resonance with a decay energy of 76(14) keV was observed in the system 18C+n corresponding to a state in 19C at an excitation energy of 653(95)keV. This resonance could correspond to the first 5/2+ state which was recently speculated to be unbound in order to describe 1n and 2n removal cross section measurements from 20C.

nucl-ex

Search for $^{21}$C and constraints on $^{22}$C

A search for the neutron-unbound nucleus $^{21}$C was performed via the single proton removal reaction from a beam of 22 N at 68 MeV/u. Neutrons were detected with the Modular Neutron Array (MoNA) in coincidence with $^{20}$C fragments. No evidence for a low-lying state was found, and the reconstructed $^{20}$C+n decay energy spectrum could be described with an s-wave line shape with a scattering length limit of |as| < 2.8 fm, consistent with shell model predictions. A comparison with a renormalized zero-range three-body model suggests that $^{22}$C is bound by less than 70 keV.

nucl-ex

Study of two-neutron radioactivity in the decay of 26O

A new technique was developed to measure the lifetimes of neutron unbound nuclei in the picosecond range. The decay of 26O -> 24O+n+n was examined as it had been predicted to have an appreciable lifetime due to the unique structure of the neutron-rich oxygen isotopes. The half-life of 26O was extracted as 4.5^{+1.1}_{-1.5}(stat.) +/- 3 (sys.) ps. This corresponds to 26O having a finite lifetime at an 82% confidence level and, thus, suggests the possibility of two-neutron radioactivity.

nucl-ex

First observation of $^{13}$Li ground state

The ground state of neutron-rich unbound $^{13}$Li was observed for the first time in a one-proton removal reaction from $^{14}$Be at a beam energy of 53.6 MeV/u. The $^{13}$Li ground state was reconstructed from $^{11}$Li and two neutrons giving a resonance energy of 120$^{+60}_{-80}$ keV. All events involving single and double neutron interactions in the Modular Neutron Array (MoNA) were analyzed, simulated, and fitted self-consistently. The three-body ($^{11}$Li+$n+n$) correlations within Jacobi coordinates showed strong dineutron characteristics. The decay energy spectrum of the intermediate $^{12}$Li system ($^{11}$Li+$n$) was described with an s-wave scattering length of greater than -4 fm, which is a smaller absolute value than reported in a previous measurement.

nucl-ex

Observation of Ground-State Two-Neutron Decay

Neutron decay spectroscopy has become a successful tool to explore nuclear properties of nuclei with the largest neutron-to-proton ratios. Resonances in nuclei located beyond the neutron dripline are accessible by kinematic reconstruction of the decay products. The development of two-neutron detection capabilities of the Modular Neutron Array (MoNA) at NSCL has opened up the possibility to search for unbound nuclei which decay by the emission of two neutrons. Specifically this exotic decay mode was observed in 16Be and 26O.

nucl-ex

Exploring the neutron dripline two neutrons at a time: The first observations of the 26O and 16Be ground state resonances

The two-neutron unbound ground state resonances of $^{26}$O and $^{16}$Be were populated using one-proton knockout reactions from $^{27}$F and $^{17}$B beams. A coincidence measurement of 3-body system (fragment + n + n) allowed for the decay energy of the unbound nuclei to be reconstructed. A low energy resonance, $<$ 200 keV, was observed for the first time in the $^{24}$O + n + n system and assigned to the ground state of $^{26}$O. The $^{16}$Be ground state resonance was observed at 1.35 MeV. The 3-body correlations of the $^{14}$Be + n + n system were compared to simulations of a phase-space, sequential, and dineutron decay. The strong correlations in the n-n system from the experimental data could only be reproduced by the dineutron decay simulation providing the first evidence for a dineutron-like decay.

nucl-ex

Spectroscopy of neutron-unbound $^{27,28}$F

The ground state of $^{28}$F has been observed as an unbound resonance $2\underline{2}0$ keV above the ground state of $^{27}$F. Comparison of this result with USDA/USDB shell model predictions leads to the conclusion that the $^{28}$F ground state is primarily dominated by $sd$-shell configurations. Here we present a detailed report on the experiment in which the ground state resonance of $^{28}$F was first observed. Additionally, we report the first observation of a neutron-unbound excited state in $^{27}$F at an excitation energy of $25\underline{0}0 (2\underline{2}0)$ keV.

nucl-ex