arXiv subjects

S. N. Liddick

Publications and source records attributed to S. N. Liddick.

At least 37 records · Page 2Linked to original sources

arXiv2019

The beta-Oslo method: experimentally constrained ($n,γ$) reaction rates relevant to the $r$-process

Unknown neutron-capture reaction rates remain a significant source of uncertainty in state-of-the-art $r$-process nucleosynthesis reaction network calculations. As the $r$-process involves highly neutron-rich nuclei for which direct ($n,γ$) cross-section measurements are virtually impossible, indirect methods are called for to constrain ($n,γ$) cross sections used as input for the $r$-process nuclear network. Here we discuss the newly developed beta-Oslo method, which is capable of providing experimental input for calculating ($n,γ$) rates of neutron-rich nuclei. The beta-Oslo method represents a first step towards constraining neutron-capture rates of importance to the $r$-process.

nucl-ex↗

arXiv2019

Novel Techniques for Constraining Neutron-Capture Rates Relevant for r-Process Heavy-Element Nucleosynthesis

The rapid-neutron capture process ($r$ process) is identified as the producer of about 50\% of elements heavier than iron. This process requires an astrophysical environment with an extremely high neutron flux over a short amount of time ($\sim$ seconds), creating very neutron-rich nuclei that are subsequently transformed to stable nuclei via $β^-$ decay. One key ingredient to large-scale $r$-process reaction networks is radiative neutron-capture ($n,γ$) rates, for which there exist virtually no data for extremely neutron-rich nuclei involved in the $r$ process. Due to the current status of nuclear-reaction theory and our poor understanding of basic nuclear properties such as level densities and average $γ$-decay strengths, theoretically estimated ($n,γ$) rates may vary by orders of magnitude and represent a major source of uncertainty in any nuclear-reaction network calculation of $r$-process abundances. In this review, we discuss new approaches to provide information on neutron-capture cross sections and reaction rates relevant to the $r$ process. In particular, we focus on indirect, experimental techniques to measure radiative neutron-capture rates. While direct measurements are not available at present, but could possibly be realized in the future, the indirect approaches present a first step towards constraining neutron-capture rates of importance to the $r$ process.

nucl-ex↗

arXiv2018

Enhanced low-energy $γ$-decay strength of $^{70}$Ni and its robustness within the shell model

Neutron-capture reactions on very neutron-rich nuclei are essential for heavy-element nucleosynthesis through the rapid neutron-capture process, now shown to take place in neutron-star merger events. For these exotic nuclei, radiative neutron capture is extremely sensitive to their $γ$-emission probability at very low $γ$ energies. In this work, we present measurements of the $γ$-decay strength of $^{70}$Ni over the wide range $1.3 \leq E_γ \leq 8 $ MeV. A significant enhancement is found in the $γ$-decay strength for transitions with $E_γ< 3$ MeV. At present, this is the most neutron-rich nucleus displaying this feature, proving that this phenomenon is not restricted to stable nuclei. We have performed $E1$-strength calculations within the quasiparticle time-blocking approximation, which describe our data above $E_γ\simeq 5$ MeV very well. Moreover, large-scale shell-model calculations indicate an $M1$ nature of the low-energy $γ$ strength. This turns out to be remarkably robust with respect to the choice of interaction, truncation and model space, and we predict its presence in the whole isotopic chain, in particular the neutron-rich $^{72,74,76}\mathrm{Ni}$.

nucl-ex↗

arXiv2018

Measurement of the $^{20}$F half-life

The half-life of the $^{20}$F ground state has been measured using a radioactive beam implanted in a plastic scintillator and recording $βγ$ coincidences together with four CsI(Na) detectors. The result, $T_{1/2} = 11.0011(69)_{\rm stat}(30)_{\rm sys}$~s, is at variance by 17 combined standard deviations with the two most precise results. The present value revives the poor consistency of results for this half-life and calls for a new measurement, with a technique having different sources of systematic effects, to clarify the discrepancy.

nucl-ex↗

arXiv2018

r-Process Nucleosynthesis: Connecting Rare-Isotope Beam Facilities with the Cosmos

This is an exciting time for the study of r-process nucleosynthesis. Recently, a neutron star merger GW170817 was observed in extraordinary detail with gravitational waves and electromagnetic radiation from radio to gamma rays. The very red color of the associated kilonova suggests that neutron star mergers are an important r-process site. Astrophysical simulations of neutron star mergers and core collapse supernovae are making rapid progress. Detection of both, electron neutrinos and antineutrinos from the next galactic supernova will constrain the composition of neutrino-driven winds and provide unique nucleosynthesis information. Finally FRIB and other rare-isotope beam facilities will soon have dramatic new capabilities to synthesize many neutron-rich nuclei that are involved in the r-process. The new capabilities can significantly improve our understanding of the r-process and likely resolve one of the main outstanding problems in classical nuclear astrophysics. However, to make best use of the new experimental capabilities and to fully interpret the results, a great deal of infrastructure is needed in many related areas of astrophysics, astronomy, and nuclear theory. We will place these experiments in context by discussing astrophysical simulations and observations of r-process sites, observations of stellar abundances, galactic chemical evolution, and nuclear theory for the structure and reactions of very neutron-rich nuclei. This review paper was initiated at a three-week International Collaborations in Nuclear Theory program in June 2016 where we explored promising r-process experiments and discussed their likely impact, and their astrophysical, astronomical, and nuclear theory context.

astro-ph.SR↗

arXiv2017

Confirmation of the isomeric state in 26P

We report the independent experimental confirmation of an isomeric state in the proton drip-line nucleus $^{26}$P. The $γ$-ray energy and half-life determined are 164.4 $\pm$ 0.3 (sys) $\pm$ 0.2 (stat) keV and 104 $\pm$ 14 ns, respectively, which are in agreement with the previously reported values. These values are used to set a semi-empirical limit on the proton separation energy of $^{26}$P, with the conclusion that it can be bound or unbound.

nucl-ex↗

arXiv2016

Isobaric multiplet mass equation in the $A=31$ $T = 3/2$ quartets

The observed mass excesses of analog nuclear states with the same mass number $A$ and isospin $T$ can be used to test the isobaric multiplet mass equation (IMME), which has, in most cases, been validated to a high degree of precision. A recent measurement [Kankainen et al., Phys. Rev. C 93 041304(R) (2016)] of the ground-state mass of $^{31}$Cl led to a substantial breakdown of the IMME for the lowest $A = 31, T = 3/2$ quartet. The second-lowest $A = 31, T = 3/2$ quartet is not complete, due to uncertainties associated with the identity of the $^{31}$S member state. Using a fast $^{31}$Cl beam implanted into a plastic scintillator and a high-purity Ge $γ$-ray detection array, $γ$ rays from the $^{31}$Cl$(βγ)$$^{31}$S sequence were measured. Shell-model calculations using USDB and the recently-developed USDE interactions were performed for comparison. Isospin mixing between the $^{31}$S isobaric analog state (IAS) at 6279.0(6) keV and a nearby state at 6390.2(7) keV was observed. The second $T = 3/2$ state in $^{31}$S was observed at $E_x = 7050.0(8)$ keV. Isospin mixing in $^{31}$S does not by itself explain the IMME breakdown in the lowest quartet, but it likely points to similar isospin mixing in the mirror nucleus $^{31}$P, which would result in a perturbation of the $^{31}$P IAS energy. USDB and USDE calculations both predict candidate $^{31}$P states responsible for the mixing in the energy region slightly above $E_x = 6400$ keV. The second quartet has been completed thanks to the identification of the second $^{31}$S $T = 3/2$ state, and the IMME is validated in this quartet.

nucl-ex↗

arXiv2016

Beta-delayed gamma decay of 26P: Possible evidence of a proton halo

Background: Measurements of $β$ decay provide important nuclear structure information that can be used to probe isospin asymmetries and inform nuclear astrophysics studies. Purpose: To measure the $β$-delayed $γ$ decay of $^{26}$P and compare the results with previous experimental results and shell-model calculations. Method: A $^{26}$P fast beam produced using nuclear fragmentation was implanted into a planar germanium detector. Its $β$-delayed $γ$-ray emission was measured with an array of 16 high-purity germanium detectors. Positrons emitted in the decay were detected in coincidence to reduce the background. Results: The absolute intensities of $^{26}$P $β$-delayed $γ$-rays were determined. A total of six new $β$-decay branches and 15 new $γ$-ray lines have been observed for the first time in $^{26}$P $β$-decay. A complete $β$-decay scheme was built for the allowed transitions to bound excited states of $^{26}$Si. $ft$ values and Gamow-Teller strengths were also determined for these transitions and compared with shell model calculations and the mirror $β$-decay of $^{26}$Na, revealing significant mirror asymmetries. Conclusions: A very good agreement with theoretical predictions based on the USDB shell model is observed. The significant mirror asymmetry observed for the transition to the first excited state ($δ=51(10)\%$) may be evidence for a proton halo in $^{26}$P.

nucl-ex↗

arXiv2016

Isospin Mixing Reveals $^{30}$P($p,γ$)$^{31}$S Resonance Influencing Nova Nucleosynthesis

The thermonuclear $^{30}$P($p,γ$)$^{31}$S reaction rate is critical for modeling the final elemental and isotopic abundances of ONe nova nucleosynthesis, which affect the calibration of proposed nova thermometers and the identification of presolar nova grains, respectively. Unfortunately, the rate of this reaction is essentially unconstrained experimentally, because the strengths of key $^{31}$S proton capture resonance states are not known, largely due to uncertainties in their spins and parities. Using the $β$ decay of $^{31}$Cl, we have observed the $β$-delayed $γ$ decay of a $^{31}$S state at $E_x = 6390.2(7)$ keV, with a $^{30}$P($p,γ$)$^{31}$S resonance energy of $E_r = 259.3(8)$ keV, in the middle of the $^{30}$P($p,γ$)$^{31}$S Gamow window for peak nova temperatures. This state exhibits isospin mixing with the nearby isobaric analog state (IAS) at $E_x = 6279.0(6)$ keV, giving it an unambiguous spin and parity of $3/2^+$ and making it an important $l = 0$ resonance for proton capture on $^{30}$P.

nucl-ex↗

arXiv2016

Digital Data Acquisition For the Low Energy Neutron Detector Array (LENDA)

A digital data acquisition system (DDAS) has been implemented for the Low Energy Neutron Detector Array (LENDA). LENDA is an array of 24 BC-408 plastic-scintillator bars designed to measure low-energy neutrons with kinetic energies in the range of 100 keV to 10 MeV from (p,n)-type charge-exchange reactions. Compared to the previous data acquisition (DAQ) system for LENDA, DDAS offers the possibility to lower the neutron detection threshold, increase the overall neutron-detection efficiency, decrease the dead time of the system, and allow for easy expansion of the array. The system utilized in this work was XIA's Digital Gamma Finder Pixie-16 250 MHz digitizers. A detector-limited timing resolution of 400 ps was achieved for a single LENDA bar. Using DDAS, the neutron detection threshold of the system was reduced compared to the previous analog system, now reaching below 100 keV. The new DAQ system was successfully used in a recent charge-exchange experiment using the $^{16}$C(p,n) reaction at the National Superconducting Cyclotron Laboratory (NSCL).

physics.ins-det↗

arXiv2015

Revalidation of the isobaric multiplet mass equation for the $A=20$ quintet

An unexpected breakdown of the isobaric multiplet mass equation in the $A=20$, $T=2$ quintet was recently reported, presenting a challenge to modern theories of nuclear structure. In the present work, the excitation energy of the lowest $T = 2$ state in $^{20}$Na has been measured to be $6498.4 \pm 0.2_{\textrm{stat}} \pm 0.4_{\textrm{syst}}$ keV by using the superallowed $0^+ \rightarrow 0^+$ beta decay of $^{20}$Mg to access it and an array of high-purity germanium detectors to detect its $γ$-ray deexcitation. This value differs by 27 keV (1.9 standard deviations) from the recommended value of $6525 \pm 14$ keV and is a factor of 28 more precise. The isobaric multiplet mass equation is shown to be revalidated when the new value is adopted.

nucl-ex↗

arXiv2015

Observation of Doppler broadening in $β$-delayed proton-$γ$ decay

Background: The Doppler broadening of $γ$-ray peaks due to nuclear recoil from $β$-delayed nucleon emission can be used to measure the energies of the nucleons. This method has never been tested using $β$-delayed proton emission or applied to a recoil heavier than $A=10$. Purpose: To test and apply this Doppler broadening method using $γ$-ray peaks from the $^{26}$P($βpγ$)$^{25}$Al decay sequence. Methods: A fast beam of $^{26}$P was implanted into a planar Ge detector, which was used as a $^{26}$P $β$-decay trigger. The SeGA array of high-purity Ge detectors was used to detect $γ$ rays from the $^{26}$P($βpγ$)$^{25}$Al decay sequence. Results: Radiative Doppler broadening in $β$-delayed proton-$γ$ decay was observed for the first time. The Doppler broadening analysis method was verified using the 1613 keV $γ$-ray line for which the proton energies were previously known. The 1776 keV $γ$ ray de-exciting the 2720 keV $^{25}$Al level was observed in $^{26}$P($βpγ$)$^{25}$Al decay for the first time and used to determine that the center-of-mass energy of the proton emission feeding the 2720-keV level is 5.1 $\pm$ 1.0 (stat.) $\pm$ 0.6 (syst.) MeV, corresponding to a $^{26}$Si excitation energy of 13.3 $\pm$ 1.0 (stat.) $\pm$ 0.6 (syst.) MeV for the proton-emitting level. Conclusions: The Doppler broadening method has been demonstrated to provide practical measurements of the energies for $β$-delayed nucleon emissions populating excited states of nuclear recoils at least as heavy as $A=25$.

nucl-ex↗

arXiv2014

Novel technique for constraining r-process (n,$γ$) reaction rates

A novel technique has been developed, which will open exciting new opportunities for studying the very neutron-rich nuclei involved in the r-process. As a proof-of-principle, the $γ$-spectra from the $β$-decay of $^{76}$Ga have been measured with the SuN detector at the National Superconducting Cyclotron Laboratory. The nuclear level density and $γ$-ray strength function are extracted and used as input to Hauser-Feshbach calculations. The present technique is shown to strongly constrain the $^{75}$Ge($n,γ$)$^{76}$Ge cross section and reaction rate.

nucl-ex↗

arXiv2014

Proton spectroscopy of 48Ni, 46Fe, and 44Cr

Results of decay spectroscopy on nuclei in vicinity of the doubly magic 48Ni are presented. The measurements were performed with a Time Projection Chamber with optical readout which records tracks of ions and protons in the gaseous volume. Six decays of 48Ni including four events of two-proton ground-state radioactivity were recorded. An advanced reconstruction procedure yielded the 2p decay energy for 48Ni of Q2p = 1.29(4) MeV. In addition, the energy spectra of \b{eta}-delayed protons emitted in the decays of 44Cr and 46Fe, as well as half-lives and branching ratios were determined. The results were found to be consistent with the previous measurements made with Si detectors. A new proton line in the decay of 44Cr corresponding to the decay energy of 760 keV is reported. The first evidence for the \b{eta}2p decay of 46 Fe, based on one clear event, is shown.

nucl-ex↗

arXiv2013

Classical-Nova Contribution to the Milky Way's $^{26}$Al Abundance: Exit Channel of the Key $^{25}$Al($p,γ$)$^{26}$Si Resonance

Classical novae are expected to contribute to the 1809-keV Galactic $γ$-ray emission by producing its precursor $^{26}$Al, but the yield depends on the thermonuclear rate of the unmeasured $^{25}$Al($p,γ$)$^{26}$Si reaction. Using the $β$ decay of $^{26}$P to populate the key $J^π=3^+$ resonance in this reaction, we report the first evidence for the observation of its exit channel via a $1741.6 \pm 0.6 (\textrm{stat}) \pm 0.3 (\textrm{syst})$ keV primary $γ$ ray, where the uncertainties are statistical and systematic, respectively. By combining the measured $γ$-ray energy and intensity with other experimental data on $^{26}$Si, we find the center-of-mass energy and strength of the resonance to be $E_r = 414.9 \pm 0.6(\textrm{stat}) \pm 0.3 (\textrm{syst}) \pm 0.6(\textrm{lit.})$ keV and $ωγ= 23 \pm 6 (\textrm{stat})^{+11}_{-10}(\textrm{lit.})$ meV, respectively, where the last uncertainties are from adopted literature data. We use hydrodynamic nova simulations to model $^{26}$Al production showing that these measurements effectively eliminate the dominant experimental nuclear-physics uncertainty and we estimate that novae may contribute up to 30% of the Galactic $^{26}$Al.

nucl-ex↗

arXiv2012

Beta decay of 71,73Co; probing single particle states approaching doubly magic 78Ni

Low-energy excited states in 71,73Ni populated via the β decay of 71,73Co were investigated in an experiment performed at the National Superconducting Cyclotron Laboratory (NSCL) at Michigan State University (MSU). Detailed analysis led to the construction of level schemes of 71,73Ni, which are interpreted using systematics and analyzed using shell model calculations. The 5/2- states attributed to the the f5/2 orbital and positive parity 5/2+ and 7/2+ states from the g9/2 orbital have been identified in both 71,73Ni. In 71Ni the location of a 1/2- β-decaying isomer is proposed and limits are suggested as to the location of the isomer in 73Ni. The location of positive parity cluster states are also identified in 71,73Ni. Beta-delayed neutron branching ratios obtained from this data are given for both 71,73Co.

nucl-ex↗

arXiv2010

Beta-Delayed Proton Emission Branches in 43Cr

The beta+ decay of very neutron deficient 43Cr has been studied by means of an imaging time projection chamber which allowed recording tracks of charged particles. Events of beta-delayed emission of one-, two-, and three protons were clearly identified. The absolute branching ratios for these channels were determined to be 81(4)%, 7.1(4)%, and 0.08(3)%, respectively. The 43Cr is thus established as the second case in which the beta-3p decay occurs. Although the feeding to the proton-bound states in 43V is expected to be negligible, the large branching ratio of 12(4)% for decays without proton emission is found.

nucl-ex↗

arXiv2010

Half-lives and branchings for β-delayed neutron emission for neutron-rich Co-Cu isotopes in the r-process

The β decays of very neutron-rich nuclides in the Co-Zn region were studied experimentally at the National Superconducting Cyclotron Laboratory using the NSCL β-counting station in conjunction with the neutron detector NERO. We measured the branchings for β-delayed neutron emission (Pn values) for 74Co (18 +/- 15%) and 75-77Ni (10 +/- 2.8%, 14 +/- 3.6%, and 30 +/- 24%, respectively) for the first time, and remeasured the Pn values of 77-79Cu, 79,81Zn, and 82Ga. For 77-79Cu and for 81Zn we obtain significantly larger Pn values compared to previous work. While the new half-lives for the Ni isotopes from this experiment had been reported before, we present here in addition the first half-life measurements of 75Co (30 +/- 11 ms) and 80Cu (170+110 -50 ms). Our results are compared with theoretical predictions, and their impact on various types of models for the astrophysical rapid neutron-capture process (r-process) is explored. We find that with our new data, the classical r-process model is better able to reproduce the A = 78-80 abundance pattern inferred from the solar abundances. The new data also influence r-process models based on the neutrino-driven high-entropy winds in core collapse supernovae.

nucl-ex↗